arXiv subjects

K. Imamura

Publications and source records attributed to K. Imamura.

13 recordsLinked to original sources

arXiv2026

High-field fate of the Kitaev quantum spin liquid in $\alpha$-RuCl$_3$

Kitaev quantum spin liquids (KQSLs) host fractionalized excitations described by itinerant Majorana quasiparticles and gapped $Z_2$ fluxes (visons), providing a platform for emergent topological matter. Whether such a state survives under strong magnetic fields, however, remains an open question. The layered honeycomb magnet $\alpha$-RuCl$_3$ is a leading candidate material: an in-plane field of $\sim$ 7 T suppresses antiferromagnetic order and induces a quantum-disordered phase exhibiting signatures consistent with Majorana excitations, including an anomalous thermal Hall effect and field-angle-dependent specific heat. At higher fields, the magnetization approaches saturation, suggesting a transition to a spin-polarized state, yet the microscopic evolution between these limits remains unresolved. Here we report high-field specific heat measurements up to 24 T that reveal a distinct crossover at $\mu_0H^*\approx$15 T, beyond which the perturbative Kitaev description breaks down. Above $H^*$, the characteristic six-fold angular modulation of the specific heat collapses and the excitation gap deviates from the predicted $H^3$ scaling. Meanwhile, the gap decreases with increasing field and the in-plane magnetization anisotropy persists up to $\sim$ 24 T, both in sharp contrast to a trivial spin-polarized state, indicating that KQSL signatures are preserved even at $\sim$ 90 % of magnetization saturation. These results reveal that the KQSL in $\alpha$-RuCl$_3$ extends well beyond the perturbative window, persisting as a nonperturbative regime in which the Majorana and vison energy scales merge, before eventually giving way to spin polarization. This thermodynamic roadmap provides a basis for understanding how fractionalized phases evolve under strong magnetic fields.

cond-mat.str-el↗

arXiv2026

Pseudo Point Nodal Superconducting Gap in Spin-Triplet UTe$_2$

The unconventional superconductor UTe$_2$ represents a rare example of spin-triplet pairing with potentially topologically protected quantum states. However, conflicting reports on its gap structure, particularly regarding point nodes, have hindered understanding of the order parameter symmetry and topological properties. Here we report high-resolution thermal conductivity measurements on high-quality UTe$_2$ single crystals down to ~50 mK that resolve the gap anisotropy through bulk directional transport. The $b$-axis thermal conductivity $\kappa_b/T$ exhibits negligible residual conductivity as $T \to 0$, and its temperature dependence is consistent with a small superconducting energy gap along the $b$-axis. Under magnetic fields, the residual $\kappa_b/T$ shows only weak field-induced enhancement. Remarkably, a threshold field emerges at low fields for $H \parallel a$, characterized by a kink that signals a change in quasiparticle transport normal to the field. Below the threshold, $\kappa_b/T$ remains isotropic for all field orientations, whereas strong anisotropy between transport along and normal to the field develops above it. These signatures strongly suggest that UTe$_2$ exhibits a fully gapped state with a pseudo point-nodal structure, where gap minima approach but never reach zero. We estimate the minimal gap $\Delta_{min}/\Delta_0 \sim 0.1$ along the $b$-axis, where $\Delta_0$ is the characteristic superconducting gap. This unusual gap structure provides crucial insights into the pairing mechanism and topology of this spin-triplet superconductor and excludes non-unitary mixing of pairing symmetries.

cond-mat.supr-con↗

arXiv2025

Impact of charge-density-wave pattern on the superconducting gap in V-based kagome superconductors

Kagome metals $A$V$_3$Sb$_5$ ($A=$ K, Rb, Cs) provide a compelling platform to explore the interplay between superconductivity (SC) and charge-density-wave (CDW) orders. While distinct CDW orders have been identified in K/RbV$_3$Sb$_5$ versus CsV$_3$Sb$_5$, their influence on the SC order parameter remains unresolved. Here, we investigate low-energy quasiparticle excitations in $A$V$_3$Sb$_5$, uncovering a striking difference in SC gap anisotropy: K/RbV$_3$Sb$_5$ exhibit fully gapped, nearly isotropic $s$-wave states, in contrast to the strongly anisotropic SC gap in CsV$_3$Sb$_5$. Contrary to previous vortex-state studies suggesting nodal SC in K/RbV$_3$Sb$_5$, our Meissner-state measurements in high-quality crystals demonstrate fully gapped states with reduced anisotropy compared to CsV$_3$Sb$_5$. Impurity scattering introduced via electron irradiation in K/RbV$_3$Sb$_5$ has a minimal impact on low-energy excitations, and it induces an increase in the SC transition temperature $T_{\rm c}$, consistent with more isotropic $s$-wave SC competing with CDW order. Our theoretical analysis attributes the observed SC gap anisotropy differences to distinct CDW modulation patterns: the star-of-David structure unique to CsV$_3$Sb$_5$ preserves van Hove singularities near the Fermi level, promoting anisotropic $s$-wave SC with enhanced $T_{\rm c}$ via bond-order fluctuations. These findings establish a systematic framework for understanding the interplay between SC and CDW orders in $A$V$_3$Sb$_5$, driven by electron correlations.

