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K. Y. Yip

Publications and source records attributed to K. Y. Yip.

13 recordsLinked to original sources

Suppression of both superconductivity and structural transition in hole-doped MoTe$_2$ induced by Ta substitution

Type-II Weyl semimetal MoTe$_2$ exhibits a first-order structural transition at $T_s$ $\sim$250~K and superconducts at $T_c$ $\sim$0.1~K at ambient pressure. Both $T_s$ and $T_c$ can be manipulated by several tuning parameters, such as hydrostatic pressure and chemical substitution. It is often reported that suppressing $T_s$ enhances $T_c$, but our study shows a different behaviour when MoTe$_2$ is hole-doped by Ta. When $T_s$ is suppressed by Ta doping, $T_c$ is also suppressed. Our findings suggest that the suppression of $T_s$ does not necessarily enhance superconductivity in MoTe$_2$. By connecting with the findings of electron-doped MoTe$_2$, we argue that varying electron carrier concentration can effectively tune $T_c$. In addition, the Hall coefficient is enhanced around the doping region, where $T_s$ is completely suppressed, suggesting that the critical scattering around the structural transition may also play a role in suppressing $T_c$.

cond-mat.supr-con

Pauli-limit violation in lanthanide infinite-layer nickelate superconductors

Superconductivity can be destroyed by a magnetic field with an upper bound known as the Pauli-limit in spin-singlet superconductors. Almost all the discovered superconductors are spin-singlet, with the highest transition temperature $T_c$ at ambient pressure achieved in the cuprate family. The closest cuprate analogue is the recently discovered infinite-layer nickelate, which hosts substantial structural and electronic similarity to the cuprate. A previous magnetotransport study on Nd$_{0.775}$Sr$_{0.225}$NiO$_2$ has observed an isotropic Pauli-limited upper critical field. Here, we report a large violation (>2 times) of Pauli-limit in every crystallographic directions in La$_{1-x}$(Ca/Sr)$_x$NiO$_2$ regardless of the doping $x$. Such a large violation of the Pauli-limit in all directions in La$_{1-x}$(Ca/Sr)$_x$NiO$_2$ is unexpected and unlikely accounted by a Fulde Ferrell-Larkin-Ovchinnikov (FFLO)-state, strong spin-orbit-coupling, strong-coupling or a large pseudogap. On the other hand, in agreement with the previous report, we observe a Pauli-limiting critical field in Nd$_{1-x}$Sr$_x$NiO$_2$ and the superconducting anisotropy decreases as doping increases, suggesting a spin-singlet pairing. Therefore, superconductivity in La$_{1-x}$(Ca/Sr)$_x$NiO$_2$ could be driven by a non-spin-singlet Cooper pairing mechanism with an attractive high-$T_c$ at 10 K, an order of magnitude higher than the known spin triplet superconductors, favourably extending the application of spin-triplet superconductivity in topological matter, non-dissipative spintronics, and quantum computing.

cond-mat.supr-con

Current-induced superconducting anisotropy of Sr$\mathsf{_2}$RuO$\mathsf{_4}$

In the unconventional superconductor Sr$\mathsf{_2}$RuO$\mathsf{_4}$, unusual first-order superconducting transition has been observed in the low-temperature and high-field region, accompanied by a four-fold anisotropy of the in-plane upper critical magnetic field $H_{c2}$. The origin of such unusual $H_{c2}$ behavior should be closely linked to the debated superconducting symmetry of this oxide. Here, toward clarification of the unusual $H_{c2}$ behavior, we performed the resistivity measurements capable of switching in-plane current directions as well as precisely controlling the field directions. Our results reveal that resistive $H_{c2}$ under the in-plane current exhibits an additional two-fold anisotropy. By systematically analyzing $H_{c2}$ data taken under various current directions, we succeeded in separating the two-fold $H_{c2}$ component into the one originating from applied current and the other originating from certain imperfection in the sample. The former component, attributable to vortex flow effect, is weakened at low temperatures where $H_{c2}$ is substantially suppressed. The latter component is enhanced in the first order transition region, possibly reflecting a change in the nature of the superconducting state under high magnetic field.

cond-mat.supr-con

Linear magnetoresistance with a universal energy scale in a strong-coupling superconductor

