arXiv subjects

K. Matsui

Publications and source records attributed to K. Matsui.

At least 19 recordsLinked to original sources

arXiv2025

High-field NMR study of field-induced states in Pb(TiO)Cu$_4$(PO$_4$)$_4$

The square cupola antiferromagnet Pb(TiO)Cu$_4$(PO$_4$)$_4$ exhibits the intriguing magnetoelectric responses arising from the consecutive change in the magnetic quadrupolar-type configuration of magnetic moments under external magnetic fields higher than 15 T. To clarify the high-field magnetic structures in Pb(TiO)Cu$_4$(PO$_4$)$_4$, an NMR measurement was performed in pulsed fields up to 32.2 T significantly extending the field range accessible by superconducting magnets. The double-peak structure of NMR spectra emerging above 29 T applied along the [001] direction evidences the successive magnetic transitions. The field dependence of NMR spectra was analyzed on the basis of cluster mean-field theory, which allows us to propose possible magnetic structures for the high-field magnetic states.

cond-mat.str-el↗

arXiv2025

Neutron emission following nuclear muon capture on palladium isotopes

The energy spectra of the neutrons emitted following nuclear muon capture on palladium isotopes ($A=104$, 105, 106, 108, and 110) were measured using isotopically enriched target. \item[Method] The experiment was performed at the MuSIC-M1 beamline at the Research Center for Nuclear Physics (RCNP), Osaka University. The neutrons and $\gamma$ rays were detected with twenty-one liquid scintillators and BaF$_2$ detectors. The time-of-flight method was used to determine the neutron energy. \item[Results] Neutron energy spectra from 1\,MeV up to 20\,MeV were measured for five palladium isotopes, providing the first systematic data in the $A\sim100$ region. The spectral shapes were compared with the previous measurement for heavy nuclei and theoretical calculations. The neutron-neutron opening angle distribution was also measured and an indication of small angle correlation was found. \item[Conclusions] The spectral shape below 4\,MeV was well explained consistently with the previous measurement by the evaporation model introducing a mass number scaling. The neutron energy spectrum around 10\,MeV plays a key role in understanding the dynamics of the nuclear muon capture reaction because it is the result of the transition from the direct and pre-equilibrium neutron emission onto the evaporation process.

nucl-ex↗

arXiv2025

Impact of newly measured $\beta$\nobreakdash-delayed neutron emitters around \myisoSimp{78}{Ni} on light element nucleosynthesis in the neutrino-wind following a neutron star merger

Neutron emission probabilities and half-lives of 37 beta-delayed neutron emitters from 75Ni to 92Br were measured at the RIKEN Nishina Center in Japan, including 11 one-neutron and 13 two-neutron emission probabilities and 6 half-lives measured for the first time, which supersede theoretical estimates. These nuclei lie in the path of the weak r-process occurring in neutrino-driven winds from the accretion disk formed after the merger of two neutron stars, synthesizing elements in the A~80 abundance peak. The presence of such elements dominates the accompanying kilonova emission over the first few days and has been identified in the AT2017gfo event, associated with the gravitational wave detection GW170817. Abundance calculations based on over 17000 simulated trajectories describing the evolution of matter properties in the merger outflows show that the new data lead to an increase of 50-70 percent in the abundance of Y, Zr, Nb, and Mo. This enhancement is large compared to the scatter of relative abundances observed in old very metal-poor stars and is therefore significant in the comparison with other possible astrophysical processes contributing to light-element production. These results underline the importance of including experimental decay data for very neutron-rich beta-delayed neutron emitters into r-process models.

nucl-ex↗

arXiv2021

Exploration of increasing drivers trust in a semi-autonomous vehicle through real time visualizations of collaborative driving dynamic

The Thinking Wave is an ongoing development of visualization concepts showing the real-time effort and confidence of semi-autonomous vehicle (AV) systems. Offering drivers access to this information can inform their decision making, and enable them to handle the situation accordingly and takeover when necessary. Two different visualizations have been designed, Concept one, Tidal, demonstrates the AV systems effort through intensified activity of a simple graphic which fluctuates in speed and frequency. Concept two, Tandem, displays the effort of the AV system as well as the handling dynamic and shared responsibility between the driver and the vehicle system. Working collaboratively with mobility research teams at the University of Tokyo, we are prototyping and refining the Thinking Wave and its embodiments as we work towards building a testable version integrated into a driving simulator. The development of the thinking wave aims to calibrate trust by increasing the drivers knowledge and understanding of vehicle handling capacity. By enabling transparent communication of the AV systems capacity, we hope to empower AV-skeptic drivers and keep over-trusting drivers on alert in the case of an emergency takeover situation, in order to create a safer autonomous driving experience.

