arXiv subjects

K. Fujita

Publications and source records attributed to K. Fujita.

At least 73 records · Page 4Linked to original sources

arXiv2009

Spectroscopic Fingerprint of Phase-Incoherent Superconductivity in the Cuprate Pseudogap State

A possible explanation for the existence of the cuprate "pseudogap" state is that it is a d-wave superconductor without quantum phase rigidity. Transport and thermodynamic studies provide compelling evidence that supports this proposal, but few spectroscopic explorations of it have been made. One spectroscopic signature of d-wave superconductivity is the particle-hole symmetric "octet" of dispersive Bogoliubov quasiparticle interference modulations. Here we report on this octet's evolution from low temperatures to well into the underdoped pseudogap regime. No pronounced changes occur in the octet phenomenology at the superconductor's critical temperature Tc, and it survives up to at least temperature T ~ 1.5Tc. In the pseudogap regime, we observe the detailed phenomenology that was theoretically predicted for quasiparticle interference in a phase-incoherent d-wave superconductor. Thus, our results not only provide spectroscopic evidence to confirm and extend the transport and thermodynamics studies, but they also open the way for spectroscopic explorations of phase fluctuation rates, their effects on the Fermi arc, and the fundamental source of the phase fluctuations that suppress superconductivity in underdoped cuprates.

cond-mat.supr-con↗

arXiv2009

Measurement of diffusion thermopower in the quantum Hall systems

We have measured diffusion thermopower in a two-dimensional electron gas at low temperature ($T$=40 mK) in the field range 0 $<B<$ 3.4 T, by employing the current heating technique. A Hall bar device is designed for this purpose, which contains two crossing Hall bars, one for the measurement and the other used as a heater, and is equipped with a metallic front gate to control the resistivity of the areas to be heated. In the low magnetic field regime ($B\leq$ 1 T), we obtain the transverse thermopower $S_{yx}$ that quantitatively agrees with the $S_{yx}$ calculated from resistivities using the generalized Mott formula. In the quantum Hall regime ($B\geq$ 1T), we find that $S_{yx}$ signal appears only when both the measured and the heater area are in the resistive (inter-quantum Hall transition) region. Anomalous gate-voltage dependence is observed above $\sim$1.8 T, where spin-splitting in the measured area becomes apparent.

cond-mat.mes-hall↗

arXiv2009

Polarization transfer measurements for $^{12}{\rm C}(\vec{p},\vec{n})^{12}{\rm N (g.s.},1^+)$ at 296 MeV and nuclear correlation effects

Differential cross sections and complete sets of polarization observables are presented for the Gamow-Teller $^{12}{\rm C}(\vec{p},\vec{n})^{12}{\rm N}({\rm g.s.},1^+)$ reaction at a bombarding energy of 296 MeV with momentum transfers $q$ of 0.1 to $2.2{\rm fm}^{-1}$. The polarization transfer observables are used to deduce the spin-longitudinal cross section, $ID_q$, and spin-transverse cross sections, $ID_p$ and $ID_n$. The data are compared with calculations based on the distorted wave impulse approximation (DWIA) using shell-model wave functions. Significant differences between the experimental and theoretical results are observed for all three spin-dependent $ID_i$ at momentum transfers of $q \gtrsim 0.5{\rm fm}^{-1}$, suggesting the existence of nuclear correlations beyond the shell model. We also performed DWIA calculations employing random phase approximation (RPA) response functions and found that the observed discrepancy is partly resolved by the pionic and rho-mesonic correlation effects.

nucl-ex↗

arXiv2009

Effects of out-of-plane disorder on the nodal quasiparticle and superconducting gap in single-layer Bi$_2$Sr$_{1.6}Ln_{0.4}$CuO$_{6+δ}$ ($Ln$ = La, Nd, Gd)

How out-of-plane disorder affects the electronic structure has been investigated for the single-layer cuprates Bi$_2$Sr$_{1.6}$$Ln$$_{0.4}$CuO$_{6+δ}$ ($Ln$ = La, Nd, Gd) by angle-resolved photoemission spectroscopy. We have observed that, with increasing disorder, while the Fermi surface shape and band dispersions are not affected, the quasi-particle width increases, the anti-nodal gap is enhanced and the superconducting gap in the nodal region is depressed. The results indicate that the superconductivity is significantly depressed by out-of-plane disorder through the enhancement of the anti-nodal gap and the depression of the superconducting gap in the nodal region.

