arXiv subjects

K. Woodruff

Publications and source records attributed to K. Woodruff.

18 recordsLinked to original sources

arXiv2022

Neutral Bremsstrahlung emission in xenon unveiled

We present evidence of non-excimer-based secondary scintillation in gaseous xenon, obtained using both the NEXT-White TPC and a dedicated setup. Detailed comparison with first-principle calculations allows us to assign this scintillation mechanism to neutral bremsstrahlung (NBrS), a process that has been postulated to exist in xenon that has been largely overlooked. For photon emission below 1000 nm, the NBrS yield increases from about 10$^{-2}$ photon/e$^{-}$ cm$^{-1}$ bar$^{-1}$ at pressure-reduced electric field values of 50 V cm$^{-1}$ bar$^{-1}$ to above 3$\times$10$^{-1}$ photon/e$^{-}$ cm$^{-1}$ bar$^{-1}$ at 500 V cm$^{-1}$ bar$^{-1}$. Above 1.5 kV cm$^{-1}$ bar$^{-1}$, values that are typically employed for electroluminescence, it is estimated that NBrS is present with an intensity around 1 photon/e$^{-}$ cm$^{-1}$ bar$^{-1}$, which is about two orders of magnitude lower than conventional, excimer-based electroluminescence. Despite being fainter than its excimeric counterpart, our calculations reveal that NBrS causes luminous backgrounds that can interfere, in either gas or liquid phase, with the ability to distinguish and/or to precisely measure low primary-scintillation signals (S1). In particular, we show this to be the case in the "buffer" and "veto" regions, where keeping the electric field below the electroluminescence (EL) threshold will not suffice to extinguish secondary scintillation. The electric field in these regions should be chosen carefully to avoid intolerable levels of NBrS emission. Furthermore, we show that this new source of light emission opens up a viable path towards obtaining S2 signals for discrimination purposes in future single-phase liquid TPCs for neutrino and dark matter physics, with estimated yields up to 20-50 photons/e$^{-}$ cm$^{-1}$.

physics.ins-det↗

arXiv2022

Simulated Thick, Fully-Depleted CCD Exposures Analyzed with Deep Learning Techniques

Thick, Charge Coupled Devices (CCDs) have recently been explored for applied physics, such as nuclear explosion monitoring, and dark matter detection purposes. When run in fully-depleted mode, these devices are sensitive detectors for energy depositions by a variety of primary particles. In this study we are interested in applying the Deep Learning (DL) technique known as panoptic segmentation to simulated CCD images to identify, attribute and measure energy depositions from radioisotopes of interest. We simulate CCD exposures of a chosen radioxenon isotope, $^{135}$Xe, and overlay a simulated cosmic muon background appropriate for a surface-lab. We show that with this DL technique we can reproduce the beta spectrum to good accuracy, while suffering expected confusion with same-topology gammas and conversion electrons and identifying cosmic muons less than optimally.

physics.ins-det↗

arXiv2021

The Dynamics of Ions on Phased Radio-frequency Carpets in High Pressure Gases and Application for Barium Tagging in Xenon Gas Time Projection Chambers

Radio-frequency (RF) carpets with ultra-fine pitches are examined for ion transport in gases at atmospheric pressures and above. We develop new analytic and computational methods for modeling RF ion transport at densities where dynamics are strongly influenced by buffer gas collisions. An analytic description of levitating and sweeping forces from phased arrays is obtained, then thermodynamic and kinetic principles are used to calculate ion loss rates in the presence of collisions. This methodology is validated against detailed microscopic SIMION simulations. We then explore a parameter space of special interest for neutrinoless double beta decay experiments: transport of barium ions in xenon at pressures from 1 to 10 bar. Our computations account for molecular ion formation and pressure dependent mobility as well as finite temperature effects. We discuss the challenges associated with achieving suitable operating conditions, which lie beyond the capabilities of existing devices, using presently available or near-future manufacturing techniques.

physics.ins-det↗

arXiv2021

Dielectric Strength of Noble and Quenched Gases for High Pressure Time Projection Chambers