cs.HC↗

arXiv2021

Isomeric states in neutron-rich nuclei around $N = 40$

Neutron-rich nuclei in the vicinity of the $N=40$ island of inversion are characterized by shell evolution and exhibit deformed ground states. In several nuclei isomeric states have been observed and attributed to excitations to the intruder neutron $1g_{9/2}$ orbital. In the present study we searched for isomeric states in nuclei around $N=40$, $Z=22$ produced by projectile fragmentation at RIBF. Delayed $\gamma$ rays were detected by the EURICA germanium detector array. High statistics data allowed for an updated decay scheme of $^{60}$V. The lifetime of an isomeric state in $^{64}$V was measured for the first time in the present experiment. A previously unobserved isomeric state was discovered in $^{58}$Sc. The measured lifetime suggests a parity changing transition, originating from an odd number of neutrons in the $1g_{9/2}$ orbital. The nature of the isomeric state in $^{58}$Sc is thus different from isomers in the less exotic V and Sc nuclei.

nucl-ex↗

arXiv2021

Persistence of the ${Z=28}$ shell gap in ${A=75}$ isobars: Identification of a possible ${(1/2^-)}$ ${\mu}$s isomer in ${^{75}}$Co and ${\beta}$ decay to ${^{75}}$Ni

Background: The evolution of shell structure around doubly magic exotic nuclei is of great interest in nuclear physics and astrophysics. In the `southwest' region of $^{78}$Ni, the development of deformation might trigger a major shift in our understanding of explosive nucleosynthesis. To this end, new spectroscopic information on key close-lying nuclei is very valuable. Purpose: We intend to measure the isomeric and $\beta$ decay of $^{75}$Co, with one-proton and two-neutron holes relative to $^{78}$Ni, to access new nuclear structure information in $^{75}$Co and its $\beta$-decay daughters $^{75}$Ni and $^{74}$Ni. Methods: The nucleus $^{75}$Co is produced in relativistic in-flight fission reactions of $^{238}$U at the Radioactive Ion Beam Factory in the RIKEN Nishina Center. Its isomeric and $\beta$ decay are studied exploiting the BigRIPS and EURICA setups. Results: We obtain partial $\beta$-decay spectra for $^{75}$Ni and $^{74}$Ni, and report a new isomeric transition in $^{75}$Co. The energy [$E_{\gamma}=1914(2)$ keV] and half-life [$t_{1/2}=13(6)$ $\mu$s] of the delayed $\gamma$ ray lend support for the existence of a $J^{\pi}=(1/2^-)$ isomeric state at 1914(2) keV. A comparison with PFSDG-U shell-model calculations provides a good account for the observed states in $^{75}$Ni, but the first calculated $1/2^-$ level in $^{75}$Co, a prolate $K=1/2$ state, is predicted about 1 MeV below the observed $(1/2^-)$ level. Conclusions: The spherical-like structure of the lowest-lying excited states in $^{75}$Ni is proved. In the case of $^{75}$Co, the results suggest that the dominance of the spherical configurations over the deformed ones might be stronger than expected below $^{78}$Ni. Further experimental efforts to discern the nature of the $J^{\pi}=(1/2^-)$ isomer are necessary.

nucl-ex↗

arXiv2019

$^{78}$Ni revealed as a doubly magic stronghold against nuclear deformation

Nuclear magic numbers, which emerge from the strong nuclear force based on quantum chromodynamics, correspond to fully occupied energy shells of protons, or neutrons inside atomic nuclei. Doubly magic nuclei, with magic numbers for both protons and neutrons, are spherical and extremely rare across the nuclear landscape. While the sequence of magic numbers is well established for stable nuclei, evidence reveals modifications for nuclei with a large proton-to-neutron asymmetry. Here, we provide the first spectroscopic study of the doubly magic nucleus $^{78}$Ni, fourteen neutrons beyond the last stable nickel isotope. We provide direct evidence for its doubly magic nature, which is also predicted by ab initio calculations based on chiral effective field theory interactions and the quasi-particle random-phase approximation. However, our results also provide the first indication of the breakdown of the neutron magic number 50 and proton magic number 28 beyond this stronghold, caused by a competing deformed structure. State-of-the-art phenomenological shell-model calculations reproduce this shape coexistence, predicting further a rapid transition from spherical to deformed ground states with $^{78}$Ni as turning point.

nucl-ex↗

arXiv2019

First spectroscopy of 61Ti and the transition to the Island of Inversion at N = 40

