arXiv subjects

K. Jin

Publications and source records attributed to K. Jin.

34 records · Page 2Linked to original sources

arXiv2017

Reemergence of high-Tc superconductivity in the (Li1-xFex)OHFe1-ySe under high pressure

The pressure-induced reemergence of the second high-Tc superconducting phase (SC-II) in the alkali-metal intercalated AxFe2-ySe2 (A = K, Rb, Cs, Tl) remains an enigma and proper characterizations on the superconducting- and normal-state properties of the SC-II phase were hampered by the intrinsic inhomogeneity and phase separation. To elucidate this intriguing problem, we performed a detailed high-pressure magnetotransport study on the recently discovered (Li1-xFex)OHFe1-ySe single crystals, which have high Tc~40 K and share similar Fermi surface topology as AxFe2-ySe2, but are free from the sample complications. We found that the ambient-pressure Tc~41 K is suppressed gradually to below 2 K upon increasing pressure to Pc ~5 GPa, above which a SC-II phase with higher Tc emerges and the Tc increases progressively to above 50 K up to 12.5 GPa. Interestingly, our high-precision resistivity data enable us to uncover the sharp transition of the normal state from a Fermi liquid for SC-I phase (0 < P < 5 GPa) to a non-Fermi-liquid for SC-II phase (P > 5GPa). In addition, the reemergence of high-Tc SC-II phase is found to accompany with a concurrent enhancement of electron carrier density. Since high-pressure structural study based on the synchrotron X-ray diffraction rules out the structural transition below 10 GPa, the observed SC-II phase with enhanced carrier density should be ascribed to an electronic origin associated with a pressure-induced Fermi surface reconstruction.

cond-mat.supr-con↗

arXiv2017

Raman study of electron-phonon coupling in thin films of LiTi$_2$O$_4$ spinel oxide superconductor

We performed a Raman scattering study of thin films of LiTi$_2$O$_4$ spinel oxide superconductor. We detected four out of five Raman active modes, with frequencies in good accordance with our first-principles calculations. Three T$_{2g}$ modes show a Fano lineshape from 5 K to 295 K, which suggests an electron-phonon coupling in LiTi$_2$O$_4$. Interestingly, the electron-phonon coupling shows an anomaly across the negative to positive magnetoresistance transition at 50 K, which may be due to the unset of other competing orders. The strength of the electron-phonon interaction estimated from the Allen's formula and the observed lineshape parameters suggests that the three T$_{2g}$ modes contribute little to superconductivity.

cond-mat.supr-con↗

arXiv2017

Bosonic excitations and electron pairing in an electron-doped cuprate superconductor

Superconductivity originates from the coupling between charge carriers and bosonic excitations of either phononic or electronic origin. Identifying the most relevant pairing glue is a key step towards a clear understanding of the unconventional superconductivity. Here, by applying the ultrafast optical spectroscopy on the electron-doped cuprates La$_{1.9}$Ce$_{0.1}$CuO$_{4\pmδ}$, we discern a bosonic mode of electronic origin that has the strongest coupling with the charge carriers near $T_c$. We argue that this mode is associated with the two-dimensional antiferromagnetic spin fluctuations, and can fully account for the superconducting pairing. Our work may help to establish a quantitative relation between bosonic excitations and superconducting pairing in electron-doped cuprates, and pave the way for systematic exploration of superconductivity and other collective phenomena in all correlated materials.

cond-mat.str-el↗

arXiv2016

Studies of relative gain and timing response of fine-mesh photomultiplier tubes in high magnetic fields

We investigated the use of Hamamatsu fine-mesh photomultiplier tube assemblies H6152-70 and H6614-70 with regards to their gain and timing resolution in magnetic fields up to 1.9 T. Our results show that the H6614-70 assembly can operate reliably in magnetic fields exceeding 1.5 T, while preserving a reasonable timing resolution even with a gain reduction of a factor of approximately 100. The reduction of the relative gain of the H6152-70 is similar to the H6614-70's near 1.5 T, but its timing resolution worsens considerably at this high field.

physics.ins-det↗

arXiv2015

Magnetism and a field-cycling induced effect in staircase Kagomé antiferromagnet PbCu$_3$TeO$_7$ revealed by NMR

