arXiv subjects

K. M. Pontoppidan

Publications and source records attributed to K. M. Pontoppidan.

At least 37 records · Page 2Linked to original sources

arXiv2011

Warm dust resolved in the cold disk around T Cha with VLTI/AMBER

The transition between massive Class II circumstellar disks and Class III debris disks, with dust residuals, has not yet been clearly understood. Disks are expected to dissipate with time, and dust clearing in the inner regions can be the consequence of several mechanisms. Planetary formation is one of them that will possibly open a gap inside the disk. According to recent models based on photometric observations, T Cha is expected to present a large gap within its disk, meaning that an inner dusty disk is supposed to have survived close to the star. We investigate this scenario with new near-infrared interferometric observations. We observed T Cha in the H and K bands using the AMBER instrument at VLTI and used the MCFOST radiative transfer code to model the SED of T Cha and the interferometric observations simultaneously and to test the scenario of an inner dusty structure. We also used a toy model of a binary to check that a companion close to the star can reproduce our observations. The scenario of a close (few mas) companion cannot satisfactorily reproduce the visibilities and SED, while a disk model with a large gap and an inner ring producing the bulk of the emission (in H and K-bands) close to 0.1 AU is able to account for all the observations. With this study, the presence of an optically thick inner dusty disk close to the star and dominating the H and K- bands emission is confirmed. According to our model, the large gap extends up to ~ 7.5 AU. This points toward a companion (located at several AU) gap-opening scenario to explain the morphology of T Cha.

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arXiv2011

Single peaked CO emission line profiles from the inner regions of protoplanetary disks

The study of warm molecular gas in the inner region (<10 AU) of circumstellar disks around young stars is of significant importance to understand how planets are forming. This inner zone of disks can now be explored in unprecedented detail with the high spectral (R=100000) and spatial resolution spectrometer CRIRES at the VLT. This paper investigates a set of disks that show CO ro-vibrational v=1-0 4.7 micron emission line profiles characterized by a single, narrow peak and a broad base extending to > 50 km/s, not readily explained by just Keplerian motions of gas in the inner disk. The line profiles are very symmetric, have high line/continuum ratios and have central velocity shifts of <5 km/s relative to the stellar radial velocity. The disks in this subsample are accreting onto their central stars at high rates relative to the parent sample. All disks show CO lines from v=2, suggesting that the lines are excited, at least in part, by UV fluorescence. Analysis of their spatial distribution shows that the lines are formed within a few AU of the central star. It is concluded that these broad centrally peaked line profiles are inconsistent with the double peaked profiles expected from just an inclined disk in Keplerian rotation. Alternative non-Keplerian line formation mechanisms are discussed, including thermally and magnetically launched winds and funnel flows. The most likely interpretation is that these profiles originate from a combination of emission from the inner part (< a few AU) of a circumstellar disk, perhaps with enhanced turbulence, and a slow moving disk wind, launched by either EUV emission or soft X-rays.

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arXiv2010

First results of the Herschel Key Program 'Dust, Ice and Gas in Time': Dust and Gas Spectroscopy of HD 100546

We present far-infrared spectroscopic observations, taken with the Photodetector Array Camera and Spectrometer (PACS) on the Herschel Space Observatory, of the protoplanetary disk around the pre-main-sequence star HD 100546. These observations are the first within the DIGIT Herschel key program, which aims to follow the evolution of dust, ice, and gas from young stellar objects still embedded in their parental molecular cloud core, through the final pre-main-sequence phases when the circumstellar disks are dissipated. Our aim is to improve the constraints on temperature and chemical composition of the crystalline olivines in the disk of HD 100546 and to give an inventory of the gas lines present in its far-infrared spectrum. The 69 μ\m feature is analyzed in terms of position and shape to derive the dust temperature and composition. Furthermore, we detected 32 emission lines from five gaseous species and measured their line fluxes. The 69 μ\m emission comes either from dust grains with ~70 K at radii larger than 50 AU, as suggested by blackbody fitting, or it arises from ~200 K dust at ~13 AU, close to the midplane, as supported by radiative transfer models. We also conclude that the forsterite crystals have few defects and contain at most a few percent iron by mass. Forbidden line emission from [CII] at 157 μ\m and [OI] at 63 and 145 μ\m, most likely due to photodissociation by stellar photons, is detected. Furthermore, five H2O and several OH lines are detected. We also found high-J rotational transition lines of CO, with rotational temperatures of ~300 K for the transitions up to J=22-21 and T~800 K for higher transitions.

