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K. W. Baldwin

Publications and source records attributed to K. W. Baldwin.

At least 91 records · Page 5Linked to original sources

Realization of a Valley Superlattice

In a number of widely-studied materials, such as Si, AlAs, Bi, graphene, MoS2, and many transition metal dichalcogenide monolayers, electrons acquire an additional, spin-like degree of freedom at the degenerate conduction band minima, also known as "valleys". External symmetry breaking fields such as mechanical strain, or electric or magnetic fields, can tune the valley-polarization of these materials making them suitable candidates for "valleytronics". Here we study a quantum well of AlAs, where the two-dimensional electrons reside in two energetically degenerate valleys. By fabricating a strain-inducing grating on the sample surface, we engineer a spatial modulation of the electron population in different valleys, i.e., a "valley superlattice" in the quantum well plane. Our results establish a novel manipulation technique of the valley degree of freedom, paving the way to realizing a valley-selective layered structure in multi-valley materials, with potential application in valleytronics.

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Direct observation of composite fermions and their fully spin-polarized Fermi sea near $ν=5/2$

The enigmatic even-denominator fractional quantum Hall state at Landau level filling factor $ν=5/2$ is arguably the most promising candidate for harboring Majorana quasi-particles with non-Abelian statistics and thus of potential use for topological quantum computing. The theoretical description of the $ν=5/2$ state is generally believed to involve a topological p-wave pairing of fully spin-polarized composite fermions through their condensation into a non-Abelian Moore-Read Pfaffian state. There is, however, no direct and conclusive experimental evidence for the existence of composite fermions near $ν=5/2$ or for an underlying fully spin-polarized Fermi sea. Here, we report the observation of composite fermions very near $ν=5/2$ through geometric resonance measurements, and find that the measured Fermi wavevector provides direct demonstration of a Fermi sea with full spin polarization. This lends crucial credence to the model of $5/2$ fractional quantum Hall effect as a topological p-wave paired state of composite fermions.

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Surface segregation and the Al problem in GaAs quantum wells

Low-defect two-dimensional electron systems (2DESs) are essential for studies of fragile many-body interactions that only emerge in nearly-ideal systems. As a result, numerous efforts have been made to improve the quality of modulation-doped Al$_x$Ga$_{1-x}$As/GaAs quantum wells (QWs), with an emphasis on purifying the source material of the QW itself or achieving better vacuum in the deposition chamber. However, this approach overlooks another crucial component that comprises such QWs, the Al$_x$Ga$_{1-x}$As barrier. Here we show that having a clean Al source and hence a clean barrier is instrumental to obtain a high-quality GaAs 2DES in a QW. We observe that the mobility of the 2DES in GaAs QWs declines as the thickness or Al content of the Al$_x$Ga$_{1-x}$As barrier beneath the QW is increased, which we attribute to the surface segregation of Oxygen atoms that originate from the Al source. This conjecture is supported by the improved mobility in the GaAs QWs as the Al cell is cleaned out by baking.

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Intersubband scattering in n-GaAs/AlGaAs wide quantum wells

Slow magnetooscilations of the conductivity are observed in a 75 nm wide quantum well at heating of the two-dimensional electrons by a high-intensity surface acoustic wave. These magnetooscillations are caused by intersubband elastic scattering between the symmetric and asymmetric subbands formed due to an electrostatic barrier in the center of the quantum well. The tunneling splitting between these subbands as well as the intersubband scattering rate are determined.

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Cyclotron Orbits of Composite Fermions in the Fractional Quantum Hall Regime

We study a bilayer GaAs hole system that hosts two distinct many-body phases at low temperatures and high perpendicular magnetic fields. The higher-density (top) layer develops a Fermi sea of composite fermions (CFs) in its half-filled lowest Landau level, while the lower-density (bottom) layer forms a Wigner crystal (WC) as its filling becomes very small. Owing to the inter-layer interaction, the CFs in the top-layer feel the periodic Coulomb potential of the WC in the bottom-layer. We measure the magnetoresistance of the top-layer while changing the bottom-layer density. As the WC layer density increases, the resistance peaks separating the adjacent fractional quantum Hall states in the top-layer change nonmonotonically and attain maximum values when the cyclotron orbit of the CFs encloses one WC lattice point. These features disappear at T = 275 mK when the WC melts. The observation of such geometric resonance features is unprecedented and surprising as it implies that the CFs retain a well-defined cyclotron orbit and Fermi wave vector even deep in the fractional quantum Hall regime, far from half-filling.

