arXiv subjects

Katja C. Nowack

Publications and source records attributed to Katja C. Nowack.

At least 19 recordsLinked to original sources

arXiv2026

Signatures of nodal superconductivity in stoichiometric FeTe

Superconductivity in stoichiometric FeTe opens access to the FeTe endpoint of the Fe(Se,Te) phase diagram, yet the nature of its superconducting pairing state remains unresolved. In this work, we combine scanning superconducting quantum interference device (SQUID) microscopy, electrical transport, scanning tunneling microscopy and spectroscopy (STM/S), and mean-field calculations to investigate the local superfluid response and pairing state of FeTe thin films with tunable stoichiometry. Even in stoichiometric FeTe, we observe micrometer-scale spatial variations in both superfluid stiffness and superconducting transition temperature $T_c$, while the London penetration depth remains non-saturating down to 0.02$T_c$ and follows a power-law temperature dependence with an exponent of approximately 1-1.5. Together with a V-shaped low-energy density of states and two-gap modeling, these results indicate a superconducting state with gap nodes or deep minima, consistent with either a $d$-wave or nodal $s$-wave superconducting state. Our findings establish stoichiometric FeTe as a distinct superconducting regime that departs from the trend toward more isotropic gaps at intermediate Se/Te compositions, providing a new benchmark for modern microscopic theories of iron-chalcogenide superconductivity. Our work also reveals a crossover from weak to rapid suppression of $T_c$ as superfluid stiffness decreases, connecting FeTe to the broader phenomenology observed in unconventional superconductors.

cond-mat.supr-con↗

arXiv2026

Imaging Harmonic Generation of Magnons

This work combines theory and experiment to examine the mechanisms underlying the harmonic generation of magnons. We develop a nonlinear spin-wave framework that is directly analogous to harmonic generation in nonlinear optics, and combine it with scanning nitrogen-vacancy (NV) center magnetometry to image and quantify magnonic harmonic generation in a Ni$_{81}$Fe$_{19}$/Pt microstripe. Within this framework, the harmonic response arises from nonlinear magnetization dynamics localized at strongly inhomogeneous textures, such as the sample edges and domain walls, that act as anharmonic confining potentials. Scanning probe imaging confirms that the harmonic response is correspondingly nonuniform and concentrated near the sample edges. We measure an expected nonlinear power-law scaling, a systematic shift toward larger wavevector excitations at higher harmonic order, and a spin-selective response indicative of an increasingly chiral harmonic stray field. These results provide a microscopic understanding of magnonic harmonic generation and highlight its potential for engineering nonlinear functionality in magnonic systems.

cond-mat.mes-hall↗

arXiv2026

Imaging the Superconducting Proximity Effect in S-S'-S Transition Edge Sensors

Proximity effects at superconducting interfaces, between different superconductors (S-S') or between superconductors and normal metals (S-N), are fundamental to the performance of superconducting electronics, yet only few experiments have directly probed the spatial structure of proximity effects within a device. This is particularly relevant for transition edge sensors (TESs), where the interplay of direct and inverse proximity effects governs detector sensitivity. Here, we use scanning superconducting interference device (SQUID) susceptometry to directly image the local diamagnetic response in functional S-S'-S TES structures. We resolve long range proximity coupling extending over tens of micrometers, revealing that the local transition temperature is dramatically tuned by neighboring regions, being either enhanced by superconducting (S) leads or suppressed by normal metal (N) contacts. Our observations are quantitatively supported by Ginzburg Landau modeling of the device geometry and calculations of the temperature dependent diamagnetism based on self-consistent Usadel equations. By providing spatially resolved measurements of the interplay of proximity effects in TES devices, this work establishes a framework for understanding and controlling superconducting states in heterogeneous superconducting structures.

