arXiv subjects

Kan Zhao

Publications and source records attributed to Kan Zhao.

11 recordsLinked to original sources

arXiv2026

1/9 Magnetization Plateau in a Classical Kagome Ising Ferromagnet with Competing Further-Neighbor Interactions

The two-dimensional kagome lattice is a paradigmatic platform for exploring geometrically frustrated magnetism. While the nearest-neighbor ferromagnetic Ising model on this lattice is theoretically trivial, competing further-neighbor interactions can reintroduce severe frustration. In this work, we systematically investigate a classical kagome Ising model with ferromagnetic nearest-neighbor (J1) and antiferromagnetic second- (J2) and third-neighbor (J3) couplings using simulated annealing Monte Carlo methods. We demonstrate that while J2 couplings merely suppress the conventional ferromagnetic order, the inclusion of J3 fundamentally reconstructs the low-temperature phase diagram. This extended geometric frustration stabilizes a novel ordered phase characterized by a robust 1/9 magnetization plateau and a massively enlarged 3 by 3 magnetic supercell. Crucially, this fractional ordered phase manifests as a stability plateau in the phase diagram, where its critical temperature becomes nearly independent of the coupling strength J3. We also calculate the corresponding static spin structure factor, revealing a distinct Z6-symmetric reciprocal-space signature for experimental identification. Our findings reveal that complex fractional magnetic orders can emerge purely from classical geometric frustration induced by competing extended interactions, providing a distinct mechanism for understanding fractionally ordered states in real frustrated magnets.

cond-mat.str-el↗

arXiv2026

Ising Supercriticality and Universal Magnetocalorics in Spiral Antiferromagnet Nd$_3$BWO$_9$

The celebrated analogy between the pressure-temperature phase diagram of a liquid-gas system and the field-temperature phase diagram of a ferromagnet has long been a cornerstone for understanding universality of phase transitions and critical phenomena. Here we extend this analogy to a highly frustrated antiferromagnet, the spiral Ising compound Nd$_3$BWO$_9$ with kagome layers. In its phase diagram, we identify a metamagnetic transition line with a critical endpoint (CEP) located at $\mu_0H_{\mathrm{c}} \simeq 1.04$ T and $T_{\mathrm{c}} \simeq 0.3$ K. Above the CEP, an Ising supercritical regime emerges with crossover lines that follow a universal scaling law, as evidenced by the specific heat, magnetic susceptibility, and magnetocaloric measurements. Remarkably, we observe highly sensitive magnetic cooling near the emergent CEP, characterized by a divergent magnetic Gr\"uneisen ratio $\Gamma_H \propto 1/t^{\beta+\gamma-1}$, with $\beta + \gamma \simeq 1.563$ the sum of critical exponents of the 3D Ising universality class and $t \equiv (T-T_{\rm c})/T_{\rm c}$ the reduced temperature. Adiabatic demagnetization from 2 K and 4 T reaches a minimum temperature of 195 mK, via a self-cascading process that combines supercritical and topological cooling. Our findings open a new avenue for studying supercritical phenomena and magnetic refrigeration with the frustrated rare-earth compounds RE$_3$BWO$_9$ and, more broadly, in Ising-anisotropic antiferromagnets such as spin ices.

cond-mat.str-el↗

arXiv2025

Antiferromagnetic ordering and critical behavior induced giant magnetocaloric effect in distorted kagome lattice Gd$_3$BWO$_9$

