arXiv subjects

K. Matsubayashi

Publications and source records attributed to K. Matsubayashi.

At least 19 recordsLinked to original sources

arXiv2026

Coupled structural and electronic evolution under pressure in CuIr2Se4, CuRh2S4, and CuRh2Se4

Spinel chalcogenides provide a platform for investigating the interplay among metallic, superconducting, and pressure-induced insulating states. Here, we combine synchrotron powder X-ray diffraction and electrical-resistivity measurements to investigate the pressure evolution of CuIr2Se4, CuRh2S4, and CuRh2Se4 over pressure ranges extending beyond those previously explored. High-pressure diffraction reveals closely related monoclinic supercells in all three compounds. For CuIr2Se4 and CuRh2S4, constrained profile fits based on structural models relaxed using density functional theory are compatible with Phase-IV-type bond-disproportionated structures, whereas the data for CuRh2Se4 establish a compatible monoclinic unit cell without resolving its atomic-scale ordering pattern. Insulating-like transport develops abruptly over a narrow pressure range in CuIr2Se4 but more gradually over broader pressure ranges in the Rh-based compounds, in close correspondence with their respective structural transformations. We also establish previously unreported bulk superconductivity in CuIr2Se4 at ambient pressure: zero resistance is attained at 0.29 K, and the accompanying ac diamagnetic response is consistent with nearly complete superconducting shielding. These results establish a close relationship between the formation of the high-pressure monoclinic phases and the evolution toward insulating transport, and demonstrate that transition-metal and chalcogen substitutions tune the characteristic pressure scales and the competition with superconductivity within a closely related structural framework.

cond-mat.mtrl-sci↗

arXiv2022

Pressure tuning of localization and superconductivity in LaOPbBiS$_{3}$ and La$_{2}$O$_{2}$Bi$_{3}$AgS$_{6}$

We report the effect of pressure on the electrical transport properties of the four-layer-type bismuth chalcogenide semiconductors LaOPbBiS$_{3}$ and La$_{2}$O$_{2}$Bi$_{3}$AgS$_{6}$ and present the discovery of a pressure-induced superconductivity. In both compounds, the semiconductorlike behavior concomitant with an anomaly in the more insulating state is gradually suppressed with increasing pressure while the superconductivity develops. The obtained phase diagrams, in sharp contrast with the interplay between the conventional charge density waves and superconductivity, suggest that the enhancement of the superconductivity is due to the disorder near the localization threshold. These results indicate that pressure tuning of the local disorder in four-layer-type bismuth chalcogenides provides an attractive opportunity to study the interplay between disorder and superconductivity.

cond-mat.supr-con↗

arXiv2019

Evolution of Magnetic Double Helix and Quantum Criticality near a Dome of Superconductivity in CrAs

At ambient pressure CrAs undergoes a first-order transition into a double-helical magnetic state at TN = 265 K, which is accompanied by a structural transition. The recent discovery of pressure-induced superconductivity in CrAs makes it important to clarify the nature of quantum phase transitions out of its coupled structural/helimagnetic order. Here we show, via neutron diffraction on the single-crystal CrAs under hydrostatic pressure (P), that the combined order is suppressed at Pc ~ 10 kbar, near which bulk superconductivity develops with a maximal transition temperature Tc ~ 2 K. We further show that the coupled order is also completely suppressed by phosphorus doping in CrAs1-xPx at a critical xc ~ 0.05, above which inelastic neutron scattering evidenced persistent antiferromagnetic correlations, providing a possible link between magnetism and superconductivity. In line with the presence of antiferromagnetic fluctuations near Pc (xc), the A coefficient of the quadratic temperature dependence of resistivity exhibits a dramatic enhancement as P (x) approaches Pc (xc), around which Res(T) has a non-Fermi-liquid form. Accordingly, the electronic specific-heat coefficient of CrAs1-xPx peaks out around xc. These properties provide clear evidences for quantum criticality, which we interpret as originating from a nearly second-order helimagnetic quantum phase transition that is concomitant with a first-order structural transition. Our findings in CrAs highlight the distinct characteristics of quantum criticality in bad metals, thereby bringing out new insights into the physics of unconventional superconductivity such as occurring in the high-Tc iron pnictides.