cond-mat.supr-con↗

arXiv2025

Topology meets time-reversal symmetry breaking in FeSe$_{1-x}$Te$_{x}$ superconductor

Time-reversal symmetry breaking (TRSB) in magnetic topological insulators induces a Dirac gap in the topological surface state (TSS), leading to exotic phenomena such as the quantum anomalous Hall effect. Yet, the interplay between TRSB and topology in superconductors remains underexplored due to limited suitable materials. Here we employ zero-field muon spin relaxation ($\mu$SR) as a sensitive probe of TRSB to map out the electronic phase diagrams of iron-chalcogenide superconductors FeSe$_{1-x}$Te$_{x}$. For the Te composition $x=0.64$ with the highest superconducting transition temperature $T_{\rm c}=14.5$ K, which is known to host a TSS and Majorana zero modes within vortices, we detect spontaneous magnetic fields below $T_{\rm c}$ distinct from a magnetic order. This signifies a TRSB superconducting state in the bulk, revealing the convergence of unconventional TRSB superconductivity with topologically nontrivial electronic structures in FeSe$_{1-x}$Te$_{x}$. Given the relatively high $T_{\rm c}$ and the tunability of the Fermi level through chemical substitution, iron-chalcogenide superconductors offer an intriguing platform for investigating the synergy between topological superconductivity and TRSB.

cond-mat.supr-con↗

arXiv2024

Magnetothermal transport in ultraclean single crystals of Kitaev magnet $\alpha$-RuCl$_3$

The layered honeycomb magnet $\alpha$-RuCl$_3$ has emerged as a promising candidate for realizing a Kitaev quantum spin liquid. Previous studies have reported oscillation-like anomalies in the longitudinal thermal conductivity and half-integer quantized thermal Hall conductivity above the antiferromagnetic critical field $H_c$, generating significant interest. However, the origins of these phenomena remain contentious due to strong sample dependence. Here we re-examine the magnetothermal transport properties using recently available ultra-pure $\alpha$-RuCl$_3$ single crystals to further elucidate potential signatures of the spin liquid state. Our findings reveal that while anomalies in thermal conductivity above $H_c$ persist even in ultraclean crystals, their magnitude is significantly attenuated, contrary to the quantum oscillations hypothesis. This suggests that the anomalies are likely attributable to localized stacking faults inadvertently introduced during magnetothermal transport measurements. The thermal Hall conductivity exhibits a half-quantized plateau, albeit with a narrower width than previously reported. This width reduction can be understood through two distinct mechanisms: sample-dependent magnetic critical fields that influence the lower boundary of the plateau region, and the decoupling between chiral Majorana edge currents and phononic thermal transport that determines the upper boundary. These results indicate that structural imperfections exert a substantial influence on both the oscillation-like anomalies and quantization effects observed in magnetothermal transport measurements of $\alpha$-RuCl$_3$.

cond-mat.str-el↗

arXiv2024

Lifting of gap nodes by disorder in ultranodal superconductor candidate FeSe1-xSx

The observation of time-reversal symmetry breaking and large residual density of states in tetragonal FeSe$_{1-x}$S$_x$ suggests a novel type of ultranodal superconducting state with Bogoliubov Fermi surfaces (BFSs). Although such BFSs in centrosymmetric superconductors are expected to be topologically protected, the impurity effect of this exotic superconducting state remains elusive experimentally. Here, we investigate the impact of controlled defects introduced by electron irradiation on the superconducting state of tetragonal FeSe$_{1-x}$S$_x$ ($0.18\le x\le 0.25$). The temperature dependence of magnetic penetration depth is initially consistent with a model with BFSs in the pristine sample. After irradiation, we observe a nonmonotonic evolution of low-energy excitations with impurity concentrations. This nonmonotonic change indicates a transition from nodal to nodeless, culminating in gapless with Andreev bound states, reminiscent of the nodal $s_\pm$ case. This points to the accidental nature of the possible BFSs in tetragonal FeSe$_{1-x}$S$_x$, which are susceptible to disruption by the disorder.

