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K. Hirose

Publications and source records attributed to K. Hirose.

At least 19 recordsLinked to original sources

Kinetic energy of fission fragments within a dynamical model

Kinetic energy of individual fission fragment for actinide nuclei is, for example, important for evaluating the prompt-neutron spectrum in the laboratory system. It is experimentally known that kinetic energy for each fragment is constant at about 100 MeV for light fragments and that for heavy fragments decreases linearly with mass number. Most of the theoretical studies carried out so far attempted to calculate the total kinetic energy of both fragments, i.e. sum of the energies of two fragments, but the kinetic energy of each fragment was not analyzed in detail as far as we recognize. We have calculated them in thermal-neutron induced fission of $^{239}\mathrm{Pu}$ with a dynamical model using Langevin equations within a three-dimensional two-center parametrization. Also fission of $^{258}\mathrm{Fm}$ was investigated. It is calculated from the Coulomb energy at the scission point and the pre-scission kinetic energy. It is found that the pre-scission kinetic energy has about 2-4% contribution in the kinetic energy. The calculated results reproduce the trend of the experimental data.

nucl-th

Neutron emission during fission and its impact on fission-fragment mass distribution studied by Langevin model

Actinide nuclei exhibit mass-asymmetric fission at low energy due to shell structure. The fission-fragment mass distributions produced at high energy tend to have a symmetric shape due to smearing of shell effects. On the other hand, the distribution can be changed by neutron emission occurring before fission, as this decreases the excitation energy of the fissioning nucleus, and thus revives the shell structure. In so called multichance fission, neutron emission is considered prior to fission at the initial nuclear shape, and competition between fission and neutron emission is determined with the framework of the statistical model. In the present work, we describe fission in the Langevin equations, and neutron emission is treated throughout the fission process. The calculation reproduces experimentally observed mass distributions, and for a wide range of initial compound-nucleus excitation energy up to 60 MeV. The results show that, while neutron emission dominates at the ground-state shape, it occurs along the shape evolution path to the scission point.

nucl-th

Giant Dipole Resonance photofission and photoneutron reactions in $^{238}$U and $^{232}$Th

New measurements of photofission and photoneutron reactions on $^{238}$U and $^{232}$Th in the Giant Dipole Resonance (GDR) energy region have been performed at the laser Compton-scattering $\gamma$-ray source of the NewSUBARU synchrotron radiation facility using a high-and-flat efficiency moderated $^3$He detection array. The neutron-multiplicity sorting of high-multiplicity fission neutron coincidence events has been performed using a dedicated energy dependent, multiple firing statistical treatment. The photoneutron $(\gamma,\,in)$ with $i$~=~1~--~3 and photofission $(\gamma,\,F)$ reactions have been discriminated by considering a Gaussian distribution of prompt-fission-neutron (PFN) multiplicities predicted by the theory of evaporation in sequential neutron emission from excited fission fragments. We report experimental $(\gamma,\,n)$, $(\gamma,\,2n)$, $(\gamma,\,3n)$ and $(\gamma,\,F)$ cross sections, average energies of PFNs and of $(\gamma,\,in)$ photoneutrons, as well as the mean number of PFNs per fission act and the width of the PFNs multiplicity distribution. Based on these primary experimental results and combined with reasonable assumptions, we extract also the first- and second-chance fission contributions. The new experimental results are compared with statistical-model calculations performed with the EMPIRE-3.2 Malta and TALYS-1.964 codes on the present data and with prompt fission emission calculations obtained with the Los Alamos model in the frame of the most probable fragmentation approach with and without sequential emission.

nucl-ex

Search for the 6$\alpha$ condensed state in $^{24}$Mg using the $^{12}\rm{C}+{}^{12}\rm{C}$ scattering

