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K. Imagawa

Publications and source records attributed to K. Imagawa.

12 recordsLinked to original sources
arXiv2025

Background stability and annual modulation test using PICOLON ultra-pure NaI(Tl) detector

The dark matter observation claimed by the DAMA/LIBRA experiment has been a long-standing puzzle within the particle physics community. NaI(Tl) crystals with radiopurity comparable to DAMA/LIBRA's are essential for adequate verification. Existing experiments using NaI(Tl) target have been hampered by the high radioactivity concentration of NaI(Tl) crystals. PICOLON experiment conducts an independent search for Weakly Interacting Massive Particles using highest purity NaI(Tl) crystals. In 2020, the NaI(Tl) crystal (Ingot#85) reached the same purity level as DAMA/LIBRA crystals. The DAMA/LIBRA group has stressed that verifying their signal requires high-purity NaI(Tl) crystals with long-term stability. Based on a six-month measurement, we have confirmed the long-term stability of its radiopurity. This stability provides a significant advantage for future efforts to adequately verify the DAMA/LIBRA result using NaI(Tl) crystal. In this paper, we present the background stability of purity in the Ingot#94 NaI(Tl) detector, which was produced using the Ingot#85 purification method, along with the first annual modulation search conducted by the PICOLON experiment.

physics.ins-det↗
arXiv2024

Radiopurity of NaI(Tl) crystals for PICOLON dark matter experiment

The dark matter observation claim by the DAMA/LIBRA collaboration has been a long-standing puzzle within the particle physics community. Efforts of other research groups to verify the claim have been insufficient by significant radioactivity of present NaI(Tl) crystals. PICOLON (Pure Inorganic Crystal Observatory for LOw-energy Neut(ra)lino) experiment conducts independent search for Weakly Interacting Massive Particles (WIMPs) using NaI(Tl) crystals. Our NaI(Tl) crystal manufactured in 2020 (Ingot #85) reached the same purity level as DAMA/LIBRA crystals. In this report, we describe the radiopurity of the new Ingot #94 crystal produced using the same purification technique as Ingot #85. The $α$-ray events were selected by pulse-shape discrimination method. The impurities in the Ingot #94, $^{232}$Th, $^{226}$Ra and $^{210}$Po radioactivity were $4.6\pm 1.2~\mathrm{μBq/kg}$, $7.9\pm 4.4~\mathrm{μBq/kg}$, and $19\pm 6~\mathrm{μBq/kg}$, which are equivalent to those of the DAMA/LIBRA crystals. The background rate in the energy region of 2-6 keV , was 2-5 events/d/kg/keV without applying a veto trigger.

physics.ins-det↗
arXiv2024

Present status of PICOLON project

The existence of cosmic dark matter and neutrino properties are long-standing problems in cosmology and particle physics. These problems have been investigated by using radiation detectors. We will discuss the application of inorganic crystal scintillators to studies on dark matter and neutrino properties. A large volume and high-purity inorganic crystal is a promising detector for investigating dark matter and neutrino.

astro-ph.IM↗
arXiv2021

PICOLON dark matter search project

PICOLON (Pure Inorganic Crystal Observatory for LOw-energy Neutr(al)ino) aims to search for cosmic dark matter by high purity NaI(Tl) scintillator. We developed extremely pure NaI(Tl) crystal by hybrid purification method. The recent result of $^{210}$Pb in our NaI(Tl) is less than 5.7 $μ$Bq/kg. We will report the test experiment in the low-background measurement at Kamioka Underground Laboratory. The sensitivity for annual modulating signals and finding dark matter particles will be discussed.

astro-ph.IM↗
arXiv2021

Dark matter search with high purity NaI(Tl) scintillator

A dark matter search project needs and extremely low background radiation detector since the expected event rate of dark matter is less than a few events in one year in one tonne of the detector mass. The authors developed a highly radiopure NaI(Tl) crystal to search for dark matter. The best combination of the purification methods was developed, resulting $^{\mathrm{nat}}$K and $^{210}$Pb were less than 20 ppb and 5.7 $μ$Bq/kg, respectively. The authors will construct a large volume detector system with high-purity NaI(Tl) crystals. The design and the performance of the prototype detector module will be reported in this article.