cond-mat.supr-con↗

arXiv2016

Competition of superconductivity with the structural transition in Mo3Sb7

Prior to the superconducting transition at Tc = 2.3 K, Mo3Sb7 undergoes a symmetry-lowering, cubic-to-tetragonal structural transition at Ts = 53 K. We have monitored the pressure dependence of these two transitions by measuring the resistivity of Mo3Sb7 single crystals under various hydrostatic pressures up to 15 GPa. The application of external pressure enhances Tc but suppresses Ts until Pc ~ 10 GPa, above which a pressure-induced first order structural transition takes place and is manifested by the phase coexistence in the pressure range 8 < P < 12 GPa. The cubic phase above 12 GPa is also found to be superconducting with a higher Tc =6 K that decreases slightly with further increasing pressure. The variations with pressure of Tc and Ts satisfy the Bilbro-McMillan equation, i.e. Tc^nTs^(1-n) = constant, thus suggesting the competition of superconductivity with the structural transition that has been proposed to be accompanied with a spin-gap formation at Ts. This scenario is supported by our first-principles calculations which imply the plausible importance of magnetism that competes with the superconductivity in Mo3Sb7.

cond-mat.supr-con↗

arXiv2016

T/B scaling without quasiparticle mass divergence: YbCo2Ge4

YbCo$_2$Ge$_4$ is a clean paramagnetic Kondo lattice which displays non-Fermi liquid behavior. We report a detailed investigation of the specific heat, magnetic Grüneisen parameter ($Γ_{\rm mag}$) and temperature derivative of the magnetization ($M$) on a high-quality single crystal at temperatures down to $0.1$~K and magnetic fields up to 7~T. $Γ_{\rm mag}$ and $dM/dT$ display a divergence upon cooling and obey $T/B$ scaling. Similar behavior has previously been found in several other Yb-based Kondo lattices and related to a zero-field quantum critical point without fine tuning of pressure or composition. However, in the approach of $B\rightarrow 0$ the electronic heat capacity coefficient of YbCo$_2$Ge$_4$ saturates at low $T$, excluding ferromagnetic quantum criticality. This indicates that $T/B$ scaling is insufficient to prove a zero-field quantum critical point.

cond-mat.str-el↗

arXiv2016

Pressure dependence of the magnetic ground states in MnP

MnP, a superconductor under pressure, exhibits a ferromagnetic order below TC~290 K followed by a helical order with the spins lying in the ab plane and the helical rotation propagating along the c axis below Ts~50 K at ambient pressure. We performed single crystal neutron diffraction experiments to determine the magnetic ground states under pressure. Both TC and Ts are gradually suppressed with increasing pressure and the helical order disappears at ~1.2 GPa. At intermediate pressures of 1.8 and 2.0 GPa, the ferromagnetic order first develops and changes to a conical or two-phase (ferromagnetic and helical) structure with the propagation along the b axis below a characteristic temperature. At 3.8 GPa, a helical magnetic order appears below 208 K, which hosts the spins in the ac plane and the propagation along the b axis. The period of this b axis modulation is shorter than that at 1.8 GPa. Our results indicate that the magnetic phase in the vicinity of the superconducting phase may have a helical magnetic correlation along the b axis.

cond-mat.supr-con↗

arXiv2015

Dome-shaped magnetic order competing with high-temperature superconductivity at high pressures in FeSe

The coexistence and competition between superconductivity and electronic orders, such as spin or charge density waves, have been a central issue in high transition-temperature (${T_{\rm c}}$) superconductors. Unlike other iron-based superconductors, FeSe exhibits nematic ordering without magnetism whose relationship with its superconductivity remains unclear. More importantly, a pressure-induced fourfold increase of ${T_{\rm c}}$ has been reported, which poses a profound mystery. Here we report high-pressure magnetotransport measurements in FeSe up to $\sim9$ GPa, which uncover a hidden magnetic dome superseding the nematic order. Above ${\sim6}$ GPa the sudden enhancement of superconductivity (${T_{\rm c}\le38.3}$ K) accompanies a suppression of magnetic order, demonstrating their competing nature with very similar energy scales. Above the magnetic dome we find anomalous transport properties suggesting a possible pseudogap formation, whereas linear-in-temperature resistivity is observed above the high-${T_{\rm c}}$ phase. The obtained phase diagram highlights unique features among iron-based superconductors, but bears some resemblance to that of high-${T_{\rm c}}$ cuprates.

