arXiv subjects

K. Watanabe

Publications and source records attributed to K. Watanabe.

At least 415 records · Page 23Linked to original sources

arXiv2010

Hunting for Monolayer Boron Nitride: Optical and Raman Signatures

We describe the identification of single- and few- layer boron nitride. Its optical contrast is much smaller than that of graphene but even monolayers are discernable by optimizing viewing conditions. Raman spectroscopy can be used to confirm BN monolayers. They exhibit an upshift in the fundamental Raman mode by up to 4 cm-1. The number of layers in thicker crystals can be counted by exploiting an integer-step increase in the Raman intensity and optical contrast.

cond-mat.mes-hall↗

arXiv2010

Boron nitride substrates for high-quality graphene electronics

Graphene devices on standard SiO2 substrates are highly disordered, exhibiting characteristics far inferior to the expected intrinsic properties of graphene[1-12]. While suspending graphene above the substrate yields substantial improvement in device quality[13,14], this geometry imposes severe limitations on device architecture and functionality. Realization of suspended-like sample quality in a substrate supported geometry is essential to the future progress of graphene technology. In this Letter, we report the fabrication and characterization of high quality exfoliated mono- and bilayer graphene (MLG and BLG) devices on single crystal hexagonal boron nitride (h-BN) substrates, by a mechanical transfer process. Variable-temperature magnetotransport measurements demonstrate that graphene devices on h-BN exhibit enhanced mobility, reduced carrier inhomogeneity, and reduced intrinsic doping in comparison with SiO2-supported devices. The ability to assemble crystalline layered materials in a controlled way sets the stage for new advancements in graphene electronics and enables realization of more complex graphene heterostructres.

cond-mat.mes-hall↗

arXiv2010

Anisotropic excitonic effects in the energy loss function of hexagonal boron nitride

We demonstrate that the valence energy-loss function of hexagonal boron nitride (hBN) displays a strong anisotropy in shape, excitation energy and dispersion for momentum transfer q parallel or perpendicular to the hBN layers. This is manifested by e.g. an energy shift of 0.7 eV that cannot be captured by single-particle approaches and is a demonstration of a strong anisotropy in the two-body electron-hole interaction. Furthermore, for in-plane directions of q we observe a splitting of the -plasmon in the M direction that is absent in the K direction and this can be traced back to band-structure effects.

cond-mat.mtrl-sci↗

arXiv2009

$^{63/65}$Cu- and $^{35/37}$Cl-NMR Studies of Triplet Localization in the Quantum Spin System NH$_4$CuCl$_3$

$^{63/65}$Cu- and $^{35/37}$Cl-NMR experiments were performed to investigate triplet localization in the $S=1/2$ dimer compound NH$_4$CuCl$_3$, which shows magnetization plateaus at one-quarter and three-quarters of the saturation magnetization. In $^{63/65}$Cu-NMR experiments, signal from only the singlet Cu site was observed, because that from the triplet Cu site was invisible due to the strong spin fluctuation of onsite 3$d$-spins. We found that the temperature dependence of the shift of $^{63/65}$Cu-NMR spectra at the singlet Cu site deviated from that of macroscopic magnetization below T=6 K. This deviation is interpreted as the triplet localization in this system. From the $^{35/37}$Cl-NMR experiments at the 1/4-plateau phase, we found the two different temperature dependences of Cl-shift, namely the temperature dependence of one deviates below T=6 K from that of the macroscopic magnetization as observed in the $^{63/65}$Cu-NMR experiments, whereas the other corresponds well with that of the macroscopic magnetization in the entire experimental temperature region. We interpreted these dependences as reflecting the transferred hyperfine field at the Cl site located at a singlet site and at a triplet site, respectively. This result also indicates that the triplets are localized at low temperatures. $^{63/65}$Cu-NMR experiments performed at high magnetic fields between the one-quarter and three-quarters magnetization plateaus have revealed that the two differently oriented dimers in the unit cell are equally occupied by triplets, the fact of which limits the theoretical model on the periodic structure of the localized triplets.

cond-mat.stat-mech↗

arXiv2008

Hollow carbon spheres as an efficient dopant for enhancing critical current density of MgB2 based tapes

A significant enhancement of Jc and Hirr in MgB2 tapes has been achieved by the in situ powder-in-tube method utilizing hollow carbon spheres (HCS) as dopants. At 4.2 K, the transport Jc for the 850C sintered samples reached 3.1x10^4, and 1.4x10^4 A/cm^2 at 10 and 12 T, respectively, and were better than those of optimal nano-SiC doped tapes. Furthermore, the Hirr for doped sample was raised up to 16.8 T at 10 K due to the carbon substitution effect. The results demonstrate that HCS is one of the most promising dopants besides nano-carbon and SiC for the enhancement of current capacity for MgB2 in high fields.

cond-mat.supr-con↗

arXiv2008

A cheap liquid additive from acetone for strong in-field Jc enhancement in MgB2 conductors