cond-mat.supr-con↗

arXiv2024

Demonstration of nuclear gamma-ray polarimetry based on a multi-layer CdTe Compton Camera

To detect and track structural changes in atomic nuclei, the systematic study of nuclear levels with firm spin-parity assignments is important. While linear polarization measurements have been applied to determine the electromagnetic character of gamma-ray transitions, the applicable range is strongly limited due to the low efficiency of the detection system. The multi-layer Cadmium-Telluride (CdTe) Compton camera can be a state-of-the-art gamma-ray polarimeter for nuclear spectroscopy with the high position sensitivity and the detection efficiency. We demonstrated the capability to operate this detector as a reliable gamma-ray polarimeter by using polarized 847-keV gamma rays produced by the $^{56}\rm{Fe}({\it p},{\it p'}\gamma)$ reaction. By combining the experimental data and simulated calculations, the modulation curve for the gamma ray was successfully obtained. A remarkably high polarization sensitivity was achieved, compatible with a reasonable detection efficiency. Based on the obtained results, a possible future gamma-ray polarimetery is discussed.

astro-ph.IM↗

arXiv2024

Two-step growth of high-quality single crystals of the Kitaev magnet $\alpha$-RuCl$_{3}$

The layered honeycomb magnet $\alpha$-RuCl$_3$ is the most promising candidate for a Kitaev quantum spin liquid (KQSL) that can host charge-neutral Majorana fermions. Recent studies have shown significant sample dependence of thermal transport properties, which are a key probe of Majorana quasiparticles in the KQSL state, highlighting the importance of preparing high-quality single crystals of $\alpha$-RuCl$_3$. Here, we present a relatively simple and reliable method to grow high-quality single crystals of $\alpha$-RuCl$_3$. We use a two-step crystal growth method consisting of a purification process by chemical vapor transport (CVT) and a main crystal growth process by sublimation. The obtained crystals exhibit a distinct first-order structural phase transition from the monoclinic ($C2/m$) to the rhombohedral ($R\bar{3}$) structure at $\sim150$ K, which is confirmed by the nuclear quadrupole resonance spectra with much sharper widths than previously reported. The Raman spectra show the absence of defect-induced modes, supporting the good crystallinity of our samples. The jumps in the thermal expansion coefficient and specific heat at the antiferromagnetic (AFM) transition at 7.6-7.7 K are larger and sharper than those of previous samples grown by the CVT and Bridgman methods and do not show any additional AFM transitions at 10-14 K due to stacking faults. The longitudinal thermal conductivity in the AFM phase is significantly larger than previously reported, indicating a very long mean free path of heat carriers. All the results indicate that our single crystals are of superior quality with good crystallinity and few stacking faults, which provides a suitable platform for studying the Kitaev physics.

cond-mat.str-el↗

arXiv2023

Defect-Induced Low-Energy Majorana Excitations in the Kitaev Magnet $\alpha$-RuCl$_3$

The excitations in the Kitaev spin liquid (KSL) can be described by Majorana fermions, which have characteristic field dependence of bulk gap and topological edge modes. In the high-field state of layered honeycomb magnet $\alpha$-RuCl$_3$, experimental results supporting these Majorana features have been reported recently. However, there are challenges due to sample dependence and the impact of inevitable disorder on the KSL is poorly understood. Here we study how low-energy excitations are modified by introducing point defects in $\alpha$-RuCl$_3$ using electron irradiation, which induces site vacancies and exchange randomness. High-resolution measurements of the temperature dependence of specific heat $C(T)$ under in-plane fields $H$ reveal that while the field-dependent Majorana gap is almost intact, additional low-energy states with $C/T=A(H)T$ are induced by introduced defects. At low temperatures, we obtain the data collapse of $C/T\sim H^{-\gamma}(T/H)$ expected for a disordered quantum spin system, but with an anomalously large exponent $\gamma$. This leads us to find a power-law relationship between the coefficient $A(H)$ and the field-sensitive Majorana gap. These results are consistent with the picture that the disorder induces low-energy linear Majorana excitations, which may be considered as a weak localization effect of Majorana fermions in the KSL.

