arXiv subjects

K. H. Kim

Publications and source records attributed to K. H. Kim.

At least 73 records · Page 4Linked to original sources

arXiv2003

A Hierarchically-Organized Phase Diagram near a Quantum Critical Point in URu2Si2

A comprehensive transport study, as a function of both temperature and magnetic field in continuous magnetic fields up to 45 T reveals that URu2Si2 possesses all the essential hallmarks of quantum criticality at temperatures above 5.5 K and fields around 38 T, but then collapses into multiple low temperature phases in a hierarchically-organized phase diagram as the temperature is reduced. Although certain generic features of the phase diagram are very similar to those in the cuprates and heavy fermion superconductors, the existence of multiple ordered hysteretic phases near the field-tuned quantum critical point is presently unique to URu2Si2. This finding suggests the existence of many competing order parameters separated by small energy difference in URu2Si2.

cond-mat.str-el↗

arXiv2002

Multi-scale Phase Modulations in Colossal Magnetoresistance Manganites

Extensive experimental results are presented on the multi-scale phase modulation phenomena observed in colossal magnetoresistance manganites. Two key types of phase inhomogeneities directly relevant to the colossal magnetoresistance (CMR) are discussed. The first type involves micrometer-scale coexistence of structurally and electronically different phases. We present extensive experimental data for a prototypical system exhibiting such a phase coexistence, (La,Pr)$_{5/8}$Ca$_{3/8}$MnO$_{3}$. These data reveal that percolative transport phenomena play the key role in the metal-insulator transition in this system, and are largely responsible for the significant magnitude of the magnetoresistance. The phase composition of the multiphase states is governed by both the electron correlations and the effects of martensitic accommodation strain. The second type of an inhomogeneous state is realized in the paramagnetic state commonly found in manganites at high-temperatures. In this state, nanometer-scale structural correlations associated with nanoscale charge/orbital ordered regions are observed. Experimental investigation of numerous manganite systems indicates that these correlations are generic in orthorhombic mixed-valent manganites, and that the correlated regions play an essential role in the CMR effect.

cond-mat.str-el↗

arXiv2002

Resonant photoemission spectroscopy study of insulator-to-metal transition in Cr- and Ru-doped Nd_{1/2}A_{1/2}Mn_{1-y} O_{3} (A=Ca, Sr)

Electronic structures of very dilute Cr- or Ru-doped Nd_{1/2}A_{1/2}MnO_{3} (NAMO; A=Ca, Sr) manganites have been investigated using the Mn and Cr 2p -> 3d resonant photoemission spectroscopy (PES). All the Cr- and Ru-doped NAMO systems exhibit the clear metallic Fermi edges in the Mn e_g spectra near E_F, consistent with their metallic ground states. The Cr 3d states with t^3_{2g} configuration are at ~ 1.3 eV below E_F, and the Cr e_{g} states do not participate in the formation of the band near E_F. Cr- and Ru-induced ferromagnetism and insulator-to-metal transitions can be understood with their measured electronic structures.

cond-mat.str-el↗

arXiv2002

High Field Studies of the Hidden Order Transition in URu$_2$Si$_2$

We studied in detail the low temperature/high magnetic field phases of URu$_{2}$Si$_{2}$ single crystals with specific heat, magnetocaloric effect, and magnetoresistance in magnetic fields up to 45 T. Data obtained down to 0.5 K, and extrapolated to T = 0, show a suppression of the hidden order phase at H$_{o}$(0) = 35.9 $\pm$ 0.35 T and the appearance of a new phase for magnetic fields in excess of H$_{1}$(0) = 36.1 $\pm$ 0.35 T observed \textit{only} at temperatures lower than 6 K. In turn, complete suppression of this high field state is attained at a critical magnetic field H$_{2}$(0) = 39.7 $\pm$ 0.35 T. No phase transitions are observed above 40 T. We discuss our results in the context of itinerant vs. localized \textit{f}-electron behavior and consider the implications for the hidden order phase.

