arXiv subjects

K. W. Brown

Publications and source records attributed to K. W. Brown.

31 records · Page 2Linked to original sources

arXiv2022

Proton and neutron exchange as a prelude to fusion at near-barrier energies

Systematic examination of fusion for $^{39,41,45,47}$K + $^{28}$Si and $^{36,44}$Ar + $^{28}$Si provides insight into the impact of neutron and proton exchange on fusion for nuclei at and near the N=20 and N=28 shells. Comparison of the reduced excitation functions reveals a marked difference between the behavior of open-shell and closed-shell systems. While coupled channels calculations provide a good description for the closed-shell nuclei they significantly under-predict the fusion cross-section for open-shell nuclei. The observed trends are examined in the context of a potential energy surface, including shell effects, and multi-nucleon exchange with consideration of Pauli-blocking.

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arXiv2022

In-flight production of an isomeric beam of $^{16}$N

An in-flight beam of $^{16}$N was produced via the single-neutron adding ($d$,$p$) reaction in inverse kinematics at the recently upgraded Argonne Tandem Linear Accelerator System (ATLAS) in-flight system. The amount of the $^{16}$N beam which resided in its excited 0.120-MeV $J^π=0^-$ isomeric state (T$_{1/2}\approx5$ $μ$s) was determined to be 40(5)% at a reaction energy of 7.9(3) MeV/$u$, and 24(2)% at a reaction energy of 13.2(2) MeV/$u$. The isomer measurements took place at an experimental station $\approx30$ m downstream of the production target and utilized an Al beam-stopping foil and a HPGe Clover detector. Composite $^{16}$N beam rate determinations were made at the experimental station and the focal plane of the Argonne in-flight radioactive ion-beam separator (RAISOR) with Si $Δ$E-E telescopes. A Distorted Wave Born Approximation (DWBA) approach was coupled with the known spectroscopic information on $^{16}$N in order to estimate the relative $^{16}$N isomer yields and composite $^{16}$N beam rates. In addition to the observed reaction-energy dependence of the isomer fraction, a large sensitivity to angular acceptance of the recoils was also observed.

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arXiv2021

Beam Particle Identification and Tagging of Incompletely Stripped Heavy Beams with HEIST

A challenge preventing successful inverse kinematics measurements with heavy nuclei that are not fully stripped is identifying and tagging the beam particles. For this purpose, the HEavy ISotope Tagger (HEIST) has been developed. HEIST utilizes two micro-channel plate timing detectors to measure time of flight, a multi-sampling ion chamber to measure energy loss, and a high purity Ge detector to identify isomer decays and calibrate the isotope identification system. HEIST has successfully identified $^{198}$Pb and other nearby nuclei at energies of about 75 MeV/A. In the experiment discussed, a typical cut containing 89\% of all $^{198}$Pb$^{+80}$ in the beam had a purity of 86\%. We examine the issues of charge state contamination. The observed charge state populations of these ions are presented and are moderately well described by the charge state model GLOBAL.

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arXiv2021

Using spin alignment of inelastically-excited fast beams to make spin assignments: the spectroscopy of 13O as a test case

Excited states in 13O were investigated using inelastic scattering of an E/A=69.5-MeV 13O beam off of a 9Be target. The excited states were identified in the invariant-mass spectra of the decay products. Both single proton and sequential two-proton decays of the excited states were examined. For a number of the excited states, the protons were emitted with strong anisotropy where emissions transverse to the beam axis are favored. The measured proton-decay angular distributions were compared to predictions from distorted-wave born-approximation (DWBA) calculations of the spin alignment which was shown to be largely independent of the excitation mechanism. The deduced $^{13}$O level scheme is compared to ab initio no-core shell model with continuum (NCSMC) predictions. The lowest-energy excited states decay isotropically consistent with predictions of strong proton 1s1/2 structure. Above these states in the level scheme, we observed a number of higher-spin states not predicted within the model. Possibly these are associated with rotational bands built on deformed cluster configurations predicted by antisymmetrized molecular dynamics (AMD) calculations. The spin alignment mechanism is shown to be useful for making spin assignments and may have widespread use.

