arXiv subjects

Katarzyna Sadecka

Publications and source records attributed to Katarzyna Sadecka.

5 recordsLinked to original sources

arXiv2026

Impact of exciton-phonon and exciton-magnon interaction on transport in anisotropic 2D magnetic semiconductors

Two-dimensional magnetic semiconductors provide a unique platform for exploring the interplay between charge, lattice, spin, and light. The strong Coulomb interaction combined with long-range magnetic order enables efficient coupling between excitons and both lattice vibrations and spin excitations, thereby strongly influencing exciton dynamics and transport in these materials. Here, we develop a microscopic many-body theory of exciton--phonon and exciton--magnon interactions in mono- and bilayer CrSBr. We demonstrate that the quasi-one-dimensional character of excitons in CrSBr gives rise to strongly anisotropic exciton--phonon and exciton--magnon scattering, resulting in direction-dependent diffusion coefficients. Furthermore, we identify a distinct temperature dependence originating from one-phonon and two-magnon scattering processes, providing characteristic signatures of the underlying microscopic interactions. Our work establishes a microscopic framework for understanding exciton transport in magnetic van der Waals semiconductors and provides guidance for future optical spectroscopy and exciton transport experiments.

cond-mat.mes-hall↗

arXiv2026

Magnetoexcitons and Massive Dirac Fermions in Monolayers of Transition Metal Dichalcogenides in a High Magnetic Field

We present a theory of the emission spectrum of magnetoexcitons interacting with a $ν= 1$ quantum Hall state of massive Dirac fermions in monolayer transition metal dichalcogenides in high magnetic fields. Using an ab initio-parametrized massive Dirac fermion model including valley and spin degrees of freedom, combined with exact diagonalization techniques, we show that interband emission from the massive Dirac Fermion magnetoexciton interacting with $ν= 1$ state directly probes intra-conduction-band excitations of the $ν= 1$. Many-body interactions with the filled massive Dirac fermion $ν= 1$ level yield a strong renormalization of the emission spectrum, including fully polarized emission, a pronounced redshift, and broadening relative to neutral and charged excitons. The calculated spectra are consistent with recent experiments [1-3], establishing magneto-spectroscopy as a probe of finite carrier densities in massive Dirac systems.

cond-mat.mes-hall↗

arXiv2024

Electrically tunable MoSe$_2$/WSe$_2$ heterostructure-based quantum dot

We describe here a theory of a quantum dot in an electrically tunable MoSe$_2$/WSe$_2$ heterostructure. Van der Waals heterostructures allow for tuning their electronic properties beyond their monolayer counterparts. We start by determining their electronic structure using density functional theory. We obtain the type-II band alignment and close in energy conduction band minima (valleys) at the $K$ and $Q$ points in the Brillouin zone. The valence band maxima, also energetically close, are located at the $K$ and $Γ$ points. By analyzing the Kohn-Sham wavefunctions, we describe the layer, spin, and orbital contributions. Next, we construct an \textit{ab initio}-based tight-binding model, which helps us to better understand the complexity of the interlayer interactions. We determine the effect of a vertical electric field, showing that vertical gating enables control of valleys extrema and their occupancy. Finally, we employ the tight-binding model to investigate laterally gated quantum dots and analyze the influence of a perpendicular electric field on their energy spectrum. Our results demonstrate that tuning the electric field enables control over the valley character of the quantum dot states, selectively localizing them in either the $K$ or $Q$ valleys, as evidenced by their characteristic degeneracies and wavefunctions.

cond-mat.mes-hall↗

arXiv2024

Optical Properties of Gated Bilayer Graphene Quantum Dots with Trigonal Warping

We determine the optical properties of gated bilayer graphene quantum dots with trigonal warping (TW) of single-particle energy spectra. The lateral structure of metallic gates confines electrons and holes in a quantum dot (QD) electrostatically. The gated bilayer graphene energy spectrum is characterized by two K-valleys surrounded by three minivalleys with energies depending on the applied vertical electric field. Employing an atomistic tight-binding model, we compute the single-particle QD states and analyze the influence of TW on the energy spectrum as the lateral confining potential depth varies. We find a regime where the QD levels are dominated by the presence of three minivalleys around each K-valley. Next, we compute dipole matrix elements and analyze the oscillator strengths and optical selection rules for optical valence to conduction band transitions. We then include electron-electron interactions by first computing the microscopic Coulomb matrix elements, electron self-energy, and solving the Bethe-Salpeter equation to obtain the excitonic spectrum. Finally, we obtain the absorption spectrum for a shallow confining potential depth, which further amplifies the effects of TW on the optical properties. Our results predict the existence of two degenerate bright exciton states, each built of the three minivalley states that do not exist in the deep confinement regime, where the effects of TW are negligible.

cond-mat.mes-hall↗

arXiv2023

Electrically Tunable Fine Structure of Negatively Charged Excitons in Gated Bilayer Graphene Quantum Dots

We predict here the fine structure of an electrically tunable negatively charged exciton (trion) composed of two electrons and a hole confined in a gated bilayer graphene quantum dot (QD). We start with an atomistic approach, allowing us to compute confined electron and confined hole QD states for a structure containing over one million atoms. Using atomistic wavefunctions we compute Coulomb matrix elements and self-energies. In the next step, by solving the Bethe-Salpeter-like equation for trions, we describe a negatively charged exciton, built as a strongly interacting interlayer complex of two electrons in the conduction band and one hole in the valence band. Unlike in conventional semiconducting QDs, we show that the trion contains a fine structure composed of ten states arising from the valley and spin degrees of freedom. Finally, we obtain absorption into and emission from the trion states. We predict the existence of bright low-energy states and propose to extract the fine structure of the trion using the temperature dependence of emission spectra.

cond-mat.mes-hall↗