We report on significant flux pinning enhancement in MgB2/Fe tapes that has been easily obtained by a simple and cheap route using acetone as both an efficient ball-milling medium and liquid additive through the in situ method. Results showed that the highly reactive C released from the decomposition of the acetone substituted into B sites, accompanied by the grain refinement effect due to the acetone doping. At 4.2 K, the transport Jc for the 5 wt % acetone doped tapes sintered at 700C reached up to 2.4x10^4 A/cm^2 at 10 T, which is even higher than that of the nano-C added samples heated at 900C.

cond-mat.supr-con↗

arXiv2008

Photon correlation in GaAs self-assembled quantum dots

We report on photon coincidence measurement in a single GaAs self-assembled quantum dot (QD) using a pulsed excitation light source. At low excitation, when a neutral exciton line was present in the photoluminescence (PL) spectrum, we observed nearly perfect single photon emission from an isolated QD at 670 nm wavelength. For higher excitation, multiple PL lines appeared on the spectra, reflecting the formation of exciton complexes. Cross-correlation functions between these lines showed either bunching or antibunching behavior, depending on whether the relevant emission was from a biexciton cascade or a charged exciton recombination.

cond-mat.other↗

arXiv2007

Strong influence of precursor powder on the critical current density of Fe-sheathed MgB2 tapes

The effect of the quality of starting powders on the microstructure and superconducting properties of in-situ processed Fe-sheathed MgB2 tapes has been investigated. Three different types of commercial atomized spherical magnesium powder and two different purities of amorphous boron powder were employed. When using the 10-micrometre magnesium as precursor powders, the Mg reacted with boron more uniformly and quickly, thus the uniformity of the fabricated MgB2 was improved and the grain size of the MgB2 was decreased, hence significant critical current density (Jc) enhancements were achieved for MgB2 tapes. Jc at 4.2 K for MgB2 tapes made from the 10 um Mg and high purity boron powders was at least a factor of ten higher than values measured for MgB2 samples made from all other starting powders. At 20 K, 5 T, the typical Jc values of the tapes were over 1.0x10^4 A/cm^2 and were much better than those of tape samples reported recently.

cond-mat.supr-con↗

arXiv2007

NMR Study on the Vortex Slush Phase in Organic Superconductor κ-(BEDT-TTF)2Cu(NCS)2

The vortex state in a single crystal of the layered organic superconductor κ-(BEDT-TTF2Cu(NCS)2, where BEDT-TTF (or ET) is bis(ethylenedithio)tetrathiafulvalene, was studied by 1H-NMR. Under a low field region around 0.75 T, the vortex glass-liquid transition was demonstrated by a diverging of the longitudinal nuclear spin relaxation rate and peak-broadening in spectra. Under a high field region near the upper critical field Hc2(0)~7 T, the curvature of nuclear spin relaxation curves showed a drastic change at the temperature where the emergence of the quantum vortex slush state was reported. The mechanism in this curvature change was discussed in terms of the fluctuating field produced by fragments of vortex glass.

cond-mat.str-el↗

arXiv2007

Relaxation and phase space singularities in time series of human magnetoencephalograms as indicator of photosensitive epilepsy

To analyze the crucial role of fluctuation and relaxation effects for the function of the human brain we studied some statistical quantifiers that support the information characteristics of neuromagnetic brain responses (magnetoencephalogram, MEG). The signals to a flickering stimulus of different color combinations have been obtained from a group of control subjects which is then contrasted with those of a patient suffering photosensitive epilepsy (PSE). We found that the existence of the specific stratification of the phase clouds and the concomitant relaxation singularities of the corresponding nonequilibrium dynamics of the chaotic behavior of the signals in separate areas in a patient provide likely indicators for the zones which are responsible for the appearance of PSE.

physics.med-ph↗

arXiv2007

Amplification of Quantum Meson Modes in the Late Time of the Chiral Phase Transition

We investigate the time evolution of the quantum meson modes in the late time of chiral phase transition. In particular, it is shown that there exists a possible solution to the equation of motion for the quantum meson modes, which reveals a parametric resonance and/or resonance through forced oscillation induced by the small oscillation of the chiral condensate. After that, we demonstrate the unstable regions for the quantum meson modes in both the cases of a uniform and spatially expanding system.

nucl-th↗

arXiv2007

Strongly enhanced critical current density in Fe-sheathed MgB2 tapes by stearic acid and stearate doping

Fe-sheathed MgB2 tapes with cheap stearic acid, Mg stearate and Zn stearate doping were prepared through the in situ powder-in-tube method. It is found that Jc, Hirr, and Hc2 were significantly enhanced by doping. Compared to the pure tapes, Jc for all the doped samples was improved by more than an order of magnitude in a high-field regime. At 4.2 K, the transport Jc reached 2.02x10^4 A/cm^2 at 10 T for the Zn stearate doped tapes and 3.72x10^3 A/cm^2 at 14 T for the stearic acid doped samples, respectively, equivalent to that of tapes achieved by nanoscale SiC or carbon doping. The improvement of Jc-H properties in doped samples can be attributed to the increase of Hc2 resulting from the incorporation of C atoms into the MgB2 crystal lattice as well as a high density of flux-pinning centers.