Isomeric states in 59,61Ti have been populated in the projectile fragmentation of a 345 AMeV 238U beam at the Radioactive Isotope Beam Factory. The decay lifetimes and delayed gamma-ray transitions were measured with the EURICA array. Besides the known isomeric state in 59Ti, two isomeric states in 61Ti are observed for the first time. Based on the measured lifetimes, transition multipolarities as well as tentative spins and parities are assigned. Large-scale shell model calculations based on the modified LNPS interaction show that both 59Ti and 61Ti belong to the Island of Inversion at N=40 with ground state configurations dominated by particle-hole excitations to the g_9/2 and d_5/2 orbits.

nucl-ex↗

arXiv2018

Low temperature magnetism of gold nano particles contained in electrochemical sugar recognition system

Low temperature magnetic properties were investigated on the gold nano particles (GNP) with an average size of 11.5 nm, assembled with molecules of ruthenium complex (Ru0) and phenylboronic acid (B0) by the proton nuclear resonance (1H-NMR) and susceptibility measurements. The temperature dependence of the NMR shift and the uniform susceptibility was described as the sum of the Curie-Weiss term and a positive constant term. From the former, the average number of Ru0 on each GNP was estimated to be 118, which is 23 % of the calculation. The finite positive constant term shows a clear contrast with the well-known fact that the bulk gold is diamagnetic. Finally, a disappearance of the motional narrowing effect in the proton NMR spectra below 60 K indicates that the wavering motion of Ru0 complexes on GNP at room temperature is frozen at low temperatures.

cond-mat.mes-hall↗

arXiv2018

Commissioning of the BRIKEN detector for the measurement of very exotic beta-delayed neutron emitters

A new detection system has been installed at the RIKEN Nishina Center (Japan) to investigate decay properties of very neutron-rich nuclei. The setup consists of three main parts: a moderated neutron counter, a detection system sensitive to the implantation and decay of radioactive ions, and gamma-ray detectors. We describe here the setup, the commissioning experiment and some selected results demonstrating its performance for the measurement of half-lives and beta-delayed neutron emission probabilities. The methodology followed in the analysis of the data is described in detail. Particular emphasis is placed on the correction of the accidental neutron background.

physics.ins-det↗

arXiv2018

Is Seniority a Partial Dynamic Symmetry in the First $νg_{9/2}$ Shell?

The low-lying structures of the midshell $νg_{9/2}$ Ni isotopes $^{72}$Ni and $^{74}$Ni have been investigated at the RIBF facility in RIKEN within the EURICA collaboration. Previously unobserved low-lying states were accessed for the first time following $β$ decay of the mother nuclei $^{72}$Co and $^{74}$Co. As a result, we provide a complete picture in terms of the seniority scheme up to the first $(8^+)$ levels for both nuclei. The experimental results are compared to shell-model calculations in order to define to what extent the seniority quantum number is preserved in the first neutron $g_{9/2}$ shell. We find that the disappearance of the seniority isomerism in the $(8^+_1)$ states can be explained by a lowering of the seniority-four $(6^+)$ levels as predicted years ago. For $^{74}$Ni, the internal de-excitation pattern of the newly observed $(6^+_2)$ state supports a restoration of the normal seniority ordering up to spin $J=4$. This property, unexplained by the shell-model calculations, is in agreement with a dominance of the single-particle spherical regime near $^{78}$Ni.

nucl-ex↗

arXiv2018

Spectroscopy of nuclei around $^{100}$Sn populated via two-neutron knockout reactions

We report on the in-beam gamma spectroscopy of $^{102}$Sn and $^{100}$Cd produced via two-neutron removal from carbon and CH$_2$ targets at about 150 MeV/nucleon beam energy. New transitions assigned to the decay of a second 2$^+$ excited state at 2470(60) keV in $^{102}$Sn were observed. Two-neutron removal cross sections from $^{104}$Sn and $^{102}$Cd have been extracted. The enhanced cross section to the 2$^+_2$ in $^{102}$Sn populated via the $(p,p2n)$ reaction is traced back to an increase of shell-model structure overlaps, consistent with the hypothesis that the proton-induced two-deeply-bound-nucleon removal mechanism is of direct nature.

nucl-ex↗

arXiv2017

Spin dynamics in the high-field phases of volborthite

We report single-crystal 51V NMR studies on volborthite Cu3V2O7(OH)2 2H2O, which is regarded as a quasi-two-dimensional frustrated magnet with competing ferromagnetic and antiferromagnetic interactions. In the 1/3 magnetization plateau above 28 T, the nuclear spin-lattice relaxation rate 1/T1 indicates an excitation gap with a large effective g factor in the range of 4.6-5.9, pointing to magnon bound states. Below 26 T where the gap has closed, the NMR spectra indicate small internal fields with a Gaussian-like distribution, whereas 1/T1 shows a power-law-like temperature dependence in the paramagnetic state, which resembles a slowing down of spin fluctuations associated with magnetic order. We discuss the possibility of an exotic spin state caused by the condensation of magnon bound states below the magnetization plateau.