We synthesize the high-quality Gd$_3$BWO$_9$ single crystal and investigate its lowtemperature magnetic and thermodynamic properties. Below $T\rm_{N}$ = 1.08 K, the anisotropic behavior of magnetic susceptibilities reveals that the Gd$^{3+}$ moments exhibit the dominant antiferromagnetic coupling along the $c$-axis, while displaying a ferromagnetic arrangement in kagome plane. With pronounced magnetic frustration, in adiabatic demagnetization refrigeration experiments starting from initial conditions of 9 T and 2 K, Gd$_3$BWO$_9$ polycrystal reaches a minimum temperature of 0.151 K, significantly lower than its $T\rm_{N}$. Due to the high density of Gd$^{3+}$ ions ($S$=7/2), the maximum magnetic entropy change reaches over 50 J kg$^{-1}$ K$^{-1}$ under fields up to 7 T in Gd$_3$BWO$_9$, nearly 1.5 times as large as commercial sub-Kelvin magnetic coolant Gd$_3$Ga$_5$O$_{12}$(GGG). The H-T phase diagram of Gd$_3$BWO$_9$ under $H$//$c$ exhibits field-induced critical behavior near the phase boundaries. This observation aligns with the theoretical scenario in which a quantum critical point acts as the endpoint of a line of classical second-order phase transitions. Such behavior suggests the importance of further investigations into the divergence of magnetic Gr\"uneisen parameter in the vicinity of critical field at ultralow temperatures.

cond-mat.str-el↗

arXiv2025

Interplay of short-range bond order and A-type antiferromagnetic order in metallic triangular lattice GdZn$_3$P$_3$

We investigate a hexagonal ScAl$_3$C$_3$-type antiferromagnet GdZn$_3$P$_3$ single crystal. Compared with antiferromagnetic topological material EuM$_2$X$_2$ (M=Zn, Cd; X=P, As), the GdZn$_3$P$_3$ features an additional ZnP$_3$ trigonal planar units. Notably, single-crystal X-ray diffraction analysis reveals that Zn and P atoms within trigonal planar layer exhibit significant anisotropic displacement parameters with a space group of P63/mmc. Meanwhile, scanning transmission electron microscopy experiment demonstrates the presence of interstitial P atoms above and below the ZnP honeycomb lattice, suggesting potential ZnP bond instability within the ZnP$_3$ trigonal layers. Concerning the triangular Gd$^{3+}$ layer, the magnetic susceptibility $\chi$$(T)$ and heat capacity measurements reveal long-range antiferromagnetic order at T$_N$ = 4.5 K. Below T$_N$, the in-plane $\chi$$(T)$ is nearly 4 times the $\chi$$(T)$ along $c$ axis, indicative of strong magnetic anisotropy. The Curie Weiss fitting to the low temperature $\chi$$(T)$ data reveals ferromagnetic interaction ($\theta$$_{CW}$ = 5.2 K) in ab-plane, and antiferromagnetic interaction ($\theta$$_{CW}$ = -1 K) along c axis, suggesting the ground state as an A-type antiferromagnetic order. Correspondingly, the density function theory calculation shows that GdZn$_3$P$_3$ is an indirect semiconductor with a band gap 0.27 eV, supported by the resistivity measurement on polycrystal sample. Interestingly, the GdZn$_3$P$_3$ single crystal exhibits metallic conductivity with an anomaly at T$_N$, likely associated with the observation of interstitial P atoms mentioned above. Therefore, our results establish GdZn$_3$P$_3$ system as a concrete example for investigating the coupling between charge carrier and triangular lattice magnetism in the two-dimensional lattice framework, on the background of short-range bond order.

cond-mat.str-el↗

arXiv2025

E-21 Level Instability Frequency Dissemination over 2067 km noisy Telecommunication Infrastructure

The realization of ultra stable optical frequency transmission through fiber networks is critical for advancing global optical frequency standards and enabling applications such as redefining the second in the International System of Units, geophysical sensing, quantum network construction, and fundamental physics experiments. However, achieving high reliability and low instability optical frequency carrier transmission links over distances exceeding thousands of kilometers remains technically challenging, thereby limiting the scalability and reliability of such networks. In this study, we experimentally demonstrate that the noise accumulation in long distance optical links can be mitigated by narrowband purification of the optical signal's phase noise, enabling optical links of theoretically unlimited length. Additionally, we implemented digital optical phase measurement and feedback technology to calibrate noise compensation deviations caused by inconsistencies in round trip optical frequencies, enhancing link stability. By adopting digital phase measurement instead of traditional phase detectors, we expanded the dynamic noise tolerance range of the optical phase-locked loop, significantly improving system reliability. Ultimately, on a 2067 km telecommunications fiber link with a noise level exceeding 5000 rad^2/Hz.km, we achieved an optical frequency transfer with a daily instability of 2.9 E-21 without experiencing any optical cycle slips maintaining continuous operation for four days. This work establishes a technical foundation for leveraging existing fiber resources to construct global scale optical frequency standard networks.