Dielectric breakdown strength is one of the critical performance metrics for gases and mixtures used in large, high pressure gas time projection chambers. In this paper we experimentally study dielectric breakdown strengths of several important time projection chamber working gases and gas-phase insulators over the pressure range 100 mbar to 10 bar, and gap sizes ranging from 0.1to 10 mm. Gases characterized include argon, xenon, CO2, CF4, and mixtures 90-10 argon-CH4,90-10 argon-CO2and 99-1 argon-CF4. We develop a theoretical model for high voltage breakdown based on microphysical simulations that use PyBoltz electron swarm Monte Carlo results as input to Townsend- and Meek-like discharge criteria. This model is shown to be highly predictive at high pressure, out-performing traditional Paschen-Townsend and Meek-Raether models significantly. At lower pressure-times-distance, the Townsend-like model is an excellent description for noble gases whereas the Meek-like model provides a highly accurate prediction for insulating gases.

physics.ins-det↗

arXiv2021

Sensitivity of the NEXT experiment to Xe-124 double electron capture

Double electron capture by proton-rich nuclei is a second-order nuclear process analogous to double beta decay. Despite their similarities, the decay signature is quite different, potentially providing a new channel to measure the hypothesized neutrinoless mode of these decays. The Standard-Model-allowed two-neutrino double electron capture ($2νECEC$) has been predicted for a number of isotopes, but only observed in $^{78}$Kr, $^{130}$Ba and, recently, $^{124}$Xe. The sensitivity to this decay establishes a benchmark for the ultimate experimental goal, namely the potential to discover also the lepton-number-violating neutrinoless version of this process, $0νECEC$. Here we report on the current sensitivity of the NEXT-White detector to $^{124}$Xe $2νECEC$ and on the extrapolation to NEXT-100. Using simulated data for the $2νECEC$ signal and real data from NEXT-White operated with $^{124}$Xe-depleted gas as background, we define an optimal event selection that maximizes the NEXT-White sensitivity. We estimate that, for NEXT-100 operated with xenon gas isotopically enriched with 1 kg of $^{124}$Xe and for a 5-year run, a sensitivity to the $2νECEC$ half-life of $6 \times 10^{22}$ y (at 90% confidence level) or better can be reached.

hep-ex↗

arXiv2021

Sensitivity of a tonne-scale NEXT detector for neutrinoless double beta decay searches

The Neutrino Experiment with a Xenon TPC (NEXT) searches for the neutrinoless double-beta decay of Xe-136 using high-pressure xenon gas TPCs with electroluminescent amplification. A scaled-up version of this technology with about 1 tonne of enriched xenon could reach in less than 5 years of operation a sensitivity to the half-life of neutrinoless double-beta decay decay better than 1E27 years, improving the current limits by at least one order of magnitude. This prediction is based on a well-understood background model dominated by radiogenic sources. The detector concept presented here represents a first step on a compelling path towards sensitivity to the parameter space defined by the inverted ordering of neutrino masses, and beyond.

physics.ins-det↗

arXiv2021

Demonstration of background rejection using deep convolutional neural networks in the NEXT experiment

Convolutional neural networks (CNNs) are widely used state-of-the-art computer vision tools that are becoming increasingly popular in high energy physics. In this paper, we attempt to understand the potential of CNNs for event classification in the NEXT experiment, which will search for neutrinoless double-beta decay in $^{136}$Xe. To do so, we demonstrate the usage of CNNs for the identification of electron-positron pair production events, which exhibit a topology similar to that of a neutrinoless double-beta decay event. These events were produced in the NEXT-White high-pressure xenon TPC using 2.6-MeV gamma rays from a $^{228}$Th calibration source. We train a network on Monte Carlo-simulated events and show that, by applying on-the-fly data augmentation, the network can be made robust against differences between simulation and data. The use of CNNs offer significant improvement in signal efficiency/background rejection when compared to previous non-CNN-based analyses.

physics.ins-det↗

arXiv2020

Dependence of polytetrafluoroethylene reflectance on thickness at visible and ultraviolet wavelengths in air

