arXiv subjects

K. T. Law

Publications and source records attributed to K. T. Law.

At least 55 records · Page 3Linked to original sources

arXiv2023

Three-Dimensional Quantum Anomalous Hall Effect in Magnetic Topological Insulator Trilayers of Hundred-Nanometer Thickness

Magnetic topological states refer to a class of exotic phases in magnetic materials with their non-trivial topological property determined by magnetic spin configurations. An example of such states is the quantum anomalous Hall (QAH) state, which is a zero magnetic field manifestation of the quantum Hall effect. Current research in this direction focuses on QAH insulators with a thickness of less than 10nm. The thick QAH insulators in the three-dimensional(3D) regime are limited, largely due to inevitable bulk carriers being introduced in thick magnetic TI samples. Here, we employ molecular beam epitaxy (MBE) to synthesize magnetic TI trilayers with a thickness of up to ~106 nm. We find these samples exhibit well-quantized Hall resistance and vanishing longitudinal resistance at zero magnetic field. By varying magnetic dopants, gate voltages, temperature, and external magnetic fields, we examine the properties of these thick QAH insulators and demonstrate the robustness of the 3D QAH effect. The realization of the well-quantized 3D QAH effect indicates that the nonchiral side surface states of our thick magnetic TI trilayers are gapped and thus do not affect the QAH quantization. The 3D QAH insulators of hundred-nanometer thickness provide a promising platform for the exploration of fundamental physics, including axion physics and image magnetic monopole, and the advancement of electronic and spintronic devices to circumvent Moore's law.

cond-mat.mes-hall↗

arXiv2023

The Ginzburg-Landau theory of flat band superconductors with quantum metric

Recent experimental study unveiled highly unconventional phenomena in the superconducting twisted bilayer graphene (TBG) with ultra flat bands, which cannot be described by the conventional BCS theory. For example, given the small Fermi velocity of the flat bands, the superconducting coherence length predicted by BCS theory is more than 20 times shorter than the measured values. A new theory is needed to understand many of the unconventional properties of flat band superconductors. In this work, we establish a Ginzburg-Landau (GL) theory from a microscopic flat band Hamiltonian. The GL theory shows how the properties of the physical quantities such as the critical temperature, the superconducting coherence length, the upper critical field and the superfluid density are governed by the quantum metric of the Bloch states. One key conclusion is that the superconducting coherence length is not determined by the Fermi velocity but by the size of the optimally localized Wannier functions which is limited by quantum metric. Applying the theory to TBG, we calculated the superconducting coherence length and the upper critical fields. The results match the experimental ones well without fine tuning of parameters. The established GL theory provides a new and general theoretical framework for understanding flat band superconductors with quantum metric.

cond-mat.supr-con↗

arXiv2023

Axion Insulator State in Hundred-Nanometer-Thick Magnetic Topological Insulator Sandwich Heterostructures

An axion insulator is a three-dimensional (3D) topological insulator (TI), in which the bulk maintains the time-reversal symmetry or inversion symmetry but the surface states are gapped by surface magnetization. The axion insulator state has been observed in molecular beam epitaxy (MBE)-grown magnetically doped TI sandwiches and exfoliated intrinsic magnetic TI MnBi2Te4 flakes with an even number layer. All these samples have a thickness of ~10 nm, near the 2D-to-3D boundary. The coupling between the top and bottom surface states in thin samples may hinder the observation of quantized topological magnetoelectric response. Here, we employ MBE to synthesize magnetic TI sandwich heterostructures and find that the axion insulator state persists in a 3D sample with a thickness of ~106 nm. Our transport results show that the axion insulator state starts to emerge when the thickness of the middle undoped TI layer is greater than ~3 nm. The 3D hundred-nanometer-thick axion insulator provides a promising platform for the exploration of the topological magnetoelectric effect and other emergent magnetic topological states, such as the high-order TI phase.