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Berry Phase and Anomalous Transport of the Composite Fermions at the Half-Filled Landau Level

The fractional quantum Hall effect (FQHE) in two-dimensional electron system (2DES) is an exotic, superfluid-like matter with an emergent topological order. From the consideration of Aharonov-Bohm interaction of electrons and magnetic field, the ground state of a half-filled lowest Landau level is mathematically transformed to a Fermi sea of composite objects of electrons bound to two flux quanta, termed composite fermions (CFs). A strong support for the CF theories comes from experimental confirmation of the predicted Fermi surface at $ν$ = 1/2 (where $ν$ is the Landau level filling factor) from the detection of the Fermi wave vector in the semi-classical geometrical resonance experiments. Recent developments in the theory of CFs have led to a prediction of a $π$ Berry phase for the CF circling around the Fermi surface at half-filling. In this paper we provide the first experimental evidence for the detection of the Berry phase of CFs in the fractional quantum Hall effect. Our measurements of the Shubnikov-de Haas oscillations of CFs as a function carrier density at a fixed magnetic field provide a strong support for an existence of a $π$ Berry phase at $ν$ = 1/2. We also discover that the conductivity of composite fermions at $ν$ = 1/2 displays an anomalous linear density dependence, whose origin remains mysterious yet tantalizing.

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Low-Frequency Microwave Induced Quantum Oscillations in A Two-Dimensional Electron System

We study the magnetoresistance of an ultrahigh mobility GaAs/AlGaAs two-dimensional electron sample in a weak magnetic field under low-frequency (f < 20 GHz) microwave (MW) irradiation. We observe that with decreasing MW frequency, microwave induced resistance oscillations (MIRO) damp and multi-photon processes become dominant. At very low MW frequency (f < 4 GHz), MIRO disappears gradually and a new SdH-like oscillation develops. The analysis indicates that the new oscillation may originate from alternating Hall-field induced resistance oscillations (ac-HIRO), or can be viewed as a multi-photon process of MIRO in low MW frequency limit. Our findings bridge the non-equilibrium states of MIRO and HIRO, which can be brought into a frame of quantum tunneling junction model.

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Interaction-induced Interlayer Charge Transfer in the Extreme Quantum Limit

An interacting bilayer electron system provides an extended platform to study electron-electron interaction beyond single layers. We report here experiments demonstrating that the layer densities of an asymmetric bilayer electron system oscillate as a function of perpendicular magnetic field that quantizes the energy levels. At intermediate fields, this interlayer charge transfer can be well explained by the alignment of the Landau levels in the two layers. At the highest fields where both layers reach the extreme quantum limit, however, there is an anomalous, enhanced charge transfer to the majority layer. Surprisingly, when the minority layer becomes extremely dilute, this charge transfer slows down as the electrons in the minority layer condense into a Wigner crystal. Furthermore, by examining the quantum capacitance of the dilute layer at high fields, the screening induced by the composite fermions in an adjacent layer is unveiled. The results highlight the influence of strong interaction in interlayer charge transfer in the regime of very high fields and low Landau level filling factors.

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Tuning of Fermi Contour Anisotropy in GaAs (001) 2D Holes via Strain

We demonstrate tuning of the Fermi contour anisotropy of two-dimensional (2D) holes in a symmetric GaAs (001) quantum well via the application of in-plane strain. The ballistic transport of high-mobility hole carriers allows us to measure the Fermi wavevector of 2D holes via commensurability oscillations as a function of strain. Our results show that a small amount of in-plane strain, on the order of $10^{-4}$, can induce significant Fermi wavevector anisotropy as large as 3.3, equivalent to a mass anisotropy of 11 in a parabolic band. Our method to tune the anisotropy \textit{in situ} provides a platform to study the role of anisotropy on phenomena such as the fractional quantum Hall effect and composite fermions in interacting 2D systems.

