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Kamran Behnia

Publications and source records attributed to Kamran Behnia.

At least 19 recordsLinked to original sources

Deviation from Fermi-liquid $T^2$ resistivity caused by collective transport

`Fermi-liquid behavior' is nowadays used as a shorthand for quadratic temperature dependence of the electrical resistivity. In a metal, for this to occur, electrons must be cooled well below the Fermi degeneracy temperature, $T_{\mathrm{F}}$. A departure from this behavior is observed at finite temperature. Here, we note that this departure has opposite signs in two distinct types of Fermi liquids. In weakly correlated ones, the upward departure implies a higher exponent of the inelastic resistivity, attributable to \textit{additional scattering} by phonons. In contrast, there is a downward deviation in strongly correlated metals, which implies either \textit{reduced scattering} or \textit{additional conduction}, as in the case of normal liquid $^3$He, in which a distinct contribution to heat transport by a sound mode has been recently identified. Such a channel of conduction smoothly transforms across $T_{\mathrm{F}}$ to the one captured by the Bridgman formula for thermal conductivity of classical liquids. In three metals (UPt$_3$, Sr$_2$RuO$_4$, and heavily overdoped LSCO), according to the available experimental data, the normalized amplitude of excess conductivity at $T/T_{\mathrm{F}}\simeq0.02$ is comparable to what has been seen in $^3$He, suggesting, without establishing, a common origin.

cond-mat.str-el

Electron-phonon coupled hydrodynamics in semimetal TaAs_2

Hydrodynamic corrections to diffusive transport can arise when momentum-conserving collisions between quasiparticles become prominent, and they have been documented for both electrons and phonons. An emerging frontier topic is coupled electron-phonon (e-ph) hydrodynamics. Here, through electrical and thermal transport measurements on TaAs2 crystals with different impurity levels, we document the emergence of an e-ph bifluid in the temperature window of 5 to 15 K. Within this range, the lattice thermal conductivity exhibits a faster-than-T^3 temperature dependence, as a consequence of non-monotonic and purity-dependent phonon mean free paths, a signature of phonon Poiseuille flow. However, strong e-ph coupling impedes the emergence of a ballistic regime. This is corroborated by the observation of quantum oscillations in the lattice thermal conductivity. Prominent phonon-mediated momentum exchange between electrons amplifies the violation of the Wiedemann-Franz law and yields a two-order-of-magnitude discrepancy between quantum and transport lifetimes, a signature of electron hydrodynamics in semimetals. Our results imply that in semimetals with optimized e-ph coupling, thanks to matching between the cryogenic phonon wave?length and the Fermi wavelength, momentum and energy flow between the electron and phonon reservoirs as frequently as within each reservoir.

cond-mat.mtrl-sci

Observation of thermal Hall effect in diamond

Numerous insulators, including non-magnetic ones, have been unexpectedly found to display a finite thermal Hall signal, which has stimulated debate about its origin. Here, we report on a study of the thermal Hall effect in two diamond single crystals. The transverse thermal conductivity (kappa_xy) was found to peak at a temperature close to that at which the longitudinal thermal conductivity (kappa_xx) reaches its maximum. The measured kappa_xy, with an amplitude of 340 W/(m K) at B = 10 T, is the largest ever observed, while the kappa_xy/kappa_xx ratio follows the phenomenological trend identified in other insulators. Our observation implies the existence of an intrinsic thermal Hall effect in a generic phonon gas. We argue that the rough amplitude of both the thermal Hall angle and the thermal Hall resistivity can be accounted for by simple arguments invoking fundamental constants and quantum-mechanical constraints on solid state cohesion.

