arXiv subjects

K. Miyagawa

Publications and source records attributed to K. Miyagawa.

At least 37 records · Page 2Linked to original sources

arXiv2014

Anisotropic charge dynamics in the quantum spin-liquid candidate $κ$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$

We have in detail characterized the anisotropic charge response of the dimer Mott insulator $κ$-(BEDT-TTF)$_2$\-Cu$_2$(CN)$_3$ by dc conductivity, Hall effect and dielectric spectroscopy. At room temperature the Hall coefficient is positive and close to the value expected from stoichiometry; the temperature behavior follows the dc resistivity $ρ(T)$. Within the planes the dc conductivity is well described by variable-range hopping in two dimensions; this model, however, fails for the out-of-plane direction. An unusually broad in-plane dielectric relaxation is detected below about 60 K; it slows down much faster than the dc conductivity following an Arrhenius law. At around 17 K we can identify a pronounced dielectric anomaly concomitantly with anomalous features in the mean relaxation time and spectral broadening. The out-of-plane relaxation, on the other hand, shows a much weaker dielectric anomaly; it closely follows the temperature behavior of the respective dc resistivity. At lower temperatures, the dielectric constant becomes smaller both within and perpendicular to the planes; also the relaxation levels off. The observed behavior bears features of relaxor-like ferroelectricity. Because heterogeneities impede its long-range development, only a weak tunneling-like dynamics persists at low temperatures. We suggest that the random potential and domain structure gradually emerge due to the coupling to the anion network.

cond-mat.str-el↗

arXiv2014

Mottness in a doped organic superconductor

We report the pressure study of a doped organic superconductor with Hall coefficient and conductivity measurements. We find that maximally enhanced superconductivity and a non-Fermi liquid appear around a certain pressure where mobile carriers increase critically, suggesting a possible quantum phase transition between strongly and weakly correlated regimes. Our description extends the conventional picture of a Mott metal-insulator transition at half filling to the case of a doped Mott insulator with tunable correlation.

cond-mat.mtrl-sci↗

arXiv2014

Evidence of Andreev bound states as a hallmark of the FFLO phase in $κ$-(BEDT-TTF)$_2$Cu(NCS)$_2$

Superconductivity is a quantum phenomena arising, in its simplest form, from pairing of fermions with opposite spin into a state with zero net momentum. Whether superconductivity can occur in fermionic systems with unequal number of two species distinguished by spin, atomic hyperfine states, flavor, presents an important open question in condensed matter, cold atoms, and quantum chromodynamics, physics. In the former case the imbalance between spin-up and spin-down electrons forming the Cooper pairs is indyced by the magnetic field. Nearly fifty years ago Fulde, Ferrell, Larkin and Ovchinnikov (FFLO) proposed that such imbalanced system can lead to exotic superconductivity in which pairs acquire finite momentum. The finite pair momentum leads to spatially inhomogeneous state consisting of of a periodic alternation of "normal" and "superconducting" regions. Here, we report nuclear magnetic resonance (NMR) measurements providing microscopic evidence for the existence of this new superconducting state through the observation of spin-polarized quasiparticles forming so-called Andreev bound states.

cond-mat.supr-con↗

arXiv2014

Systematic Variations in the Charge-Glass-Forming Ability of Geometrically Frustrated $θ$-(BEDT-TTF)$_2X$ Organic Conductors

The critical cooling rate $R_{\rm c}$ above which charge ordering is kinetically avoided upon cooling, which results in charge-glass formation, was investigated for the geometrically frustrated system $θ$-(BEDT-TTF)$_2X$. X-ray diffraction experiments revealed that $θ$-(BEDT-TTF)$_2$TlCo(SCN)$_4$ exhibits a horizontally charge-ordered state, and kinetic avoidance of this state requires rapid cooling of faster than 150 K/min. This value is markedly higher than that reported for two other isostructural $θ$-type compounds, thus demonstrating the lower charge-glass-forming ability of $X$ $=$ TlCo(SCN)$_4$. In accounting for the systematic variations of $R_{\rm c}$ among the three $θ$-(BEDT-TTF)$_2X$, we found that stronger charge frustration leads to superior charge-glass former. Our results suggest that charge frustration tends to slow the kinetics of charge ordering.

cond-mat.str-el↗

arXiv2014

Emergence of non-equilibrium charge dynamics in a charge-cluster glass

Non-equilibrium charge dynamics, such as cooling-rate-dependent charge vitrification and physical aging, have been demonstrated for a charge-cluster glass in $θ$-(BEDT-TTF)$_2$CsZn(SCN)$_4$ using electron transport measurements. The temperature evolution of the relaxation time obeys the Arrhenius law, indicating that the glass-forming charge liquid can be classified as a "`strong" liquid in the scheme of canonical structural-glass formers. X-ray diffuse scattering further reveals that the spatial growth of charge clusters in the charge liquid is frozen below the glass transition temperature, indicating an intrinsic relationship between dynamics and structure in the charge-cluster glass.

