arXiv subjects

K. Ikeda

Publications and source records attributed to K. Ikeda.

16 recordsLinked to original sources

arXiv2021

Magnetic anisotropy of the van der Waals ferromagnet Cr$_2$Ge$_2$Te$_6$ studied by angular-dependent XMCD

The van der Waals ferromagnet Cr$_2$Ge$_2$Te$_6$ (CGT) has a two-dimensional crystal structure where each layer is stacked through van der Waals force. We have investigated the nature of the ferromagnetism and the weak perpendicular magnetic anisotropy (PMA) of CGT by means of X-ray absorption spectroscopy and X-ray magnetic circular dichroism (XMCD) studies of CGT single crystals. The XMCD spectra at the Cr $L_{2,3}$ edge for different magnetic field directions were analyzed on the basis of the cluster-model multiplet calculation. The Cr valence is confirmed to be 3+ and the orbital magnetic moment is found to be nearly quenched, as expected for the high-spin $t_{2g}$$^3$ configuration of the Cr$^{3+}$ ion. A large ($\sim 0.2$ eV) trigonal crystal-field splitting of the $t_{2g}$ level caused by the distortion of the CrTe$_6$ octahedron has been revealed, while the single-ion anisotropy (SIA) of the Cr atom is found to have a sign {\it opposite} to the observed PMA and too weak compared to the reported anisotropy energy. The present result suggests that anisotropic exchange coupling between the Cr atoms through the ligand Te $5p$ orbitals having strong spin-orbit coupling has to be invoked to explain the weak PMA of CGT, as in the case of the strong PMA of CrI$_3$.

cond-mat.mtrl-sci↗

arXiv2021

Hard x-ray photoemission study on strain effect in LaNiO$_3$ thin films

The strain effect from a substrate is an important experimental route to control electronic and magnetic properties in transition-metal oxide (TMO) thin films. Using hard x-ray photoemission spectroscopy, we investigate the strain dependence of the valence states in LaNiO$_{3}$ thin films, strongly correlated perovskite TMO, grown on four substrates: LaAlO$_{3}$, (LaAlO$_{3}$)$_{0.3}$(SrAl$_{0.5}$Ta$_{0.5}$O$_{3}$)$_{0.7}$, SrTiO$_{3}$, and DyScO$_{3}$. A Madelung potential analysis of core-level spectra suggests that the point-charge description is valid for the La ions while it breaks down for Ni and O ions due to a strong covalent bonding between the two. A clear x-ray photon-energy dependence of the valence spectra is analyzed by the density functional theory, which points to a presence of the La 5$p$ state near the Fermi level.

cond-mat.str-el↗

arXiv2020

Development and application of a $^3$He Neutron Spin Filter at J-PARC

We are developing a neutron polarizer with polarized $^3$He gas, referred to as a $^3$He spin filter, based on the Spin Exchange Optical Pumping (SEOP) for polarized neutron scattering experiments at Materials and Life Science Experimental Facility (MLF) of Japan Proton Accelerator Research Complex (J-PARC). A $^3$He gas-filling station was constructed at J-PARC, and several $^3$He cells with long spin relaxation times have been fabricated using the gas-filling station. A laboratory has been prepared in the MLF beam hall for polarizing $^3$He cells, and compact pumping systems with laser powers of 30~W and 110~W, which can be installed onto a neutron beamline, have been developed. A $^3$He polarization of 85% was achieved at a neutron beamline by using the pumping system with the 110~W laser. Recently, the first user experiment utilizing the $^3$He spin filter was conducted, and there have been several more since then. The development and utilization of $^3$He spin filters at MLF of J-PARC are reported.

physics.ins-det↗

arXiv2018

Anisotropic spin-density distribution and magnetic anisotropy of strained La$_{1-x}$Sr$_x$MnO$_3$ thin films: Angle-dependent x-ray magnetic circular dichroism

Magnetic anisotropies of ferromagnetic thin films are induced by epitaxial strain from the substrate via strain-induced anisotropy in the orbital magnetic moment and that in the spatial distribution of spin-polarized electrons. However, the preferential orbital occupation in ferromagnetic metallic La$_{1-x}$Sr$_x$MnO$_3$ (LSMO) thin films studied by x-ray linear dichroism (XLD) has always been found out-of-plane for both tensile and compressive epitaxial strain and hence irrespective of the magnetic anisotropy. In order to resolve this mystery, we directly probed the preferential orbital occupation of spin-polarized electrons in LSMO thin films under strain by angle-dependent x-ray magnetic circular dichroism (XMCD). Anisotropy of the spin-density distribution was found to be in-plane for the tensile strain and out-of-plane for the compressive strain, consistent with the observed magnetic anisotropy. The ubiquitous out-of-plane preferential orbital occupation seen by XLD is attributed to the occupation of both spin-up and spin-down out-of-plane orbitals in the surface magnetic dead layer.