cond-mat.mtrl-sci

Electron-electron and electron-phonon collision cross sections in CsV3Sb5

AV3Sb5 (A=K, Rb, Cs) are kagome metals and superconductors, attracting much recent attention as nexus of multiple quantum states. Here, through a systematic study of electric and thermal transport of CsV3Sb5, we identify it as a metallic Fermi liquid with moderate electronic correlations ans strong electron-phonon (e-ph) collision cross section. We observe contributions to the inelastic electrical resistivity, each dominating within a distinct temperature window. The prefactor of the T2 is consistent with the Kadowaki-Woods scaling for a Fermi liquid with moderate correlation. By performing thermal conductivity measurements at zero and finite magnetic field, we separate the electronic and the lattice contributions to the thermal conductivity. The Wiedemann-Franz law is satisfied in the zero-temperature limit, while a downward deviation emerges at finite temperature due to the mismatch between the prefactors of the electrical and thermal quadratic resistivities, as reported in other metals. The Bloch-Grüneisen description of electron-phonon scattering successfully accounts for both electronic thermal and electrical transport, indicating a remarkably large e-ph collision cross section in CsV3Sb5.

cond-mat.str-el

Hydrodynamics of the viscous electron fluid in cadmium

Thanks to electron-electron ($e$-$e$) collisions conserving momentum, metallic electron fluids are viscous. Yet, this viscosity is rarely detectable in bulk transport. Here, we report on the canonical realization of the Gurzhi effect in an elemental three-dimensional metal: cadmium. Using focused ion beam microstructuring to tune the effective thickness, we detected a low-temperature size-dependent resistivity upturn in a finite window sandwiched between ballistic and diffusive regimes. Within this window, the electrical conductivity displays a simultaneous quadratic dependence on both sample size and temperature -- fingerprint of a hydrodynamic flow. This leads us to quantify the amplitude and the temperature dependence of kinematic and dynamic viscosity of the electron fluid. In cadmium, in contrast with graphene and $^3$He, the rate of momentum-conserving $e$-$e$ collisions is not set by the main Fermi energy, but by Lilliputian energy scales and inter-valley bottlenecks.

cond-mat.str-el

Interaction driven transverse thermal resistivity in a phonon gas

The amplitude of the Hall response of electrons can be understood without invoking interactions. Most theories of the phonon thermal Hall effect have likewise opted for a non-interacting picture. Here, we challenge this approach. Our study of WS$_2$, a transition metal dichalcogenide (TMD) insulator, finds that longitudinal, $κ_{xx}$, and transverse, $κ_{xy}$, thermal conductivities peak at almost the same temperature. Their ratio obeys an upper bound, as in other insulators. We then compare transverse thermal transport in a phonon gas and in a molecular gas. In the latter, the Senftleben-Beenakker effect is driven by the competition between molecular collisions and applied magnetic field in setting the distribution of molecular angular momenta. An off-diagonal transport response arises thanks to interactions between non-spherical particles, which do not need to be chiral. By analogy, we argue that in a phonon gas, magnetic field will influence phonon-phonon interactions, and generates a transverse thermal \emph{resistivity}, whose order of magnitude can be accounted for by invoking a Berry force on the drift velocity of the nuclei in the presence of a finite heat. This simple picture gives a reasonable account of the experimentally measured transverse thermal resistivity of seven different crystalline insulators.

cond-mat.mtrl-sci

Phonon Thermal Hall Effect in quartz and its absence in silica

The observation of a misalignment between the applied heat flux and the measured temperature gradient in insulating solids induced by magnetic field has become a subject of experimental investigation, theoretical speculation, and unsettled controversy. To identify the origin of this phonon thermal Hall effect, we performed a comparative study of longitudinal and transverse heat transport in crystalline (quartz) and vitreous (silica) SiO$_2$ using identical experimental set-ups and thermometers. A finite signal was detected in the crystalline samples and none in the amorphous sample, within our resolution. The cleaner crystal exhibited a larger thermal Hall conductivity than the dirtier one, ruling out disorder as the driver of the effect. On the other hand, the amplitude of the transverse thermal resistivity is almost identical in the two crystalline samples (W$_{\perp}$/B$\approx 10^{-6}$ m.K.W$^{-1}$.T$^{-1}$). We show that in a phonon gas, as in a molecular gas displaying the Senftleben-Beenakker effect, heat is conducted through two channels, and argue that a thermal Hall response is unavoidable whenever these channels differ both in entropy production and in their coupling to the magnetic field. Under such conditions, the conserved energy current and the non-conserved entropy current cease to be parallel. Finally, the magnitude of the transverse thermal resistivity can be accounted for by a surprisingly simple picture. The heat flux induces a tiny drift velocity of the lattice nuclei, the magnetic field exerts a transverse Berry force on this drift, and this force is balanced by an entropic restoring force.