We searched for the 6$\alpha$-condensed state in $^{24}$Mg by measuring the $^{12}\rm{C}+{}^{12}\rm{C}$ scattering with the SAKRA Si detector array at $E_\rm{cm}$ = 17.5-25.0 MeV. By using the invariant-mass method for the detected 3$\alpha$ particles, the inclusive cross sections for the $^{12}\rm{C}+{}^{12}\rm{C}\to{}^{12}\rm{C}(0^+_2)+X$ and $^{12}\rm{C}(3^-_1)+X$ reactions were determined. In addition, the missing-mass spectroscopy was successfully utilized to determine the excitation energy of the residual $^{12}\rm{C}$ nucleus and the exclusive cross sections for the $^{12}\rm{C}+{}^{12}\rm{C}\to{}^{12}\rm{C}(0^+_2)+{}^{12}\rm{C}(0^+_1)$, $^{12}\rm{C}(0^+_2)+{}^{12}\rm{C}(2^+_1)$, and $^{12}\rm{C}(0^+_2)+{}^{12}\rm{C}(0^+_2)$ reactions. In both the inclusive $^{12}\rm{C}(0^+_2)+X$ channel and the exclusive $^{12}\rm{C}(0^+_2)+{}^{12}\rm{C}(0^+_1)$ channel, the cross section peaked at $E_rm{cm}$ = 19.4 MeV, which correspond to the excitation energy of $E_x$ = 33.3 MeV in $^{24}\rm{Mg}$. This 19.4-MeV state is a candidate for the 6$\alpha$-condensed state because of the agreement of the excitation energy with the theoretical value and its decay property. In the exclusive $^{12}\rm{C}(0^+_2)+{}^{12}\rm{C}(0^+_2)$ channel, a broad state was observed at $E_\rm{cm}$ = 22.5 MeV, which correspond to the excitation energy of $E_x$ = 36.4 MeV in $^{24}\rm{Mg}$. From the angular distribution of the differential cross section, the spin and parity of this 22.5-MeV state was assigned to be $4^+$. In addition, a $2^+$ state was suggested at the low-energy side of the 22.5-MeV state. Because their excitation energies are higher than the theoretical value of the 6$\alpha$-condensed state, these states might be excited states of the 6$\alpha$-condensed state such as the $2^+_2$ and $4^+_1$ states in $^{12}\rm{C}$.

nucl-ex

The $^{59}$Fe(n, γ)$^{60}$Fe Cross Section from the Surrogate Ratio Method and Its Effect on the $^{60}$Fe Nucleosynthesis

The long-lived $^{60}$Fe (with a half-life of 2.62 Myr) is a crucial diagnostic of active nucleosynthesis in the Milky Way galaxy and in supernovae near the solar system. The neutron-capture reaction $^{59}$Fe(n,$γ$)$^{60}$Fe on $^{59}$Fe (half-life = 44.5 days) is the key reaction for the production of $^{60}$Fe in massive stars. This reaction cross section has been previously constrained by the Coulomb dissociation experiment, which offered partial constraint on the $E$1 $γ$-ray strength function but a negligible constraint on the $M$1 and $E$2 components. In this work, for the first time, we use the surrogate ratio method to experimentally determine the $^{59}$Fe(n,$γ$)$^{60}$Fe cross sections in which all the components are included. We derived a Maxwellian-averaged cross section of 27.5 $\pm$ 3.5 mb at $kT$= 30 keV and 13.4 $\pm$ 1.7 mb at $kT$= 90 keV, roughly 10 - 20% higher than previous estimates. We analyzed the impact of our new reaction rates in nucleosynthesis models of massive stars and found that uncertainties in the production of $^{60}$Fe from the $^{59}$Fe(n,$γ$)$^{60}$Fe rate are at most of 25%. We conclude that stellar physics uncertainties now play a major role in the accurate evaluation of the stellar production of $^{60}$Fe.

astro-ph.GA

Estimation of the detected background by the future gamma-ray transient mission CAMELOT