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arXiv2021

Value-assigned pulse shape discrimination for neutron detectors

Using the waveforms from a digital electronic system, an offline analysis technique on pulse shape discrimination (PSD) has been developed to improve the neutron-gamma separation in a bar-shaped NE-213 scintillator that couples to a photomultiplier tube (PMT) at each end. The new improved method, called the ``valued-assigned PSD'' (VPSD), assigns a normalized fitting residual to every waveform as the PSD value. This procedure then facilitates the incorporation of longitudinal position dependence of the scintillator, which further enhances the PSD capability of the detector system. In this paper, we use radiation emitted from an AmBe neutron source to demonstrate that the resulting neutron-gamma identification has been much improved when compared to the traditional technique that uses the geometric mean of light outputs from both PMTs. The new method has also been modified and applied to a recent experiment at the National Superconducting Cyclotron Laboratory (NSCL) that uses an analog electronic system.

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arXiv2020

Isotopically resolved neutron total cross sections at intermediate energies

The neutron total cross sections $σ_{tot}$ of $^{16,18}$O, $^{58,64}$Ni, $^{103}$Rh, and $^{112,124}$Sn have been measured at the Los Alamos Neutron Science Center (LANSCE) from low to intermediate energies (3 $\leq E_{lab} \leq$ 450 MeV) by leveraging waveform-digitizer technology. The $σ_{tot}$ relative differences between isotopes are presented, revealing additional information about the isovector components needed for an accurate optical-model description away from stability. Digitizer-enabled $σ_{tot}$-measurement techniques are discussed and a series of uncertainty-quantified dispersive optical model (DOM) analyses using these new data is presented, validating the use of the DOM for modeling light systems ($^{16,18}$O) and systems with open neutron shells ($^{58,64}$Ni and $^{112,124}$Sn). The valence-nucleon spectroscopic factors extracted for each isotope reaffirm the usefulness of high-energy proton reaction cross sections for characterizing depletion from the mean-field expectation.

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arXiv2020

Particle decays of levels in $^{11,12}$N and $^{12}$O investigated with the invariant-mass method

Particle-decaying states of the light nuclei $^{11,12}$N and $^{12}$O were studied using the invariant-mass method. The decay energies and intrinsic widths of a number of states were measured, and the momentum correlations of three-body decaying states were considered. A second 2$p$-decaying 2$^+$ state of $^{12}$O was observed for the first time, and a higher energy $^{12}$O state was observed in the 4$p$+2$α$ decay channel. This 4$p$+2$α$ channel also contains contributions from fission-like decay paths, including $^6$Be$_{g.s.}$+$^{6}$Be$_{g.s.}$. Analogs to these states in $^{12}$O were found in $^{12}$N in the 2$p$+$^{10}$B and 2$p$+$α$+$^6$Li channels. The momentum correlations for the prompt 2$p$ decay of $^{12}$O$_{g.s.}$ were found to be nearly identical to those of $^{16}$Ne$_{g.s.}$, and the correlations for the new 2$^+$ state were found to be consistent with sequential decay through excited states in $^{11}$N. The momentum correlations for the 2$^+_1$ state in $^{12}$O provide a new value for the $^{11}$N ground-state energy. The states in $^{12}$N/$^{12}$O that belong to the $A$=12 isobaric sextet do not deviate from the quadratic isobaric multiplet mass equation (IMME) form.

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arXiv2019

Invariant-mass spectroscopy of $^{14}$O excited states

Excited states in $^{14}$O have been investigated both experimentally and theoretically. Experimentally, these states were produced via neutron-knockout reactions with a fast $^{15}$O beam and the invariant-mass technique was employed to isolate the 1$p$ and 2$p$ decay channels and determine their branching ratios. The spectrum of excited states was also calculated with the Shell Model Embedded in the Continuum that treats bound and scattering states in a unified model. By comparing energies, widths and decay branching patterns, spin and parity assignments for all experimentally observed levels below 8 MeV are made. This includes the location of the second 2$^{+}$ state that we find is in near degeneracy with the third 0$^{+}$ state. An interesting case of sequential 2$p$ decay through a pair of degenerate $^{13}$N excited states with opposite parities was found where the interference between the two sequential decay pathways produces an unusual relative-angle distribution between the emitted protons.