Polytetrafluoroethylene (PTFE) is an excellent diffuse reflector widely used in light collection systems for particle physics experiments. However, the reflectance of PTFE is a function of its thickness. In this work, we investigate this dependence in air for light of wavelengths 260 nm and 450 nm using two complementary methods. We find that PTFE reflectance for thicknesses from 5 mm to 10 mm ranges from 92.5% to 94.5% at 450 nm, and from 90.0% to 92.0% at 260 nm. We also see that the reflectance of PTFE of a given thickness can vary by as much as 2.7% within the same piece of material. Finally, we show that placing a specular reflector behind the PTFE can recover the loss of reflectance in the visible without introducing a specular component in the reflectance.

physics.ins-det↗

arXiv2020

Barium Selective Chemosensing by Diazacrown Ether Naphthalimide Turn-on Fluorophores for Single Ion Barium Tagging

Single molecule fluorescence detection of barium is investigated for enhancing the sensitivity and robustness of a neutrinoless double beta decay ($0νββ$) search in $^{136}$Xe, the discovery of which would alter our understanding of the nature of neutrinos and the early history of the Universe. A key developmental step is the synthesis of barium-selective chemosensors capable of incorporation into ongoing experiments in high-pressure $^{136}$Xe gas. Here we report turn-on fluorescent naphthalimide chemosensors containing monoaza- and diaza-crown ethers as agents for single Ba$^{2+}$ detection. Monoaza-18-crown-6 ether naphthalimide sensors showed sensitivity primarily to Ba$^{2+}$ and Hg$^{2+}$, whereas two diaza-18-crown-6 ether naphthalimides revealed a desirable selectivity toward Ba$^{2+}$. Solution-phase fluorescence and NMR experiments support a photoinduced electron transfer mechanism enabling turn-on fluorescence sensing in the presence of barium ions. Changes in ion-receptor interactions enable effective selectivity between competitive barium, mercury, and potassium ions, with detailed calculations correctly predicting fluorescence responses. With these molecules, dry-phase single Ba$^{2+}$ ion imaging with turn-on fluorescence is realized using oil-free microscopy techniques. This represents a significant advance toward a practical method of single Ba$^{2+}$ detection within large volumes of $^{136}$Xe, plausibly enabling a background-free technique to search for the hypothetical process of $0νββ$.

physics.ins-det↗

arXiv2020

Mitigation of Backgrounds from Cosmogenic $^{137}$Xe in Xenon Gas Experiments using $^{3}$He Neutron Capture

\Xe{136} is used as the target medium for many experiments searching for \bbnonu. Despite underground operation, cosmic muons that reach the laboratory can produce spallation neutrons causing activation of detector materials. A potential background that is difficult to veto using muon tagging comes in the form of \Xe{137} created by the capture of neutrons on \Xe{136}. This isotope decays via beta decay with a half-life of 3.8 minutes and a \Qb\ of $\sim$4.16 MeV. This work proposes and explores the concept of adding a small percentage of \He{3} to xenon as a means to capture thermal neutrons and reduce the number of activations in the detector volume. When using this technique we find the contamination from \Xe{137} activation can be reduced to negligible levels in tonne and multi-tonne scale high pressure gas xenon neutrinoless double beta decay experiments running at any depth in an underground laboratory.

physics.ins-det↗

arXiv2020

Radio Frequency and DC High Voltage Breakdown of High Pressure Helium, Argon, and Xenon

Motivated by the possibility of guiding daughter ions from double beta decay events to single-ion sensors for barium tagging, the NEXT collaboration is developing a program of R&D to test radio frequency (RF) carpets for ion transport in high pressure xenon gas. This would require carpet functionality in regimes at higher pressures than have been previously reported, implying correspondingly larger electrode voltages than in existing systems. This mode of operation appears plausible for contemporary RF-carpet geometries due to the higher predicted breakdown strength of high pressure xenon relative to low pressure helium, the working medium in most existing RF carpet devices. In this paper we present the first measurements of the high voltage dielectric strength of xenon gas at high pressure and at the relevant RF frequencies for ion transport (in the 10 MHz range), as well as new DC and RF measurements of the dielectric strengths of high pressure argon and helium gases at small gap sizes. We find breakdown voltages that are compatible with stable RF carpet operation given the gas, pressure, voltage, materials and geometry of interest.

