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K. T. Flanagan

Publications and source records attributed to K. T. Flanagan.

At least 19 recordsLinked to original sources

Energies and lifetimes of the 9p and 10p excited states in atomic francium

We present the first measurement of 9p 2P1/2,3/2 and 10p 2P1/2,3/2 excited levels absolute wavenumbers and radiative lifetime in francium. We used the Collinear Resonance Ionization Spectroscopy (CRIS) technique, applied on a beam of 221Fr atoms. Prior to this work, no experimental data existed for francium p-states with n > 8. The results provide a precision experimental test of relativistic coupled-cluster theory for the heaviest alkali, showing good agreement for lifetimes and relative excitation energies, despite a residual global offset in absolute energies.

physics.atom-ph

Charge Radii Measurements of Exotic Tin Isotopes in the Proximity of $N=50$ and $N=82$

We report nuclear charge radii for the isotopes $^{104-134}$Sn, measured using two different collinear laser spectroscopy techniques at ISOLDE-CERN. These measurements clarify the arch-like trend in charge radii along the isotopic chain and reveal an odd-even staggering that is more pronounced near the $N=50$ and $N=82$ shell closures. The observed local trends are well described by both nuclear density functional theory and valence space in-medium similarity renormalization group calculations. Both theories predict appreciable contributions from beyond-mean-field correlations to the charge radii of the neutron-deficient tin isotopes. The models, however, fall short of reproducing the magnitude of the known $B(E2)$ transition probabilities, highlighting the remaining challenges in achieving a unified description of both ground-state properties and collective phenomena.

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Observation of the distribution of nuclear magnetization in a molecule

Rapid progress in the experimental control and interrogation of molecules, combined with developments in precise calculations of their structure, are enabling new opportunities in the investigation of nuclear and particle physics phenomena. Molecules containing heavy, octupole-deformed nuclei such as radium are of particular interest for such studies, offering an enhanced sensitivity to the properties of fundamental particles and interactions. Here, we report precision laser spectroscopy measurements and theoretical calculations of the structure of the radioactive radium monofluoride molecule, $^{225}$Ra$^{19}$F. Our results allow fine details of the short-range electron-nucleus interaction to be revealed, indicating the high sensitivity of this molecule to the distribution of magnetization, currently a poorly constrained nuclear property, within the radium nucleus. These results provide a direct and stringent test of the description of the electronic wavefunction inside the nuclear volume, highlighting the suitability of these molecules to investigate subatomic phenomena.

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$^{61}$Cr as a Doorway to the N = 40 Island of Inversion

This paper reports on the measurement of the ground-state spin and nuclear magnetic dipole moment of $^{61}$Cr. The radioactive ion beam was produced at the CERN-ISOLDE facility and was probed using high-resolution resonance ionization laser spectroscopy with the CRIS apparatus. The present ground-state spin measurement $I = \frac{1}{2}$, differing from the previously adopted $I =(\frac{5}{2})$, has significant consequences on the interpretation of existing beta decay data and nuclear structure in the region. The structure and shape of $^{61}$Cr is interpreted with state-of-the-art Large-Scale Shell Model and Discrete-Non-Orthogonal Shell Model calculations. From the measured magnetic dipole moment $μ(^{61}$Cr$)=+0.539(7)~μ_N$ and the theoretical findings, its configuration is understood to be driven by 2 particle - 2 hole neutron excitations with an unpaired $1p_{1/2}$ neutron. This establishes the western border of the $N=40$ Island Of Inversion (IoI), characterized by 4 particle - 4 hole neutron components. We discuss the shape evolution along the Cr isotopic chain as a quantum phase transition at the entrance of the $N=40$ IoI.

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Laser spectroscopy and CP-violation sensitivity of actinium monofluoride

The apparent invariance of the strong nuclear force under combined charge conjugation and parity (CP) remains an open question in modern physics. Precision experiments with heavy atoms and molecules can provide stringent constraints on CP violation via searches for effects due to permanent electric dipole moments and other CP-odd properties in leptons, hadrons, and nuclei. Radioactive molecules have been proposed as highly sensitive probes for such searches, but experiments with most such molecules have so far been beyond technical reach. Here we report the first production and spectroscopic study of a gas-phase actinium molecule, $^{227}$AcF. We observe the predicted strongest electronic transition from the ground state, which is necessary for efficient readout in searches of symmetry-violating interactions. Furthermore, we perform electronic- and nuclear-structure calculations for $^{227}$AcF to determine its sensitivity to various CP-violating parameters, and find that a realistic, near-term experiment with a precision of 1 mHz would improve current constraints on the CP-violating parameter hyperspace by three orders of magnitude. Our results thus highlight the potential of $^{227}$AcF for exceptionally sensitive searches of CP violation.