cond-mat.supr-con↗

arXiv2015

Kondo effect in CeX$_{c}$ (X$_{c}$=S, Se, Te) studied by electrical resistivity under high pressure

We have measured the electrical resistivity of cerium monochalcogenices, CeS, CeSe, and CeTe, under high pressures up to 8 GPa. Pressure dependences of the antiferromagnetic ordering temperature $T_{N}$, crystal field splitting, and the $\ln T$ anomaly of the Kondo effect have been studied to cover the whole region from the magnetic ordering regime at low pressure to the Fermi liquid regime at high pressure. $T_{N}$ initially increases with increasing pressure, and starts to decrease at high pressure as expected from the Doniach's diagram. Simultaneously, the $\ln T$ behavior in the resistivity is enhanced, indicating the enhancement of the Kondo effect by pressure. It is also characteristic in CeX$_{c}$ that the crystal field splitting rapidly decreases at a common rate of $-12.2$ K/GPa. This leads to the increase in the degeneracy of the $f$ state and further enhancement of the Kondo effect. It is shown that the pressure dependent degeneracy of the $f$ state is a key factor to understand the pressure dependence of $T_{N}$, Kondo effect, magnetoresistance, and the peak structure in the temperature dependence of resistivity.

cond-mat.str-el↗

arXiv2015

Pressure-Induced Valence Crossover and Novel Metamagnetic Behavior near the Antiferromagnetic Quantum Phase Transition of YbNi$_{3}$Ga$_{9}$

We report electrical resistivity, ac magnetic susceptibility and X-ray absorption spectroscopy measurements of intermediate valence YbNi$_{3}$Ga$_{9}$ under pressure and magnetic field. We have revealed a characteristic pressure-induced Yb valence crossover within the temperature-pressure phase diagram, and a first-order metamagnetic transition is found below $P_{\rm c}$ $\sim$ 9 GPa where the system undergoes a pressure-induced antiferromagnetic transition. As a possible origin of the metamagnetic behavior, a critical valence fluctuation emerging near the critical point of the first-order valence transition is discussed on the basis of the temperature-field-pressure phase diagram.

cond-mat.str-el↗

arXiv2014

Pressure induced superconductivity on the border of magnetic order in MnP

We report the discovery of superconductivity on the border of long-range magnetic order in the itinerant-electron helimagnet MnP via the application of high pressure. Superconductivity with Tsc~1 K emerges and exists merely near the critical pressure Pc~8 GPa, where the long-range magnetic order just vanishes. The present finding makes MnP the first Mn-based superconductor. The close proximity of superconductivity to a magnetic instability suggests an unconventional pairing mechanism. Moreover, the detailed analysis of the normal-state transport properties evidenced non-Fermi-liquid behavior and the dramatic enhancement of the quasi-particle effective mass near Pc associated with the magnetic quantum fluctuations.

cond-mat.supr-con↗

arXiv2014

Quantum Criticality Based on Large Ising Spins: YbCo$_2$Ge$_4$ with New 1-2-4 Structure Type

We present a new type of quantum critical material YbCo$_2$Ge$_4$, having the largest quantum-critical pseudospin size ever. The YbCo$_2$Ge$_4$-type structure is new, forms in the orthorhombic $Cmcm$ system, and is related to the well-known ThCr$_2$Si$_2$ structure. Heavy rare earth (Tm,Yb,Lu, or Y) members are also possible to be grown. YbCo$_2$Ge$_4$ possesses the Ising-type ground-state doublet, namely the simplest ones of uniaxially up or down, $|\pm \sim 7/2\rangle$. It is clearly manifested through comprehensive resistivity, magnetization, specific heat, and NQR/NMR experiments. Large pseudospin state usually tends to order in simple magnetisms, or hard to be screened by Kondo effect. Therefore, the discovery of the quantum criticality of the fluctuating large spins opens a new door to new-material search and theoretical studies.