We report $^{125}$Te and $^{63,65}$Cu nuclear magnetic resonance (NMR) studies on single crystals of staircase Kagomé antiferromagnet PbCu3TeO7 ($T_{N1}\approx$ 36 K). A Curie constant as large as $Θ$~140 K is obtained by a Curie-Weiss fitting of the high-temperature Knight shift. The frustration factor f (= $Θ/T_N $)$\approx$ 4 implies intermediate frustration in this system. From the high-temperature Knight shift data of $^{125}$Te, its hyperfine coupling constant is estimated to be $^{125}A_{hf}$ = -67 kOe/$μ_B$, which suggests a strong interlayer coupling bridging the neighboring Kagomé layers. At $T$= 2 K, we find two types of zero-field NMR signals. One has no dependence on the history of the field treatment, which is consistent with Cu NMR signals from inequivalent Cu sites with different internal hyperfine fields. The other one is only seen after a field-cycling process, which is consistent with domain wall contributions in this frustrated antiferromagnet.

cond-mat.str-el↗

arXiv2014

The Phase Diagram in Electron-Doped LCCO

Superconductors are a striking example of a quantum phenomenon in which electrons move coherently over macroscopic distances without scattering. The high-temperature superconducting oxides(cuprates) are the most studied class of superconductors, composed of two-dimensional CuO2 planes separated by other layers which control the electron concentration in the planes. A key unresolved issue in cuprates is the relationship between superconductivity and magnetism. In this paper, we report a sharp phase boundary of static three-dimensional magnetic order in the electron-doped superconductor La2-xCexCuO4-d where small changes in doping or depth from the surface switch the material from superconducting to magnetic. Using low-energy spin polarized muons, we find static magnetism disappears close to where superconductivity begins and well below the doping where dramatic changes in the transport properties are reported. These results indicate a higher degree of symmetry between the electron and hole-doped cuprates than previously thought.

cond-mat.supr-con↗

arXiv2011

Quantum critical scaling at the edge of Fermi liquid stability in a cuprate superconductor

In the high temperature cuprate superconductors, the pervasiveness of anomalous electronic transport properties suggests that violation of conventional Fermi liquid behavior is closely tied to superconductivity. In other classes of unconventional superconductors, atypical transport is well correlated with proximity to a quantum critical point, but the relative importance of quantum criticality in the cuprates remains uncertain. Here we identify quantum critical scaling in the electron-doped cuprate material La2-xCexCuO4 with a line of quantum critical points that surrounds the superconducting phase as a function of magnetic field and charge doping. This zero-temperature phase boundary, which delineates a metallic Fermi liquid regime from an extended non-Fermi liquid ground state, closely follows the upper critical field of the overdoped superconducting phase and gives rise to an expanse of distinct non Fermi liquid behavior at finite temperatures. Together with signatures of two distinct flavors of quantum fluctuations, this suggests that quantum criticality plays a significant role in shaping the anomalous properties of the cuprate phase diagram.

cond-mat.str-el↗

arXiv2011

Sign reversal of the Hall resistance in the mixed-state of La$_{1.89}$ Ce$_{0.11}$CuO$_{4}$ and La$_{1.89}$Ce$_{0.11}$(Cu$_{0.99}$Co$_{0.01}$)O$_{4} $ thin films

The transport properties of La$_{1.89}$Ce$_{0.11}$CuO$_{4}$(LCCO) and La$_{1.89}$Ce$_{0.11}$(Cu$_{0.99}$Co$_{0.01}$)O$_{4}$ (LCCO:Co) superconducting thin films are investigated. When the external field $\bf H$ is applied along the crystallographic c-axis, a double sign reversal of the Hall voltage in the mixed state of LCCO:Co thin films is observed whereas a single sign reversal is detected in LCCO. A double sign reversal of the Hall signal in LCCO can be recovered if the magnetic field is tilted away from the plane of the film. We find that the transition from one to two of the Hall sign reversal coincides with the change in the pinning from strong to weak. This temperature/field induced transition is caused either by the magnetic impurities in LCCO:Co or by the coupling between the pancake vortices and the in-plane Josephson vortices in LCCO. These results are in agreement with early theoretical and numerical predictions.

cond-mat.supr-con↗

arXiv2011

First-principles study on oxidation effects in uranium oxides and high-pressure high-temperature behavior of point defects in uranium dioxide