cond-mat.supr-con↗

arXiv2009

Enhancement of the superconducting critical temperature in Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ by controlling disorder outside CuO$_2$ planes

We investigate the effect of disorder at various lattice sites outside the CuO$_2$ plane on the superconducting critical temperature $T_c$ of the cuprate superconductor Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ (Bi2212). The most effective disorder turns out to be that at the Sr site in the neighboring blocks, which contain apical-oxygen atoms. The Sr-site disorder reduces $T_c$ and also produces a residual component ($ρ_0$) in the in-plane resistivity, the magnitude of which is found to be proportional to the magnitude of $T_c$ reduction. We demonstrate that both $T_c$-degradation rate and $ρ_0$ decrease as the number of the CuO$_2$ planes increases in the unit cell, that is, as the number of the neighboring SrO blocks decreases. In real crystals of Bi-based cuprates, main source of disorder is Bi atoms randomly occupying the Sr sites. We have succeeded in reducing the Bi content at Sr-sites as much as possible and achieved $T_c$=98K, a high-$T_c$ record in Bi2212.

cond-mat.supr-con↗

arXiv2008

Imaging the impact on cuprate superconductivity of varying the inter-atomic distances within individual crystal unit-cells

Many theoretical models of high temperature superconductivity focus only on the doping dependence of the CuO2 plane electronic structure. But such models are manifestly insufficient to explain the strong variations in superconducting critical temperature Tc among cuprates which have identical hole-density but are crystallographically different outside the CuO2 plane. A key challenge, therefore, has been to identify a predominant out-of-plane influence controlling the superconductivity - with much attention focusing on the distance $d_A$ between the apical oxygen and the planar copper atom. Here we report direct determination of how variations of inter-atomic distances within individual crystalline unit cells, affect the superconducting energy-gap maximum $Δ$ of Bi2Sr2CaCu2O8. In this material, quasi-periodic variations of unit cell geometry occur in the form of a bulk crystalline 'supermodulation'. Within each supermodulation period, we find a $\sim 9\pm1%$ co-sinusoidal variation in local $Δ$ that is anti-correlated with the associated $d_A$ variations. Furthermore, we show that phenomenological consistency would exist between these effects and the random $Δ$ variations found near dopant atoms if the primary effect of the interstitial dopant atom is to displace the apical oxygen so as to diminish $d_A$ or tilt the CuO5 pyramid. Thus we reveal a strong non-random out-of-plane effect on cuprate superconductivity at atomic scale.

cond-mat.supr-con↗

arXiv2008

How Cooper pairs vanish approaching the Mott insulator in Bi2Sr2CaCu2O8+d

The antiferromagnetic ground state of copper oxide Mott insulators is achieved by localizing an electron at each copper atom in real space (r-space). Removing a small fraction of these electrons (hole doping) transforms this system into a superconducting fluid of delocalized Cooper pairs in momentum space (k-space). During this transformation, two distinctive classes of electronic excitations appear. At high energies, the enigmatic 'pseudogap' excitations are found, whereas, at lower energies, Bogoliubov quasi-particles -- the excitations resulting from the breaking of Cooper pairs -- should exist. To explore this transformation, and to identify the two excitation types, we have imaged the electronic structure of Bi2Sr2CaCu2O8+d in r-space and k-space simultaneously. We find that although the low energy excitations are indeed Bogoliubov quasi-particles, they occupy only a restricted region of k-space that shrinks rapidly with diminishing hole density. Concomitantly, spectral weight is transferred to higher energy r-space states that lack the characteristics of excitations from delocalized Cooper pairs. Instead, these states break translational and rotational symmetries locally at the atomic scale in an energy independent fashion. We demonstrate that these unusual r-space excitations are, in fact, the pseudogap states. Thus, as the Mott insulating state is approached by decreasing the hole density, the delocalized Cooper pairs vanish from k-space, to be replaced by locally translational- and rotational-symmetry-breaking pseudogap states in r-space.

cond-mat.supr-con↗

arXiv2007

Evolution of the electronic excitation spectrum with strongly diminishing hole-density in superconducting Bi_{2}Sr_{2}CaCu_{2}O_{8+δ}