cond-mat.mtrl-sci

T-square electric resistivity and its thermal counterpart in RuO$_2$

We present a study of low-temperature electric and thermal transport in RuO$_2$, a metallic oxide which has attracted much recent attention. Careful scrutiny of electric resistivity reveals a quadratic temperature dependence below $\sim$ 20 K undetected in previous studies of electronic transport in this material. The prefactor of this T$^2$ resistivity, given the electronic specific heat, corresponds to what is expected by the Kadowaki-Woods scaling. The variation of its amplitude across 4 different samples is negligible despite an eightfold variation of residual resistivity. There is also a T$^5$ resistivity due to scattering by phonons. By measuring thermal conductivity, $κ$, at zero field and at 12 T, we separated its electronic and the phononic components and found that the electronic component respects the Wiedemann-Franz law at zero temperature and deviates downward at finite temperature. The latter corresponds to a threefold discrepancy between the prefactors of the two (thermal and electric) T-square resistivities. Our results, establishing RuO$_2$ as a weakly correlated Fermi liquid, provide new input for the ongoing theoretical attempt to give a quantitative account of electron-electron scattering in metallic oxides starting from first principles.

cond-mat.str-el

Thermal Hall conductivity of semimetallic graphite dominated by ambipolar phonon drag

It is now known that in addition to electrons, other quasi-particles such as phonons and magnons can also generate a thermal Hall signal. Graphite is a semimetal with extremely mobile charge carriers of both signs and a large lattice thermal conductivity. We present a study of the thermal Hall effect in highly oriented pyrolytic graphite (HOPG) samples with electronic, phononic and phonon drag contributions to the thermal Hall signal. The measured thermal Hall conductivity ($κ_{xy}$) is two orders of magnitude higher than what is expected by electronic carriers according to the electrical Hall conductivity and the Wiedemann-Franz law, yielding a record Hall Lorenz number of $164.9\times10^{-8}V^2 K^{-2}$ ($\sim$67$L_0$) - the largest ever observed in a metal. The temperature dependence of the thermal Hall conductivity significantly differs from its longitudinal counterpart, ruling out a purely phononic origin of the non-electronic component. Based on the temperature dependence and the amplitudes of the Seebeck and Nernst responses, we demonstrate that ambipolar phonon drag dominates the thermal Hall response of graphite.

cond-mat.mes-hall

Incipient modulated phase in Sr$_{1-x}$Ca$_{x}$TiO$_3$

Nanometer-scale modulations can spontaneously emerge in complex materials when multiple degrees of freedom interact. Here we demonstrate that ferroelectric Sr$_{1-x}$Ca$_x$TiO$_3$ lies in close proximity to an incipient structurally modulated phase. Using inelastic neutron and X-ray scattering, we show that upon cooling, dipolar fluctuations strongly couple to and soften the $c_{44}$ transverse acoustic mode. We identify the wavevector at which this softening is maximal, thereby defining the characteristic length scale of the modulation. Calcium substitution enhances both the amplitude and the wavevector of the softening by strengthening the ferroelectric and antiferrodistortive instabilities. Our results demonstrate that nonlinear flexoelectric phonon coupling tends to stabilize a modulated state that cooperates with, rather than competes against, the other lattice instabilities in SrTiO$_3$.

cond-mat.mtrl-sci

Phonon Thermal Hall Effect: The Roles of Disorder, Annealing, and Metallic Contacts