cond-mat.str-el↗

arXiv2013

Environmental Effects on the Star Formation Activity at z~0.9 in the COSMOS Field

We investigated the fraction of [OII] emitters in galaxies at z~0.9 as a function of the local galaxy density in the Hubble Space Telescope (HST) COSMOS 2 square degree field. [OII] emitters are selected by the narrow-band excess technique with the NB711-band imaging data taken with Suprime-Cam on the Subaru telescope. We carefully selected 614 photo-z selected galaxies with M_U3500 < -19.31 at z=0.901-0.920, which includes 195 [OII] emitters, to directly compare results with our previous study at z~1.2. We found that the fraction is almost constant at 0.3 Mpc^-2 < Sigma_10th < 10 Mpc^-2. We also checked the fraction of galaxies with blue rest-frame colors of NUV-R < 2 in our photo-z selected sample, and found that the fraction of blue galaxies does not significantly depend on the local density. On the other hand, the semi-analytic model of galaxy formation predicted that the fraction of star-forming galaxies at z~0.9 decreases with increasing the projected galaxy density even if the effects of the projection and the photo-z error in our analysis were taken into account. The fraction of [OII] emitters decreases from ~60% at z~1.2 to ~30% at z~0.9 independent of the galaxy environment. The decrease of the [OII] emitter fraction could be explained mainly by the rapid decrease of the star formation activity in the universe from z~1.2 to z~0.9.

astro-ph.CO↗

arXiv2012

Ionization Source of a Minor-axis Cloud in the Outer Halo of M82

The M82 `cap' is a gas cloud at a projected radius of 11.6 kpc along the minor axis of this well known superwind source. The cap has been detected in optical line emission and X-ray emission and therefore provides an important probe of the wind energetics. In order to investigate the ionization source of the cap, we observed it with the Kyoto3DII Fabry-Perot instrument mounted on the Subaru Telescope. Deep continuum, Ha, [NII]6583/Ha, and [SII]6716,6731/Ha maps were obtained with sub-arcsecond resolution. The superior spatial resolution compared to earlier studies reveals a number of bright Ha emitting clouds within the cap. The emission line widths (< 100 km s^-1 FWHM) and line ratios in the newly identified knots are most reasonably explained by slow to moderate shocks velocities (v_shock = 40--80 km s^-1) driven by a fast wind into dense clouds. The momentum input from the M82 nuclear starburst region is enough to produce the observed shock. Consequently, earlier claims of photoionization by the central starburst are ruled out because they cannot explain the observed fluxes of the densest knots unless the UV escape fraction is very high (f_esc > 60%), i.e., an order of magnitude higher than observed in dwarf galaxies to date. Using these results, we discuss the evolutionary history of the M82 superwind. Future UV/X-ray surveys are expected to confirm that the temperature of the gas is consistent with our moderate shock model.

astro-ph.GA↗

arXiv2012

Microwave Surface Impedance Measurements of the Electronic State and Dissipation of Magnetic Vortices in Superconducting Iron-Based LiFeAs Single Crystals

LiFeAs is one of the iron-based superconductors having multiple gaps with the possible sign reversal. To clarify how those novel natures affect the energy dissipation of magnetic vortices, we investigated the microwave surface impedance of LiFeAs single crystals under finite magnetic fields. The flux-flow resistivity enhanced rapidly at low magnetic fields, which is similar to the case of MgB$_{2}$. This is probably the consequence of the multiple-gap nature and the gap anisotropy. This suggest that the sign-reversal is not important for the flux-flow even for multiple-gap superconductors. As for the electronic state, the vortex core of LiFeAs turned out to be "moderately clean". Furthermore, the mean free path inside the vortex core was much shorter than that outside, and was close to the core radius. These results strongly suggest a process specific to the core boundary is important for a scattering mechanism inside the vortex core.

cond-mat.supr-con↗

arXiv2012

Post-starburst Tidal Tails in the Archetypical Ultra Luminous Infrared Galaxy Arp 220