cond-mat.str-el↗

arXiv2017

Structure of 55Sc and development of the N=34 subshell closure

The low-lying structure of $^{55}$Sc has been investigated using in-beam $γ$-ray spectroscopy with the $^{9}$Be($^{56}$Ti,$^{55}$Sc+$γ$)$X$ one-proton removal and $^{9}$Be($^{55}$Sc,$^{55}$Sc+$γ$)$X$ inelastic-scattering reactions at the RIKEN Radioactive Isotope Beam Factory. Transitions with energies of 572(4), 695(5), 1539(10), 1730(20), 1854(27), 2091(19), 2452(26), and 3241(39) keV are reported, and a level scheme has been constructed using $γγ$ coincidence relationships and $γ$-ray relative intensities. The results are compared to large-scale shell-model calculations in the $sd$-$pf$ model space, which account for positive-parity states from proton-hole cross-shell excitations, and to it ab initio shell-model calculations from the in-medium similarity renormalization group that includes three-nucleon forces explicitly. The results of proton-removal reaction theory with the eikonal model approach were adopted to aid identification of positive-parity states in the level scheme; experimental counterparts of theoretical $1/2^{+}_{1}$ and $3/2^{+}_{1}$ states are suggested from measured decay patterns. The energy of the first $3/2^{-}$ state, which is sensitive to the neutron shell gap at the Fermi surface, was determined. The result indicates a rapid weakening of the $N=34$ subshell closure in $pf$-shell nuclei at $Z>20$, even when only a single proton occupies the $πf_{7/2}$ orbital.

nucl-ex↗

arXiv2016

Possible quantum liquid crystal phases of helium monolayers

The second-layer phase diagrams of $^4$He and $^3$He adsorbed on graphite are investigated. Intrinsically rounded specific-heat anomalies are observed at 1.4 and 0.9 K, respectively, over extended density regions in between the liquid and incommensurate solid phases. They are identified to anomalies associated with the Kosterlitz-Thouless-Halperin-Nelson-Young type two-dimensional melting. The prospected low temperature phase (C2 phase) is a commensurate phase or a $\textit{quantum hexatic}$ phase with quasi-bond-orientational order, both containing $\textit{zero}$-$\textit{point}$ defectons. In either case, this would be the first atomic realization of the $\textit{quantum liquid crystal}$, a new state of matter. From the large enhancement of the melting temperature over $^3$He, we propose to assign the observed anomaly of $^4$He-C2 phase at 1.4 K to the hypothetical supersolid or superhexatic transition.

cond-mat.other↗

arXiv2013

Intermediate-energy Coulomb excitation of 104Sn: Moderate E2 strength decrease approaching 100Sn

The reduced transition probability B(E2) of the first excited 2+ state in the nucleus 104Sn was measured via Coulomb excitation in inverse kinematics at intermediate energies. A value of 0.163(26) e^2b^2 was extracted from the absolute cross-section on a Pb target, while the method itself was verified with the stable 112Sn isotope. Our result deviates significantly from the earlier reported value of 0.10(4) e^2b^2 and corresponds to a moderate decrease of excitation strength relative to the almost constant values observed in the proton-rich, even-A 106-114Sn isotopes. Present state-of-the-art shell-model predictions, which include proton and neutron excitations across the N=Z=50 shell closures as well as standard polarization charges, underestimate the experimental findings

nucl-ex↗

arXiv2012

Preliminary Heat Capacity and Vapor Pressure Measurements of 2D 4He on ZYX Graphite

We report preliminary heat capacity and vapor pressure measurements of the first and second layers of 4He adsorbed on ZYX graphite. ZYX is known to have much better crystallinity than Grafoil, the most commonly-used exfoliated graphite substrate, such as a ten-times larger platelet size. This allows us to distinguish different phases in 2D helium-4 much more clearly and may provide qualitatively different insights into this system. We found a significantly asymmetric density-dependence of the heat-capacity peak associated with the 1/3 phase formation comparing with that obtained with Grafoil. The 2nd-layer promotion density is determined as 11.8+-0.3 nm-2 from the heat-capacity measurement of low density samples in the 2nd layer and vapor pressure measurement.

cond-mat.other↗

arXiv2012

Millikelvin LEED apparatus: a feasibility study

A low-energy electron diffraction (LEED) apparatus which works at temperatures down to about 100 mK is designed to obtain structural information of 2D helium on graphite. This very low temperature system can be realized by reducing the thermal inflow from the LEED optics to the sample which is cooled by cryogen-free dilution refrigerator. The atomic scattering factor of He is also estimated using a kinematical model, which suggests that the diffraction signal from He atom can well be obtained by using a delay-line detector instead of a fluorescent screen.

cond-mat.mtrl-sci↗