cond-mat.str-el↗

arXiv2013

Charge-cluster glass in an organic conductor

Geometrically frustrated spin systems often do not exhibit long-range ordering, resulting in either quantum-mechanically disordered states, such as quantum spin liquids, or classically disordered states, such as spin ices or spin glasses. Geometric frustration may play a similar role in charge ordering, potentially leading to unconventional electronic states without long-range order; however, there are no previous experimental demonstrations of this phenomenon. Here, we show that a charge-cluster glass evolves upon cooling in the absence of long-range charge ordering for an organic conductor with a triangular lattice, theta-(BEDT-TTF)2RbZn(SCN)4. A combination of time-resolved transport measurements and x-ray diffraction reveal that the charge-liquid phase has charge clusters that fluctuate extremely slowly (<10-100 Hz) and heterogeneously. Upon further cooling, the cluster dynamics freeze, and a charge-cluster glass is formed. Surprisingly, these observations correspond to recent ideas regarding the structural glass formation of supercooled liquids, indicating that a glass-forming charge liquid relates correlated-electron physics to glass physics in soft matter.

cond-mat.str-el↗

arXiv2012

Precise calculation of the two-step process for K- d -> pi Sigma N in the Lambda (1405) resonance region

The reaction K- d -> pi Sigma N is investigated taking into account single scattering and the two-step process due to Kbar N -> pi Sigma rescattering. The influence of some common approximations are examined. It is found that the treatment of the kinematics in the Green's function that appears in the loop integral of the rescattering process has a rather strong impact on the resulting lineshape of the pi Sigma invariant mass spectrum. Specifically, a calculation with correct kinematics where the three-body unitarity cut due to the nK- p threshold occurs at the physical value yields a pronounced peak in the invariant mass spectrum at this threshold and, at the same time, suppresses the signal in the region of the Lambda(1405) resonance. On the other hand, an approximation applied in past calculations shifts that threshold down and, consequently, leads to an accidental and therefore erroneous enhancement of the signal of the Lambda(1405) in the pi Sigma invariant mass spectrum.

nucl-th↗

arXiv2011

Role of the $K_1$ meson in $K^0$ photoproduction off the deuteron

Neutral kaon photoproduction off the nucleon and deuteron has been reinvestigated by utilizing the new experimental data on both targets. An isobar model for elementary operator and impulse approximation for the reaction on the deuteron have been used. The available free parameters in the elementary model have been extracted from both elementary and deuteron data. In contrast to the elementary reaction, fitting the deuteron data requires an inclusion of weighting factor. The result indicates that the angular distribution of the elementary $K^0Λ$ process does not show backward peaking behavior.

nucl-th↗

arXiv2010

$^{13}$C NMR Study on Zero-Gap State in the Organic Conductor $θ$-(BEDT-TTF)$_{2}$I$_{3}$ under Pressure

We present the results of our $^{13}$C NMR study of the quasi-two-dimensional organic conductor $θ$-(BEDT-TTF)$_2$I$_{3}$ under pressure, which is suggested to be a zero-gap conductor by transport measurements. We found that NMR spin shift is proportional to $T$ and that spin-lattice relaxation rate follows the power law $T^α$ ($α=3 \sim 4$), where $T$ is the temperature. This behavior is consistent with the cone-like band dispersion and provides microscopic evidence for the realization of the zero-gap state in the present material under pressure.

cond-mat.mes-hall↗

arXiv2009

Neutral kaon photoproduction on the deuteron

Neutral kaon photoproduction on the deuteron has been investigated by including the final state effects and compared with the experimental data. Comparison shows that the models used in this calculation can reproduce the data in the $Σ$ channel regions fairly well but still give over predictions in the $Λ$ channel. It seems that the tensor target asymmetries are more suitable for studying the final state effects. The extractions of the elementary photoproduction amplitude are also demonstrated.

nucl-th↗

arXiv2009

Field-induced staggered magnetic moment in the quasi-two-dimensional organic Mott insulator $κ$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Cl

We investigated the magnetism under a magnetic field in the quasi-two-dimensional organic Mott insulator $κ$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Cl through magnetization and $^{13}$C-NMR measurements. We found that in the nominally paramagnetic phase (i.e., above Néel temperature) the field-induced local moments have a staggered component perpendicular to the applied field. As a result, the antiferromagnetic transition well defined at a zero field becomes crossover under a finite field. This unconventional behavior is qualitatively reproduced by the molecular-field calculation for Hamiltonian including the exchange, Dzyaloshinsky-Moriya (DM), and Zeeman interactions. This calculation also explains other unconventional magnetic features in $κ$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Cl reported in the literature. The present results highlight the importance of the DM interaction in field-induced magnetism in a nominally paramagnetic phase, especially in low-dimensional spin systems.

cond-mat.str-el↗

arXiv2008

NMR Evidence for Antiferromagnetic Transition in the Single-Component Molecular Conductor, [Au(tmdt)_{2}] at 110 K