physics.optics↗

arXiv2025

3D XY Universality and Nonlinear magnetic susceptibility in a kagome ice compound

Kagome spin ice is an intriguing class of spin systems constituted by in-plane Ising spins with ferromagnetic interaction residing on the kagome lattice, theoretically predicted to host a plethora of magnetic transitions and excitations. In particular, different variants of kagome spin ice models can exhibit different sequences of symmetry breaking upon cooling from the paramagnetic to the fully ordered ground state. Recently, it has been demonstrated that the frustrated intermetallic HoAgGe stands as a faithful solid-state realization of kagome spin ice. Here we use single crystal neutron diffuse scattering to map the spin ordering of HoAgGe at various temperatures more accurately and surprisingly find that the ordering sequence appears to be different from previously known scenarios: From the paramagnetic state, the system first enters a partially ordered state with fluctuating magnetic charges, in contrast to a charge-ordered paramagnetic phase before reaching the fully ordered state. Through state-of-the-art Monte Carlo simulations and scaling analyses using a quasi-2D model for the distorted Kagome spin ice in HoAgGe, we elucidate a single three-dimensional (3D) XY phase transition into the ground state with broken time-reversal symmetry (TRS). However, the 3D XY transition has a long crossover tail before the fluctuating magnetic charges fully order. More interestingly, we find both experimentally and theoretically that the TRS breaking phase of HoAgGe features an unusual, hysteretic response: In spite of their vanishing magnetization, the two time-reversal partners are distinguished and selected by a nonlinear magnetic susceptibility tied to the kagome ice rule. Our discovery not only unveils a new symmetry breaking hierarchy of kagome spin ice, but also demonstrates the potential of TRS-breaking frustrated spin systems for information technology applications.

cond-mat.str-el↗

arXiv2023

Time-reversal-like degeneracies distinguished by the anomalous Hall effect in a metallic kagome ice compound

In magnetic crystals, despite the explicit breaking of time-reversal symmetry, two equilibrium states related by time reversal are always energetically degenerate. In ferromagnets such time-reversal degeneracy can be manifested by hysteresis loops in the magnetic field dependence of the magnetization and, if metallic, in the anomalous Hall effect. Importantly, both quantities simply change signs but not their absolute sizes under time reversal, which follows from their fundamental definitions. Our integral experimental and theoretical study shows that in the metallic kagome spin ice HoAgGe subject to finite magnetic fields parallel to the kagome plane, an emergent time-reversal-like degeneracy appears between magnetic states that have the same energy and net magnetization, but different sizes of the anomalous Hall effect. These degeneracies are unraveled by finite hysteresis in the field-dependent anomalous Hall effect contrasted with the vanishing hysteresis in the magnetization, which appears only at low-temperatures T$<$4K when the kagome spin ice is fully ordered into $\sqrt{3}$$\times$$\sqrt{3}$ state. By explicitly determining the degenerate states and calculating the corresponding physical properties using a tight-binding model, we nailed down the time-reversal-like operation that transforms these degenerate states into each other. The operation is related to the nontrivial distortion of the kagome lattice in HoAgGe and is effective only because of the richness of degenerate states unique to kagome spin ice. Our work points to the powerful role of the anomalous Hall effect to diagnose hidden symmetries in frustrated spin systems.

cond-mat.str-el↗

arXiv2023

Magnetic tuning of band topology evidenced by exotic quantum oscillations in the Dirac semimetal EuMnSb$_2$

