Searcharxiv⌕ Search

arXiv subjects

K. Richter

Publications and source records attributed to K. Richter.

36 records · Page 2Linked to original sources

Thermopower of a superconducting single-electron transistor

We present a linear-response theory for the thermopower of a single-electron transistor consisting of a superconducting island weakly coupled to two normal-conducting leads (NSN SET). The thermopower shows oscillations with the same periodicity as the conductance and is rather sensitive to the size of the superconducting gap. In particular, the previously studied sawtooth-like shape of the thermopower for a normal-conducting single-electron device is qualitatively changed even for small gap energies.

cond-mat.mes-hall↗

Semiclassical form factor for spectral and matrix element fluctuations of multi-dimensional chaotic systems

We present a semiclassical calculation of the generalized form factor which characterizes the fluctuations of matrix elements of the quantum operators in the eigenbasis of the Hamiltonian of a chaotic system. Our approach is based on some recently developed techniques for the spectral form factor of systems with hyperbolic and ergodic underlying classical dynamics and f=2 degrees of freedom, that allow us to go beyond the diagonal approximation. First we extend these techniques to systems with f>2. Then we use these results to calculate the generalized form factor. We show that the dependence on the rescaled time in units of the Heisenberg time is universal for both the spectral and the generalized form factor. Furthermore, we derive a relation between the generalized form factor and the classical time-correlation function of the Weyl symbols of the quantum operators.

nlin.CD↗

Supporting random wave models: a quantum mechanical approach

We show how two-point correlation functions derived within non-isotropic random wave models are in fact quantum results that are obtained in the appropriate limit in terms of the exact Green function of the quantum system. Since no statistical model is required for this derivation, this shows that taking the wave functions as Gaussian processes is the only assumption of those random wave models. We also show how for clean systems the two-point correlation function defined through an energy average defines a Gaussian theory which substantially reduces the spurious contributions coming from the normalisation problem.

nlin.CD↗

Leading off-diagonal contribution to the spectral form factor of chaotic quantum systems

We semiclassically derive the leading off-diagonal correction to the spectral form factor of quantum systems with a chaotic classical counterpart. To this end we present a phase space generalization of a recent approach for uniformly hyperbolic systems (M. Sieber and K. Richter, Phys. Scr. T90, 128 (2001); M. Sieber, J. Phys. A: Math. Gen. 35, L613 (2002)). Our results coincide with corresponding random matrix predictions. Furthermore, we study the transition from the Gaussian orthogonal to the Gaussian unitary ensemble.

nlin.CD↗

Conductance of a molecular junction mediated by unconventional metal-induced gap states

The conductance of a molecular junction is commonly determined by either charge-transfer-doping, where alignment of the Fermi energy to the molecular levels is achieved, or tunnelling through the tails of molecular resonances within the highest-occupied and lowest-unoccupied molecular-orbital gap. Here, we present an alternative mechanism where electron transport is dominated by electrode surface states. They give rise to metallization of the molecular bridge and additional, pronounced conductance resonances allowing for substantial tailoring of its electronic properties via, e.g. a gate voltage. This is demonstrated in a field-effect geometry of a fullerene-bridge between two metallic carbon nanotubes.

cond-mat.mes-hall↗

Fingerprints of mesoscopic leads in the conductance of a molecular wire

The influence of contacts on linear transport through a molecular wire attached to mesoscopic tubule leads is studied. It is shown that low dimensional leads, such as carbon nanotubes, in contrast to bulky electrodes, strongly affect transport properties. By focusing on the specificity of the lead-wire contact, we show, in a fully analytical treatment, that the geometry of this hybrid system supports a mechanism of channel selection and a sum rule, which is a distinctive hallmark of the mesoscopic nature of the electrodes.

cond-mat.mes-hall↗

A molecular wire sandwiched between nanotube leads: analytic results for the conductance

Analytic results for the conductance of a molecular wire attached to mesoscopic tubule leads are obtained. They permit to study linear transport in presence of low dimensional leads in the whole range of parameters. In particular contact effects can be addressed in detail. By focusing on the specificity of the lead-wire contact, we show that the geometry of this hybrid system supports a mechanism of channel selection, which is a distinctive hallmark of the mesoscopic nature of the electrodes.