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arXiv2010

Dust, Ice and Gas in Time (DIGIT) Herschel program first results: A full PACS-SED scan of the gas line emission in protostar DK Cha

DK Cha is an intermediate-mass star in transition from an embedded configuration to a star plus disk stage. We aim to study the composition and energetics of the circumstellar material during this pivotal stage. Using the Range Scan mode of PACS on the Herschel Space Observatory, we obtained a spectrum of DK Cha from 55 to 210 micron as part of the DIGIT Key Program. Almost 50 molecular and atomic lines were detected, many more than the 7 lines detected in ISO-LWS. Nearly the entire ladder of CO from J=14-13 to 38-37 (E_u/k = 4080 K), water from levels as excited as E_u/k = 843 K, and OH lines up to E_u/k = 290 K were detected. The continuum emission in our PACS SED scan matches the flux expected from a model consisting of a star, a surrounding disk of 0.03 Solar mass, and an envelope of a similar mass, supporting the suggestion that the object is emerging from its main accretion stage. Molecular, atomic, and ionic emission lines in the far-infrared reveal the outflow's influence on the envelope. The inferred hot gas can be photon-heated, but some emission could be due to C-shocks in the walls of the outflow cavity.

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arXiv2010

Evidence for episodic warm outflowing CO gas from the intermediate mass young stellar object IRAS 08470-4321

We present a R=10,000 M-band spectrum of LLN19 (IRAS 08470-4321), a heavily embedded intermediate-mass young stellar object located in the Vela Molecular Cloud, obtained with VLT-ISAAC. The data were fitted by a 2-slab cold-hot model and a wind model. The spectrum exhibits deep broad ro-vibrational absorption lines of 12CO v=1<-0 and 13CO v=1<-0. A weak CO ice feature at 4.67 micron is also detected. Differences in velocity indicate that the warm gas is distinct from the cold millimeter emitting gas, which may be associated with the absorption by cooler gas (45K). The outflowing warm gas at 300-400K and with a mass-loss rate varying between 0.48E-7 and 4.2E-7 MSun /yr can explain most of the absorption. Several absorption lines were spectrally resolved in subsequent spectra obtained with the VLT-CRIRES instrument. Multiple absorption substructures in the high-resolution (R=100,000) spectra indicate that the mass-loss is episodic with at least two major events that occurred recently (<28 years). The discrete mass-loss events together with the large turbulent width of the gas (dv=10-12 km/s) are consistent with the predictions of the Jet-Bow shock outflow and the wide-angle wind model. The CO gas/solid column density ratio of 20-100 in the line-of-sight confirms that the circumstellar environment of LLN~19 is warm. We also derive a 12C/13C ratio of 67 +/- 3, consistent with previous measurements in local molecular clouds but not with the higher ratios found in the envelope of other young stellar objects.

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arXiv2009

Radiative transfer models of mid-infrared H2O lines in the Planet-forming Region of Circumstellar Disks

The study of warm molecular gas in the inner regions of protoplanetary disks is of key importance for the study of planet formation and especially for the transport of H2O and organic molecules to the surfaces of rocky planets/satellites. Recent Spitzer observations have shown that the mid-infrared spectra of protoplanetary disks are covered in emission lines due to water and other molecules. Here, we present a non-LTE 2D radiative transfer model of water lines in the 10-36 mum range that can be used to constrain the abundance structure of water vapor, given an observed spectrum, and show that an assumption of local thermodynamic equilibrium (LTE) does not accurately estimate the physical conditions of the water vapor emission zones. By applying the model to published Spitzer spectra we find that: 1) most water lines are subthermally excited, 2) the gas-to-dust ratio must be one to two orders of magnitude higher than the canonical interstellar medium ratio of 100-200, and 3) the gas temperature must be higher than the dust temperature, and 4) the water vapor abundance in the disk surface must be truncated beyond ~ 1 AU. A low efficiency of water formation below ~ 300 K may naturally result in a lower water abundance beyond a certain radius. However, we find that chemistry, may not be sufficient to produce an abundance drop of many orders of magnitude and speculate that the depletion may also be caused by vertical turbulent diffusion of water vapor from the superheated surface to regions below the snow line, where the water can freeze out and be transported to the midplane as part of the general dust settling. Such a vertical cold finger effect is likely to be efficient due to the lack of a replenishment mechanism of large, water-ice coated dust grains to the disk surface.