cond-mat.str-el↗

arXiv2002

Effects of unreacted Mg impurities on the transport properties of MgB2

We synthesized polycrystalline MgB2 from a stoichiometric mixture of Mg and the 11 B isotope under different conditions. All the samples showed bulk superconductivity with Tc = 38~39 K. The samples containing the least amount of unreacted Mg showed the highest Tc and the sharpest transition width (Delta_Tc). A residual resistivity ratio (RRR) of ~ 5.8, and a magnetoresistance (MR), at 40 K, of 12% were obtained for these samples. Moreover, there was no upturn of resistivity in a low temperature region at 10 Tesla. The samples containing appreciable amounts of unreacted Mg showed quite different behaviors; the values of Delta_Tc, RRR, and MR were much larger. An upturn appeared in resistivity of the samples below about 50 K at 10 T and is thought to be due to the unreacted Mg.

cond-mat.supr-con↗

arXiv2002

Photoemission Line shape Study on La$_{0.7}$Sr$_{0.3}$Mn$_{1-δ}$Al$_δ$O$_{3}$ ($δ$ = 0, 0.03, 0.06)

We have studied the line shapes of ultraviolet photoemission spectra of La$_{0.7}$Sr$_{0.3}$Mn$_{1-δ}$Al$_δ$O$_3$ ($δ$ = 0, 0.03, 0.06) systems to test the extrinsic image charge screening effect on photoemission spectra recently suggested by R. Joynt (Science {\bf 284}, 777 (1999)), who argued that the photoemission spectrum near the Fermi energy, specially for poorly conducting system, can be very different from the intrinsic density of states because the outgoing electron has probability of losing its kinetic energy due to the image force. We tested this argument in real materials experimentally by measuring the photoemission line shapes of La$_{0.7}$Sr$_{0.3}$Mn$_{1-δ}$Al$_δ$O$_3$ systems, for which all the requirements of this theory are satisfied and sample resistivities change systematically. We found that experimental photoemission spectra do not show the change of line shapes expected from the extrinsic image force effect and we conclude that the influence of this long range interaction is not so large as suggested in that paper.

cond-mat.str-el↗

arXiv2002

Bulk-sensitive photoemission spectroscopy of A_2FeMoO_6 double perovskites (A=Sr, Ba)

Electronic structures of Sr_2FeMoO_6 (SFMO) and Ba_2FeMoO_6 (BFMO) double perovskites have been investigated using the Fe 2p->3d resonant photoemission spectroscopy (PES) and the Cooper minimum in the Mo 4d photoionization cross section. The states close to the Fermi level are found to have strongly mixed Mo-Fe t_{2g} character, suggesting that the Fe valence is far from pure 3+. The Fe 2p_{3/2} XAS spectra indicate the mixed-valent Fe^{3+}-Fe^{2+} configurations, and the larger Fe^{2+} component for BFMO than for SFMO, suggesting a kind of double exchange interaction. The valence-band PES spectra reveal good agreement with the LSDA+U calculation.

cond-mat.mtrl-sci↗

arXiv2002

Spin/Orbital Pattern-Dependent Polaron Absorption in Nd(1-x)Sr(x)MnO3

We investigated optical properties of Nd(1-x)Sr(x)MnO3 (x= 0.40, 0.50, 0.55, and 0.65) single crystals. In the spin/orbital disordered state, their conductivity spectra look quite similar, and the strength of the mid-infrared absorption peak is proportional to x(1-x) consistent with the polaron picture. As temperature lowers, the Nd(1-x)Sr(x)MnO3 samples enter into various spin/orbital ordered states, whose optical responses are quite different. These optical responses can be explained by the spin/orbital ordering pattern-dependent polaron hopping.