cond-mat.mes-hall↗

arXiv2023

Valley-polarized Josephson Junctions as gate-tunable $0$-$π$ qubit platforms

Recently, gate-defined Josephson junctions based on magic-angle twisted bilayer graphene (MATBG) have been fabricated. In such a junction, local electrostatic gating can create two superconducting regions connected by an interaction-driven valley-polarized state as the weak link. Due to the spontaneous time-reversal and inversion symmetry breaking of the valley-polarized state, novel phenomena such as the Josephson diode effect have been observed without applying external fields. Importantly, when the so-called nonreciprocity efficiency (which measures the sign and strength of the Josephson effect) changes sign, the energy-phase relation of the junction is approximate $F(ϕ) \approx \cos(2ϕ)$ where $F$ is the free energy and $ϕ$ is the phase difference of the two superconductors. In this work, we show that such a MATBG-based Josephson junction, when shunted by a capacitor, can be used to realize the long-sought-after $0$-$π$ qubits which are protected from local perturbation-induced decoherence. Interestingly, by changing the junction parameters, transmon-like qubits with large anharmonicity can also be realized. In short, by utilizing the novel interaction-driven valley-polarized state in MATBG, a single gate-defined Josephson junction can be used to replace complicated superconducting circuits for realizing qubits that are protected from local perturbations.

cond-mat.supr-con↗

arXiv2023

Orbital Fulde-Ferrell pairing state in moiré Ising superconductors

In this work, we study superconducting moiré homobilayer transition metal dichalcogenides where the Ising spin-orbit coupling (SOC) is much larger than the moiré bandwidth. We call such noncentrosymmetric superconductors, moiré Ising superconductors. Due to the large Ising SOC, the depairing effect caused by the Zeeman field is negligible and the in-plane upper critical field ($B_{c2}$) is determined by the orbital effects. This allows us to study the effect of large orbital fields. Interestingly, when the applied in-plane field is larger than the conventional orbital $B_{c2}$, a finite-momentum pairing phase would appear which we call the orbital Fulde-Ferrell (FF) state. In this state, the Cooper pairs acquire a net momentum of $2q_B$ where $2q_B=eBd$ is the momentum shift caused by the magnetic field $B$ and $d$ denotes the layer separation. This orbital field-driven FF state is different from the conventional FF state driven by Zeeman effects in Rashba superconductors. Remarkably, we predict that the FF pairing would result in a giant superconducting diode effect under electric gating when layer asymmetry is induced. An upturn of the $B_{c2}$ as the temperature is lowered, coupled with the giant superconducting diode effect, would allow the detection of the orbital FF state.

cond-mat.supr-con↗

arXiv2023

Heesch Weyl Fermions in inadmissible chiral antiferromagnets

Symmetry is a crucial factor in determining the topological properties of materials. In nonmagnetic chiral crystals, the existence of the Kramers Weyl fermions reveals the topological nature of the Kramers degeneracy at time-reversal-invariant momenta (TRIMs). However, it is not clear whether Weyl nodes can also be pinned at points of symmetry in magnetic materials where the time-reversal is spontaneously broken. In this study, we introduce a new type of Weyl fermions, called Heesch Weyl fermions (HWFs), which are stabilized and pinned at points of symmetry by the Heesch groups in inadmissible chiral antiferromagnets. The emergence of HWFs is fundamentally different from that of Kramers Weyl fermions, as it does not rely on any anti-unitary symmetry $\mathcal{A}$ that satisfies $\mathcal{A}^2=-1$. Importantly, the emergence of HWFs is closely related to the antiferromagnetic order, as they are generally obscured by nodal lines in the parent nonmagnetic state. Using group theory analysis, we classify all the magnetic little co-groups of momenta where Heesch Weyl nodes are enforced and pinned by symmetry. With the guidance of this classification and first-principles calculations, we identify antiferromagnetic (AFM) materials such as YMnO$_3$ and Mn$_3$IrGe as candidate hosts for the AFM-order-induced HWFs.We also explore novel properties of Heesch Weyl antiferromagnets, such as nonlinear anomalous Hall effects and axial movement of Heesch Weyl nodes. Our findings shed new light on the role of symmetry in determining and stabilizing topological properties in magnetic materials, and open up new avenues for the design and exploration of topological materials.

cond-mat.mtrl-sci↗

arXiv2023

$φ_0$-Josephson junction in twisted bilayer graphene induced by a valley-polarized state

Recently, gate-defined Josephson junctions in magic angle twisted bilayer graphene (MATBG) were studied experimentally and highly unconventional Fraunhofer patterns were observed. In this work, we show that an interaction-driven valley-polarized state connecting two superconducting regions of MATBG would give rise to a long-sought-after purely electric controlled $φ_0$-junction in which the two superconductors acquire a finite phase difference $φ_0$ in the ground state. We point out that the emergence of the $φ_0$-junction stems from the valley-polarized state which breaks time-reversal symmetry and trigonal warping effects which break the intravalley inversion symmetry. Importantly, a spatially non-uniform valley polarization order parameter at the junction can explain the highly unconventional Fraunhofer patterns observed in the experiment. Our work explores the novel transport properties of the valley-polarized state and suggests that gate-defined MATBG Josephson junctions could realize the first purely electric controlled $φ_0$-junctions with applications in superconducting devices.