physics.ins-det↗

arXiv2019

Low-diffusion Xe-He gas mixtures for rare-event detection: Electroluminescence Yield

High pressure xenon Time Projection Chambers (TPC) based on secondary scintillation (electroluminescence) signal amplification are being proposed for rare event detection such as directional dark matter, double electron capture and double beta decay detection. The discrimination of the rare event through the topological signature of primary ionisation trails is a major asset for this type of TPC when compared to single liquid or double-phase TPCs, limited mainly by the high electron diffusion in pure xenon. Helium admixtures with xenon can be an attractive solution to reduce the electron diffusion significantly, improving the discrimination efficiency of these optical TPCs. We have measured the electroluminescence (EL) yield of Xe-He mixtures, in the range of 0 to 30% He and demonstrated the small impact on the EL yield of the addition of helium to pure xenon. For a typical reduced electric field of 2.5 kV/cm/bar in the scintillation region, the EL yield is lowered by ~ 2%, 3%, 6% and 10% for 10%, 15%, 20% and 30% of helium concentration, respectively. This decrease is less than what has been obtained from the most recent simulation framework in the literature. The impact of the addition of helium on EL statistical fluctuations is negligible, within the experimental uncertainties. The present results are an important benchmark for the simulation tools to be applied to future optical TPCs based on Xe-He mixtures.

physics.ins-det↗

arXiv2019

Energy calibration of the NEXT-White detector with 1% resolution near Q$_{ββ}$ of $^{136}$Xe

Excellent energy resolution is one of the primary advantages of electroluminescent high pressure xenon TPCs, and searches for rare physics events such as neutrinoless double-beta decay ($β\beta0ν$) require precise energy measurements. Using the NEXT-White detector, developed by the NEXT (Neutrino Experiment with a Xenon TPC) collaboration, we show for the first time that an energy resolution of 1% FWHM can be achieved at 2.6 MeV, establishing the present technology as the one with the best energy resolution of all xenon detectors for $β\beta0ν$ searches.

physics.ins-det↗

arXiv2019

Barium Chemosensors with Dry-Phase Fluorescence for Neutrinoless Double Beta Decay

The nature of the neutrino is one of the major open questions in experimental nuclear and particle physics. The most sensitive known method to establish the Majorana nature of the neutrino is detection of the ultra-rare process of neutrinoless double beta decay. However, identification of one or a handful of decay events within a large mass of candidate isotope, without obfuscation by backgrounds is a formidable experimental challenge. One hypothetical method for achieving ultra-low-background neutrinoless double beta decay sensitivity is the detection of single $^{136}$Ba ions produced in the decay of $^{136}$Xe (`barium tagging'). To implement such a method, a single-ion-sensitive barium detector must be developed and demonstrated in bulk liquid or dry gaseous xenon. This paper reports on the development of two families of dry-phase barium chemosensor molecules for use in high pressure xenon gas detectors, synthesized specifically for this purpose. One particularly promising candidate, an anthracene substituted aza-18-crown-6 ether, is shown to respond in the dry phase with almost no intrinsic background from the unchelated state, and to be amenable to barium sensing through fluorescence microscopy. This interdisciplinary advance, paired with earlier work demonstrating sensitivity to single barium ions in solution, opens a new path toward single ion detection in high pressure xenon gas.

physics.ins-det↗

arXiv2019

Demonstration of the event identification capabilities of the NEXT-White detector

In experiments searching for neutrinoless double-beta decay, the possibility of identifying the two emitted electrons is a powerful tool in rejecting background events and therefore improving the overall sensitivity of the experiment. In this paper we present the first measurement of the efficiency of a cut based on the different event signatures of double and single electron tracks, using the data of the NEXT-White detector, the first detector of the NEXT experiment operating underground. Using a \TO\ calibration source to produce signal-like and background-like events with energies near 1.6 MeV, a signal efficiency of $71.6 \pm 1.5_{\textrm{ stat}} \pm 0.3_{\textrm{ sys}} \%$ for a background acceptance of $20.6 \pm 0.4_{\textrm{ stat}} \pm 0.3_{\textrm{ sys}} \%$ is found, in good agreement with Monte Carlo simulations. An extrapolation to the energy region of the neutrinoless double beta decay by means of Monte Carlo simulations is also carried out, and the results obtained show an improvement in background rejection over those obtained at lower energies.