cond-mat.mtrl-sci↗

arXiv2017

Multi-cluster dynamics in $^{13}_Λ{\rm C}$ and analogy to clustering in $^{12}{\rm C}$

We investigate structure of $^{13}_Λ{\rm C}$ and discuss the difference and similarity between the structures of $^{12}{\rm C}$ and $^{13}_Λ{\rm C}$ by answering the questions if the linear-chain and gaslike cluster states, which are proposed to appear in $^{12}{\rm C}$, survives, or new structure states appear or not. We introduce a microscopic cluster model called, Hyper-Tohsaki-Horiuchi-Schuck-Röpke (H-THSR) wave function, which is an extended version of the THSR wave function so as to describe $Λ$ hypernuclei. We obtained two bound states and two resonance (quasi-bound) states for $J^π=0^+$ in $^{13}_Λ{\rm C}$, corresponding to the four $0^+$ states in $^{12}{\rm C}$. However, the inversion of level ordering between the spectra of $^{12}{\rm C}$ and $^{13}_Λ{\rm C}$, i.e. that the $0_3^+$ and $0_4^+$ states in $^{13}_Λ{\rm C}$ correspond to the $0_4^+$ and $0_3^+$ states in $^{12}{\rm C}$, respectively, is shown to occur. The additional $Λ$ particle reduces sizes of the $0_2^+$ and $0_3^+$ states in $^{13}_Λ{\rm C}$ very much, but the shrinkage of the $0_4^+$ state is only a half of the other states. In conclusion, the Hoyle state becomes quite a compact object with ${^{9}_Λ{\rm Be}}+α$ configuration in $^{13}_Λ{\rm C}$ and is no more gaslike state composed of the $3α$ clusters. Instead, the $0_4^+$ state in $^{13}_Λ{\rm C}$, coming from the $^{12}{\rm C}(0_3^+)$ state, appears as a gaslike state composed of $α+α+^{5}_Λ{\rm He}$ configuration, i.e. the Hoyle analog state. A linear-chain state in a $Λ$ hypernucleus is for the first time predicted to exist as the $0_3^+$ state in $^{13}_Λ{\rm C}$ with more shrunk arrangement of the $3α$ clusters along $z$-axis than the $3α$ linear-chain configuration realized in the $^{12}{\rm C}(0_4^+)$ state.

nucl-th↗

arXiv2017

Magnetic anisotropy of $L1_0$-ordered FePt thin films studied by Fe and Pt $L_{2,3}$-edges x-ray magnetic circular dichroism

The strong perpendicular magnetic anisotropy of $L{\rm1_0}$-ordered FePt has been the subject of extensive studies for a long time. However, it is not known which element, Fe or Pt, mainly contributes to the magnetic anisotropy energy (MAE). We have investigated the anisotropy of the orbital magnetic moments of Fe 3$d$ and Pt 5$d$ electrons in $L{\rm1_0}$-ordered FePt thin films by Fe and Pt $L_{2,3}$-edge x-ray magnetic circular dichroism (XMCD) measurements for samples with various degrees of long-range chemical order $S$. Fe $L_{2,3}$-edge XMCD showed that the orbital magnetic moment was larger when the magnetic field was applied perpendicular to the film than parallel to it, and that the anisotropy of the orbital magnetic moment increased with $S$. Pt $L_{2,3}$-edge XMCD also showed that the orbital magnetic moment was smaller when the magnetic field was applied perpendicular to the film than parallel to it, opposite to the Fe $L_{2,3}$-edge XMCD results although the anisotropy of the orbital magnetic moment increases with $S$ like the Fe edge. These results are qualitatively consistent with the first-principles calculation by Solovyev ${\it et\ al.}$ [Phys. Rev. B $\bf{52}$, 13419 (1995).], which also predicts the dominant contributions of Pt 5$d$ to the magnetic anisotropy energy rather than Fe 3$d$ due to the strong spin-orbit coupling and the small spin splitting of the Pt 5$d$ bands in $L{\rm1_0}$-ordered FePt.

cond-mat.mtrl-sci↗

arXiv2015

High-resolution structure studies and magnetoelectric coupling of relaxor multiferroic Pb(Fe$_{0.5}$Nb$_{0.5}$)O$_3$