cond-mat.supr-con↗

arXiv2006

Final-state read-out of exciton qubits by observing resonantly excited photoluminescence in quantum dots

We report on a new approach to detect excitonic qubits in semiconductor quantum dots by observing spontaneous emissions from the relevant qubit level. The ground state of excitons is resonantly excited by picosecond optical pulses. Emissions from the same state are temporally resolved with picosecond time resolution. To capture weak emissions, we greatly suppress the elastic scattering of excitation beams, by applying obliquely incident geometry to the micro photoluminescence set-up. Rabi oscillations of the ground-state excitons appear to be involved in the dependence of emission intensity on excitation amplitude.

cond-mat.mtrl-sci↗

arXiv2006

Improved critical current densities in MgB2 tapes with ZrB2 doping

MgB2/Fe tapes with 2.5-15 at.% ZrB2 additions were prepared through the in situ powder-in-tube method. Compared to the pure tape, a significant improvement in the in-field critical current density Jc was observed, most notably for 10 at.% doping, while the critical temperature decreased slightly. At 4.2 K, the transport Jc for the 10 at.% doped sample increased by more than an order of magnitude than the undoped one in magnetic fields above 9 T. Nanoscale segregates or defects caused by the ZrB2 additions which act as effective flux pinning centers are proposed to be the main reason for the improved Jc field performance.

cond-mat.supr-con↗

arXiv2006

Improved properties of epitaxial YNixMn1-xO3 films by annealing under high magnetic fields

The effect of annealing under a magnetic field on the microstructure and properties of YNixMn1-xO3 (x=0.33 and 0.5) films has been investigated. It is found that the ferromagnetic transition temperature is significantly enhanced after post annealing in the presence of an 8 T magnetic field. Characterization study shows that the microstructure is affected, obtaining larger grains of uniform size when films are annealed under a magnetic field. The improvement in the ordering temperature of all films is interpreted in terms of the grain growth caused by the magnetic-field driving force for boundary motion where the exchange coupling is high.

cond-mat.mtrl-sci↗

arXiv2006

Cu-NMR study on the disordered quantum spin magnet with the Bose-glass ground state

Cu-NMR study has been performed on the disordered spin-gap system Tl1-xKxCuCl3 In the high-field H > HC=Δ/μ_B, where Δis the spin-gap, the hyperfine field becomes extremely inhomogeneous at low temperatures due to the field-induced magnetic order, indicating that the ordered spin state must be different from the pure TlCuCl3. In the low field H < HC, a saturating behavior in the longitudinal nuclear spin relaxation rate 1/T1 was observed at low temperatures, indicating existence of the magnetic ground state proposed to be Bose-glass phase by Fisher.

cond-mat.str-el↗

arXiv2006

Large irreversibility field in nanoscale C-doped MgB2/Fe tape conductors

We investigated the effect of nanoscale-C doping on the critical current density Jc and irreversibility field Birr of Fe-sheathed MgB2 tapes prepared by the in-situ powder-in-tube method. The tapes were heat treated at 600-950C for 1 h. Higher values of Jc and Birr were seen for 5 at.%C-doped MgB2 tapes at higher sintering temperatures, where substantial substitution of boron for carbon occurred. The C-doped samples sintered at 950C showed the highest Birr, for example, at 4.2 K, the Birr reached 22.9 T. In particular, at 20 K, Birr for the C-doped tape achieved 9 T, which is comparable to the upper critical field of the commercial NbTi at 4.2 K. This role of nano-sized C particles can be very beneficial in the fabrication of MgB2 tapes for magnetic resonance imaging applications at 20 K.

cond-mat.supr-con↗

arXiv2006

Discovery of Li2(Pd,Pt)3B superconductors

Critical temperature Tc of the Li2(Pd1-xPtx)3B was reported to be 7-8K for x=0 and 2.2-2.8K for x=1. In this article we present our preliminary results on behavior of magnetization-temperature curves with starting composition of Pd-B precursor, y-Li concentration in LiyPd3B and post-annealing of the Pd-end compound. Results suggest that to maximize Tc ratio Pd:B should be close to 3:1, while y-Li has to be optimum. The lowest Tc for LiyPd3B was 4.4-4.6K, while post-annealings at 560 deg. C allowed enhancement of Tc up to 8.2-8.4K. Compositions Li2Z3B with Z=Ni, Ru, Rh, Re, Ag are not superconducting down to 1.8K. Exception is composition with Re showing superconductivity due to Re3B compound. All samples were prepared by arc melting.

cond-mat.supr-con↗