arXiv subjects

K. Totsuka

Publications and source records attributed to K. Totsuka.

At least 19 recordsLinked to original sources

arXiv2024

Gapless spin excitations in a quantum spin liquid state of S=1/2 perfect kagome antiferromagnet

Quantum spin liquids (QSLs) represent an exotic quantum many-body state characterized by the suppression of long-range magnetic order due to strong quantum fluctuations. The kagome spin-1/2 antiferromagnet (AFM) is a prime candidate for realizing QSLs, but its ground state remains an unresolved conundrum. Here we investigate the recently discovered perfect kagome AFM YCu$_3$(OH)$_{6.5}$Br$_{2.5}$ to elucidate two central enigmas surrounding the kagome AFM. Ultra-sensitive torque magnetometry experiments reveal that the intrinsic magnetic susceptibility arising from the kagome layer remains nearly temperature-independent down to exceedingly low temperatures. This observation seemingly implies the emergence of gapless fermionic spin excitations akin to Pauli paramagnetism in metals. However, most strikingly, these results stand in stark contrast to the conspicuous absence of a temperature-linear contribution to the specific heat. These findings appear irreconcilable with the widely-discussed theoretical frameworks assuming fermionic quasiparticles (QPs), instead suggesting a transition of bosonic QPs into a superfluid state with a gapless Goldstone mode. Furthermore, magnetocaloric measurements evince an entropy anomaly, constituting thermodynamic evidence that magnetic fields instigate the opening of a spin gap, driving a quantum phase transition into a 1/9 magnetization plateau state. These results shed light on the nature of the low-energy excitations in zero and strong magnetic fields, providing crucial insights into the long-standing unresolved issues of the ground state of the kagome AFM.

cond-mat.str-el↗

arXiv2023

Emergent spin-gapped magnetization plateaus in a spin-1/2 perfect kagome antiferromagnet

The two-dimensional (2D) spin-1/2 kagome Heisenberg antiferromagnet is believed to host quantum spin liquid (QSL) states with no magnetic order, but its ground state remains largely elusive. An important outstanding question concerns the presence or absence of the 1/9 magnetization plateau, where exotic quantum states, including topological ones, are expected to emerge. Here we report the magnetization of a recently discovered kagome QSL candidate YCu$_3$(OH)$_{6.5}$Br$_{2.5}$ up to 57 T. Above 50 T, a clear magnetization plateau at 1/3 of the saturation moment of Cu$^{2+}$ ions is observed, supporting that this material provides an ideal platform for the kagome Heisenberg antiferromagnet. Remarkably, we found another magnetization plateau around 20 T, which is attributed to the 1/9 plateau. The temperature dependence of this plateau reveals the distinct spin gap, whose magnitude estimated by the plateau width is approximately 10% of the exchange interaction. The observation of 1/9 and 1/3 plateaus highlights the emergence of novel states in quantum spin systems.

cond-mat.str-el↗

arXiv2022

Intrinsic suppression of topological thermal Hall effect in an exactly solvable quantum magnet

In contrast to electron (fermion) systems, topological phases of charge neutral bosons have been poorly understood despite recent extensive research on insulating magnets. The most important unresolved issue is how the inevitable inter-bosonic interactions influence the topological properties. It has been proposed that the quantum magnet SrCu$_2$(BO$_3$)$_2$ with an exact ground state serves as an ideal platform for this investigation, as the system is expected to be a magnetic analogue of a Chern insulator with electrons replaced by bosonic magnetic excitations (triplons). Here, in order to examine topologically protected triplon chiral edge modes in SrCu$_2$(BO$_3$)$_2$, we measured and calculated the thermal Hall conductivity $κ_{xy}$. Our calculations show that the sign of $κ_{xy}$ is negative, which is opposite to the previous calculations, and its magnitude is 2$π$ times smaller. No discernible $κ_{xy}$ was observed, which is at most 20-30% of our calculations if present. This implies that even relatively weak inter-particle interactions seriously influence the topological transport properties at finite temperatures. These demonstrate that, in contrast to fermionic cases, the picture of non-interacting topological quasi-particles cannot be naively applied to bosonic systems, calling special attention to the interpretation of the topological bosonic excitations reported for various insulating magnets.

cond-mat.str-el↗

arXiv2019

From coupled-wire construction of quantum Hall states to wave functions and hydrodynamics

In this paper we use a close connection between the coupled wire construction (CWC) of Abelian quantum Hall states and the theory of composite bosons to extract the Laughlin wave function and the hydrodynamic effective theory in the bulk, including the Wen-Zee topological action, directly from the CWC. We show how rotational invariance can be recovered by fine-tuning the interactions. A simple recipe is also given to construct general Abelian quantum Hall states desceibed by the multi-component Wen-Zee action.