The recent discovery of a nonsaturating linear magnetoresistance in several correlated electron systems near a quantum critical point has revealed an interesting interplay between the linear magnetoresistance and the zero-field linear-in-temperature resistivity. These studies suggest a possible role of quantum criticality on the observed linear magnetoresistance. Here, we report our discovery of a nonsaturating, linear magnetoresistance in Mo$_8$Ga$_{41}$, a nearly isotropic strong electron-phonon coupling superconductor with a linear-in-temperature resistivity from the transition temperature to $\sim$55 K. The growth of the resistivity in field is comparable to that in temperature, provided that both quantities are measured in the energy unit. Our datasets are remarkably similar to magnetoresistance data of the optimally doped La$_{2-x}$Sr$_x$CuO$_4$, despite the clearly different crystal and electronic structures, and the apparent absence of quantum critical physics in Mo$_8$Ga$_{41}$. A new empirical scaling formula is developed, which is able to capture the key features of the low-temperature magnetoresistance data of Mo$_8$Ga$_{41}$, as well as the data of La$_{2-x}$Sr$_x$CuO$_4$.

cond-mat.supr-con

Stabilization of antiferromagnetism in 1T-Fe$_{0.05}$TaS$_2$

1T-TaS$_2$ is a prototypical charge-density-wave (CDW) system with a Mott insulating ground state. Usually, a Mott insulator is accompanied by an antiferromagnetic state. However, the antiferromagnetic order had never been observed in 1T-TaS$_2$. Here, we report the stabilization of the antiferromagnetic order by the intercalation of a small amount of Fe into the van der Waals gap of 1T-TaS$_2$, i.e. forming 1T-Fe$_{0.05}$TaS$_2$. Upon cooling from 300~K, the electrical resistivity increases with a decreasing temperature before reaching a maximum value at around 15~K, which is close to the Neel temperature determined from our magnetic susceptibility measurement. The antiferromagnetic state can be fully suppressed when the sample thickness is reduced, indicating that the antiferromagnetic order in Fe$_{0.05}$TaS$_2$ has a non-negligible three-dimensional character. For the bulk Fe$_{0.05}$TaS$_2$, a comparison of our high pressure electrical transport data with that of 1T-TaS$_2$ indicates that, at ambient pressure, Fe$_{0.05}$TaS$_2$ is in the nearly commensurate charge-density-wave (NCCDW) phase near the border of the Mott insulating state. The temperature-pressure phase diagram thus reveals an interesting decoupling of the antiferromagnetism from the Mott insulating state.

cond-mat.str-el

Detection of hole pockets in the candidate type-II Weyl semimetal MoTe$_2$ from Shubnikov-de Haas quantum oscillations

The bulk electronic structure of $T_d$-MoTe$_2$ features large hole Fermi pockets at the Brillouin zone center ($Γ$) and two electron Fermi surfaces along the $Γ-X$ direction. However, the large hole pockets, whose existence has important implications for the Weyl physics of $T_d$-MoTe$_2$, has never been conclusively detected in quantum oscillations. This raises doubt about the realizability of Majorana states in $T_d$-MoTe$_2$, because these exotic states rely on the existence of Weyl points, which originated from the same band structure predicted by density functional theory (DFT). Here, we report an unambiguous detection of these elusive hole pockets via Shubnikov-de Haas (SdH) quantum oscillations. At ambient pressure, the quantum oscillation frequencies for these pockets are 988 T and 1513 T, when the magnetic field is applied along the $c$-axis. The quasiparticle effective masses $m^*$ associated with these frequencies are 1.50 $m_e$ and 2.77 $m_e$, respectively, indicating the importance of Coulomb interactions in this system. We further measure the SdH oscillations under pressure. At 13 kbar, we detected a peak at 1798 T with $m^*$ = 2.86 $m_e$. Relative to the oscillation data at a lower pressure, the amplitude of this peak experienced an enhancement, which can be attributed to the reduced curvature of the hole pockets under pressure. Combining our experimental data with DFT + $U$ calculations, where $U$ is the Hubbard parameter, our results shed light on why these important hole pockets have not been detected until now.

cond-mat.supr-con

Spectroscopic Fingerprint of Chiral Majorana Modes at the Edge of a Quantum Anomalous Hall Insulator / Superconductor Heterostructure

