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K. F. Allison

Publications and source records attributed to K. F. Allison.

2 recordsLinked to original sources

Dynamic polarization of graphene by moving external charges: random phase approximation

We evaluate the stopping and image forces on a charged particle moving parallel to a doped sheet of graphene by using the dielectric response formalism for graphene's $π$-electron bands in the random phase approximation (RPA). The forces are presented as functions of the particle speed and the particle distance for a broad range of charge-carrier densities in graphene. A detailed comparison with the results from a kinetic equation model reveal the importance of inter-band single-particle excitations in the RPA model for high particle speeds. We also consider the effects of a finite gap between graphene and a supporting substrate, as well as the effects of a finite damping rate that is included through the use of Mermin's procedure. The damping rate is estimated from a tentative comparison of the Mermin loss function with a HREELS experiment. In the limit of low particle speeds, several analytical results are obtained for the friction coefficient that show an intricate relationship between the charge-carrier density, the damping rate, and the particle distance, which may be relevant to surface processes and electrochemistry involving graphene.

cond-mat.mtrl-sci

Friction force on slow charges moving over supported graphene

We provide a theoretical model that describes the dielectric coupling of a 2D layer of graphene, represented by a polarization function in the Random Phase Approximation, and a semi-infinite 3D substrate, represented by a surface response function in a non-local formulation. We concentrate on the role of the dynamic response of the substrate for low-frequency excitations of the combined graphene-substrate system, which give rise to the stopping force on slowly moving charges above graphene. A comparison of the dielectric loss function with experimental HREELS data for graphene on a SiC substrate is used to estimate the damping rate in graphene and to reveal the importance of phonon excitations in an insulating substrate. A signature of the hybridization between graphene's pi plasmon and the substrate's phonon is found in the stopping force. A friction coefficient that is calculated for slow charges moving above graphene on a metallic substrate shows an interplay between the low-energy single-particle excitations in both systems.

cond-mat.mes-hall