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K. Litzius

Publications and source records attributed to K. Litzius.

2 recordsLinked to original sources

Nanoscale imaging of spin textures with locally varying altermagnetic response in $\alpha$-Fe$_2$O$_3$

Altermagnetism is a recently identified magnetic state in which time-reversal symmetry is broken despite a collinear compensated spin structure. The response of altermagnets is determined not only by their $d$-, $g$-, or $i$-wave spin order, but also the orientation of their N\'eel vector $\mathbf{L}$. Therefore, accessing a response that fundamentally depends on the orientation of $\mathbf{L}$, such as the anomalous Hall effect, remains experimentally challenging in particular at the nanoscale. Here, we harness nano-spectroscopic X-ray magnetic circular dichroism (XMCD) to investigate nanoscale modulated altermagnetic responses in $\alpha$-Fe$_2$O$_3$ (Hematite). By performing spectroscopy across the temperature-induced $\mathbf{L}$-reorientation Morin transition, we observe the on-and-off switching of XMCD, in agreement with our theoretical calculations. Although the bulk XMCD vanishes below the Morin temperature, we confirm the reorientation of $\mathbf{L}$ by harnessing polarization-independent X-ray absorption spectroscopy. Moreover, we observe a finite XMCD signal in nanoscale domain walls with locally modulated N\'eel vectors, while the surrounding domains exhibit no XMCD. At room temperature, we instead identify altermagnetic meron spin textures that exhibit XMCD in their planar regions but no XMCD in their nanoscopic cores. Our results establish a pathway to harness complex spin textures with nanoscale functionalities in a broader class of altermagnets with various $\mathbf{L}$-orientations and using light, earth-abundant elements.

cond-mat.mtrl-sci

Investigation of the Dzyaloshinskii-Moriya interaction and room temperature skyrmions in W/CoFeB/MgO thin films and microwires

Recent studies have shown that material structures, which lack structural inversion symmetry and have high spin-orbit coupling can exhibit chiral magnetic textures and skyrmions which could be a key component for next generation storage devices. The Dzyaloshinskii-Moriya Interaction (DMI) that stabilizes skyrmions is an anti-symmetric exchange interaction favoring non-collinear orientation of neighboring spins. It has been shown that material systems with high DMI can lead to very efficient domain wall and skyrmion motion by spin-orbit torques. To engineer such devices, it is important to quantify the DMI for a given material system. Here we extract the DMI at the Heavy Metal (HM) /Ferromagnet (FM) interface using two complementary measurement schemes namely asymmetric domain wall motion and the magnetic stripe annihilation. By using the two different measurement schemes, we find for W(5 nm)/Co20Fe60B20(0.6 nm)/MgO(2 nm) the DMI to be 0.68 +/- 0.05 mJ/m2 and 0.73 +/- 0.5 mJ/m2, respectively. Furthermore, we show that this DMI stabilizes skyrmions at room temperature and that there is a strong dependence of the DMI on the relative composition of the CoFeB alloy. Finally we optimize the layers and the interfaces using different growth conditions and demonstrate that a higher deposition rate leads to a more uniform film with reduced pinning and skyrmions that can be manipulated by Spin-Orbit Torques.

cond-mat.mtrl-sci