A complete knowledge of its excitation spectrum could greatly benefit efforts to understand the unusual form of superconductivity occurring in the lightly hole-doped copper-oxides. Here we use tunnelling spectroscopy to measure the T\to 0 spectrum of electronic excitations N(E) over a wide range of hole-density p in superconducting Bi_{2}Sr_{2}CaCu_{2}O_{8+/delta}. We introduce a parameterization for N(E) based upon an anisotropic energy-gap /Delta (\vec k)=/Delta_{1}(Cos(k_{x})-Cos(k_{y}))/2 plus an effective scattering rate which varies linearly with energy /Gamma_{2}(E) . We demonstrate that this form of N(E) allows successful fitting of differential tunnelling conductance spectra throughout much of the Bi_{2}Sr_{2}CaCu_{2}O_{8+/delta} phase diagram. The resulting average /Delta_{1} values rise with falling p along the familiar trajectory of excitations to the 'pseudogap' energy, while the key scattering rate /Gamma_{2}^{*}=/Gamma_{2}(E=/Delta_{1}) increases from below ~1meV to a value approaching 25meV as the system is underdoped from p~16% to p<10%. Thus, a single, particle-hole symmetric, anisotropic energy-gap, in combination with a strongly energy and doping dependent effective scattering rate, can describe the spectra without recourse to another ordered state. Nevertheless we also observe two distinct and diverging energy scales in the system: the energy-gap maximum /Delta_{1} and a lower energy scale /Delta_{0} separating the spatially homogeneous and heterogeneous electronic structures.

cond-mat.supr-con↗

arXiv2007

Bogoliubov angle and visualization of particle-hole mixture in superconductors

Superconducting excitations --Bogoliubov quasiparticles -- are the quantum mechanical mixture of negatively charged electron (-e) and positively charged hole (+e). Depending on the applied voltage bias in STM one can sample the particle and hole content of such a superconducting excitation. Recent Scanning Tunneling Microscope (STM) experiments offer a unique insight into the inner workings of the superconducting state of superconductors. We propose a new observable quantity for STM studies that is the manifestation of the particle-hole dualism of the quasiparticles. We call it a {\em Bogoliubov angle}. This angle measures the relative weight of particle and hole amplitude in the superconducting (Bogoliubov) quasiparticle. We argue that this quantity can be measured locally by comparing the ratio of tunneling currents at positive and negative biases. This Bogoliubov angle allows one to measure directly the energy and position dependent particle-hole admixture and therefore visualize robustness of superconducting state locally. It may also allow one to measure the particle-hole admixture of excitations in normal state above critical temperature and thus may be used to measure superconducting correlations in pseudogap state.

cond-mat.supr-con↗

arXiv2007

Study of nuclear correlation effects via 12C(p,n)12N(g.s.,1+) at 296 MeV

We report measurements of the cross section and a complete set of polarization observables for the Gamow--Teller ${}^{12}{\rm C}(\vec{p},\vec{n}){}^{12}{\rm N}({\rm g.s.},1^+)$ reaction at a bombarding energy of 296 MeV. The data are compared with distorted wave impulse approximation calculations employing transition form factors normalized to reproduce the observed beta-decay $ft$ value. The cross section is significantly under-predicted by the calculations at momentum transfers $q \gtrsim $ 0.5 ${\rm fm^{-1}}$. The discrepancy is partly resolved by considering the non-locality of the nuclear mean field. However, the calculations still under-predict the cross section at large momentum transfers of $q$ $\simeq$ 1.6 ${\rm fm^{-1}}$. We also performed calculations employing random phase approximation response functions and found that the observed enhancement can be attributed in part to pionic correlations in nuclei.

nucl-ex↗

arXiv2007

Complete Set of Polarization Transfer Observables for the $^{12}{\rm C}(p,n)$ Reaction at 296 MeV and 0$^{\circ}$