physics.atom-ph

Reduction in nuclear size and quadrupole deformation of high-spin isomers of 127,129In

We employed laser spectroscopy of atomic transitions to measure the nuclear charge radii and electromagnetic properties of the high-spin isomeric states in neutron-rich indium isotopes (Z = 49) near the closed proton and neutron shells at Z = 50 and N = 82. Our data reveal a reduction in the nuclear charge radius and intrinsic quadrupole moment when protons and neutrons are fully aligned in 129In(N = 80), to form the high spin isomer. Such a reduction is not observed in 127In(N = 78), where more complex configurations can be formed by the existence of four neutron-holes. These observations are not consistently described by nuclear theory.

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Charge radii of neutron-rich scandium isotopes and the seniority symmetry in the $0f_{7/2}$ shell

Nuclear charge radii of neutron-rich $^{47-49}$Sc isotopes were measured using collinear laser spectroscopy at CERN-ISOLDE. The new data reveal that the charge radii of scandium isotopes exhibit a distinct trend between $N=20$ and $N=28$, with $^{41}$Sc and $^{49}$Sc isotopes having similar values, mirroring the closeness of the charge radii of $^{40}$Ca and $^{48}$Ca. Theoretical models that successfully interpret the radii of calcium isotopes could not account for the observed behavior in scandium radii, in particular the reduced odd-even staggering. Remarkably, the inclusion of the new $^{49}$Sc radius data has unveiled a similar trend in the charge radii of $N=28$ isotones and $Z=20$ isotopes when adding the neutrons atop the $^{40}$Ca core and the protons atop the $^{48}$Ca core, respectively. We demonstrate that this trend is consistent with the prediction of the seniority model.

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Pinning down electron correlations in RaF via spectroscopy of excited states and high-accuracy relativistic quantum chemistry

We report the spectroscopy of the 14 lowest excited electronic states in the radioactive molecule radium monofluoride (RaF). The observed excitation energies are compared with fully relativistic state-of-the-art Fock-space coupled cluster (FS-RCC) calculations, which achieve an agreement of >=99.64% (within ~12 meV) with experiment for all states. Guided by theory, a firm assignment of the angular momentum and term symbol is made for 10 states and a tentative assignment for 4 states. The role of high-order electron correlation and quantum electrodynamics effects in the excitation energy of excited states is studied, found to be important for all states. Establishing the simultaneous accuracy and precision of calculations is an important step for research at the intersection of particle, nuclear, and chemical physics, including searches of physics beyond the Standard Model, for which RaF is a promising probe.

physics.atom-ph

Ionization potential of radium monofluoride

The ionization potential (IP) of radium monofluoride (RaF) was measured to be 4.969(2)[10] eV, revealing a relativistic enhancement in the series of alkaline earth monofluorides. The results are in agreement with a relativistic coupled-cluster prediction of 4.969[7] eV, incorporating up to quantum electrodynamics corrections. Using the same computational methodology, an improved calculation for the dissociation energy ($D_{0}$) of 5.54[5] eV is presented. This confirms that radium monofluoride joins the small group of diatomic molecules for which $D_{0}>\mathrm{IP}$, paving the way for precision control and interrogation of its Rydberg states.

physics.atom-ph

Electromagnetic Properties of Indium Isotopes Elucidate the Doubly Magic Character of $^{100}$Sn

Our understanding of nuclear properties in the vicinity of $^{100}$Sn, suggested to be the heaviest doubly magic nucleus with equal numbers of protons (Z=50) and neutrons (N=50), has been a long-standing challenge for experimental and theoretical nuclear physics. Contradictory experimental evidence exists on the role of nuclear collectivity in this region of the nuclear chart. Using precision laser spectroscopy, we measured the ground-state electromagnetic moments of indium (Z=49) isotopes approaching the N=50 neutron number down to 101In, and nuclear charge radii of 101-131In spanning almost the complete range between the two major neutron closed-shells at N=50 and N=82. Our results for both nuclear charge radii and quadrupole moments reveal striking parabolic trends as a function of the neutron number, with a clear reduction toward these two neutron closed-shells, thus supporting a doubly magic character of $^{100}$Sn. Two complementary nuclear many-body frameworks, density functional theory and ab initio methods, elucidate our findings. A detailed comparison with our experimental results exposes deficiencies of nuclear models, establishing a benchmark for future theoretical developments.