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arXiv2008

Lack of PAH emission toward low-mass embedded young stellar objects

PAHs have been detected toward molecular clouds and some young stars with disks, but have not yet been associated with embedded young stars. We present a sensitive mid-IR spectroscopic survey of PAH features toward a sample of low-mass embedded YSOs. The aim is to put constraints on the PAH abundance in the embedded phase of star formation using radiative transfer modeling. VLT-ISAAC L-band spectra for 39 sources and Spitzer IRS spectra for 53 sources are presented. Line intensities are compared to recent surveys of Herbig Ae/Be and T Tauri stars. The radiative transfer codes RADMC and RADICAL are used to model the PAH emission from embedded YSOs consisting of a PMS star with a circumstellar disk embedded in an envelope. The dependence of the PAH feature on PAH abundance, stellar radiation field, inclination and the extinction by the surrounding envelope is studied. The 3.3 micron PAH feature is undetected for the majority of the sample (97%), with typical upper limits of 5E-16 W/m^2. Compact 11.2 micron PAH emission is seen directly towards 1 out of the 53 Spitzer Short-High spectra, for a source that is borderline embedded. For all 12 sources with both VLT and Spitzer spectra, no PAH features are detected in either. In total, PAH features are detected toward at most 1 out of 63 (candidate) embedded protostars (<~ 2%), even lower than observed for class II T Tauri stars with disks (11-14%). Assuming typical class I stellar and envelope parameters, the absence of PAHs emission is most likely explained by the absence of emitting carriers through a PAH abundance at least an order of magnitude lower than in molecular clouds but similar to that found in disks. Thus, most PAHs likely enter the protoplanetary disks frozen out in icy layers on dust grains and/or in coagulated form.

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arXiv2008

Characterizing the nature of embedded young stellar objects through silicate, ice and millimeter observations

(Abridged) Classification schemes for YSOs are based on evaluating the degree of dissipation of the surrounding envelope, whose main effects are the extinction of the optical radiation from the central YSO and re-emission in the far-infrared. Since extinction is a property of column density along the line of sight, the presence of a protoplanetary disk may lead to a misclassification when the system is viewed edge-on. We performed radiative transfer calculations, using the axysimmetric 3D radiative transfer codes RADMC and RADICAL, to show the effects of different geometries on the main indicators of YSO evolutionary stage, like the slope of the flux between 2 and 24mum, the bolometric temperature and the optical depth of silicates and ices. We show that for systems viewed at intermediate angles the 'classical' indicators of evolution accurately trace the envelope column density, and they all agree with each other. On the other hand, edge-on system are misclassified for inclinations larger than ~65deg. In particular, silicate emission, typical of pre-main sequence stars with disks, turns into absorption when the disk column density reaches 1e22cm-2, corresponding e.g. to a 5e-3 Msun flaring disk viewed at 64deg. A similar effect is noticed in all the other classification indicators studied alpha, Tbol, and the H2O and CO2 ices absorption strengths. This misclassification has a big impact on the nature of the flat-spectrum sources (alpha ~0), whose number can be explained by simple geometrical arguments without invoking evolution. A reliable classification scheme using a minimal number of observations is constituted by observations of the mm-flux with both a single dish and an interferometer.

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arXiv2008

H2O and OH gas in the terrestrial planet-forming zones of protoplanetary disks

We present detections of numerous 10-20 micron H2O emission lines from two protoplanetary disks around the T Tauri stars AS 205A and DR Tau, obtained using the InfraRed Spectrograph on the Spitzer Space Telescope. Follow-up 3-5 micron Keck-NIRSPEC data confirm the presence of abundant water and spectrally resolve the lines. We also detect the P4.5 (2.934 micron) and P9.5 (3.179 micron) doublets of OH and 12CO/13CO v=1-0 emission in both sources. Line shapes and LTE models suggest that the emission from all three molecules originates between ~0.5 and 5 AU, and so will provide a new window for understanding the chemical environment during terrestrial planet formation. LTE models also imply significant columns of H2O and OH in the inner disk atmospheres, suggesting physical transport of volatile ices either vertically or radially; while the significant radial extent of the emission stresses the importance of a more complete understanding of non-thermal excitation processes.