This study presents a background estimation for the Cubesats Applied for MEasuring and LOcalising Transients (CAMELOT), which is a proposed fleet of nanosatellites for the all-sky monitoring and timing based localization of gamma-ray transients with precise localization capability at low Earth orbits. CAMELOT will allow to observe and precisely localize short gamma-ray bursts (GRBs) associated with kilonovae, long GRBs associated with core-collapse massive stars, magnetar outbursts, terrestrial gamma-ray flashes, and gamma-ray counterparts to gravitational wave sources. The fleet of at least nine 3U CubeSats is proposed to be equipped with large and thin CsI(Tl) scintillators read out by multi-pixel photon counters (MPPC). A careful study of the radiation environment in space is necessary to optimize the detector casing, estimate the duty cycle due to the crossing of the South Atlantic Anomaly and polar regions, and to minimize the effect of the radiation damage of MPPCs.

astro-ph.HE

First observation of the competing fission modes in the neutron-deficient sub-lead region

Fragment mass distributions from fission of excited compound nucleus $^{178}$Pt have been deduced from the measured fragment velocities. The $^{178}$Pt nucleus was created at the JAEA tandem facility in a complete fusion reaction $^{36}$Ar + $^{142}$Nd, at beam energies of 155, 170 and 180 MeV. The data are indicative of a mixture of the mass-asymmetric and mass-symmetric fission modes associated with higher and lower total kinetic energies of the fragments, respectively. The measured fragment yields are dominated by asymmetric mass splits, with the symmetric mode contributing at the level of $\approx1/3$. This constitutes the first observation of a multimodal fission in the sub-lead region. Most probable experimental fragment-mass split of the asymmetric mode, $A_{L}/A_{H}\approx 79/99$, is well reproduced by nuclear density functional theory using the UNEDF1-HFB and D1S potentials. The symmetric mode is associated by theory with very elongated fission fragments, which is consistent with the observed total kinetic energy/fragment mass correlation.

nucl-ex

Core-exsolved SiO$_2$ dispersal in the Earth's mantle

SiO$_2$ may have been expelled from the core directly following core formation in the early stages of Earth's accretion and onwards through the present day. On account of SiO$_2$'s low density with respect to both the core and the lowermost mantle, we examine the process of SiO$_2$ accumulation at the core-mantle boundary (CMB) and its incorporation into the mantle by buoyant rise. Today, if SiO$_2$ is 100-10000 times more viscous than lower mantle material, the dimensions of SiO$_2$ diapirs formed by the viscous Rayleigh-Taylor instability at the CMB would cause them to be swept into the mantle as inclusions of 100 m - 10 km diameter. Under early Earth conditions of rapid heat loss after core formation, SiO$_2$ diapirs of ~1 km diameter could have risen independently of mantle flow to their level of neutral buoyancy in the mantle, trapping them there due to a combination of intrinsically high viscosity and neutral buoyancy. We examine the SiO$_2$ yield by assuming Si+O saturation at the conditions found at the base of a magma ocean and find that for a range of conditions, dispersed bodies could reach as high as 8.5 vol.% in parts of the lower mantle. At such low concentration, their effect on aggregate seismic wavespeeds is within observational seismology uncertainty. However, their presence can account for small-scale scattering in the lower mantle due to the bodies' large velocity contrast. We conclude that the shallow lower mantle (700-1500 km depth) could harbor SiO$_2$ released in early Earth times.

astro-ph.EP

Neutral Kaon Spectrometer 2

A large-acceptance spectrometer, Neutral Kaon Spectrometer 2 (NKS2), was newly constructed to explore various photoproduction reactions in the gigaelectronvolt region at the Laboratory of Nuclear Science (LNS, currently ELPH), Tohoku University. The spectrometer consisted of a dipole magnet, drift chambers, and plastic scintillation counters. NKS2 was designed to separate pions and protons in a momentum range of less than 1 GeV/$c$, and was placed in a tagged photon beamline. A cryogenic H$_{2}$/D$_{2}$ target fitted to the spectrometer were designed. The design and performance of the detectors are described. The results of the NKS2 experiment on analyzing strangeness photoproduction data using a 0.8--1.1 GeV tagged photon beam are also presented.

physics.ins-det

The 95zr(n, gamma)96zr cross section from the surrogate ratio method and its effect on the s-process nucleosynthesis