With the recent discovery of the quantum anomalous Hall insulator (QAHI), which exhibits the conductive quantum Hall edge states without external magnetic field, it becomes possible to create a novel topological superconductor (SC) by introducing superconductivity into these edge states. In this case, two distinct topological superconducting phases with one or two chiral Majorana edge modes were theoretically predicted, characterized by Chern numbers (N ) of 1 and 2, respectively. We present spectroscopic evidence from Andreev reflection experiments for the presence of chiral Majorana modes in a Nb / (Cr0.12Bi0.26Sb0.62)2Te3 heterostructure with distinct signatures attributed to two different topological superconducting phases. The results are in qualitatively good agreement with the theoretical predictions.

cond-mat.supr-con

Angular dependence of the upper critical field in the high-pressure $1T'$ phase of MoTe$_2$

Superconductivity in the type-II Weyl semimetal candidate MoTe$_2$ has attracted much attention due to the possible realization of topological superconductivity. Under applied pressure, the superconducting transition temperature is significantly enhanced, while the structural transition from the high-temperature 1$T'$ phase to the low-temperature $T_d$ phase is suppressed. Hence, applying pressure allows us to investigate the dimensionality of superconductivity in 1$T'$-MoTe$_2$. We have performed a detailed study of the magnetotransport properties and upper critical field $H_{c2}$ of MoTe$_2$ under pressure. The magnetoresistance (MR) and Hall coefficient of MoTe$_2$ are found to be decreasing with increasing pressure. In addition, the Kohler's scalings for the MR data above $\sim$11 kbar show a change of exponent whereas the data at lower pressure can be well scaled with a single exponent. These results are suggestive of a Fermi surface reconstruction when the structure changes from the $T_d$ to 1$T'$ phase. The $H_{c2}$-temperature phase diagram constructed at 15 kbar, with $H\parallel ab$ and $H\perp ab$, can be satisfactorily described by the Werthamer-Helfand-Hohenberg model with the Maki parameters $α\sim$ 0.77 and 0.45, respectively. The relatively large $α$ may stem from a small Fermi surface and a large effective mass of semimetallic MoTe$_2$. The angular dependence of $H_{c2}$ at 15 kbar can be well fitted by the Tinkham model, suggesting the two-dimensional nature of superconductivity in the high-pressure 1$T'$ phase.

cond-mat.supr-con

Anisotropic two-gap superconductivity and the absence of a Pauli paramagnetic limit in single-crystalline LaO$_{0.5}$F$_{0.5}$BiS$_2$

Ambient-pressure-grown LaO$_{0.5}$F$_{0.5}$BiS$_2$ with a superconducting transition temperature $T_{c}\sim$3K possesses a highly anisotropic normal state. By a series of electrical resistivity measurements with a magnetic field direction varying between the crystalline $c$-axis and the $ab$-plane, we present the first datasets displaying the temperature dependence of the out-of-plane upper critical field $H_{c2}^{\perp}(T)$, the in-plane upper critical field $H_{c2}^{\parallel}(T)$, as well as the angular dependence of $H_{c2}$ at fixed temperatures for ambient-pressure-grown LaO$_{0.5}$F$_{0.5}$BiS$_2$ single crystals. The anisotropy of the superconductivity, $H_{c2}^{\parallel}/H_{c2}^{\perp}$, reaches $\sim$16 on approaching 0 K, but it decreases significantly near $T_{c}$. A pronounced upward curvature of $H_{c2}^{\parallel}(T)$ is observed near $T_{c}$, which we analyze using a two-gap model. Moreover, $H_{c2}^{\parallel}(0)$ is found to exceed the Pauli paramagnetic limit, which can be understood by considering the strong spin-orbit coupling associated with Bi as well as the breaking of the local inversion symmetry at the electronically active BiS$_2$ bilayers. Hence, LaO$_{0.5}$F$_{0.5}$BiS$_2$ with a centrosymmetric lattice structure is a unique platform to explore the physics associated with local parity violation in the bulk crystal.

cond-mat.supr-con

Nearly isotropic superconductivity in layered Weyl semimetal WTe$_2$ at 98.5 kbar