cond-mat.str-el↗

arXiv2017

"Haldane" phases with ultracold fermionic atoms in double-well optical lattices

We propose to realize one-dimensional topological phases protected by SU($N$) symmetry using alkali or alkaline-earth atoms loaded into a bichromatic optical lattice. We derive a realistic model for this system and investigate it theoretically. Depending on the parity of $N$, two different classes of symmetry-protected topological (SPT) phases are stabilized at half-filling for physical parameters of the model. For even $N$, the celebrated spin-1 Haldane phase and its generalization to SU($N$) are obtained with no local symmetry breaking. In stark contrast, at least for $N=3$, a new class of SPT phases, dubbed chiral Haldane phases, that spontaneously break inversion symmetry, emerge with a two-fold ground-state degeneracy. The latter ground states with open-boundary conditions are characterized by different left and right boundary spins which are related by conjugation. Our results show that topological phases are within close reach of the latest experiments on cold fermions in optical lattices.

cond-mat.str-el↗

arXiv2016

Phases of one-dimensional SU(N) cold atomic Fermi gases --from molecular Luttinger liquids to topological phases

Alkaline-earth and ytterbium cold atomic gases make it possible to simulate SU(N)-symmetric fermionic systems in a very controlled fashion. Such a high symmetry is expected to give rise to a variety of novel phenomena ranging from molecular Luttinger liquids to (symmetry- protected) topological phases. We review some of the phases that can be stabilized in a one dimensional lattice. The physics of this multicomponent Fermi gas turns out to be much richer and more exotic than in the standard SU(2) case. For N > 2, the phase diagram is quite rich already in the case of the single-band model, including a molecular Luttinger liquid (with dominant superfluid instability in the N-particle channel) for incommensurate fillings, as well as various Mott-insulating phases occurring at commensurate fillings. Particular attention will be paid to the cases with additional orbital degree of freedom (which is accessible experimentally either by taking into account two atomic states or by putting atoms in the p-band levels). We introduce two microscopic models which are relevant for these cases and discuss their symmetries and strong coupling limits. More intriguing phase diagrams are then presented including, for instance, symmetry protected topological phases characterized by non-trivial edge states.

cond-mat.quant-gas↗

arXiv2015

Magnetization plateaus of an easy-axis Kagomé antiferromagnet with extended interactions

We investigate the properties in finite magnetic field of an extended anisotropic XXZ spin-1/2 model on the Kagome lattice, originally introduced by Balents, Fisher, and Girvin [Phys. Rev. B, 65, 224412 (2002)]. The magnetization curve displays plateaus at magnetization m=1/6 and 1/3 when the anisotropy is large. Using low-energy effective constrained models (quantum loop and quantum dimer models), we discuss the nature of the plateau phases, found to be crystals that break discrete rotation and/or translation symmetries. Large-scale quantum Monte-Carlo simulations were carried out in particular for the m=1/6 plateau. We first map out the phase diagram of the effective quantum loop model with an additional loop-loop interaction to find stripe order around the point relevant for the original model as well as a topological Z2 spin liquid. The existence of a stripe crystalline phase is further evidenced by measuring both standard structure factor and entanglement entropy of the original microscopic model.

cond-mat.str-el↗

arXiv2015

Magnetic excitations from an S=1/2 diamond-shaped tetramer compound Cu2PO4OH

Inelastic neutron scattering experiments have been carried out on a powder sample of Cu2PO4OH, which consists of diamond-shaped tetramer spin units with S=1/2. We have observed two nearly dispersionless magnetic excitations at E1~12 and E2~20 meV, whose energy width are broader than the instrumental resolution. The simplest square tetramer model with one dominant interaction, which predicts two sharp excitation peaks at E1 and E2(=2E1), does not explain the experimental result. We found that two diagonal intratetramer interactions compete with the main interaction and weak intertetramer interactions connect the tetramers. The main intratetramer interaction is found to split into two inequivalent ones due to a structural distortion below 160 K. Cu2PO4OH is considered to be a good material to study the S=1/2 Heisenberg tetramer system.

cond-mat.mtrl-sci↗

arXiv2015

Symmetry-protected topological order in SU(N) Heisenberg magnets --quantum entanglement and non-local order parameters