Formation Gibbs free energy of point defects and oxygen clusters in uranium dioxide at high-pressure high-temperature conditions are calculated from first principles, using the LSDA+U approach for the electronic structure and the Debye model for the lattice vibrations. The phonon contribution on Frenkel pairs is found to be notable, whereas it is negligible for the Schottky defect. Hydrostatic compression changes the formation energies drastically, making defect concentrations depend more sensitively on pressure. Calculations show that, if no oxygen clusters are considered, uranium vacancy becomes predominant in overstoichiometric UO2 with the aid of the contribution from lattice vibrations, while compression favors oxygen defects and suppresses uranium vacancy greatly. At ambient pressure, however, the experimental observation of predominant oxygen defects in this regime can be reproduced only in a form of cuboctahedral clusters, underlining the importance of defect clustering in UO2+x. Making use of the point defect model, an equation of state for non-stoichiometric oxides is established, which is then applied to describe the shock Hugoniot of UO2+x. Furthermore, the oxidization and compression behavior of uranium monoxide, triuranium octoxide, uranium trioxide, and a series of defective UO2 at zero Kelvin are investigated. The evolution of mechanical properties and electronic structures with an increase of the oxidation degree are analyzed, revealing the transition of the groundstate of uranium oxides from metallic to Mott insulator and then to charge-transfer insulator due to the interplay of strongly correlated effects of 5f orbitals and the shift of electrons from uranium to oxygen atoms.

cond-mat.mtrl-sci↗

arXiv2011

Link between spin fluctuations and Cooper pairing in copper oxide superconductors

Although it is generally accepted that superconductivity (SC) is unconventional in the high- transition temperature copper oxides (high-Tc cuprates), the relative importance of phenomena such as spin and charge (stripe) order, SC fluctuations, proximity to a Mott insulator, a pseudogap phase, and quantum criticality are still a matter of great debate1. In electron-doped cuprates, the absence of an anomalous pseudogap phase in the underdoped region of the phase diagram2 and weaker electron correlations3,4, suggest that Mott physics and other unidentified competing orders are less relevant and that antiferromagnetic (AFM) spin fluctuations are the dominant feature. Here we demonstrate that a linear-temperature (T-linear) scattering rate - a key feature of the anomalous normal state properties of the cuprates - is correlated with the Cooper pairing (SC). Through a study of magnetotransport in thin films of the electron-doped cuprate La2 xCexCuO4 (LCCO), we show that an envelope of T-linear scattering surrounds the SC phase, and survives to zero temperature when superconductivity is suppressed by magnetic fields. Comparison with similar behavior found in organic superconductors5 strongly suggests that the T-linear resistivity is caused by spin-fluctuation scattering. Our results establish a fundamental connection between AFM spin fluctuations and the pairing mechanism of high temperature superconductivity in the cuprates.

cond-mat.supr-con↗

arXiv2011

Anomalous Enhancement of the Superconducting Transition Temperature in Electron-Doped Cuprate Heterostructures

The superconducting transition temperature $T_{c}$ of multilayers of electron-doped cuprates, composed of underdoped (or undoped) and overdoped La% $_{2-x}$Ce$_{x}$CuO$_{4}$ (LCCO) and Pr$_{2-x}$Ce$_{x}$CuO$_{4}$ (PCCO) thin films, is found to increase significantly with respect to the $T_{c}$ of the corresponding single-phase films. By investigating the critical current density of superlattices with different doping levels and layer thicknesses, we find that the $T_{c}$ enhancement is caused by a redistribution of charge over an anomalously large distance.

cond-mat.supr-con↗

arXiv2009

Preparation of electron-doped La(2-x)CexCuO4 thin films with various Ce doping by dc magnetron sputtering

A series of c-axis oriented electron-doped high-Tc superconducting La(2-x)CexCuO4 thin films, from heavily underdoped x=0.06 to heavily overdoped x=0.19, have been synthesized by dc magnetron sputtering technique on (100) SrTiO3 substrates. The influence of various fabrication conditions, such as the deposition temperature and the deposition rate, etc., on the quality of the thin films has been scrutinized. We find that the quality of the films is less sensitive to the deposition temperature in the overdoped region than that in the underdoped region. In the phase diagram of Tc(x), the superconducting dome indicates that the optimally doping level is at the point x=0.105 with the transition temperature Tc0 = 26.5 K. Further more, both the disappearance of the upturn in the $ρ_{xx}$(T) curve at low temperature under H=10 T and the positive differential Hall coefficient, $R_H'=d ρ_{xy}/dH$, are observed around x = 0.15, implying a possible rearrangement of Fermi surface at this doping level.