physics.ins-det↗

arXiv2019

Barium Tagging with Selective, Dry-Functional, Single Molecule Sensitive On-Off Fluorophores for the NEXT Experiment

In the search for neutrinoless double beta decay, understanding and reducing backgrounds is crucial for success. An advance that could drive backgrounds to negligible levels would be the ability to efficiently detect the barium daughter in $^{136}$Xe to $^{136}$Ba double beta decay, since no conventional radioactive process can produce barium ions or atoms in xenon at significant rates. In xenon gas, the barium daughter most likely survives as a dication. An approach under development by the NEXT collaboration involves transporting this ion from the active medium onto a coated transparent plane supporting a barium-sensitive fluorescent dye, monitored via fluorescence microscopy. Upon exposure to a barium dication, the dye will begin fluorescing, which, when correlated with the detection of a double electron signal at the anode, would confirm double beta decay.Our results have shown that a single barium ion can be resolved via Single Molecule Fluorescent Imaging (SMFI). The next challenge is a realization of this technique within in a large volume of xenon gas. Significant advances have recently been made: custom barium-tagging molecules that fluoresce strongly in the dry state when exposed to barium have been demonstrated, and devices constructed that can observe fluorescence via in-vacuum or in-gas Total Internal Reflection Fluorescence Microscopy. We present the status of this technique and the outlook for barium tagging with On-Off switchable fluorophores, including new results with a Ba$^{2+}$-selective dye that functions under our desired conditions in the visible region and with single ion sensitivity.

physics.ins-det↗

arXiv2019

Radiogenic backgrounds in the NEXT double beta decay experiment

Natural radioactivity represents one of the main backgrounds in the search for neutrinoless double beta decay. Within the NEXT physics program, the radioactivity-induced backgrounds are measured with the NEXT-White detector. Data from 37.9 days of low-background operations at the Laboratorio Subterráneo de Canfranc with xenon depleted in $^{136}$Xe are analyzed to derive a total background rate of (0.84$\pm$0.02) mHz above 1000 keV. The comparison of data samples with and without the use of the radon abatement system demonstrates that the contribution of airborne-Rn is negligible. A radiogenic background model is built upon the extensive radiopurity screening campaign conducted by the NEXT Collaboration. A spectral fit to this model yields the specific contributions of $^{60}$Co, $^{40}$K, $^{214}$Bi and $^{208}$Tl to the total background rate, as well as their location in the detector volumes. The results are used to evaluate the impact of the radiogenic backgrounds in the double beta decay analyses, after the application of topological cuts that reduce the total rate to (0.25$\pm$0.01) mHz. Based on the best-fit background model, the NEXT-White median sensitivity to the two-neutrino double beta decay is found to be 3.5$σ$ after 1 year of data taking. The background measurement in a Q$_{ββ}\pm$100 keV energy window validates the best-fit background model also for the neutrinoless double beta decay search with NEXT-100. Only one event is found, while the model expectation is (0.75$\pm$0.12) events.

physics.ins-det↗

arXiv2019

Electron Drift and Longitudinal Diffusion in High Pressure Xenon-Helium Gas Mixtures

We report new measurements of the drift velocity and longitudinal diffusion coefficients of electrons in pure xenon gas and in xenon-helium gas mixtures at 1-9 bar and electric field strengths of 50-300 V/cm. In pure xenon we find excellent agreement with world data at all $E/P$, for both drift velocity and diffusion coefficients. However, a larger value of the longitudinal diffusion coefficient than theoretical predictions is found at low $E/P$ in pure xenon, below the range of reduced fields usually probed by TPC experiments. A similar effect is observed in xenon-helium gas mixtures at somewhat larger $E/P$. Drift velocities in xenon-helium mixtures are found to be theoretically well predicted. Although longitudinal diffusion in xenon-helium mixtures is found to be larger than anticipated, extrapolation based on the measured longitudinal diffusion coefficients suggest that the use of helium additives to reduce transverse diffusion in xenon gas remains a promising prospect.

physics.ins-det↗