cond-mat.mes-hall↗

Molecular wire-nanotube interfacial effects on electron transport

We discuss the conductance of a molecular bridge between mesoscopic electrodes supporting low-dimensional transport and bearing an internal structure. As an example for such nanoelectrodes we assume semi-infinite (carbon) nanotubes. In the Landauer scattering matrix approach, we show that the conductance of this hybrid is very sensitive to the geometry of the contact unlike the usual behaviour in the presence of bulk electrodes.

cond-mat.mes-hall↗

Fullerene based devices for molecular electronics

We have investigated the electronic properties of a C_60 molecule in between carbon nanotube leads. This problem has been tackled within a quantum chemical treatment utilizing a density functional theory-based LCAO approach combined with the Landauer formalism. Owing to low-dimensionality, electron transport is very sensitive to the strength and geometry of interfacial bonds. Molecular contact between interfacial atoms and electrodes gives rise to a complex conductance dependence on the electron energy exhibiting spectral features of both the molecule and electrodes. These are attributed to the electronic structure of the C_60 molecule and to the local density of states of the leads, respectively.

cond-mat.mes-hall↗

An `all-carbon' molecular device

We have performed parameter-free calculations of electron transport across a carbon molecular junction consisting of a C$_{60}$ molecule sandwiched between two semi-infinite metallic carbon nanotubes. It is shown that the Landauer conductance of this carbon hybrid system can be tuned within orders of magnitude not only by varying the tube-C$_{60}$ distance, but more importantly at fixed distances by i) changing the orientation of the Buckminsterfullerene or ii) rotating one of the tubes around its cylinder axis. Furthermore, it is explicitely shown that structural relaxation determines qualitatively the transmission spectrum of such devices.

cond-mat.mes-hall↗

Conductance of a molecular wire attached to mesoscopic leads: contact effects

We study linear electron transport through a molecular wire sandwiched between nanotube leads. We show that the presence of such electrodes strongly influences the calculated conductance. We find that depending on the quality and geometry of the contacts between the molecule and the tubular reservoirs, linear transport can be tuned between an effective Newns spectral behavior and a more structured one. The latter strongly depends on the topology of the leads. We also provide analytical evidence for an anomalous behavior of the conductance as a function of the contact strength.

cond-mat.mes-hall↗

Electron transport in nanotube--molecular wire hybrids

We study contact effects on electron transport across a molecular wire sandwiched between two semi-infinite (carbon) nanotube leads as a model for nanoelectrodes. Employing the Landauer scattering matrix approach we find that the conductance is very sensitive to parameters such as the coupling strength and geometry of the contact. The conductance exhibits markedly different behavior in the two limiting scenarios of single contact and multiple contacts between the molecular wire and the nanotube interfacial atoms. In contrast to a single contact the multiple-contact configuration acts as a filter selecting single transport channels. It exhibits a scaling law for the conductance as a function of coupling strength and tube diameter. We also observe an unusual narrow-to-broad-to-narrow behavior of conductance resonances upon decreasing the coupling.

cond-mat.mes-hall↗

Mechanical Mixing in Nonlinear Nanomechanical Resonators

Nanomechanical resonators, machined out of Silicon-on-Insulator wafers, are operated in the nonlinear regime to investigate higher-order mechanical mixing at radio frequencies, relevant to signal processing and nonlinear dynamics on nanometer scales. Driven by two neighboring frequencies the resonators generate rich power spectra exhibiting a multitude of satellite peaks. This nonlinear response is studied and compared to $n^{th}$-order perturbation theory and nonperturbative numerical calculations.