A complete set of polarization transfer observables has been measured for the $^{12}{\rm C}(p,n)$ reaction at $T_p=296 {\rm MeV}$ and $θ_{\rm lab}=0^{\circ}$. The total spin transfer $Σ(0^{\circ})$ and the observable $f_1$ deduced from the measured polarization transfer observables indicate that the spin--dipole resonance at $E_x \simeq 7 {\rm MeV}$ has greater $2^-$ strength than $1^-$ strength, which is consistent with recent experimental and theoretical studies. The results also indicate a predominance of the spin-flip and unnatural-parity transition strength in the continuum. The exchange tensor interaction at a large momentum transfer of $Q \simeq 3.6 {\rm fm}^{-1}$ is discussed.

nucl-ex↗

arXiv2007

An Intrinsic Bond-Centered Electronic Glass with Unidirectional Domains in Underdoped Cuprates

Removing electrons from the CuO2 plane of cuprates alters the electronic correlations sufficiently to produce high-temperature superconductivity. Associated with these changes are spectral weight transfers from the high energy states of the insulator to low energies. In theory, these should be detectable as an imbalance between the tunneling rate for electron injection and extraction - a tunneling asymmetry. We introduce atomic-resolution tunneling-asymmetry imaging, finding virtually identical phenomena in two lightly hole-doped cuprates: Ca1.88Na0.12CuO2Cl2 and Bi2Sr2Dy0.2Ca0.8Cu2O8+d. Intense spatial variations in tunneling asymmetry occur primarily at the planar oxygen sites; their spatial arrangement forms a Cu-O-Cu bond centered electronic pattern without long range order but with 4a0-wide unidirectional electronic domains dispersed throughout (a0: the Cu-O-Cu distance). The emerging picture is then of a partial hole-localization within an intrinsic electronic glass evolving, at higher hole-densities, into complete delocalization and highest temperature superconductivity.

cond-mat.supr-con↗

arXiv2006

The hierarchy of multiple many-body interaction scales in high-temperature superconductors

To date, angle-resolved photoemission spectroscopy has been successful in identifying energy scales of the many-body interactions in correlated materials, focused on binding energies of up to a few hundred meV below the Fermi energy. Here, at higher energy scale, we present improved experimental data from four families of high-Tc superconductors over a wide doping range that reveal a hierarchy of many-body interaction scales focused on: the low energy anomaly ("kink") of 0.03-0.09eV, a high energy anomaly of 0.3-0.5eV, and an anomalous enhancement of the width of the LDA-based CuO2 band extending to energies of ~ 2 eV. Besides their universal behavior over the families, we find that all of these three dispersion anomalies also show clear doping dependence over the doping range presented.

cond-mat.supr-con↗

arXiv2006

Evidence for an alpha cluster condensed state in 16O(alpha,alpha') at 400 MeV

Inelastic $α$ scattering on 16O is studied at 400 MeV by using an ice target. Near the 4-alpha breakup threshold of 14.4 MeV, a broad peak is observed at an excitation energy of 13.6+/-0.2 MeV with a width of 0.6+/-0.2 MeV. The spin-parity is estimated to be 0+ from the momentum-transfer dependence. The observed width is significantly larger than those of the neighboring 0+ states indicating a state with a well-developed alpha cluster structure. The magnitude of the cross section is sensitive to the density distribution of the constituent alpha clusters. The observed cross section is consistent with the theoretical prediction for the alpha cluster condensed state characterized by its dilute density distribution with a large root-mean-square radius of about 4.3 fm.

nucl-ex↗

arXiv2006

Enhancement of electronic inhomogeneities due to out-of-plane disorder in Bi_2Sr_2CuO_{6+delta} superconductors observed by scanning tunneling spectroscopy

Nanoscale electronic inhomogeneity in optimally doped single-layer Bi_2Sr_{1.6}L_{0.4}CuO_{6+delta}, (L-Bi2201, L=La and Gd) as well as bilayer Bi_2Sr_2CaCu_2O_{8+delta} (Bi2212), superconductors has been investigated by the low-temperature scanning-tunneling-microscopy and spectroscopy. The inhomogeneous gap structures are observed above and below Tc on Gd-Bi2201. Increasing the out-of-plane disorder which is controlled by mismatch of the ionic radius between Sr and Ln results in the enhancement of pseudogap region with suppressed coherence peaks in the conductance spectrum, making the gap average larger and the gap distribution wider. The degree of electronic inhomogeneity measured by the distribution width of the gap amplitude is shown to have a correlation with Tc in optimally doped Bi2201 and Bi2212.