The 95Zr(n,gamma)96Zr reaction cross section is crucial in the modelling of s-process nucleosynthesis in asymptotic giant branch stars because it controls the operation of the branching point at the unstable 95Zr and the subsequent production of 96Zr. We have carried out the measurement of the 94Zr(18O,16O) and 90Zr(18O,16O) reactions and obtained the gamma-decay probability ratio of 96Zr* and 92Zr* to determine the 95Zr(n,gamma)96Zr reaction cross sections with the surrogate ratio method. Our deduced maxwellian-averaged cross section of 66+-16 mb at 30 keV is close to the value recommended by Bao et al. (2000), but 30% and more than a factor of two larger than the values proposed by Toukan & Kappeler (1990) and Lugaro et al. (2014), respectively, and routinely used in s-process models. We tested the new rate in stellar models with masses between 2 and 6 Msun and metallicities 0.014 and 0.03. The largest changes - up 80% variations in 96Zr - are seen in models of mass 3-4 Msun, where the 22Ne neutron source is mildly activated. The new rate can still provide a match to data from meteoritic stardust silicon carbide grains, provided the maximum mass of the parent stars is below 4 Msun, for a metallicity of 0.03.

nucl-ex

Near threshold angular distributions of the $^2$H$(γ,Λ)$X reaction

A study of the $^2$H$(γ,Λ)$X reaction was performed using a tagged photon beam at the Research Center for Electron Photon Science (ELPH), Tohoku University. The photoproduced $Λ$ was measured in the $p{π^{-}}$ decay channel by the upgraded Neutral Kaon Spectrometer (NKS2+). The momentum integrated differential cross section was determined as a function of the scatting angle of $Λ$ in the laboratory frame for five energy bins. Our results indicated a peak in the cross section at angles smaller than cos$θ^{LAB}_Λ$ = $0.96$. The experimentally obtained angular distributions were compared to isobar models, Kaon-Maid (KM) and Saclay-Lyon A (SLA), in addition to the composite Regge-plus-resonance (RPR) model. Both SLA(r$K_{1}K_γ$ = $-1.4$) and RPR describe the data quite well in contrast to the KM model, which substantially under predicted the cross section at the most forward angles. With the anticipated finalized data on $Λ$ integrated and momentum dependent differential cross sections of $^2$H$(γ,Λ)$X~\cite{Kaneta_Beckford}, we present our findings on the angular distributions in this report.

nucl-ex

Measurements of the photon induced production of $Λ$ in the $^2$H$(γ,Λ)$X process at threshold energies

An experiment was carried out with the NKS2+ in 2010 at the Research Center for Electron Photon Science (ELPH), in which tagged photon beams in the range of 0.8 $\le$ $E_γ$ $\le$ 1.1 GeV were impinged on a liquid $^2$H target positioned at the center of the NKS2+. The produced $Λ$ was subsequently detected by the $p{π^{-}}$ decay channel. Integrated cross sections of the $^2$H$(γ,Λ)$X in the angular region of 0.9 $\le$ $\cosθ_Λ^{LAB}$ $\le$ 1.0 was derived and compared with preceding experimental results of the NKS2 collaboration. In addition, the momentum spectra for two photon energy regions were also procured. The $Λ$ angle dependent cross sections as a function of the scattering angle in the laboratory system was additionally deduced. We present the latest results on the excitation function of $Λ$ photoproduction, the momentum distributions, angular distributions, and polarization.

nucl-ex

Report on strangeness photoproduction experiments performed with the Neutral Kaon Spectrometer 2

An experiment designed to investigate the strangeness photoproduction process using a tagged photon beam in the energy range of 0.90 -1.08 GeV incident on a liquid deuterium target was successfully performed. The purpose of the experiment was to measure the production of neutral kaons and the lambda particles on a deuteron. The generation of photo produced particles was verified by the measurement of their decayed charged particles in the Neutral Kaon Spectrometer 2. The reconstructed invariant mass distributions were achieved by selecting events where two or more particles tracks were identified. Preliminary results are presented here.

nucl-ex

Photoproduction of neutral kaons on the liquid deuterium target in the threshold region