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Search for Composite Fermions at Filling Factor 5/2: Role of Landau Level and Subband Index

The pairing of composite fermions (CFs), electron-flux quasi-particles, is commonly proposed to explain the even-denominator fractional quantum Hall state observed at $ν=5/2$ in the first excited ($N=1$) Landau level (LL) of a two-dimensional electron system (2DES). While well-established to exist in the lowest ($N=0$) LL, much is unknown about CFs in the $N=1$ LL. Here we carry out geometric resonance measurements to detect CFs at $ν=5/2$ by subjecting the 2DES to a one-dimensional density modulation. Our data, taken at a temperature of 0.3 K, reveal no geometric resonances for CFs in the $N=1$ LL. In stark contrast, we observe clear signatures of such resonances when $ν=5/2$ is placed in the $N=0$ LL of the anti-symmetric subband by varying the 2DES width. This finding implies that the CFs' mean-free-path is significantly smaller in the $N=1$ LL compared to the $N=0$ LL. Our additional data as a function of in-plane magnetic field highlight the role of subband index and establish that CFs at $ν=5/2$ in the $N=0$ LL are more anisotropic in the symmetric subband than in the anti-symmetric subband.

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Full Momentum and Energy Resolved Spectral Function of a 2D Electronic System

The single-particle spectral function measures the density of electronic states (DOS) in a material as a function of both momentum and energy, providing central insights into phenomena such as superconductivity and Mott insulators. While scanning tunneling microscopy (STM) and other tunneling methods have provided partial spectral information, until now only angle-resolved photoemission spectroscopy (ARPES) has permitted a comprehensive determination of the spectral function of materials in both momentum and energy. However, ARPES operates only on electronic systems at the material surface and cannot work in the presence of applied magnetic fields. Here, we demonstrate a new method for determining the full momentum and energy resolved electronic spectral function of a two-dimensional (2D) electronic system embedded in a semiconductor. In contrast with ARPES, the technique remains operational in the presence of large externally applied magnetic fields and functions for electronic systems with zero electrical conductivity or with zero electron density. It provides a direct high-resolution and high-fidelity probe of the dispersion and dynamics of the interacting 2D electron system. By ensuring the system of interest remains under equilibrium conditions, we uncover delicate signatures of many-body effects involving electron-phonon interactions, plasmons, polarons, and a novel phonon analog of the vacuum Rabi splitting in atomic systems.

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Fine structure of high-power microwave-induced resistance oscillations

We report on observation of a fine structure of microwave-induced resistance oscillations in an ultraclean two-dimensional electron gas. This fine structure is manifested by multiple secondary sharp extrema, residing beside the primary ones, which emerge at high radiation power. Theoretical considerations reveal that this fine structure originates from multiphoton-assisted scattering off short-range impurities. Unique properties of the fine structure allow us to access all experimental parameters, including microwave power, and to separate different contributions to photoresistance. Furthermore, we show that the fine structure offers a convenient means to quantitatively assess the correlation properties of the disorder potential in high-quality systems, allowing separation of short- and long-range disorder contributions to the electron mobility.

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Transference of Fermi Contour Anisotropy to Composite Fermions

There has been a surge of recent interest in the role of anisotropy in interaction-induced phenomena in two-dimensional (2D) charged carrier systems. A fundamental question is how an anisotropy in the energy-band structure of the carriers at zero magnetic field affects the properties of the interacting particles at high fields, in particular of the composite fermions (CFs) and the fractional quantum Hall states (FQHSs). We demonstrate here tunable anisotropy for holes and hole-flux CFs confined to GaAs quantum wells, via applying \textit{in situ} in-plane strain and measuring their Fermi wavevector anisotropy through commensurability oscillations. For strains on the order of $10^{-4}$ we observe significant deformations of the shapes of the Fermi contours for both holes and CFs. The measured Fermi contour anisotropy for CFs at high magnetic field ($α_\mathrm{CF}$) is less than the anisotropy of their low-field hole (fermion) counterparts ($α_\mathrm{F}$), and closely follows the relation: $α_\mathrm{CF} = \sqrt{α_\mathrm{F}}$. The energy gap measured for the $ν= 2/3$ FQHS, on the other hand, is nearly unaffected by the Fermi contour anisotropy up to $α_\mathrm{F} \sim 3.3$, the highest anisotropy achieved in our experiments.