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arXiv2007

Spatially extended PAHs in circumstellar disks around T Tauri and Herbig Ae stars

Our aim is to determine the presence and location of the emission from polycyclic aromatic hydrocarbons (PAHs) towards low and intermediate mass young stars with disks using large aperture telescopes. VLT-VISIR N-band spectra and VLT-ISAAC and VLT-NACO L-band spectra of 29 sources are presented, spectrally resolving the 3.3, 8.6, 11.2, and 12.6 micron PAH features. Spatial-extent profiles of the features and the continuum emission are derived and used to associate the PAH emission with the disks. The results are discussed in the context of recent PAH-emission disk models. The 3.3, 8.6, and 11.2 micron PAH features are detected toward a small fraction of the T Tauri stars, with typical upper limits between 1E-15 and 5E-17 W/m^2. All 11.2 micron detections from a previous Spitzer survey are confirmed with (tentative) 3.3 micron detections, and both the 8.6 and the 11.2 micron features are detected in all PAH sources. For 6 detections, the spatial extent of the PAH features is confined to scales typically smaller than 0.12-0.34'', consistent with the radii of 12-60 AU disks at their distances (typically 150 pc). For 3 additional sources, WL 16, HD 100546, and TY CrA, one or more of the PAH features are more extended than the hot dust continuum of the disk, whereas for Oph IRS 48, the size of the resolved PAH emission is confirmed as smaller than for the large grains. For HD 100546, the 3.3 micron emission is confined to a small radial extent of 12 +- 3 AU, most likely associated with the outer rim of the gap in this disk. Gaps with radii out to 10-30 AU may also affect the observed PAH extent for other sources. For both Herbig Ae and T Tauri stars, the small measured extents of the 8.6 and 11.2 micron features are consistent with larger (>= 100 carbon atoms) PAHs.

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arXiv2007

Cold Disks: Spitzer Spectroscopy of Disks around Young Stars with Large Gaps

We have identified four circumstellar disks with a deficit of dust emission from their inner 15-50 AU. All four stars have F-G spectral type, and were uncovered as part of the Spitzer Space Telescope ``Cores to Disks'' Legacy Program Infrared Spectrograph (IRS) first look survey of ~100 pre-main sequence stars. Modeling of the spectral energy distributions indicates a reduction in dust density by factors of 100-1000 from disk radii between ~0.4 and 15-50 AU, but with massive gas-rich disks at larger radii. This large contrast between the inner and outer disk has led us to use the term `cold disks' to distinguish these unusual systems. However, hot dust [0.02-0.2 Mmoon] is still present close to the central star (R ~0.8 AU). We introduce the 30/13 micron, flux density ratio as a new diagnostic for identifying cold disks. The mechanisms for dust clearing over such large gaps are discussed. Though rare, cold disks are likely in transition from an optically thick to an optically thin state, and so offer excellent laboratories for the study of planet formation.

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arXiv2007

Evolution of dust and ice features around FU Orionis objects

(abridged) We present spectroscopy data for a sample of 14 FUors and 2 TTauri stars observed with the Spitzer Space Telescope or with the Infrared Space Observatory (ISO). Based on the appearance of the 10 micron silicate feature we define 2 categories of FUors. Objects showing the silicate feature in absorption (Category 1) are still embedded in a dusty and icy envelope. The shape of the 10 micron silicate absorption bands is compared to typical dust compositions of the interstellar medium and found to be in general agreement. Only one object (RNO 1B) appears to be too rich in amorphous pyroxene dust, but a superposed emission feature can explain the observed shape. We derive optical depths and extinction values from the silicate band and additional ice bands at 6.0, 6.8 and 15.2 micron. In particular the analysis of the CO_2 ice band at 15.2 micron allows us to search for evidence for ice processing and constrains whether the absorbing material is physically linked to the central object or in the foreground. For objects showing the silicate feature in emission (Category 2), we argue that the emission comes from the surface layer of accretion disks. Analyzing the dust composition reveals that significant grain growth has already taken place within the accretion disks, but no clear indications for crystallization are present. We discuss how these observational results can be explained in the picture of a young, and highly active accretion disk. Finally, a framework is proposed as to how the two categories of FUors can be understood in a general paradigm of the evolution of young, low-mass stars. Only one object (Parsamian 21) shows PAH emission features. Their shapes, however, are often seen toward evolved stars and we question the object's status as a FUor and discuss other possible classifications.