cond-mat.mes-hall↗

Semiclassical Theory of Integrable and Rough Andreev Billiards

We study the effect on the density of states in mesoscopic ballistic billiards to which a superconducting lead is attached. The expression for the density of states is derived in the semiclassical S-matrix formalism shedding insight into the origin of the differences between the semiclassical theory and the corresponding result derived from random matrix models. Applications to a square billiard geometry and billiards with boundary roughness are discussed. The saturation of the quasiparticle excitation spectrum is related to the classical dynamics of the billiard. The influence of weak magnetic fields on the proximity effect in rough Andreev billiards is discussed and an analytical formula is derived. The semiclassical theory provides an interpretation for the suppression of the proximity effect in the presence of magnetic fields as a coherence effect of time reversed trajectories, similar to the weak localisation correction of the magneto-resistance in chaotic mesoscopic systems. The semiclassical theory is shown to be in good agreement with quantum mechanical calculations.

cond-mat.supr-con↗

Semiclassical Approach to Orbital Magnetism of Interacting Diffusive Quantum Systems

We study interaction effects on the orbital magnetism of diffusive mesoscopic quantum systems. By combining many-body perturbation theory with semiclassical techniques, we show that the interaction contribution to the ensemble averaged quantum thermodynamic potential can be reduced to an essentially classical operator. We compute the magnetic response of disordered rings and dots for diffusive classical dynamics. Our semiclassical approach reproduces the results of previous diagrammatic quantum calculations.

cond-mat.mes-hall↗

Chaos and Interacting Electrons in Ballistic Quantum Dots

We show that the classical dynamics of independent particles can determine the quantum properties of interacting electrons in the ballistic regime. This connection is established using diagrammatic perturbation theory and semiclassical finite-temperature Green functions. Specifically, the orbital magnetism is greatly enhanced over the Landau susceptibility by the combined effects of interactions and finite size. The presence of families of periodic orbits in regular systems makes their susceptibility parametrically larger than that of chaotic systems, a difference which emerges from correlation terms.

cond-mat.mes-hall↗

Orbital Magnetism in the Ballistic Regime: Geometrical Effects

We present a general semiclassical theory of the orbital magnetic response of noninteracting electrons confined in two-dimensional potentials. We calculate the magnetic susceptibility of singly-connected and the persistent currents of multiply-connected geometries. We concentrate on the geometric effects by studying confinement by perfect (disorder free) potentials stressing the importance of the underlying classical dynamics. We demonstrate that in a constrained geometry the standard Landau diamagnetic response is always present, but is dominated by finite-size corrections of a quasi-random sign which may be orders of magnitude larger. These corrections are very sensitive to the nature of the classical dynamics. Systems which are integrable at zero magnetic field exhibit larger magnetic response than those which are chaotic. This difference arises from the large oscillations of the density of states in integrable systems due to the existence of families of periodic orbits. The connection between quantum and classical behavior naturally arises from the use of semiclassical expansions. This key tool becomes particularly simple and insightful at finite temperature, where only short classical trajectories need to be kept in the expansion. In addition to the general theory for integrable systems, we analyze in detail a few typical examples of experimental relevance: circles, rings and square billiards. In the latter, extensive numerical calculations are used as a check for the success of the semiclassical analysis. We study the weak-field regime where classical trajectories remain essentially unaffected, the intermediate field regime where we identify new oscillations characteristic for ballistic mesoscopic structures, and the high-field regime where the typical de Haas-van Alphen oscillations exhibit finite-size corrections. We address the comparison with experimental data obtained in high-mobility semiconductor microstructures discussing the differences between individual and ensemble measurements, and the applicability of the present model.

cond-mat↗

Integrability and Disorder in Mesoscopic Systems: Application to Orbital Magnetism

We present a semiclassical theory of weak disorder effects in small structures and apply it to the magnetic response of non-interacting electrons confined in integrable geometries. We discuss the various averaging procedures describing different experimental situations in terms of one- and two-particle Green functions. We demonstrate that the anomalously large zero-field susceptibility characteristic of clean integrable structures is only weakly suppressed by disorder. This damping depends on the ratio of the typical size of the structure with the two characteristic length scales describing the disorder (elastic mean-free-path and correlation length of the potential) in a power-law form for the experimentally relevant parameter region. We establish the comparison with the available experimental data and we extend the study of the interplay between disorder and integrability to finite magnetic fields.

cond-mat↗