Interplay between magnetism and electronic band topology is of central current interest in topological matter research. We use quantum oscillations as powerful tool to probe the evolution of band topology in the Dirac semimetal EuMnSb$_2$. The Eu local 4f magnetic moments display different antiferromagnetic states below 25 K and a field-polarized phase above 16 T. Upon cooling from 65 K into the field-polarized state, an exotic temperature dependent shift of oscillation peaks arises, accompanied by the development of non-zero Berry phase and a huge unconventional splitting of the oscillations. Band-structure calculations confirm the change from trivial to non-trivial band topology induced by the ferromagnetic Eu state, classifying EuMnSb$_2$ as unique magnetic topological semimetal.

cond-mat.str-el↗

arXiv2021

Gapless Spin Liquid Behavior in A Kagome Heisenberg Antiferromagnet with Randomly Distributed Hexagons of Alternate Bonds

We demonstrate that the new single crystal of YCu$_3$[OH(D)]$_{6.5}$Br$_{2.5}$ (YCOB) is a kagome Heisenberg antiferromagnet (KHA) without evident orphan spins ($\ll$ 0.8\%). The site mixing between polar OH$^-$ and non-polar Br$^-$ causes local distortions of Cu-O-Cu exchange paths, and gives rise to 70(2)\% of randomly distributed hexagons of alternate bonds ($\sim$ $J_1-ΔJ$ and $J_1+ΔJ$) and the rest of almost uniform hexagons ($\sim$ $J_1$) on the kagome lattice. Simulations of the random exchange model with $ΔJ$/$J_1$ = 0.7(1) show good agreement with the experimental observations, including the weak upturn seen in susceptibility and the slight polarization in magnetization. Despite the average antiferromagnetic coupling of $J_1$ $\sim$ 60 K, no conventional freezing is observed down to $T$ $\sim$ 0.001$J_1$, and the raw specific heat exhibits a nearly quadratic temperature dependence below 1 K $\sim$ 0.02$J_1$, phenomenologically consistent with a gapless (spin gap $\leq$ 0.025$J_1$) Dirac quantum spin liquid (QSL). Our result sheds new light on the theoretical understanding of the randomness-relevant gapless QSL behavior in YCOB, as well as in other relevant materials.

cond-mat.str-el↗

arXiv2020

Anisotropic spin distribution and perpendicular magnetic anisotropy in the layered ferromagnetic semiconductor (Ba,K)(Zn,Mn)$_{2}$As$_{2}$

Perpendicular magnetic anisotropy of the new ferromagnetic semiconductor (Ba,K)(Zn,Mn)$_{2}$As$_{2}$ is studied by angle-dependent x-ray magnetic circular dichroism measurements. The large magnetic anisotropy with the anisotropy field of 0.85 T is deduced by fitting the Stoner-Wohlfarth model to the magnetic-field-angle dependence of the projected magnetic moment. Transverse XMCD spectra highlights the anisotropic distribution of Mn 3$d$ electrons, where the $d_{xz}$ and $d_{yz}$ orbitals are less populated than the $d_{xy}$ state because of the $D_{2d}$ splitting arising from the elongated MnAs$_{4}$ tetrahedra. It is suggested that the magnetic anisotropy originates from the degeneracy lifting of $p$-$d_{xz}$, $d_{yz}$ hybridized states at the Fermi level and resulting energy gain due to spin-orbit coupling when spins are aligned along the $z$ direction.

cond-mat.str-el↗

arXiv2020

Realization of the kagome spin ice state in a frustrated intermetallic compound

Spin ices are exotic phases of matter characterized by frustrated spins obeying local ice rules, in analogy with the electric dipoles in water ice. In two dimensions, one can similarly define ice rules for in-plane Ising-like spins arranged on a kagome lattice. These ice rules require each triangle plaquette to have a single monopole, and can lead to various unique orders and excitations. Using experimental and theoretical approaches including magnetometry, thermodynamic measurements, neutron scattering and Monte Carlo simulations, we establish HoAgGe as a crystalline (i.e. non-artificial) system that realizes the kagome spin ice state. The system features a variety of partially and fully ordered states and a sequence of field-induced phases at low temperatures, all consistent with the kagome ice rule.

cond-mat.str-el↗