In this paper, we investigate topological properties of the ground state of the SU(N) Heisenberg chain, which is argued to be relevant to the Mott-insulating phase of alkaline-earth cold fermions in a one-dimensional optical lattice. By calculating the entanglement spectrum, we show that the ground state is in one of the topological phases protected by SU(N) symmetry. We then discuss an alternative characterization of it with non-local string order parameters. We also consider how the reduction of the protecting symmetry affects the topological phase paying particular attention to the entanglement spectrum.

cond-mat.str-el↗

arXiv2015

Phase diagrams of one-dimensional half-filled two-orbital SU(N) cold fermions systems

We investigate possible realizations of exotic SU(N) symmetry-protected topological (SPT) phases with alkaline-earth cold fermionic atoms loaded into one-dimensional optical lattices. A thorough study of two-orbital generalizations of the standard SU(N) Fermi-Hubbard model, directly relevant to recent experiments, is performed. Using state-of-the-art analytical and numerical techniques, we map out the zero-temperature phase diagrams at half-filling and identify several Mott-insulating phases. While some of them are rather conventional (non-degenerate, charge-density-wave or spin-Peierls like), we also identify, for even-N, two distinct types of SPT phases: an orbital-Haldane phase, analogous to a spin-N/2 Haldane phase, and a topological SU(N) phase, which we fully characterize by its entanglement properties. We also propose sets of non-local order parameters that characterize the SU(N) topological phases found here.

cond-mat.str-el↗

arXiv2013

Symmetry-protected topological phases of alkaline-earth cold fermionic atoms in one dimension

We investigate the existence of symmetry-protected topological phases in one-dimensional alkaline-earth cold fermionic atoms with general half-integer nuclear spin I at half filling. In this respect, some orbital degrees of freedom are required. They can be introduced by considering either the metastable excited state of alkaline-earth atoms or the p-band of the optical lattice. Using complementary techniques, we show that SU(2) Haldane topological phases are stabilised from these orbital degrees of freedom. On top of these phases, we find the emergence of topological phases with enlarged SU(2I+1) symmetry which depend only on the nuclear spin degrees of freedom. The main physical properties of the latter phases are further studied using a matrix-product state approach. On the one hand, we find that these phases are symmetry-protected topological phases, with respect to inversion symmetry, when I=1/2,5/2,9/2,..., which is directly relevant to ytterbium and strontium cold fermions. On the other hand, for the other values of I(=half-odd integer), these topological phases are stabilised only in the presence of exact SU(2I+1)-symmetry.

cond-mat.str-el↗

arXiv2012

Semiclassical Approach to Competing Orders in Two-leg Spin Ladder with Ring-Exchange

We investigate the competition between different orders in the two-leg spin ladder with a ring-exchange interaction by means of a bosonic approach. The latter is defined in terms of spin-1 hardcore bosons which treat the Néel and vector chirality order parameters on an equal footing. A semiclassical approach of the resulting model describes the phases of the two-leg spin ladder with a ring-exchange. In particular, we derive the low-energy effective actions which govern the physical properties of the rung-singlet and dominant vector chirality phases. As a by-product of our approach, we reveal the mutual induction phenomenon between spin and chirality with, for instance, the emergence of a vector-chirality phase from the application of a magnetic field in bilayer systems coupled by four-spin exchange interactions.

cond-mat.str-el↗

arXiv2010

Dilute-Bose-Gas Approach to ground state phases of 3D quantum helimagnets under high magnetic field

We study high-field phase diagram and low-energy excitations of three-dimensional quantum helimagnets. Slightly below the saturation field, the emergence of magnetic order may be mathematically viewed as Bose-Einstein condensation (BEC) of magnons. The method of dilute Bose gas enables an unbiased quantitative analysis of quantum effects in three-dimensional helimagnets and thereby three phases are found: cone, coplanar fan and an attraction-dominant one. To investigate the last phase, we extend the usual BEC approach so that we can handle 2-magnon bound states. In the case of 2-magnon BEC, the transverse magnetization vanishes and long-range order occurs in the quadrupolar channel (spin-nematic phase). As an application, we map out the phase diagram of a 3D helimagnet which consists of frustrated J1-J2 chains coupled by an interchain interaction J3.