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Radiative lifetime of the A 2Π1/2 state in RaF with relevance to laser cooling

The radiative lifetime of the $A$ $^2 Π_{1/2}$ (v=0) state in radium monofluoride (RaF) is measured to be 35(1) ns. The lifetime of this state and the related decay rate $Γ= 2.86(8) \times 10^7$ $s^{-1}$ are of relevance to the laser cooling of RaF via the optically closed $A$ $^2 Π_{1/2} \leftarrow X$ $^2Σ_{1/2}$ transition, which makes the molecule a promising probe to search for new physics. RaF is found to have a comparable photon-scattering rate to homoelectronic laser-coolable molecules. Thanks to its highly diagonal Franck-Condon matrix, it is expected to scatter an order of magnitude more photons than other molecules when using just 3 cooling lasers, before it decays to a dark state. The lifetime measurement in RaF is benchmarked by measuring the lifetime of the $8P_{3/2}$ state in Fr to be 83(3) ns, in agreement with literature.

physics.atom-ph

Electromagnetic moments of scandium isotopes and $N=28$ isotones in the distinctive $0f_{7/2}$ orbit

The electric quadrupole moment of $^{49}$Sc was measured by collinear laser spectroscopy at CERN-ISOLDE to be $Q_{\rm s}=-0.159(8)$ $e$b, and a nearly tenfold improvement in precision was reached for the electromagnetic moments of $^{47,49}$Sc. The single-particle behavior and nucleon-nucleon correlations are investigated with the electromagnetic moments of $Z=21$ isotopes and $N=28$ isotones as valence neutrons and protons fill the distinctive $0f_{7/2}$ orbit, respectively, located between magic numbers, 20 and 28. The experimental data are interpreted with shell-model calculations using an effective interaction, and ab-initio valence-space in-medium similarity renormalization group calculations based on chiral interactions. These results highlight the sensitivity of nuclear electromagnetic moments to different types of nucleon-nucleon correlations, and establish an important benchmark for further developments of theoretical calculations.

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Charge radii, moments and masses of mercury isotopes across the N = 126 shell closure

Combining laser spectroscopy in a Versatile Arc Discharge and Laser Ion Source, with Penning-trap mass spectrometry at the CERN-ISOLDE facility, this work reports on mean-square charge radii of neutron-rich mercury isotopes across the $N = 126$ shell closure, the electromagnetic moments of $^{207}$Hg and more precise mass values of $^{206-208}$Hg. The odd-even staggering (OES) of the mean square charge radii and the kink at $N = 126$ are analyzed within the framework of covariant density functional theory (CDFT), with comparisons between different functionals to investigate the dependence of the results on the underlying single-particle structure. The observed features are defined predominantly in the particle-hole channel in CDFT, since both are present in the calculations without pairing. However, the magnitude of the kink is still affected by the occupation of the $1i_{11/2}$ and $2g_{9/2}$ orbitals with a dependence on the relative energies as well as pairing.

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Isotope Shifts of Radium Monofluoride Molecules

Isotope shifts of $^{223-226,228}$Ra$^{19}$F were measured for different vibrational levels in the electronic transition $A^{2}{}Π_{1/2}\leftarrow X^{2}{}Σ^{+}$. The observed isotope shifts demonstrate the particularly high sensitivity of radium monofluoride to nuclear size effects, offering a stringent test of models describing the electronic density within the radium nucleus. Ab initio quantum chemical calculations are in excellent agreement with experimental observations. These results highlight some of the unique opportunities that short-lived molecules could offer in nuclear structure and in fundamental symmetry studies.

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Laser spectroscopy of neutron-rich $^{207,208}$Hg isotopes: Illuminating the kink and odd-even staggering in charge radii across the $N=126$ shell closure

The mean-square charge radii of $^{207,208}$Hg ($Z=80, N=127,128$) have been studied for the first time and those of $^{202,203,206}$Hg ($N=122,123,126$) remeasured by the application of in-source resonance-ionization laser spectroscopy at ISOLDE (CERN). The characteristic \textit{kink} in the charge radii at the $N=126$ neutron shell closure has been revealed, providing the first information on its behavior below the $Z=82$ proton shell closure. A theoretical analysis has been performed within relativistic Hartree-Bogoliubov and non-relativistic Hartree-Fock-Bogoliubov approaches, considering both the new mercury results and existing lead data. Contrary to previous interpretations, it is demonstrated that both the kink at $N=126$ and the odd-even staggering (OES) in its vicinity can be described predominately at the mean-field level, and that pairing does not need to play a crucial role in their origin. A new OES mechanism is suggested, related to the staggering in the occupation of the different neutron orbitals in odd- and even-$A$ nuclei, facilitated by particle-vibration coupling for odd-$A$ nuclei.