Pb(Fe$_{0.5}$Nb$_{0.5}$)O$_3$ (PFN), one of the few relaxor multiferroic systems, has a $G$-type antiferromagnetic transition at $T_N$ = 143 K and a ferroelectric transition at $T_C$ = 385 K. By using high-resolution neutron-diffraction experiments and a total scattering technique, we paint a comprehensive picture of the long- and short-range structures of PFN: (i) a clear sign of short-range structural correlation above $T_C$, (ii) no sign of the negative thermal expansion behavior reported in a previous study, and (iii) clearest evidence thus far of magnetoelectric coupling below $T_N$. We conclude that at the heart of the unusual relaxor multiferroic behavior lies the disorder between Fe$^{3+}$ and Nb$^{5+}$ atoms. We argue that this disorder gives rise to short-range structural correlations arising from O disorder in addition to Pb displacement.

cond-mat.mtrl-sci↗

arXiv2014

Container structure of alpha alpha Lambda clusters in $_Λ^9$Be

New concept of clustering is discussed in $Λ$ hypernuclei using a new-type microscopic cluster model wave function, which has a structure that constituent clusters are confined in a container, whose size is a variational parameter and which we refer to as Hyper-Tohsaki-Horiuchi-Schuck-Röpke (Hyper-THSR) wave function. By using the Hyper-THSR wave function, $2α+ Λ$ cluster structure in ${^{9}_Λ{\rm Be}}$ is investigated. We show that full microscopic solutions in the $2α+ Λ$ cluster system, which are given as $2α+ Λ$ Brink-GCM wave functions, are almost perfectly reproduced by the single configurations of the Hyper-THSR wave function. The squared overlaps between the both wave functions are calculated to be $99.5$%, $99.4$%, and $97.7$% for $J^π=0^+$, $2^+$, and $4^+$ states, respectively. We also simulate the structural change by adding the $Λ$ particle, by varying the $ΛN$ interaction artificially. As the increase of the $ΛN$ interaction, the $Λ$ particle gets to move more deeply inside the core and invokes strongly the spatial core shrinkage, and accordingly distinct localized $2α$ clusters appear in the nucleonic intrinsic density, though in ${^{8}{\rm Be}}$ rather gaslike $2α$-cluster structure is shown. The origin of the localization is associated with the strong effect of Pauli principle. We conclude that the container picture of the $2α$ and $Λ$ clusters is essential in understanding the cluster structure in ${^{9}_Λ{\rm Be}}$, in which the very compact spatial localization of clusters is shown in the density distribution.

nucl-th↗

arXiv2012

Possible evidence of tensor interactions in 16O observed via (p,d) reaction

We have measured 16O(p,d) reaction using 198-, 295- and 392-MeV proton beams to search for a direct evidence on the effect of the tensor interactions in light nucleus. Differential cross sections of the one-neutron transfer reactions populating the ground states and several low-lying excited states in 15O were measured. Comparing the ratios of the cross sections for each excited state to the one for the ground state over a wide range of momentum transfer, we found a marked enhancement for the positive-parity state(s). The observation indicates large components of high-momentum neutrons in the initial ground-state configurations, due possibly to the tensor interactions.

nucl-ex↗

arXiv2011

Isoscalar monopole excitations in $^{16}$O: $α$-cluster states at low energy and mean-field-type states at higher energy

Isoscalar monopole strength function in $^{16}$O up to $E_{x}\simeq40$ MeV is discussed. We found that the fine structures at the low energy region up to $E_{x} \simeq 16$ MeV in the experimental monopole strength function obtained by the $^{16}$O$(α,α^{\prime})$ reaction can be rather satisfactorily reproduced within the framework of the $4α$ cluster model, while the gross three bump structures observed at the higher energy region ($16 \lesssim E_{x} \lesssim 40$ MeV) look likely to be approximately reconciled by the mean-field calculations such as RPA and QRPA. In this paper, it is emphasized that two different types of monopole excitations exist in $^{16}$O; one is the monopole excitation to cluster states which is dominant in the lower energy part ($E_{x} \lesssim 16$ MeV), and the other is the monopole excitation of the mean-field type such as one-particle one-hole ($1p1h$) which {is attributed} mainly to the higher energy part ($16 \lesssim E_{x} \lesssim 40$ MeV). It is found that this character of the monopole excitations originates from the fact that the ground state of $^{16}$O with the dominant doubly closed shell structure has a duality of the mean-field-type {as well as} $α$-clustering {character}. This dual nature of the ground state seems to be a common feature in light nuclei.

nucl-th↗

arXiv2004

Application of the generalized two-center cluster model to 10Be

A generalized two-center cluster model (GTCM), including various partitions of the valence nucleons around two alpha-cores, is proposed for studies on the exotic cluster structures of Be isotopes. This model is applied to the 10Be = alpha + alpha + n + n system and the adiabatic energy surfaces for alpha-alpha distances are calculated. It is found that this model naturally describes the formation of the molecular orbitals as well as that of asymptotic cluster states dependeing on their relative distance. In the negative-parity state, a new type of the alpha + 6He cluster structure is also predicted.