The photoproduction process of neutral kaons on a liquid deuterium target is investigated near the threshold region, Egamma = 0.8-1.1 GeV. K0 events are reconstructed from positive and negative pions, and differential cross sections are derived. Experimental momentum spectra are compared with those calculated in the spectator model using a realistic deuteron wave function. Elementary amplitudes as given by recent isobar models and a simple phenomenological model are used to study the effect of the new data on the angular behavior of the elementary cross section. The data favor a backward-peaked angular distribution of the elementary n(gamma,K0)Lambda process, which provides additional constraints on current models of kaon photoproduction. The present study demonstrates that the n(gamma,K0)Lambda reaction can provide key information on the mechanism of the photoproduction of strangeness.

nucl-ex

Effects of carbon incorporation on doping state of YBa2Cu3Oy

Effects of carbon incorporation on the doping state of YBa2Cu3Oy (Y-123) were investigated. Quantitative carbon analysis revealed that carbon could be introduced into Y-123 from both the precursor and the sintering gas. Nearly carbon-free (< 200 ppm) samples were prepared from a vacuum-treated precursor by sintered at 900 ˚C and cooling with 20 ˚C /min in flowing oxygen gas. The lower Tc (= 88 K) and higher oxygen content (y = 6.98) strongly suggested the overdoping state, which was supported by the temperature dependence of resisitivity and thermoelectric power. The nuclear quadrapole resonance spectra and the Raman scattering spectra indicated that there was almost no oxygen defect in the Cu-O chain in these samples. On the other hand, in the same cooling condition, the samples sintered in air stayed at optimal doping level with Tc = 93 K, and the intentionally carbon-doped sample was in the underdoping state. It is revealed that about 60% of incorporated carbon was substituted for Cu at the chain site in the form of CO32+, and the rest remains at the grain boundary as carbonate impurities. Such incorporation affected the oxygen absorption process in Y-123. It turned out that the oxygen content in Y-123 cannot be controlled only by the annealing temperature and the oxygen partial pressure but also by the incorporated carbon concentration.

cond-mat.supr-con

First-Principles Study on Electron Conduction in Sodium Nanowire

We present detailed first-principles calculations of the electron-conduction properties of a three-sodium-atom nanowire suspended between semi-infinite crystalline Na(001) electrodes during its elongation. Our investigations reveal that the conductance is ~1 G0 before the nanowire breaks and only one channel with the characteristic of the $3s$ orbital of the center atom in the nanowire contributes to the electron conduction. Moreover, the channel fully opens around the Fermi level, and the behavior of the channel-current density is insensitive to the structural deformation of the nanowire. These results verify that the conductance trace as a function of the electrode spacing exhibits a flat plateau at ~1 G0 during elongation.

cond-mat.mtrl-sci

Even-Odd Oscillation in Conductance of Single-Row Sodium Nanowire

We present a first-principles calculation of the electronic conduction properties of single-row sodium nanowires suspended between semi-infinite electrodes. The conductance of the nanowire is ~1 G0 (=2e^2/h) and oscillates with a two-atom period as the number of the atoms within the nanowire varies. Moreover, we observed bunches of high electron density with a two atom-lengths in the channel density distribution. The relation between the period of the conductance oscillation and the length of bunches are examined by using simplified models and is found to be largely affected by the characteristics of the infinite wire.

cond-mat.mtrl-sci

The Low-Temperature Fate of the 0.7 Structure in a Point Contact: A Kondo-like Correlated State in an Open System

Besides the usual conductance plateaus at multiples of 2e2/h, quantum point contacts typically show an extra plateau at ~ 0.7(2e2/h), believed to arise from electron-electron interactions that prohibit the two spin channels from being simultaneously occupied. We present evidence that the disappearance of the 0.7 structure at very low temperature signals the formation of a Kondo-like correlated spin state. Evidence includes a zero-bias conductance peak that splits in a parallel field, scaling of conductance to a modified Kondo form, and consistency between peak width and the Kondo temperature.

cond-mat.mes-hall