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Karel Prokeš

Publications and source records attributed to Karel Prokeš.

5 recordsLinked to original sources

A fluctuation-free pathway for a topological magnetic phase transition

Topological magnetic textures are particle-like spin configurations stabilized by competing interactions. Their formation is commonly attributed to fluctuation-driven, first-order nucleation processes requiring activation over a topological energy barrier. Here, we demonstrate an alternative barrier- and fluctuation-free pathway for nucleating topological magnetic textures, triggered in our experiments by an excitation-induced spin reorientation transition. By combining x-ray imaging, scattering and micromagnetic simulations, we show that the system follows a deterministic cascade of symmetry-breaking phase transitions after excitation. First, the system undergoes a second-order phase transition from a homogeneous state to weak stripe domains, then a first-order transition to topologically trivial bubbles, and finally a topological switching event into skyrmionic textures. Through simulations, we generalize our findings and demonstrate that this pathway is active in a vast range of low-anisotropy materials. This previously unrecognized, spontaneous transition pathway suggests strategies for rapid, low-energy generation of topological spin textures and points to a general role of intrinsic modulational instabilities in phase transitions beyond magnetism.

cond-mat.mtrl-sci↗

Direct observation of Néel-type skyrmions and domain walls in a ferrimagnetic DyCo$_3$ thin film

Isolated magnetic skyrmions are stable, topologically protected spin textures that are at the forefront of research interests today due to their potential applications in information technology. A distinct class of skyrmion hosts are rare earth - transition metal (RE-TM) ferrimagnetic materials. To date, the nature and the control of basic traits of skyrmions in these materials are not fully understood. We show that for an archetypal ferrimagnetic material DyCo$_3$ that exhibits a strong perpendicular anisotropy, the ferrimagnetic skyrmion size can be tuned by an external magnetic field. Moreover, by taking advantage of the high spatial resolution of scanning transmission X-ray microscopy (STXM) and utilizing a large x-ray magnetic linear dichroism (XMLD) contrast that occurs naturally at the RE resonant edges, we resolve the nature of the magnetic domain walls of ferrimagnetic skyrmions. We demonstrate that through this method one can easily discriminate between Bloch and Néel type domain walls for each individual skyrmion. For all isolated ferrimagnetic skyrmions, we observe that the domain walls are of Néel-type. This key information is corroborated with results of micromagnetic simulations and allows us to conclude on the nature of the Dzyaloshinskii-Moriya interaction (DMI) which concurs to the stabilisation of skyrmions in this ferrimagnetic system. Establishing that an intrinsic DMI occurs in RE-TM materials will also be beneficial towards a deeper understanding of chiral spin texture control in ferrimagnetic materials.

cond-mat.mtrl-sci↗

Evolution of the partially frustrated magnetic order in CePd$_{1-x}$Ni$_x$Al

We report on a single-crystal neutron diffraction study of the evolution of the antiferromagnetic order in the heavy-fermion compound CePd$_{1-x}$Ni$_x$Al which exhibits partial geometric frustration due to its distorted Kagomé structure. The magnetic structure is found to be unchanged with a propagation vector $Q_\mathrm{AF} \approx (0.5~0~0.35)$ for all Ni concentrations $x$ up to $x_c \approx 0.14$. Upon approaching the quantum critical concentration $x_c$, the ordered moment vanishes linearly with Néel temperature $T_{\rm N}$, in good agreement with CePdAl under hydrostatic pressure. For all Ni concentrations, substantial short-range magnetic correlations are observed above $T_{\rm N}$ as a result of frustration.

cond-mat.str-el↗

Magnetic structures in the rich magnetic phase diagram of Ho$_2$RhIn$_8$

The magnetic phase diagram of the tetragonal Ho$_2$RhIn$_8$ compound has similar features to many related systems, revealing a zero magnetic field AF1 and a field-induced AF2 phases. Details of the magnetic order in the AF2 phase were not reported yet for any of the related compounds. In addition, only the Ho$_2$RhIn$_8$ phase diagram contains a small region of the incommensurate zero-field AF3 phase. We have performed a number of neutron diffraction experiments on single crystals of Ho$_2$RhIn$_8$ using several diffractometers including experiments in both horizontal and vertical magnetic fields up to 4 T. We present details of the magnetic structures in all magnetic phases of the rich phase diagram of Ho$_2$RhIn$_8$. The Ho magnetic moments point along the tetragonal $c$ axis in every phase. The ground-state AF1 phase is characterized by propagation vector $\textbf{k}$ = (1/2, 0, 0). The more complex ferrimagnetic AF2 phase is described by four propagation vectors $\textbf{k}_{0}$ = (0, 0, 0), $\textbf{k}_{1}$ = (1/2, 0, 0), $\textbf{k}_{2}$ = (0, 1/2, 1/2), $\textbf{k}_{3}$ = (1/2, 1/2, 1/2). The magnetic structure in the AF3 phase is incommensurate with $\textbf{k}_{AF3}$ = (0.5, $δ$, 0). Our results are consistent with theoretical calculations based on crystal field theory.

cond-mat.str-el↗

Low magnetic field phase diagram of UCoGe

We propose an alternate scenario for the relation between ferromagnetism (FM) and superconductivity (SC) in UCoGe at ambient pressure. On the basis of neutron polarimetry measurement performed in strictly zero field on a single-crystal at ambient pressure, we claim that the SC phase does exist in spite of lack of long-range FM order. Moreover, the SC regime dominates to the paramagnetic (PM) state in small external magnetic fields. Above the critical SC temperature, TSC = 0.64 K, the zero-field state is characterized by a regime with strong FM spin fluctuations, suggesting the proximity of the FM quantum critical point. We present an ambient-pressure phase diagram of UCoGe based on our resistivity, magnetization and neutron polarimetry results.

cond-mat.supr-con↗