physics.ins-det↗
arXiv2021

Development of highly radiopure NaI(Tl) scintillator for PICOLON dark matter search project

The highly radiopure NaI(Tl) was developed to search for particle candidates of dark matter. The optimized methods were combined to reduce various radioactive impurities. The $^{40}$K was effectively reduced by the re-crystallization method. The progenies of the decay chains of uranium and thorium were reduced by appropriate resins. The concentration of natural potassium in NaI(Tl) crystal was reduced down to 20 ppb. Concentrations of alpha-ray emitters were successfully reduced by appropriate selection of resin. The present concentration of thorium series and 226Ra were $1.2 \pm1.4$ $μ$Bq/kg and $13\pm4$ $μ$Bq/kg, respectively. No significant excess in the concentration of $^{210}$Pb was obtained, and the upper limit was 5.7 $μ$Bq/kg at 90% C. L. The achieved level of radiopurity of NaI(Tl) crystals makes construction of a dark matter detector possible.

physics.ins-det↗
arXiv2017

Search for cosmic dark matter by means of ultra high purity NaI(Tl) scintillator

The dark matter search project by means of ultra high purity NaI(Tl) scintillator is now underdevelopment. An array of large volume NaI(Tl) detectors whose volume is 12.7 cm$ϕ\times$12.7 cm is applied to search for dark matter signal. To remove radioactive impurities in NaI(Tl) crystal is one of the most important task to find small number of dark matter signals. We have developed high purity NaI(Tl) crystal which contains small amounts of radioactive impurities, $<4$ ppb of $^{nat}$K, 0.3 ppt of Th chain, 58 $μ$Bq/kg of $^{226}$Ra and 30 $μ$Bq/kg of $^{210}$Pb. Future prospects to search for dark matter by means of a large volume and high purity NaI(Tl) scintillator is discussed.

physics.ins-det↗
arXiv2015

Dark matter search project PICO-LON

The PICO-LON project aims at search for cold dark matter by means of highly radio-pure and large volume NaI(Tl) scintillator. The NaI powder was purifed by chemical processing to remove lead isotopes and selecting a high purity graphite crucible. The concentrations of radioactive impurities of $^{226}$Ra and $^{228}$Th were effectively reduced to 58$\pm$4 $μ$Bq/kg and 1.5$\pm$1.9 $μ$Bq/kg, respectively. It should be remarked that the concentration of $^{210}$Pb, which is crucial for the sensitivity to dark matter, was reduced to 24$\pm$2 $μ$Bq/kg. The total background rate at 10 keVee was as low as 8 keV$^{-1}$kg$^{-1}$day$^{-1}$, which was sufficiently low to search for dark matter. Further purification of NaI(Tl) ingot and future prospect of PICO-LON project is discussed.

astro-ph.IM↗
arXiv2014

KamLAND-PICO project to search for cosmic dark matter

KamLAND-PICO project aims to search for WIMPs dark matter by means of NaI(Tl) scintillator. To investigate the WIMPs candidate whose cross section is as small as $10^{-9}$ pb, a pure NaI(Tl) crystal was developed by chemical processing and taking care of surroundings. The concentration of U and Th chain was reduced to $5.4\pm0.9$ ppt and $3.3\pm2.2$ ppt, respectively. It should be remarked that the concentration of $^{210}$Pb which was difficult to reduce reached to the high purity as $58\pm26$ $μ$Bq/kg.

astro-ph.IM↗
arXiv2006

The performance of thin NaI(Tl) scintillator plate for dark matter search

A thin (0.05cm) and wide area (5cmX5cm) NaI(Tl) scintillator was developed. The performance of the thin NaI(Tl) plate, energy resolution, single photoelectron energy and position sensitivity were tested. An excellent energy resolution of 20% (FWHM) at 60keV was obtained. The single photoelectron energy was calculated to be approximately 0.42 0.02keV. Position information in the 5cmx5cm area of the detector was also obtained by analyzing the ratio of the number of photons collected at opposite ends of the detector. The position resolution was obtained to be 1cm (FWHM) in the 5cmx5cm area.

nucl-ex↗