The phonon thermal Hall effect (THE) is a ubiquitous yet poorly understood phenomenon in insulators. Its microscopic origin remains debated, partly due to significant sample-dependent variations that hint at uncontrolled experimental parameters. Using SrTiO$_3$ as a model system, we identify disorder and uncontrolled strain as suppressors of a thermal Hall signal. Crystals with high thermal conductivity exhibit a substantial thermal Hall angle $\nabla T_y / \nabla T_x$ (up to 0.3\% at 9 T), whereas the effect is virtually absent in disordered samples. Crucially, annealing (in air atmosphere) these disordered samples partially restores the THE (approximately 0.1\% at 9 T) with little effect on the longitudinal thermal conductivity. This decoupling reveals that the amplitude of THE is not simply set by the phonon mean free path. Furthermore, measurements performed with metallic and insulating contacts yield identical results on the same sample. This definitively rules out parasitic signals as the effect's origin. Our work, by establishing the phonon THE as an intrinsic property of the crystal lattice and extremely sensitive to disorder, sharply constrains theoretical scenarios.

cond-mat.str-el

Deep-lying semi-Dirac fermions in hexagonal close-packed cadmium

Semi-Dirac fermions are massless in one direction and massive in the perpendicular directions. Such quasiparticles have been proposed in various contexts in condensed matter. Using first principles calculations, we identify a pair of semi-Dirac bands anti-crossing at $-3$ eV below the Fermi level in the electronic structure of hexagonal close-packed cadmium. The linear out-of-plane dispersion is kept up to the Fermi level. We demonstrate that the dichotomy between the linear and quadratic dispersions is driven by an orientation-sensitive hybridization between the $s$ and $p_z$ orbitals. The upper semi-Dirac band produces a lens-shaped nonellipsoidal Fermi sheet whose cross-section area has a $k$-dependence that is in excellent agreement with the experimentally measured period of Sondheimer oscillations.

cond-mat.mtrl-sci

Nernst effect and its thickness dependence in superconducting NbN films

Superconducting thin films and layered crystals display a Nernst signal generated by short-lived Cooper pairs above their critical temperature. Several experimental studies have broadly verified the standard theory invoking Gaussian fluctuations of a two-dimensional superconducting order parameter. Here, we present a study of the Nernst effect in granular NbN thin films with a thickness varying from 4 to 30 nm, exceeding the short superconducting coherence length and putting the system in the three-dimensional limit. We find that the Nernst conductivity decreases linearly with reduced temperature ($α_{xy}\propto \frac{T-T_c}{T_c}$), but the amplitude of $α_{xy}$ scales with thickness. While the temperature dependence corresponds to what is expected in a 2D picture, scaling with thickness corresponds to a 3D picture. We argue that this behavior indicates a 2+1D situation, in which the relevant coherence length along the thickness of the film has no temperature dependence. We find no visible discontinuity in the temperature dependence of the Nernst conductivity across T$_c$. Explaining how the response of the superconducting vortices evolves to the one above the critical temperature of short-lived Cooper pairs emerges as a challenge to the theory.

cond-mat.supr-con

Phonon thermal Hall as a lattice Aharonov-Bohm effect

In a growing list of insulators, experiments find that magnetic field induces a misalignment between the heat flux and the thermal gradient vectors. This phenomenon, known as the phonon thermal Hall effect, implies energy flow without entropy production along the orientation perpendicular to the temperature gradient. The experimentally-measured thermal Hall angle in various insulators does not exceed a bound and becomes maximal at the temperature of peak longitudinal thermal conductivity. The present paper aims to propose a scenario providing and explanation for these two experimental facts. It begins by noticing that at this temperature, $T_{max}$, Normal phonon-phonon collisions become most frequent in comparison with Umklapp and boundary scattering events. Furthermore, the Born-Oppenheimer approximated molecular wave functions are known to acquire a phase in the presence of a magnetic field. In an anharmonic crystal, in which tensile and compressive strain do not cancel out, this field-induced atomic phase gives rise to a phonon Berry phase and generates phonon-phonon interference. The rough amplitude of the thermal Hall angle expected in this picture is set by the phonon wavelength, $λ_{ph}$, and the crest atomic displacement, $δu_m$ at $T_{max}$. The derived expression is surprisingly close to what has been experimentally found in black phosphorus, germanium and silicon.