cond-mat.str-el↗

arXiv2002

Charge Ordering Fluctuation and Optical Pseudogap in La$_{1-x}$Ca$_{x}$MnO$_{3}$

Optical spectroscopy was used to investigate the optical gap (2$Δ$) due to charge ordering (CO) and related pseudogap developments with x and temperature (T) in La$_{1-x}$Ca$_{x}$MnO$_{3}$ (0.48 <= x <= 0.67). Surprisingly, we found 2$Δ$/k_{B}T_{CO} is as large as 30 for x ~0.5, and decreases rapidly with increasing x. Simultaneously, the optical pseudogap, possibly starting from T^* far above T_{CO} becomes drastically enhanced near x=0.5, producing non-BCS T-dependence of 2$Δ$ with the large magnitude far above T_{CO}, and systematic increase of T^* for x~0.5. These results unequivocally indicate systematically-enhanced CO correlation when x approaches 0.5 even though T_{CO} decreases.

cond-mat.str-el↗

arXiv2002

Optical Evidence of Multiphase Coexistence in Single Crystalline (La,Pr,Ca)MnO3

We investigated temperature (T)- and magnetic field-dependent optical conductivity spectra (\s\w) of a La_5/8-yPr_yCa_3/8MnO_3 (y~0.35) single crystal, showing intriguing phase coexistence at low T. At T_C < T < T_CO, a dominant charge-ordered phase produces a large optical gap energy of ~0.4 eV. At T < T_C, at least two absorption bands newly emerge below 0.4 eV. Analyses of (\s\w) indicate that the new bands should be attributed to a ferromagnetic metallic and a charge-disordered phase that coexist with the charge-ordered phase. This optical study clearly shows that La_5/8-yPrCa_3/8MnO_3 (y~0.35) is composed of multiphases that might have different lattice strains.

cond-mat.str-el↗

arXiv2001

Development of the Simulator for the Global Orbit Feedback System Using EPICS

We have carried out the basic research for the accelerator and tokamak control system based on the Experimental Physics and Industrial Control System (EPICS). We have used the process database and the state notation language (SNL) in the EPICS to develop the simulator which represents as a virtual machine. In this paper, we introduce the simulator of the global orbit feedback system as an example. This simulates the global orbit feedback system under the constraint conditions for Pohang Light Source (PLS) storage ring. We describe the details of the feedback algorithm and the realization of the simulator.

nucl-ex↗

arXiv2000

Raman scattering study of anomalous charge-, spin-, and lattice-dynamics in the charge-ordered phase of ${\bf Bi}_{1-x}{\bf Ca}_x{\bf MnO}_3$ ($x>0.5$)

We report an inelastic light scattering study of the effects of charge-ordering on the spin-, charge-, and lattice-dynamics in ${\rm Bi}_{1-x}{\rm Ca}_{x}{\rm MnO}_3$ $(x>0.5)$. We find that charge-ordering results in anomalous phonon behavior, such as the appearance of `activated' modes. More significantly, however, the transition to the CO phase results in the appearance of a quasielastic scattering response with the symmetry of the spin chirality operator ($T_{1g}$); this scattering response is thus indicative of magnetic or chiral spin fluctuations in the AFM charge-ordered phase.

cond-mat.str-el↗

arXiv2000

High Temperature Charge-Ordering Fluctuation in Manganites

High temperature (T) studies of La_{1-x}Ca_{x}MnO_{3} show that charge and phonon transport is significantly suppressed in a narrow doping region of x~1/2 and in a wide T range up to 900 K, which accompanies anomalous broadening of x-ray Bragg peaks. Contrarily, ferromagnetic (FM) correlation above Curie T is sharply enhanced at x~3/8. All these observations indicate the presence of short-range charge ordering (CO) correlation at high T, possibly in the form of a FM "zigzag", a small segment of the CE-type CO state. The decoupling and coupling of the FM zigzags for x~3/8 and 1/2, respectively, is consistent with our results.