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arXiv2019

Non-linearity effects on the light-output calibration of light charged particles in CsI(Tl) scintillator crystals

The light output produced by light ions (Z<=4) in CsI(Tl) crystals is studied over a wide range of detected energies (E<=300 MeV). Energy-light calibration data sets are obtained with the 10 cm crystals in the recently upgraded High-Resolution Array (HiRA10). We use proton recoil data from 40,48Ca + CH2 at 28 MeV/u, 56.6 MeV/u, 39 MeV/u and 139.8 MeV/u and data from a dedicated experiment with direct low-energy beams. We also use the punch through points of p, d, and t particles from 40,48Ca + 58,64Ni, 112,124Sn collisions reactions at 139.8 MeV/u. Non-linearities, arising in particular from Tl doping and light collection efficiency in the CsI crystals, are found to significantly affect the light output and therefore the calibration of the detector response for light charged particles, especially the hydrogen isotopes. A new empirical parametrization of the hydrogen light output, L(E,Z=1,A), is proposed to account for the observed effects. Results are found to be consistent for all 48 CsI(Tl) crystals in a cluster of 12 HiRA10 telescopes.

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arXiv2019

First observation of unbound $^{11}$O, the mirror of the halo nucleus $^{11}$Li

The structure of the extremely proton-rich nucleus $^{11}_{~8}$O$_3$, the mirror of the two-neutron halo nucleus $^{11}_{~3}$Li$_8$, has been studied experimentally for the first time. Following two-neutron knockout reactions with a $^{13}$O beam, the $^{11}$O decay products were detected after two-proton emission and used to construct an invariant-mass spectrum. A broad peak of width $\sim$3\,MeV was observed. Within the Gamow coupled-channel approach, it was concluded that this peak is a multiplet with contributions from the four-lowest $^{11}$O resonant states: $J^π$=3/2$^-_1$, 3/2$^-_2$, 5/2$^+_1$, and 5/2$^+_2$. The widths and configurations of these states show strong, non-monotonic dependencies on the depth of the $p$-$^9$C potential. This unusual behavior is due to the presence of a broad threshold resonant state in $^{10}$N, which is an analog of the virtual state in $^{10}$Li in the presence of the Coulomb potential. After optimizing the model to the data, only a moderate isospin asymmetry between ground states of $^{11}$O and $^{11}$Li was found.

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arXiv2018

Invariant-mass spectroscopy of $^{18}$Ne, $^{16}$O, and $^{10}$C excited states formed in neutron transfer reactions

Neutron transfer reactions with fast secondary beams of $^{17}$Ne, $^{15}$O, and $^9$C have been studied with the HiRA and CAESAR arrays. Excited states of $^{18}$Ne, $^{16}$O, and $^{10}$C in the continuum have been identified using invariant-mass spectroscopy. The best experimental resolution of these states is achieved by selecting events where the decay fragments are emitted transverse to the beam direction. We have confirmed a number of spin assignments made in previous works for the negative-parity states of $^{18}$Ne. In addition we have found new higher-lying excited states in $^{16}$O and $^{18}$Ne, some of which fission into two ground-state $^8$Be fragments. Finally for $^{10}$C, a new excited state was observed. These transfer reactions were found to leave the remnant of the $^9$Be target nuclei at very high excitation energies and maybe associated with the pickup of a deeply-bound $^9$Be neutron.

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arXiv2018

On Determining Dead Layer and Detector Thicknesses for a Position-Sensitive Silicon Detector

In this work, two particular properties of the position-sensitive, thick silicon detectors (known as the "E" detectors) in the High Resolution Array (HiRA) are investigated: the thickness of the dead layer on the front of the detector, and the overall thickness of the detector itself. The dead layer thickness for each E detector in HiRA is extracted using a measurement of alpha particles emitted from a $^{212}$Pb pin source placed close to the detector surface. This procedure also allows for energy calibrations of the E detectors, which are otherwise inaccessible for alpha source calibration as each one is sandwiched between two other detectors. The E detector thickness is obtained from a combination of elastically scattered protons and an energy-loss calculation method. Results from these analyses agree with values provided by the manufacturer.

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arXiv2017

Disentangling the role of vibration, rotation, and neutron transfer in the fusion of neutron-rich mid-mass nuclei

We report the first measurement of the fusion excitation functions for $^{39,47}$K + $^{28}$Si at near-barrier energies. Evaporation residues resulting from the fusion process were identified by direct measurement of their energy and time-of-flight with high geometric efficiency. At the lowest incident energy, the cross-section measured for the neutron-rich $^{47}$K induced reaction is ~6 times larger than that of the $β$-stable system. The experimental data are compared with both a dynamical deformation model and coupled channels calculations (CCFULL).

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