cond-mat.str-el↗

arXiv2023

Majorana-fermion origin of the planar thermal Hall effect in the Kitaev magnet $\alpha$-RuCl$_3$

The field-induced quantum disordered state of layered honeycomb magnet $\alpha$-RuCl$_3$ is a prime candidate for Kitaev spin liquids hosting Majorana fermions and non-Abelian anyons. Recent observations of anomalous planar thermal Hall effect demonstrate a topological edge mode, but whether it originates from Majorana fermions or bosonic magnons remains controversial. Here we distinguish these origins from low-temperature measurements of high-resolution specific heat and thermal Hall conductivity with rotating in-plane fields. In the honeycomb bond direction, a distinct closure of the low-energy bulk gap is observed concomitantly with the sign reversal of the Hall effect. General discussions of topological bands show that this is the hallmark of an angle-rotation-induced topological transition of fermions, providing conclusive evidence for the Majorana-fermion origin of the thermal Hall effect in $\alpha$-RuCl$_3$.

cond-mat.str-el↗

arXiv2023

Anisotropic Enhancement of Lower Critical Field in Ultraclean Crystals of Spin-Triplet Superconductor UTe2

The paramagnetic spin-triplet superconductor UTe$_2$ has attracted significant attention because of its exotic superconducting properties including an extremely high upper critical field and possible chiral superconducting states. Recently, ultraclean single crystals of UTe$_2$ have become available, and thus measurements on these crystals are crucial to elucidate the intrinsic superconducting properties. Here, we report the thermodynamic critical field $H_{\rm c}$, the lower critical field $H_{\rm c1}$, and the upper critical field $H_{\rm c2}$ at low fields of these high-quality single crystals. From the comparison of the anisotropies in $H_{\rm c1}$ and $H_{\rm c2}$, we find that the experimental $H_{\rm c1}$ values with the magnetic field along $b$- and $c$-axes are anomalously enhanced, showing unusual low-temperature upturns. We propose an effect of the strong Ising-like ferromagnetic fluctuations on the vortex line energy as the origin of the anisotropic enhancement of $H_{\rm c1}$.

cond-mat.supr-con↗

arXiv2019

Interplay between nuclear shell evolution and shape deformation revealed by magnetic moment of 75Cu

Exotic nuclei are characterized by a number of neutrons (or protons) in excess relative to stable nuclei. Their shell structure, which represents single-particle motion in a nucleus, may vary due to nuclear force and excess neutrons, in a phenomenon called shell evolution. This effect could be counterbalanced by collective modes causing deformations of the nuclear surface. Here, we study the interplay between shell evolution and shape deformation by focusing on the magnetic moment of an isomeric state of the neutron-rich nucleus 75Cu. We measure the magnetic moment using highly spin-controlled rare-isotope beams and achieving large spin alignment via a two-step reaction scheme that incorporates an angular-momentum-selecting nucleon removal. By combining our experiments with numerical simulations of many-fermion correlations, we find that the low-lying states in 75Cu are, to a large extent, of single-particle nature on top of a correlated 74Ni core. We elucidate the crucial role of shell evolution even in the presence of the collective mode, and within the same framework, we consider whether and how the double magicity of the 78Ni nucleus is restored, which is also of keen interest from the perspective of nucleosynthesis in explosive stellar processes.

nucl-ex↗

arXiv1996

Transition between Atomic and Molecular Hydrogen in the Galaxy: Vertical Variation of the Molecular Fraction

We derive radial and vertical distributions of HI and H2 gas densities in our Galaxy by using the terminal velocity method. We calculate the molecular fraction (f_mol) defined as the ratio of the molecular hydrogen to total hydrogen gas density at galactic longitude l= 33 to 64 deg and galactic latitude b=-2 to +2 deg. The thickness of the molecular dominant region f_mol > 0.8 is approximately constant (109 +/- 12 pc) at galactocentric distance R = 4.7 to 7.2 kpc. The molecular fraction decreases suddenly at a critical height from the galactic plane, below which the gas disk is almost totally molecular, while it is almost atomic beyond this height. We show that the vertical f_mol variation can be reproduced by a model which takes into account the phase transition between HI and H2 gases in the interstellar matter. Key words: Atomic Hydrogen --- the Galaxy --- Interstellar Matter --- Molecular Hydrogen

astro-ph↗