We present our new deep optical imaging and long-slit spectroscopy for Arp 220 that is the archetypical ULIRG in the local universe. Our sensitive Ha imaging has newly revealed large-scale, Ha absorption, i.e., post-starburst regions in this merger; one is found in the eastern superbubble and the other is in the two tidal tails that are clearly reveled in our deep optical imaging. The size of Ha absorption region in the eastern bubble is 5 kpc x 7.5 kpc and the observed Ha equivalent widths are ~2 A +- 0.2 A. The sizes of the northern and southern Ha-absorption tidal tails are ~5 kpc x 10 kpc and ~6 kpc x 20 kpc, respectively. The observed Ha equivalent widths range from 4 A to 7 A. In order to explain the presence of the two post-starburst tails, we suggest a possible multiple-merger scenario for Arp 220 in which two post-starburst disk-like structures merged into one, and then caused the two tails. This favors that Arp 220 is a multiple merging system composed of four or more galaxies, arising from a compact group of galaxies. Taking our new results into account, we discuss a star formation history in the last 1 Gyr in Arp 220.

astro-ph.CO↗

arXiv2012

Scanning Tunneling Microscopy/Spectroscopy of Vortices in LiFeAs

We investigate vortices in LiFeAs using scanning tunneling microscopy/spectroscopy. Zero-field tunneling spectra show two superconducting gaps without detectable spectral weight near the Fermi energy, evidencing fully-gapped multi-band superconductivity. We image vortices in a wide field range from 0.1 T to 11 T by mapping the tunneling conductance at the Fermi energy. A quasi-hexagonal vortex lattice at low field contains domain boundaries which consist of alternating vortices with unusual coordination numbers of 5 and 7. With increasing field, the domain boundaries become ill-defined, resulting in a uniformly disordered vortex matter. Tunneling spectra taken at the vortex center are characterized by a sharp peak just below the Fermi energy, apparently violating particlehole symmetry. The image of each vortex shows energy-dependent 4-fold anisotropy which may be associated with the anisotropy of the Fermi surface. The vortex radius shrinks with decreasing temperature and becomes smaller than the coherence length estimated from the upper critical field. This is direct evidence of the Kramer-Pesch effect expected in a clean superconductor.

cond-mat.supr-con↗

arXiv2012

Determination of spin Hamiltonian in the Ni$_4$ magnetic molecule

Magnetic excitations in a Ni$_4$ magnetic molecule were investigated by inelastic neutron scattering and bulk susceptibility ($χ_\text{bulk}$) techniques. The magnetic excitation spectrum obtained from the inelastic neutron scattering experiments exhibits three modes at energy transfers of $\hbarω=0.5$, 1.35, and 1.6 meV. We show that the energy, momentum, and temperature dependences of the inelastic neutron scattering data and $χ_\text{bulk}$ can be well reproduced by an effective spin Hamiltonian consisted of intra-molecule exchange interactions, a single-ionic anisotropy, biquadratic interactions, and Zeeman term. Under a hydrostatic pressure, the bulk magnetization decreases with increasing pressure, which along with the biquadratic term indicates spin-lattice coupling present in this system.

cond-mat.str-el↗

arXiv2011

Pressure-induced changes in the magnetic and valence state of EuFe2As2

We present the results of electrical resistivity, ac specific heat, magnetic susceptibility, X-ray absorption spectroscopy (XAS) and X-ray magnetic circular dichroism (XMCD) of the ternary iron arsenide EuFe2As2 single crystal under pressure. Applying pressure leads to a continuous suppression of the antiferromagnetism associated with Fe moments and the antiferromagnetic transition temperature becomes zero in the vicinity of a critical pressure Pc ~2.5-2.7 GPa. Pressure-induced re-entrant superconductivity, which is highly sensitive to the homogeneity of the pressure, only appears in the narrow pressure region in the vicinity of Pc due to the competition between superconductivity and the antiferromagnetic ordering of Eu2+ moments. The antiferromagnetic state of Eu2+ moments changes to the ferromagnetic state above 6 GPa. We also found that the ferromagnetic order is suppressed with further increasing pressure, which is connected with a valence change of Eu ions.

cond-mat.supr-con↗