cond-mat.supr-con↗

arXiv2009

Thickness-induced insufficient oxygen reduction in La(2-x)CexCuO4 thin films

A series of electron-doped cuprate La(2-x)CexCuO4 thin films with different thicknesses have been fabricated and their annealing time are adjusted carefully to ensure the highest superconducting transition temperature. The transport measurements indicate that, with the increase of the film thickness (<100 nm), the residual resistivity increases and the Hall coefficient shifts in the negative direction. Further more, the X-ray diffraction data reveal that the c-axis lattice constant c0 increases with the decrease of film thickness. These abnormal phenomena can be attributed to the insufficient oxygen reduction in the thin films. Considering the lattice mismatching in the ab-plane between the SrTiO3 substrates and the films, the compressive stress from the substrates may be responsible for the more difficult reduction of the oxygen in the thin films.

cond-mat.supr-con↗

arXiv2009

Evidence for Antiferromagnetic Order in La$_{2-x}$Ce$_{x}$CuO$_{4}$ from Angular Magnetoresistance Measurements

We investigated the in-plane angular magnetoresistivity (AMR) of $% T^{^{\prime}}$-phase La$_{2-x}$Ce$_{x}$CuO$_{4}$ (LCCO) thin films ($% x=0.06-0.15$) fabricated by a pulsed laser deposition technique. The in-plane AMR with $\mathbf{H}\parallel ab$ shows a twofold symmetry instead of the fourfold behavior found in other electron-doped cuprates such as Pr$% _{2-x}$Ce$_{x}$CuO$_{4}$ and Nd$_{2-x}$Ce$_{x}$CuO$_{4}$. The twofold AMR disappears above a certain temperature, $T_{D}$. The $T_{D}(x)$ is well above $T_{c}(x)$ for $x=0.06$ ($\sim 110$ K), and decreases with increasing doping, until it is no longer observed above $T_{c}(x)$ at $x=0.15$. This twofold AMR below $T_{D}(x)$ is suggested to originate from an antiferromagnetic or spin density wave order.

cond-mat.supr-con↗

arXiv2006

Ferroelectric switched all-metallic-oxide $p$-$n$ junctions

We report the first formation of the metallic $p$-$n$ junctions, the ferroelectric (Ba,Sr)TiO$_3$ (BST) switched optimally electron-doped ($n$-type) metallic T'-phase superconductor, (La,Ce)$_2$CuO$_4$ (LCCO), and hole-doped ($p$-type) metallic CMR manganite (La,Sr)MnO$_3$ (LSMO) junctions. In contrast with the previous semiconductor $p$-$n$ ($p$-$I$-$n$) junctions which are switched by the built-in field $V_0$, the present metallic oxides $p$-$I$-$n$ junctions are switched by double barrier fields, the built-in field $V_0$, and the ferroelectric reversed polarized field $V_{rp}$, both take together to lead the junctions to possess definite parameters, such as definite negligible reversed current ($10^{-9}$ A), large breakdown voltage ($>$7 V), and ultrahigh rectification ($>2\times10^4$) in the bias voltage 1.2 V to 2.0 V and temperature range from 5 to over 300 K. The related transport feature, barrier size effect, and temperature effect are also observed and defined.

cond-mat.mtrl-sci↗

arXiv2006

Coexistence of Superconductivity and Ferromagnetism in Dilute Co-doped $La_{1.89} Ce_{0.11} Cu O_{4\pm\d}$ System

Thin films of the optimally electron-doped $T'$-phase superconductor La$_{1.89}$Ce$_{0.11}$CuO$_{4\pm \d}$ are investigated by dilute Co doping, formed as La$_{1.89}$Ce$_{0.11}$(Cu$_{1-x}$Co$_{x}$)O$_{4\pm\d}$ (LCCCO) with $x$ = 0.01 -- 0.05. The following results are obtained for the first time: for the whole dilute Co doping range, LCCCO thin films show long-range ferromagnetic ordering at the temperature range from 5 K to 300 K, which is likely due to the RKKY interaction; in the very dilute Co doping, $x$ = 0.01 and 0.02, the superconductivity is maitained, the system shows the coexistence of superconductivity and ferromagnetism in the CuO$_{2}$ plane. This may be based on the nature of the charge carriers in electron-doped high-$T_{c}$ cuprate superconductors.

cond-mat.supr-con↗