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arXiv2007

Spatial separation of small and large grains in the transitional disk around the young star IRS 48

We present spatially resolved mid-infrared images of the disk surrounding the young star IRS 48 in the Ophiuchus cloud complex. The disk exhibits a ring-like structure at 18.7 micron, and is dominated by very strong emission from polycyclic aromatic hydrocarbons at shorter wavelengths. This allows a detailed study of the relative distributions of small and large dust grains. Images of IRS 48 in 5 mid-infrared bands from 8.6 to 18.7 micron as well as a low resolution N-band spectrum are obtained with VLT-VISIR. Optical spectroscopy is used to determine the spectral type of the central star and to measure the strength of the Halpha line. The 18.7 micron ring peaks at a diameter of 110 AU, with a gap of ~ 60 AU. The shape of the ring is consistent with an inclination of i = 48 +- 8 degrees. In contrast, the 7.5-13 micron PAH emission bands are centered on the source and appear to fill the gap within the ring. The measured PAH line strengths are 10-100x stronger than those typically measured for young M0 stars and can only be explained with a high PAH abundance and/or strong excess optical/UV emission. The morphology of the images, combined with the absence of a silicate emission feature, imply that the inner disk has been cleared of micron-sized dust but with a significant population of PAHs remaining. We argue that the gap can be due to grain growth and settling or to clearing by an unseen planetary or low-mass companion. IRS 48 may represent a short-lived transitional phase from a classical to a weak-line T Tauri star.

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arXiv2007

Abundant crystalline silicates in the disk of a very low mass star

We announce the discovery of SST-Lup3-1, a very low mass star close to the brown dwarf boundary in Lupus III with a circum(sub)stellar disk, discovered by the `Cores to Disks' Spitzer Legacy Program from mid-, near-infrared and optical data, with very conspicuous crystalline silicate features in its spectrum. It is the first of such objects with a full 5 to 35 micron spectrum taken with the IRS and it shows strong 10 and 20 micron silicate features with high feature to continuum ratios and clear crystalline features out to 33 micron. The dust in the disk upper layer has a crystalline silicate grain fraction between 15% and 33%, depending on the assumed dust continuum. The availability of the full Spitzer infrared spectrum allows an analysis of the dust composition as a function of temperature and position in the disk. The hot (~ 300 K) dust responsible for the 10 micron feature consists of a roughly equal mix of small (~ 0.1 micron) and large (~ 1.5 micron) grains, whereas the cold (~ 70 K) dust responsible for the longer wavelength silicate features contains primarily large grains (> 1 micron). Since the cold dust emission arises from deeper layers in the inner (< 3 AU) disk as well as from the surface layers of the outer (3-5 AU) disk, this provides direct evidence for combined grain growth and settling in the disk. The inferred crystalline mass fractions in the two components are comparable. Since only the inner 0.02 AU of the disk is warm enough to anneal the amorphous silicate grains, even the lowest fraction of 15% of crystalline material requires either very efficient mixing or other formation mechanisms.

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arXiv2007

PAH chemistry and IR emission from circumstellar disks

Aims. The chemistry of, and infrared (IR) emission from, polycyclic aromatic hydrocarbons (PAHs) in disks around Herbig Ae/Be and T Tauri stars are investigated. The equilibrium distribution of the PAHs over all accessible charge/hydrogenation states depends on the size and shape of the PAHs and on the physical properties of the star and surrounding disk. Methods. A chemistry model is created to calculate this equilibrium distribution. Destruction of PAHs by ultraviolet (UV) photons, possibly in multi-photon absorption events, is taken into account. The chemistry model is coupled to a radiative transfer code to provide the physical parameters and to combine the PAH emission with the spectral energy distribution (SED) from the star+disk system. Results. Normally hydrogenated PAHs in Herbig Ae/Be disks account for most of the observed PAH emission, with neutral and positively ionized species contributing in roughly equal amounts. Close to the midplane, the PAHs are more strongly hydrogenated and negatively ionized, but these species do not contribute to the overall emission because of the low UV/optical flux deep inside the disk. PAHs of 50 carbon atoms are destroyed out to 100 AU in the disk's surface layer, and the resulting spatial extent of the emission does not agree well with observations. Rather, PAHs of about 100 carbon atoms or more are predicted to cause most of the observed emission. The emission is extended on a scale similar to that of the size of the disk. Furthermore, the emission from T Tauri disks is much weaker and concentrated more towards the central star than that from Herbig Ae/Be disks. Positively ionized PAHs are predicted to be largely absent in T Tauri disks because of the weaker radiation field.