cond-mat.supr-con↗

arXiv2006

Interplay of electron-lattice interactions and superconductivity in Bi2Sr2CaCu2O8+d

Formation of electron pairs is essential to superconductivity. For conventional superconductors, tunnelling spectroscopy has established that pairing is mediated by bosonic modes (phonons); a peak in the second derivative of tunnel current d2I/dV2 corresponds to each phonon mode . For high-transition-temperature (high-Tc) superconductivity, however, no boson mediating electron pairing has been identified. One explanation could be that electron pair formation and related electron-boson interactions are heterogeneous at the atomic scale and therefore challenging to characterize. However, with the latest advances in d2I/dV2 spectroscopy using scanning tunnelling microscopy, it has become possible to study bosonic modes directly at the atomic scale . Here we report d2I/dV2 imaging studies of the high-Tc superconductor Bi2Sr2CaCu2O8+d. We find intense disorder of electron-boson interaction energies at the nanometre scale, along with the expected modulations in d2I/dV2 (refs 9,10). Changing the density of holes has minimal effects on both the average mode energies and the modulations, indicating that the bosonic modes are unrelated to electronic or magnetic structure. Instead, the modes appear to be local lattice vibrations, as substitution of 18O for 16O throughout the material reduces the average mode energy by approximately 6 per cent - the expected effect of this isotope substitution on lattice vibration frequencies. Significantly, the mode energies are always spatially anticorrelated with the superconducting pairing-gap energies, suggesting an interplay between these lattice vibration modes and the superconductivity.

cond-mat.supr-con↗

arXiv2005

Effect of disorder outside the CuO$_{2}$ planes on $T_{c}$ of copper oxide superconductors

The effect of disorder on the superconducting transition temperature $T_{c}$ of cuprate superconductors is examined. Disorder is introduced into the cation sites in the plane adjacent to the CuO$_{2}$ planes of two single-layer systems, Bi$_{2.0}$Sr$_{1.6}$Ln$_{0.4}$CuO$_{6+δ}$ and La$_{1.85-y}$Nd$_{y}$Sr$_{0.15}$CuO$_{4}$. Disorder is controlled by changing rare earth (Ln) ions with different ionic radius in the former, and by varying the Nd content in the latter with the doped carrier density kept constant. We show that this type of disorder works as weak scatterers in contrast to the in-plane disorder produced by Zn, but remarkably reduces $T_{c}$ suggesting novel effects of disorder on high-$T_{c}$ superconductivity.

cond-mat.supr-con↗

arXiv2005

Performance of the neutron polarimeter NPOL3 for high resolution measurements

We describe the neutron polarimeter NPOL3 for the measurement of polarization transfer observables $D_{ij}$ with a typical high resolution of $\sim$300 keV at $T_n$ $\simeq$ 200 MeV. The NPOL3 system consists of three planes of neutron detectors. The first two planes for neutron polarization analysis are made of 20 sets of one-dimensional position-sensitive plastic scintillation counters with a size of 100 cm $\times$ 10 cm $\times$ 5 cm, and they cover the area of 100 $\times$ 100 $\mathrm{cm}^2$. The last plane for detecting doubly scattered neutrons or recoiled protons is made of the two-dimensional position-sensitive liquid scintillation counter with a size of 100 cm $\times$ 100 cm $\times$ 10 cm. The effective analyzing powers $A_{y;\mathrm{eff}}$ and double scattering efficiencies $ε_{\mathrm{D.S.}}$ were measured by using the three kinds of polarized neutrons from the ${}^{2}{\rm H}(\vec{p},\vec{n})pp$, ${}^{6}{\rm Li}(\vec{p},\vec{n}){}^{6}{\rm Be}(\mathrm{g.s.})$, and ${}^{12}{\rm C}(\vec{p},\vec{n}){}^{12}{\rm N}(\mathrm{g.s.})$ reactions at $T_p$ = 198 MeV. The performance of NPOL3 defined as $ε_{\mathrm{D.S.}}(A_{y;\mathrm{eff}})^2$ are similar to that of the Indiana Neutron POLarimeter (INPOL) by taking into account for the counter configuration difference between these two neutron polarimeters.

nucl-ex↗