cond-mat.str-el↗

arXiv2000

Optical Studies of a Layered Manganite La_{1.2}Sr_{1.8}Mn_2O_7 : Polaron Correlation Effect

Optical conductivity spectra of a cleaved ab-plane of a La_{1.2}Sr_{1.8}Mn_2O_7 single crystal exhibit a small polaron absorption band in the mid-infrared region at overall temperatures. With decreasing temperature (T) to Curie temperature (T_C), the center frequency of the small polaron band moves to a higher frequency, resulting in a gap-like feature, and that it collapses to a lower frequency below T_C. Interestingly, with decreasing T, the stretching phonon mode hardens above T_C and softens below T_C. These concurring changes of lattice and electronic structure indicate that short range polaron correlation exist above T_C but disappear with a magnetic ordering.

cond-mat.str-el↗

arXiv2000

Anomalous field-dependent specific heat in charge-ordered Pr$_{1-x}$Ca$_x$MnO$_3$ and La$_{0.5}$Ca$_{0.5}$MnO$_3$

We report low temperature specific heat measurements of Pr$_{1-x}$Ca$_{x}$MnO$_{3}$ ($0.3\leq x \leq 0.5$) and La$_{0.5}$Ca$_{0.5}$MnO$_{3}$ with and without applied magnetic field. An excess specific heat, $C^{\prime}(T)$, of non-magnetic origin associated with charge ordering is found for all the samples. A magnetic field sufficient to induce the transition from the charge-ordered state to the ferromagnetic metallic state does not completely remove the $C^{\prime}$ contribution. This suggests that the charge ordering is not completely destroyed by a "melting" magnetic field. In addition, the specific heat of the Pr$_{1-x}$Ca$_{x}$MnO$_{3}$ compounds exhibit a large contribution linear in temperature ($γT$) originating from magnetic and charge disorder.

cond-mat.str-el↗

arXiv2000

Thermal/Electronic Transport Properties and Two-Phase Mixtures in La_{5/8-x}Pr_{x}Ca_{3/8}MnO_{3}

We measured thermal conductivity, k, thermoelectric power, S, and dc electric conductivity, sigma, of La_{5/8-x}Pr_{x}Ca_{3/8}MnO_{3}, showing an intricate interplay between metallic ferromagnetism (FM) and charge ordering (CO) instability. The change of k, S and sigma with temperature (T) and x agrees well with the effective medium theories for binary metal-insulator mixtures. This agreement clearly demonstrates that with the variation of T as well as x, the relative volumes of FM and CO phases drastically change and percolative metal-insulator transition occurs in the mixture of FM and CO domains.

cond-mat.str-el↗

arXiv1999

Electrodynamics of Nd0.7Sr0.3MnO3 Single Crystal investigated by Optical Conductivity Analyses

We investigated temperature dependent optical conductivity spectra of Nd0.7Sr0.3MnO3 single crystal. We found that polishing and surface scattering effects on the Nd0.7Sr0.3MnO3 crystal surfaces could significantly distort the optical responses, especially in the mid-infrared region. However, oxygen annealing and gold normalization processes seemed to remedy the distortions. We found that the spectral weight of Nd0.7Sr0.3MnO3 in the metallic state might be composed of a Drude carrier term and a strong incoherent mid-infrared absorptions. The temperature dependence of the spectral weight suggests that the electron-lattice coupling should be important in optical properties of colossal magnetoresistance manganites.

cond-mat.str-el↗

arXiv1998

Optical Investigations of La_{7/8}Sr_{1/8}MnO_3

We investigated temperature dependent optical conductivity spectra of La_{7/8}Sr_{1/8}MnO_3. Its phonon bending mode starts to be splitted near a structural phase transition temperature. With further cooling, strength of a mid-infrared small polaron peak, which is located at 0.4 eV, becomes increased. These temperature dependent changes in the phonon spectra and the polaron absorption peaks were explained by a phase separation and a percolation-type transition.

cond-mat.str-el↗