nucl-th↗

arXiv2003

Chiral Sigma Model with Pion Mean Field in Finite Nuclei

The properties of infinite matter and finite nuclei are studied by using the chiral sigma model in the framework of the relativistic mean field theory. We reconstruct an extended chiral sigma model in which the omega meson mass is generated dynamically by the sigma condensation in the vacuum in the same way as the nucleon mass. All the parameters of chiral sigma model are essentially fixed from the hadron properties in the free space. In nuclear matter, the saturation property comes out right, but the incompressibility is too large and the scalar and vector potentials are about a half of the phenomenological ones, respectively. This fact is reflected to the properties of finite nuclei. We calculate N = Z even-even mass nuclei between N = 16 and N = 34. The extended chiral sigma model without the pion mean field leads to the result that the magic number appears at N = 18 instead of N = 20 and the magic number does not appear at N = 28 due to the above mentioned nuclear matter properties. The latter problem, however, could be removed by the introduction of the finite pion mean field with the appearance of the magic number at N = 28. We find that the energy differences between the spin-orbit partners are reproduced by the finite pion mean field which is completely a different mechanism from the standard spin-orbit interaction.

nucl-th↗

arXiv2003

Three-body Coulomb breakup of 11Li in the complex scaling method

Coulomb breakup strengths of 11Li into a three-body 9Li+n+n system are studied in the complex scaling method. We decompose the transition strengths into the contributions from three-body resonances, two-body ``10Li+n'' and three-body ``9Li+n+n'' continuum states. In the calculated results, we cannot find the dipole resonances with a sharp decay width in 11Li. There is a low energy enhancement in the breakup strength, which is produced by both the two- and three-body continuum states. The enhancement given by the three-body continuum states is found to have a strong connection to the halo structure of 11Li. The calculated breakup strength distribution is compared with the experimental data from MSU, RIKEN and GSI.

nucl-th↗

arXiv2001

Triaxial deformation in 10Be

The triaxial deformation in $^{10}$Be is investigated using a microscopic $α+α+n+n$ model. The states of two valence neutrons are classified based on the molecular-orbit (MO) model, and the $π$-orbit is introduced about the axis connecting the two $α$-clusters for the description of the rotational bands. There appear two rotational bands comprised mainly of $K^π= 0^+$ and $K^π= 2^+$, respectively, at low excitation energy, where the two valence neutrons occupy $K^π= 3/2^-$ or $K^π= 1/2^-$ orbits. The triaxiality and the $K$-mixing are discussed in connection to the molecular structure, particularly, to the spin-orbit splitting. The extent of the triaxial deformation is evaluated in terms of the electro-magnetic transition matrix elements (Davydov-Filippov model, Q-invariant model), and density distribution in the intrinsic frame. The obtained values turned out to be $γ= 15^o \sim 20^o$.

nucl-th↗

arXiv2000

Important role of the spin-orbit interaction in forming the 1/2^+ orbital structure in Be isotopes

The structure of the second 0^+ state of ^{10}Be is investigated using a microscopic $α+α+n+n$ model based on the molecular-orbit (MO) model. The second 0^+ state, which has dominantly the (1/2^+)^2 configuration, is shown to have a particularly enlarged $α-α$ structure. The kinetic energy of the two valence neutrons occupying along the $α-α$ axis is reduced remarkably due to the strong $α$ clustering and, simultaneously, the spin-orbit interaction unexpectedly plays important role to make the energy of this state much lower. The mixing of states with different spin structure is shown to be important in negative-parity states. The experimentally observed small-level spacing between 1^- and 2^- (~ 300 keV) is found to be an evidence of this spin-mixing effect. ^{12}{Be} is also investigated using $α+α+4n$ model, in which four valence neutrons are considered to occupy the (3/2^-)^2(1/2^+)^2 configuration. The energy surface of ^{12}Be is shown to exhibit similar characteristics, that the remarkable $α$ clustering and the contribution of the spin-orbit interaction make the binding of the state with (3/2^-)^2(1/2^+)^2 configuration properly stronger in comparison with the closed p-shell (3/2^-)^2(1/2^-)^2 configuration.

nucl-th↗

arXiv1998

Numerical Computation of Thermoelectric and Thermomagnetic Effects

Phenomenological equations describing the Seebeck, Hall, Nernst, Peltier, Ettingshausen, and Righi-Leduc effects are numerically solved for the temperature, electric current, and electrochemical potential distributions of semiconductors under magnetic field. The results are compared to experiments.

cond-mat.mtrl-sci↗