We present the results of a ^{1}H NMR study of the single-component molecular conductor, [Au(tmdt)_{2}]. A steep increase in the NMR line width and a peak formation of the nuclear spin-lattice relaxation rate, 1/T_{1}, were observed at around 110 K. This behavior provides clear and microscopic evidences for a magnetic phase transition at considerably high temperature among organic conductors. The observed variation in 1/T_{1} with respect to temperature indicates the highly correlated nature of the metallic phase.

cond-mat.str-el↗

arXiv2007

Addendum: Triton and hypertriton binding energies calculated from SU_6 quark-model baryon-baryon interactions

Previously we calculated the binding energies of the triton and hypertriton, using an SU_6 quark-model interaction derived from a resonating-group method of two baryon clusters. In contrast to the previous calculations employing the energy-dependent interaction kernel, we present new results using a renormalized interaction, which is now energy independent and reserves all the two-baryon data. The new binding energies are slightly smaller than the previous values. In particular the triton binding energy turns out to be 8.14 MeV with a charge-dependence correction of the two-nucleon force, 190 keV, being included. This indicates that about 350 keV is left for the energy which is to be accounted for by three-body forces.

nucl-th↗

arXiv2007

Lambda-N scattering length from the reaction gamma d -> K^+ Lambda n

The perspects of utilizing the strangeness-production reaction gamma d -> K^+ Lambda n for the determination of the Lambda n low-energy scattering parameters are investigated. The spin observables that need to be measured in order to isolate the Lambda n singlet (1S0) and triplet (3S1) states are identified. Possible kinematical regions where the extraction of the Lambda n scattering lengths might be feasible are discussed.

nucl-th↗

arXiv2006

Polarization observables in exclusive kaon photoproduction on the deuteron

Single and double polarization observables for kaon photoproduction on the deuteron are studied theoretically with modern hyperon-nucleon forces. The kinematical region of the kaon scattered forward with large momentum is thoroughly investigated where either the quasifree scattering leading to the kaon and hyperon or the final-state interaction between hyperon and nucleon are expected. The quasifree scatterings show characteristic peaks in the inclusive cross sections. The final-state interaction effects are significant, especially around the Lambda-N and Sigma-N thresholds. The double polarization C_z is found to be sensitive to the final-state interaction effects. Precise data would help to clarify the property of the Lambda-N--Sigma-N interaction and also help to extract the information on the elementary amplitude from the quasifree scattering region.

nucl-th↗

arXiv2006

K0 photoproduction on the deuteron and the extraction of the elementary amplitude

The photoproduction of K0 on the deuteron has been investigated with the inclusion of YN and KN final-state interaction (FSI), as well as the pion-mediated process gamma d --> pi NN --> KYN. The YN rescattering effects for the inclusive cross section are found to be large in the threshold regions. Polarization observables show sizable FSI effects at larger kaon and hyperon angles. It is shown that the extraction of the elementary gamma N --> KY amplitude is possible in the quasi-free scattering region where FSI effects are negligible. Furthermore, the cross sections in this region are large, indicating that measurements in this kinematical region are favored.

nucl-th↗

arXiv2006

Unconventional critical behaviour in a quasi-two-dimensional organic conductor

Changing the interactions between particles in an ensemble-by varying the temperature or pressure, for example-can lead to phase transitions whose critical behaviour depends on the collective nature of the many-body system. Despite the diversity of ingredients, which include atoms, molecules, electrons and their spins, the collective behaviour can be grouped into several families (called 'universality classes') represented by canonical spin models1. One kind of transition, the Mott transition2, occurs when the repulsive Coulomb interaction between electrons is increased, causing wave-like electrons to behave as particles. In two dimensions, the attractive behaviour responsible for the superconductivity in high-transition temperature copper oxide3,4 and organic5-7 compounds appears near the Mott transition, but the universality class to which two-dimensional, repulsive electronic systems belongs remains unknown. Here we present an observation of the critical phenomena at the pressure-induced Mott transition in a quasi-two-dimensional organic conductor using conductance measurements as a probe. We find that the Mott transition in two dimensions is not consistent with known universality classes, as the observed collective behaviour has previously not been seen. This peculiarity must be involved in any emergent behaviour near the Mott transition in two dimensions.

cond-mat.str-el↗

arXiv2005

Mott Transition from a Spin Liquid to a Fermi Liquid in the Spin-Frustrated Organic Conductor kappa-(ET)2Cu2(CN)3

Pressure-temperature phase diagram of the organic Mott insulator $κ$-(ET)$_2$Cu$_2$(CN)$_3$, a model system of the spin liquid on triangular lattice, has been investigated by $^1$H NMR and resistivity measurements. The spin-liquid phase is persistent before the Mott transition to the metal or superconducting phase under pressure. At the Mott transition, the spin fluctuations are rapidly suppressed and the Fermi-liquid features are observed in the temperature dependence of the spin-lattice relaxation rate and resistivity. The characteristic curvature of Mott boundary in the phase diagram highlights a crucial effect of the spin frustration on the Mott transition.

cond-mat.str-el↗