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arXiv2006

Spitzer-IRS spectra of disks around T Tauri stars II. PAH emission features

Aims: We search for PAH features towards T Tauri stars and compare them with surveys of Herbig Ae/Be stars. The presence and strength of the PAH features are interpreted with disk radiative transfer models exploring the PAH feature dependence on the incident UV radiation, PAH abundance and disk parameters. Methods: Spitzer Space Telescope 5-35 micron spectra of 54 pre-main sequence stars with disks were obtained, consisting of 38 T Tauri, 7 Herbig Ae/Be and 9 stars with unknown spectral type. Results: Compact PAH emission is detected towards at least 8 sources of which 5 are Herbig Ae/Be stars. The 11.2 micron PAH feature is detected in all of these sources, as is the 6.2 micron PAH feature where short wavelength data are available. However, the 7.7 and 8.6 micron features appear strongly in only 1 of these 4 sources. PAH emission is observed towards at least 3 T Tauri stars (8% detection rate). The lowest mass source with PAHs in our sample is T Cha (G8). All 4 sources in our sample with evidence for dust holes in their inner disk show PAH emission, increasing the feature/continuum ratio. Typical 11.2 micron line intensities are an order of magnitude lower than those observed for the more massive Herbig Ae/Be stars. Measured line fluxes indicate PAH abundances that are factors of 10-100 lower than standard interstellar values. Conversely, PAH features from disks exposed to stars with Teff<=4200K without enhanced UV are predicted to be below the current detection limit, even for high PAH abundances. Disk modeling shows that the 6.2 and 11.2 micron features are the best PAH tracers for T Tauri stars, whereas the 7.7 and 8.6 micron bands have low feature over continuum ratios due to the strongly rising silicate emission.

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arXiv2006

Low-mass star formation in R Coronae Australis: Observations of organic molecules with the APEX telescope

This paper presents new APEX submillimetre molecular line observations of three low-mass protostars, IRS7A, IRS7B, and IRAS32, in the R Coronae Australis molecular cloud complex. The molecular excitation analysis is performed using a statistical equilibrium radiative transfer code. The derived beam averaged fractional abundances vary by less than a factor of two among the three sources, except those of H2CO and CH3OH, which show differences of about an order of magnitude. The molecular abundances are similar to those typically found in other star-forming regions in the Galaxy, such as the $ρ$~Oph and Perseus molecular clouds. There is a marked difference in the kinetic temperatures derived for the protobinary source IRS7 from H2CO (40-60 K) and CH3OH (20 K), possibly indicating a difference in origin of the emission from these two molecules.

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arXiv2006

Spatial mapping of ices in the Oph-F core: A direct measurement of CO depletion and the formation of CO2

Aims: Ices in dense star-forming cores contain the bulk of volatile molecules apart from H2 and thus represent a large fraction of dark cloud chemistry budget.To directly constrain the freeze-out profile of CO, the formation route of CO2 and the carrier of the 6.8 micron band, the spatial distribution of the CO/CO2 ice system and the 6.8 micron band carrier are measured in a nearby dense core. Methods: VLT-ISAAC, ISOCAM-CVF and Spitzer-IRS archival mid-infrared (3-20 micron) spectroscopy of young stellar objects is used to construct a map of the abundances of CO and CO2 ices in the Oph-F star-forming core, probing core radii from 2 10^3 to 14 10^3 AU or densities from 5 10^4 to 5 10^5 cm^-3 with a resolution of ~ 3000 AU. Results: The line-of-sight averaged abundances relative to water ice of both CO and CO2 ices increase monotonously with decreasing distance to the core center. The map traces the shape of the CO abundance profile between freeze-out ratios of 5-60% and shows that the CO2 ice abundance increases by a factor of 2 as the CO freezes out. It is suggested that this indicates a formation route of CO2 on a CO ice surface to produce a CO2 component dilute in CO ice, in addition to a fraction of the CO2 formed at lower densities along with the water ice mantle. It is predicted that the CO2 bending mode band profile should reflect a high CO:CO2 number ratio in the densest parts of dark clouds. In contrast to CO and CO2, the abundance of the carrier of the 6.8 micron band remains relatively constant throughout the core. A simple freeze-out model of the CO abundance profile is used to estimate the binding energy of CO on a CO ice surface to 814+/-30 K.

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