cond-mat.mes-hall↗

arXiv2023

Berry curvature, spin Hall effect and nonlinear optical response in moiré transition metal dichalcogenide heterobilayers

Recently, the topological flat bands and spin Hall effect have been experimentally observed in the AB-stacked MoTe$_2$/WSe$_2$ heterostructures. In this work, we systematically study the Berry curvature effects in moiré transition metal dichalcogenide (TMD) heterobilayers. We point out that the moiré potential of the remote conduction bands would induce a sizable periodic pseudo-magnetic field (PMF) on the valence band. This periodic PMF creates net Berry curvature flux in each valley of the moiré Brillouin zone. The combination of the effect of the Berry curvature and the spin-valley locking can induce the spin Hall effect being observed in the experiment. Interestingly, the valley-contrasting Berry curvature distribution generated by the PMF can be probed through shift currents, which are DC currents induced by linearly polarized lights through nonlinear responses. Our work shed lights on the novel quantum phenomena induced by Berry curvatures in moiré TMD heterobilayers.

cond-mat.mes-hall↗

arXiv2022

Nonlinear Hall Effects in Strained Twisted Bilayer WSe$_2$

Recently, it has been pointed out that the twisting of bilayer WSe$_2$ would generate topologically non-trivial flat bands near the Fermi energy. In this work, we show that twisted bilayer WSe$_2$ (tWSe$_2$) with uniaxial strain exhibits a large nonlinear Hall (NLH) response due to the non-trivial Berry curvatures of the flat bands. Moreover, the NLH effect is greatly enhanced near the topological phase transition point which can be tuned by a vertical displacement field. Importantly, the nonlinear Hall signal changes sign across the topological phase transition point and provides a way to identify the topological phase transition and probe the topological properties of the flat bands. The strong enhancement and high tunability of the NLH effect near the topological phase transition point renders tWSe$_2$ and related moire materials new platforms for rectification and second harmonic generations.

cond-mat.mes-hall↗

arXiv2022

Valley-Polarized Quantum Anomalous Hall State in Moiré MoTe$_2$/WSe$_2$ Heterobilayers

Moiré heterobilayer transition metal dichalcogenides (TMDs) emerge as an ideal system for simulating the single-band Hubbard model and interesting correlated phases have been observed in these systems. Nevertheless, the moiré bands in heterobilayer TMDs were believed to be topologically trivial. Recently, it was reported that both a quantum valley Hall insulating state at filling $ν=2$ (two holes per moiré unit cell) and a valley-polarized quantum anomalous Hall state at filling $ν=1$ were observed in AB stacked moiré MoTe$_2$/WSe$_2$ heterobilayers. However, how the topologically nontrivial states emerge is not known. In this work, we propose that the pseudo-magnetic fields induced by lattice relaxation in moiré MoTe$_2$/WSe$_2$ heterobilayers could naturally give rise to moiré bands with finite Chern numbers. We show that a time-reversal invariant quantum valley Hall insulator is formed at full-filing $ν=2$, when two moiré bands with opposite Chern numbers are filled. At half-filling $ν=1$, Coulomb interaction lifts the valley degeneracy and results in a valley-polarized quantum anomalous Hall state, as observed in the experiment. Our theory identifies a new way to achieve topologically non-trivial states in heterobilayer TMD materials.

cond-mat.mes-hall↗

arXiv2021

Topological superconductivity in EuS/Au/superconductor heterostructures

In a recent work, signatures of a pair of Majorana bound states (MBS) were found in a new experimental platform formed by EuS islands deposited on top of a gold surface which was made superconducting through proximity coupling to a superconductor. In this work, we provide a theoretical understanding for how MBS can be formed in EuS/Au/superconductor heterostructures. We focus on the strip geometry where a narrow ferromagnetic strip is deposited on a planar structure. We first explicitly map out the topological phase diagram of the EuS/Au/superconductor heterostructure using the lattice Green's function method. Importantly, we find that the chemical potential step between the region with and without EuS covering is a crucial ingredient for the creation of MBS of this set-up. Next, we focus on the Bogoliugov quasi-particles that are bound to the region under the EuS by Andreev reflections from the surrounding superconductors. Moreover, we obtain the topological regimes analytically using the scattering matrix method. Notably, we confirm that the normal reflections induced by the chemical potential step are essential for creating finite topological regimes. Furthermore, the area of the topological regimes shows periodic oscillation as a function of chemical potential as well as the sample width.

