arXiv subjects

Karolina Waszkowska

Publications and source records attributed to Karolina Waszkowska.

2 recordsLinked to original sources

arXiv2026

Cavity-mediated coherence protection and one-axis twisting for spins in solids

Long-range interactions between emitters give rise to collective phenomena, including superradiance, spin squeezing, and coherence protection, that are important to both fundamental physics and quantum technologies. Despite progress in cold atoms, coherent cavity-mediated all-to-all interactions have not yet been realized in a solid-state ensemble. Here we demonstrate such interactions in a $^{171}$Yb$^{3+}$:CaWO$_4$ crystal coupled to a microwave resonator, observing superradiant emission on resonance and unitary one-axis twisting dynamics in the dispersive regime. The same interaction also opens a many-body energy gap that suppresses inhomogeneous dephasing, extending the ensemble Ramsey coherence time from tens of microseconds to milliseconds without decoupling pulses. These results establish a solid-state platform for collective many-body physics with direct implications for quantum technologies. Specifically, the observed one-axis twisting dynamics opens a path towards spin squeezing for entanglement-enhanced quantum metrology, and the extended coherence due to gap-protection is relevant for both microwave photon storage and precision measurement.

quant-ph↗

arXiv2021

Anisotropic Confinement of Chromophores Induces Second-Order Nonlinear Optics in a Nanoporous Photonic Metamaterial

Second-order nonlinear optics is the base for a large variety of devices aimed at the active manipulation of light. However, physical principles restrict its occurrence to non-centrosymmetric, anisotropic matter. This significantly limits the number of base materials exhibiting nonlinear optics. Here, we show that embedding chromophores in an array of conical channels 13 nm across in monolithic silica results in mesoscopic anisotropic matter and thus in a hybrid material showing second-harmonic generation (SHG). This non-linear optics is compared to the one achieved in corona-poled polymer films containing the identical chromophores. It originates in confinement-induced orientational order of the elongated guest molecules in the nanochannels. This leads to a non-centrosymmetric dipolar order and hence to a non-linear light-matter interaction on the sub-wavelength, single-pore scale. Our study demonstrates that the advent of large-scale, self-organised nanoporosity in monolithic solids along with confinement-controllable orientational order of chromophores at the single-pore scale provides a reliable and accessible tool to design materials with a nonlinear meta-optics.

physics.optics↗