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Charge radii of exotic potassium isotopes challenge nuclear theory and the magic character of $N = 32$

Nuclear charge radii are sensitive probes of different aspects of the nucleon-nucleon interaction and the bulk properties of nuclear matter; thus, they provide a stringent test and challenge for nuclear theory. The calcium region has been of particular interest, as experimental evidence has suggested a new magic number at $N = 32$ [1-3], while the unexpectedly large increases in the charge radii [4,5] open new questions about the evolution of nuclear size in neutron-rich systems. By combining the collinear resonance ionization spectroscopy method with $β$-decay detection, we were able to extend the charge radii measurement of potassium ($Z =19$) isotopes up to the exotic $^{52}$K ($t_{1/2}$ = 110 ms), produced in minute quantities. Our work provides the first charge radii measurement beyond $N = 32$ in the region, revealing no signature of the magic character at this neutron number. The results are interpreted with two state-of-the-art nuclear theories. For the first time, a long sequence of isotopes could be calculated with coupled-cluster calculations based on newly developed nuclear interactions. The strong increase in the charge radii beyond $N = 28$ is not well captured by these calculations, but is well reproduced by Fayans nuclear density functional theory, which, however, overestimates the odd-even staggering effect. These findings highlight our limited understanding on the nuclear size of neutron-rich systems, and expose pressing problems that are present in some of the best current models of nuclear theory.

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Laser spectroscopy of indium Rydberg atom bunches by electric field ionization

This work reports on the application of a novel electric field-ionization setup for high-resolution laser spectroscopy measurements on bunched fast atomic beams in a collinear geometry. In combination with multi-step resonant excitation to Rydberg states using pulsed lasers, the field ionization technique demonstrates increased sensitivity for isotope separation and measurement of atomic parameters over non-resonant laser ionization methods. The setup was tested at the Collinear Resonance Ionization Spectroscopy experiment at ISOLDE-CERN to perform high-resolution measurements of transitions in the indium atom from the 5s$^2$5d~$^2$D$_{5/2}$ and 5s$^2$5d~$^2$D$_{3/2}$ states to 5s$^2$($n$)p~$^2$P and 5s$^2$($n$)f~$^2$F Rydberg states, up to a principal quantum number of $n$ = 72. The extracted Rydberg level energies were used to re-evaluate the ionization potential of the indium atom to be 46670.1055(21) cm$^{-1}$. The nuclear magnetic dipole and nuclear electric quadrupole hyperfine structure constants and level isotope shifts of the 5s$^2$5d~$^2$D$_{5/2}$ and 5s$^2$5d~$^2$D$_{3/2}$ states were determined for $^{113,115}$In. The results are compared to calculations using relativistic coupled-cluster theory. A good agreement is found with the ionization potential and isotope shifts, while disagreement of hyperfine structure constants indicates an increased importance of electron correlations in these excited atomic states. With the aim of further increasing the detection sensitivity for measurements on exotic isotopes, a systematic study of the field-ionization arrangement implemented in the work was performed and an improved design was simulated and is presented. The improved design offers increased background suppression independent of the distance from field ionization to ion detection.

physics.atom-ph

Measurement and microscopic description of odd-even staggering of charge radii of exotic copper isotopes

The mesoscopic nature of the atomic nucleus gives rise to a wide array of macroscopic and microscopic phenomena. The size of the nucleus is a window into this duality: while the charge radii globally scale as $A^{1/3}$, their evolution across isotopic chains reveals unanticipated structural phenomena [1-3]. The most ubiquitous of these is perhaps the Odd-Even Staggering (OES) [4]: isotopes with an odd number of neutrons are usually smaller in size than the trend of their even-neutron neighbours suggests. This OES effect varies with the number of protons and neutrons and poses a significant challenge for nuclear theory [5-7]. Here, we examine this problem with new measurements of the charge radii of short-lived copper isotopes up to the very exotic $^{78}$Cu $(Z=29, N=49)$, produced at only 20 ions/s, using the highly-sensitive Collinear Resonance Ionisation Spectroscopy (CRIS) method at ISOLDE-CERN. Due to the presence of a single proton outside of the closed Z=28 shell, these measurements provide crucial insights into the single-particle proton structure and how this affects the charge radii. We observe an unexpected reduction in the OES for isotopes approaching the $N=50$ shell gap. To describe the data, we applied models based on nuclear Density Functional Theory [2,8] (DFT) and ab-initio Valence-Space In-Medium Similarity Renormalization Group (VS-IMSRG) theory [9,10]. Through these comparisons, we demonstrate a relation between the global behavior of charge radii and the saturation density of nuclear matter, and show that the local charge radii variations, which reflect the many-body polarization effects due to the odd neutron, naturally emerge from the VS-IMSRG calculations.

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