Layered transition metal dichalcogenide WTe$_2$ has recently attracted significant attention due to the discovery of an extremely large magnetoresistance, a predicted type-II Weyl semimetallic state, and the pressure-induced superconducting state. By a careful measurement of the superconducting upper critical fields as a function of the magnetic field angle at a pressure as high as 98.5 kbar, we provide the first detailed examination of the dimensionality of the superconducting condensate in WTe$_2$. Despite the layered crystal structure, the upper critical field exhibits a negligible field anisotropy. The angular dependence of the upper critical field can be satisfactorily described by the anisotropic mass model from 2.2 K ($T/T_c\sim0.67$) to 0.03 K ($T/T_c\sim0.01$), with a practically identical anisotropy factor $γ\sim1.7$. The temperature dependence of the upper critical field, determined for both $H\perp ab$ and $H\parallel ab$, can be understood by a conventional orbital depairing mechanism. Comparison of the upper critical fields along the two orthogonal field directions results in the same value of $γ\sim1.7$, leading to a temperature independent anisotropy factor from near $T_c$ to $<0.01T_c$. Our findings thus identify WTe$_2$ as a nearly isotropic superconductor, with an anisotropy factor among one of the lowest known in superconducting transition metal dichalcogenides.

cond-mat.supr-con

Maximizing Tc by tuning nematicity and magnetism in FeSe1-xSx superconductors

A fundamental issue concerning iron-based superconductivity is the roles of electronic nematicity and magnetism in realising high transition temperature ($T_{\rm c}$). To address this issue, FeSe is a key material, as it exhibits a unique pressure phase diagram involving nonmagnetic nematic and pressure-induced antiferromagnetic ordered phases. However, as these two phases in FeSe overlap with each other, the effects of two orders on superconductivity remain perplexing. Here we construct the three-dimensional electronic phase diagram, temperature ($T$) against pressure ($P$) and isovalent S-substitution ($x$), for FeSe$_{1-x}$S$_{x}$, in which we achieve a complete separation of nematic and antiferromagnetic phases. In between, an extended nonmagnetic tetragonal phase emerges, where we find a striking enhancement of $T_{\rm c}$. The completed phase diagram uncovers two superconducting domes with similarly high $T_{\rm c}$ on both ends of the dome-shaped antiferromagnetic phase. The $T_{\rm c}(P,x)$ variation implies that nematic fluctuations unless accompanying magnetism are not relevant for high-$T_{\rm c}$ superconductivity in this system.

cond-mat.supr-con

Weakening of the diamagnetic shielding in FeSe$_{1-x}$S$_x$ at high pressures

The superconducting transition of FeSe$_{1-x}$S$_x$ with three distinct sulphur concentrations $x$ was studied under hydrostatic pressure up to $\sim$70 kbar via bulk AC susceptibility. The pressure dependence of the superconducting transition temperature ($T_c$) features a small dome-shaped variation at low pressures for $x=0.04$ and $x=0.12$, followed by a more substantial $T_c$ enhancement to a value of around 30 K at moderate pressures. In $x=0.21$, a similar overall pressure dependence of $T_c$ is observed, except that the small dome at low pressures is flattened. For all three concentrations, a significant weakening of the diamagnetic shielding is observed beyond the pressure around which the maximum $T_c$ of 30 K is reached near the verge of pressure-induced magnetic phase. This observation points to a strong competition between the magnetic and high-$T_c$ superconducting states at high pressure in this system.

cond-mat.supr-con

Quasilinear quantum magnetoresistance in pressure-induced nonsymmorphic superconductor CrAs

In conventional metals, modification of electron trajectories under magnetic field gives rise to a magnetoresistance that varies quadratically at low field, followed by a saturation at high field for closed orbits on the Fermi surface. Deviations from the conventional behaviour, e.g. the observation of a linear magnetoresistance, or a non-saturating magnetoresistance, have been attributed to exotic electron scattering mechanisms. Recently, linear magnetoresistance has been observed in many Dirac materials, in which the electron-electron correlation is relatively weak. The strongly correlated helimagnet CrAs undergoes a quantum phase transition to a nonmagnetic superconductor under pressure. Near the magnetic instability, we observe a large and non-saturating quasilinear magnetoresistance from the upper critical field to 14 T at low temperatures. We show that the quasilinear magnetoresistance arises from an intricate interplay between a nontrivial band crossing protected by nonsymmorphic crystal symmetry and strong magnetic fluctuations

cond-mat.supr-con