cond-mat.supr-con↗

arXiv2021

Magnetic Josephson Junctions and Superconducting Diodes in Magic Angle Twisted Bilayer Graphene

The simultaneous co-existence and gate-tuneability of the superconducting (SC), magnetic and topological orders in magic angle twisted bilayer graphene (MATBG) open up entirely new possibilities for the creation of complex hybrid Josephson junctions (JJ). Here we report on the creation of gate-defined, magnetic Josephson junctions in MATBG, where the weak link is gate-tuned close to the correlated state at a moiré filling factor of ν=-2. A highly unconventional Fraunhofer pattern emerges, which is phase-shifted and asymmetric with respect to the current and magnetic field directions, and shows a pronounced magnetic hysteresis. Interestingly, our theoretical calculations of the JJ with a valley polarized ν=-2 with orbital magnetization as the weak link explain most of these unconventional features without fine tuning the parameters. While these unconventional Josephson effects persist up to the critical temperature Tc ~ 3.5K of the superconducting state, at temperatures below T < 800mK, we observed a pronounced magnetic hysteresis possibly due to further spin-polarization of the ν=-2 state. We demonstrate how the combination of magnetization and its current induced magnetization switching in the MATBG JJ allows us to realize a programmable zero field superconducting diode, which represents a major building block for a new generation of superconducting quantum electronics.

cond-mat.supr-con↗

arXiv2021

Superconducting Orbital Magnetoelectric Effect and its Evolution across the Superconductivity Normal Metal Phase Transition

Superconducting magnetoelectric effect, which is the current-induced magnetization in a superconductor, mainly focused on the spin magnetization in previous studies, but ignore the effect of the orbital magnetic moments carried by the paired Bloch electrons. In this work, we show that orbital magnetic moments in superconductors can induce large orbital magnetization in the presence of a current. We constructed a unified description for the current-induced spin and orbital magnetization across the superconductivity normal metal phase transition. We find that in a superconductor with uniform pairing, the current-induced magnetization at a given current density is the same as that in its normal metal state, while with the nonuniform superconducting pairing, the current-induced magnetization exhibits an abrupt change in magnitude near the superconductivity normal metal phase transition. Importantly, our theory predicts the orbital magnetoelectric effect in superconducting twisted bilayer graphene which has paired Bloch electrons with large orbital magnetic moments and negligible spin-orbit coupling. We propose that the measurement of the current-induced orbital magnetoelectric effect can be used to detect the possible nonuniform pairings in twisted bilayer graphene and other newly discovered superconductors with non-trivial Berry curvatures.

cond-mat.mes-hall↗

arXiv2021

Topological Superconductivity in Multifold Fermion Metals

Recently, multifold fermions characterized by band crossings with multifold degeneracy and Fermi surfaces with nontrivial Chern numbers have been discovered experimentally in AlPt[arXiv:1812.03310] and XSi(X=Rh,Co)[arXiv:1812.04466][arXiv:1901.03358][arXiv:1809.01312]. In this work, we largely expand the family of multifold fermion materials by pointing out that several well-studied noncentrosymmetric superconductors are indeed multifold fermion metals. Importantly, their normal state topological properties, which have been ignored in previous studies, play an important role in the superconducting properties. Taking Li$_2$Pd$_3$B and Li$_2$Pt$_3$B as examples, we found a large number of unconventional degenerate points, such as double spin-1, spin-3/2, Weyl and double Weyl topological band crossing points near the Fermi energy, which result in finite Chern numbers on Fermi surfaces. Long Fermi arc states in Li$_2$Pd$_3$B, originating from the nontrivial band topology were found. Importantly, it has been shown experimentally that Li$_2$Pd$_3$B and Li$_2$Pt$_3$B are fully gapped and gapless superconductors, respectively. By analyzing the possible pairing symmetries, we suggest that Li$_2$Pd$_3$B can be a DIII class topological superconductor with Majorana surface states, even though the spin-orbit coupling in Li$_2$Pd$_3$B is negligible. Interestingly, Li$_2$Pt$_3$B, being gapless, is likely to be a nodal topological superconductor with dispersionless surface Majorana modes. We further identified that several noncentrosymmetric superconductors, such as Mo$_3$Al$_2$C, PdBiSe, Y$_2$C$_3$ and La$_2$C$_3$, are multifold fermion superconductors whose normal state topological properties have been ignored in previous experimental and theoretical studies.