cond-mat.mes-hall

Comment on `High-resolution Measurements of Thermal Conductivity Matrix and Search for Thermal Hall Effect in La$_2$CuO$_4$'

Recently, Jiayi Hu and co-workers reported that they did not resolve any thermal Hall signal in La$_2$CuO$_4$ by `high resolution' measurements, setting an upper bound of $|κ_{xy}| <2\times 10^{-3}~$Wm$^{-1}$K$^{-1}$ at 20 K. Two points have apparently escaped their attention. First, thermal Hall signals with an amplitude well below this resolution bound have been detected in disordered perovskites. Second, the longitudinal thermal conductivity of their sample is significantly lower than the La$_2$CuO$_4$ sample displaying a thermal Hall signal. We find that a moderate reduction of $κ_{xx}$ in SrTiO$_3$ is concomitant with a drastic attenuation of $κ_{xy}$. A trend emerges across several families of insulators: the amplitude of $κ_{xy}$ anti-correlates with disorder.

cond-mat.mtrl-sci

Scalable Sondheimer oscillations driven by commensurability between two quantizations

The electrical conductivity of metallic crystals exhibits size effects when the electron mean free path exceeds the sample thickness. One such phenomenon, known as Sondheimer oscillations, was discovered decades ago. These oscillations, periodic in magnetic field, have been hitherto treated with no reference to Landau quantization. Here, we present a study of longitudinal and transverse conductivity in cadmium single crystals with thicknesses ranging from 12.6 to 475 $μ$m, and demonstrate that the amplitude of the first ten oscillations is determined by the quantum of conductance and a length scale that depends on the sample thickness, the magnetic length and the Fermi surface geometry. We argue that this scaling is unexpected in semiclassical scenarios and it arises from the degeneracy of the momentum derivative of the cross-sectional area $A$ along the orientation of the magnetic field $\frac{\partial A}{\partial k_z}$ in cadmium, which couples Landau quantization to the discretization of $k_z$ imposed by the finite sample thickness. We show that the oscillating component of the conductivity is uniquely governed by fundamental constants and the ratio of two degeneracies, which acts as an inverted filling factor. Our conjecture is supported by the absence of such scaling in thin copper crystals.

cond-mat.mes-hall

Angle-dependent planar thermal Hall effect by quasi-ballistic phonons in black phosphorus

The origin of the phonon thermal Hall effect in insulators is a matter of ongoing debate. The large amplitude of the signal in an elemental non-magnetic solid, such as black phosphorus (BP), calls for a minimal mechanism not invoking the spin degree of freedom. Here, we show that a longitudinal heat flow generates a transverse temperature gradient in BP even when the magnetic field, the heat current and the thermal gradient lie in the same plane. The phonon mean-free-path is close to the sample thickness. Therefore, it is unlikely that scattering by point-like symmetry-breaking defects play a major role. We show that the angular dependence of the signal can be mapped to the sum of two sinusoidal components each peaking when the magnetic field is parallel to a high symmetry. We propose that anharmonicity may play a major role and argue that the magnetic field can exert a torque on electric dipolar waves traveling with phonons.

cond-mat.str-el

Comment on Unusual violation of the Wiedemann-Franz law at ultralow temperatures in topological compensated semimetals

Recently, Wang et al. [1] reported on an unusual violation of Wiedemann-Franz law in three semimetals. We compare their observations to our observations in a variety of systems, where the apparent WF law violations in the same temperature range arise as a consequence of electron-phonon decoupling. Given the empirical similarity of their data with these cases, the most plausible explanation for the reported violation is an experimental artefact.

cond-mat.str-el