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Interplay between Quantum Well Width and Interface Roughness for Electron Transport Mobility in GaAs Quantum Wells

We report transport mobility measurements for clean, two-dimensional (2D) electron systems confined to GaAs quantum wells (QWs), grown via molecular beam epitaxy, in two families of structures, a standard, symmetrically-doped GaAs set of QWs with Al$_{0.32}$Ga$_{0.68}$As barriers, and one with additional AlAs cladding surrounding the QWs. Our results indicate that the mobility in narrow QWs with no cladding is consistent with existing theoretical calculations where interface roughness effects are softened by the penetration of the electron wave function into the adjacent low barriers. In contrast, data from AlAs-clad wells show a number of samples where the 2D electron mobility is severely limited by interface roughness. These measurements across three orders of magnitude in mobility provide a road map of reachable mobilities in the growth of GaAs structures of different electron densities, well widths, and barrier heights.

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Photovoltage Detection of Edge Magnetoplasmon Oscillations and Giant Magnetoplasmon Resonances in A Two-Dimensional Hole System

In our high mobility p-type AlGaAs/GaAs two-dimensional hole samples, we originally observe the B-periodic oscillation induced by microwave (MW) in photovoltage (PV) measurements. In the frequency range of our measurements (5 - 40 GHz), the period (ΔB) is inversely proportional to the microwave frequency (f). The distinct oscillations come from the edge magnetoplasmon (EMP) in the high quality heavy hole system. In our hole sample with a very large effective mass, the observation of the EMP oscillations is in neither the low frequency limit nor the high frequency limit, and the damping of the EMP oscillations is very weak under high magnetic fields. Simultaneously, we observe the giant plasmon resonance signals in our measurements on the shallow two-dimensional hole system (2DHS).

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Geometric Resonance of Composite Fermions near Bilayer Quantum Hall States

Via the application of parallel magnetic field, we induce a single-layer to bilayer transition in two-dimensional electron systems confined to wide GaAs quantum wells, and study the geometric resonance of composite fermions (CFs) with a periodic density modulation in our samples. The measurements reveal that CFs exist close to bilayer quantum Hall states, formed at Landau level filling factors $ν=1$ and 1/2. Near $ν=1$, the geometric resonance features are consistent with half the total electron density in the bilayer system, implying that CFs prefer to stay in separate layers and exhibit a two-component behavior. In contrast, close to $ν=1/2$, CFs appear single-layer-like (single-component) as their resonance features correspond to the total density.

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Reorientation of the stripe Phase of 2D Electrons by a Minute Density Modulation

Interacting two-dimensional electrons confined in a GaAs quantum well exhibit isotropic transport when the Fermi level resides in the first excited ($N=1$) Landau level. Adding an in-plane magnetic field ($B_{||}$) typically leads to an anisotropic, stripe-like (nematic) phase of electrons with the stripes oriented perpendicular to the $B_{||}$ direction. Our experimental data reveal how a periodic density modulation, induced by a surface strain grating from strips of negative electron-beam resist, competes against the $B_{||}$-induced orientational order of the stripe phase. Even a minute ($<0.25\%$) density modulation is sufficient to reorient the stripes along the direction of the surface grating.

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Anisotropic composite fermions and fractional quantum Hall effect

We study the role of anisotropy on the transport properties of composite fermions near Landau level filling factor $ν=1/2$ in two-dimensional holes confined to a GaAs quantum well. By applying a parallel magnetic field, we tune the composite fermion Fermi sea anisotropy and monitor the relative change of the transport scattering time at $ν=1/2$ along the principal directions. Interpreted in a simple Drude model, our results suggest that the scattering time is longer along the longitudinal direction of the composite fermion Fermi sea. Furthermore, the measured energy gap for the fractional quantum Hall state at $ν=2/3$ decreases when anisotropy becomes significant. The decrease, however, might partly stem from the charge distribution becoming bilayer-like at very large parallel magnetic fields.

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