cond-mat.str-el↗

arXiv2009

Suzaku X-Ray Imaging and Spectroscopy of Cassiopeia A

Suzaku X-ray observations of a young supernova remnant, Cassiopeia A, were carried out. K-shell transition lines from highly ionized ions of various elements were detected, including Chromium (Cr-Kalpha at 5.61 keV). The X-ray continuum spectra were modeled in the 3.4--40 keV band, summed over the entire remnant, and were fitted with a simplest combination of the thermal bremsstrahlung and the non-thermal cut-off power-law models. The spectral fits with this assumption indicate that the continuum emission is likely to be dominated by the non-thermal emission with a cut-off energy at > 1 keV. The thermal-to-nonthermal fraction of the continuum flux in the 4-10 keV band is best estimated as ~0.1. Non-thermal-dominated continuum images in the 4--14 keV band were made. The peak of the non-thermal X-rays appears at the western part. The peak position of the TeV gamma-rays measured with HEGRA and MAGIC is also shifted at the western part with the 1-sigma confidence. Since the location of the X-ray continuum emission was known to be presumably identified with the reverse shock region, the possible keV-TeV correlations give a hint that the accelerated multi-TeV hadrons in Cassiopeia A are dominated by heavy elements in the reverse shock region.

astro-ph.HE↗

arXiv2009

Supersolid phase of Three-dimensional spin and hardcore-boson models

We study the stability of solid- and supersolid (SS) phases of a three-dimensional spin- and a hardcore-Bose-Hubbard models on a body-centered cubic lattice. To see the quantum effects on the stability of the SS phase, we model the vacancies (interstitials) introduced in the solid, which are believed responsible for the appearance of the SS phase, by spinwave bosons and adopt the interaction between the condensed bosons as a criterion. A repulsive nature of the low-energy effective interaction is the necessary condition for a second-order solid-SS transition and, when this condition is met, normally the SS phase is expected. In calculating the effective interaction, we use expansions from the semiclassical- (i.e. large-S) and the Ising limit combined with the ladder approximation. The impact of quantum fluctuations crucially depends on the energy of the solid phase and that of the superfluid phase at half filling. As an application to 4He, we study the parameter region in the vicinity of the fitting parameter set given by Liu and Fisher. For this parameters set, quantum fluctuations at the second order in 1/S destabilize the solid phase, which is supposed to be stable within the mean field theory.

cond-mat.quant-gas↗

arXiv2009

Magnon BEC and various phases of 3D quantum helimagnets under high magnetic field

We study high-field phase diagram and low-energy excitations of three-dimensional quantum helimagnets. Slightly below the saturation field, the emergence of magnetic order may be viewed as Bose-Einstein condensation (BEC) of magnons. The method of dilute Bose gas enables a quantitative analysis of quantum effects in these helimagnets and thereby three phases are found: cone, coplanar fan and a phase-separated one. As an application, we map out the phase diagram of a 3D helimagnet which consists of frustrated J1-J2 chains as a function of frustration and an interchain coupling. Moreover, we also calculate the stability of the 2-magnon bound state to investigate the possibility of the bound-magnon BEC.

cond-mat.str-el↗

arXiv2007

Ground-state phase diagram and magnetic properties of a tetramerized spin-1/2 J_1-J_2 model: BEC of bound magnons and absence of the transverse magnetization

We study the ground state and the magnetization process of a spin-1/2 $J_1$-$J_2$ model with a plaquette structure by using various methods. For small inter-plaquette interaction, this model is expected to have a spin-gap and we computed the first- and the second excitation energies. If the gap of the lowest excitation closes, the corresponding particle condenses to form magnetic orders. By analyzing the quintet gap and magnetic interactions among the quintet excitations, we find a spin-nematic phase around $J_1/J_2\sim -2$ due to the strong frustration and the quantum effect. When high magnetic moment is applied, not the spin-1 excitations but the spin-2 ones soften and dictate the magnetization process. We apply a mean-field approximation to the effective Hamiltonian to find three different types of phases (a conventional BEC phase, ``striped'' supersolid phases and a 1/2-plateau). Unlike the BEC in spin-dimer systems, this BEC phase is not accompanied by transverse magnetization. Possible connection to the recently discovered spin-gap compound (CuCl)LaNb2O7 is discussed.

cond-mat.str-el↗

arXiv2006

Competing Orders and Hidden Duality Symmetries in Two-leg Spin Ladder Systems

A unifying approach to competing quantum orders in generalized two-leg spin ladders is presented. Hidden relationship and quantum phase transitions among the competing orders are thoroughly discussed by means of a low-energy field theory starting from an SU(4) quantum multicritical point. Our approach reveals that the system has a relatively simple phase structure in spite of its complicated interactions. On top of the U(1)-symmetry which is known from previous studies to mixes up antiferromagnetic order parameter with that of the p-type nematic, we find an emergent U(1)-symmetry which mixes order parameters dual to the above. On the basis of the field-theoretical- and variational analysis, we give a qualitative picture for the global structure of the phase diagram. Interesting connection to other models (e.g. bosonic t-J model) is also discussed.

cond-mat.str-el↗