cond-mat.supr-con↗

arXiv2021

Creating Localized Majorana Zero Modes in Quantum Anomalous Hall Insulator/Superconductor Heterostructures with a Scissor

In this work, we demonstrate that making a cut (a narrow vacuum regime) in the bulk of a quantum anomalous Hall insulator (QAHI) creates a topologically protected single helical channel with counter-propagating electron modes, and inducing superconductivity on the helical channel through proximity effect will create Majorana zero energy modes (MZMs) at the ends of the cut. In this geometry, there is no need for the proximity gap to overcome the bulk insulating gap of the QAHI to create MZMs as in the two-dimensional QAHI/superconductor (QAHI/SC) heterostructures. Therefore, the topological regime with MZMs is greatly enlarged. Furthermore, due to the presence of a single helical channel, the generation of low energy in-gap bound states caused by multiple conducting channels is avoided such that the MZMs can be well separated from other in-gap excitations in energy. This simple but practical approach allows the creation of a large number of MZMs in devices with complicated geometry such as hexons for measurement-based topological quantum computation. We further demonstrate how braiding of MZMs can be performed by controlling the coupling strength between the counter-propagating electron modes.

cond-mat.mes-hall↗

arXiv2021

Kramers Nodal Line Metals

Recently, it was pointed out that all chiral crystals with spin-orbit coupling (SOC) can be Kramers Weyl semimetals (KWSs) which possess Weyl points pinned at time-reversal invariant momenta. In this work, we show that all achiral non-centrosymmetric materials with SOC can be a new class of topological materials, which we term Kramers nodal line metals (KNLMs). In KNLMs, there are doubly degenerate lines, which we call Kramers nodal lines (KNLs), connecting time-reversal invariant momenta. The KNLs create two types of Fermi surfaces, namely, the spindle torus type and the octdong type. Interestingly, all the electrons on octdong Fermi surfaces are described by two-dimensional massless Dirac Hamiltonians. These materials support quantized optical conductance in thin films. We further show that KNLMs can be regarded as parent states of KWSs. Therefore, we conclude that all non-centrosymmetric metals with SOC are topological, as they can be either KWSs or KNLMs.

cond-mat.mes-hall↗

arXiv2021

Kramers Weyl Semimetals as Quantum Solenoids and Their Applications in Spin-Orbit Torque Devices

Kramers Weyl semimetals are Weyl semimetals that have Weyl points pinned at the time reversal invariant momenta. Recently it has been discovered that all chiral crystals host Weyl points at time reversal invariant momenta, so metals with chiral lattice symmetry all belong to the category of Kramers Weyl semimetals. In this work, we show that due to the chiral lattice symmetry, Kramers Weyl semimetals have the unique longitudinal magnetoelectric effect in which the charge current induced spin and orbital magnetization is parallel to the direction of the current. This feature allows Kramers Weyl semimetals to act as nanoscale quantum solenoids with both orbital and spin magnetization. As the moving electrons of Kramers Weyl semimetal can generate longitudinal magnetization, Kramers Weyl semimetals can be used for new designs of spin-orbit torque devices with all electric control of magnetization switching for magnets with perpendicular magnetic anisotropy.

cond-mat.mes-hall↗

arXiv2021

Higher-Order Nonlinear Anomalous Hall Effects Induced by Berry Curvature Multipoles

In recent years, it has been shown that Berry curvature monopoles and dipoles play essential roles in the anomalous Hall effect and the nonlinear Hall effect respectively. In this work, we demonstrate that Berry curvature multipoles (the higher moments of Berry curvatures at the Fermi energy) can induce higher-order nonlinear anomalous Hall (NLAH) effect. Specifically, an AC Hall voltage perpendicular to the current direction emerges, where the frequency is an integer multiple of the frequency of the applied current. Importantly, by analyzing the symmetry properties of all the 3D and 2D magnetic point groups, we note that the quadrupole, hexapole and even higher Berry curvature moments can cause the leading-order frequency multiplication in certain materials. To provide concrete examples, we point out that the third-order NLAH voltage can be the leading-order Hall response in certain antiferromagnets due to Berry curvature quadrupoles, and the fourth-order NLAH voltage can be the leading response in the surface states of topological insulators induced by Berry curvature hexapoles. Our results are established by symmetry analysis, effective Hamiltonian and first-principles calculations. Other materials which support the higher-order NLAH effect are further proposed, including 2D antiferromagnets and ferromagnets, Weyl semimetals and twisted bilayer graphene near the quantum anomalous Hall phase.

cond-mat.mes-hall↗