cond-mat.supr-con↗

arXiv2025

Unconventional polaronic ground state in superconducting LiTi$_2$O$_4$

Geometrically frustrated lattices can display a range of correlated phenomena, ranging from spin frustration and charge order to dispersionless flat bands due to quantum interference. One particularly compelling family of such materials is the half-valence spinel Li$B_2$O$_4$ materials. On the $B$-site frustrated pyrochlore sublattice, the interplay of correlated metallic behavior and charge frustration leads to a superconducting state in LiTi$_2$O$_4$ and heavy fermion behavior in LiV$_2$O$_4$. To date, however, LiTi$_2$O$_4$ has primarily been understood as a conventional BCS superconductor despite a lattice structure that could host more exotic groundstates. Here, we present a multimodal investigation of LiTi$_2$O$_4$, combining ARPES, RIXS, proximate magnetic probes, and ab-initio many-body theoretical calculations. Our data reveals a novel mobile polaronic ground state with spectroscopic signatures that underlie co-dominant electron-phonon coupling and electron-electron correlations also found in the lightly doped cuprates. The cooperation between the two interaction scales distinguishes LiTi$_2$O$_4$ from other superconducting titanates, suggesting an unconventional origin to superconductivity in LiTi$_2$O$_4$. Our work deepens our understanding of the rare interplay of electron-electron correlations and electron-phonon coupling in unconventional superconducting systems. In particular, our work identifies the geometrically frustrated, mixed-valence spinel family as an under-explored platform for discovering unconventional, correlated ground states.

cond-mat.supr-con↗

arXiv2025

Flux trapping in NbTiN strips

We use scanning superconducting quantum interference device (SQUID) microscopy to image individual vortices in superconducting strips fabricated from NbTiN thin films. By repeatedly field-cooling strips of different widths in applied magnetic fields, we extract the threshold field at which the first vortex enters a strip, as well as the number and spatial configuration of vortices beyond this threshold. We model vortex behavior with and without considering the effect of pinning by numerically minimizing the Gibbs free energy of vortices in the strips. Our measurements provide a first experimental benchmark for understanding the flux trapping properties of NbTiN thin films, directly relevant to NbTiN-based superconducting circuits and devices.

cond-mat.supr-con↗

arXiv2025

Visualizing the breakdown of the quantum anomalous Hall effect

The creation of topologically non-trivial matter across electronic, mechanical, cold-atom, and photonic platforms is advancing rapidly, yet understanding the breakdown of topological protection remains a major challenge. In this work, we use magnetic imaging combined with global electrical transport measurements to visualize the current-induced breakdown of the quantum anomalous Hall effect (QAHE) in a magnetically doped topological insulator. We find that dissipation emerges at localized hot spots near electrical contacts, where an abrupt change in Hall angle leads to significant distortions of the current density. Using the local magnetization as a proxy for electron temperature, we directly observe that the electrons are driven out of equilibrium with the lattice at the hot spots and throughout the device in the breakdown regime. By characterizing energy relaxation processes in our device, we show that the breakdown of quantization is governed entirely by electron heating, and that a vanishing thermal relaxation strength at millikelvin temperatures limits the robustness of the QAHE. Our findings provide a framework for diagnosing energy relaxation in topological materials and will guide realizing robust topological protection in magnetic topological insulators.

cond-mat.mes-hall↗

arXiv2025

Imaging signatures of edge currents in a magnetic topological insulator

Magnetic topological insulators (MTIs) host topologically protected edge states, but the role that these edge states play in electronic transport remains unclear. Using scanning superconducting quantum interference device (SQUID) microscopy, we performed local measurements of the current distribution in a quantum anomalous Hall (QAH) insulator at large bias currents, where the quantization of the conductivity tensor breaks down. We find that bulk currents in the channel interior coexist with edge currents at the sample boundary. While the position of the edge current changes with the reversal of the magnetic field, it does not depend on the current direction. To understand our observations, we introduce a model which includes contributions from both the sample magnetization and currents driven by chemical potential gradients. To parameterize our model, we use local measurements of the chemical potential induced changes in the sample magnetization. Our model reveals that the observed edge currents can be understood as changes in the magnetization generated by the electrochemical potential distribution in the sample under bias. Our work underscores the complexity of electronic transport in MTIs and highlights both the value and challenges of using magnetic imaging to disentangle various contributions to the electronic transport signatures.

cond-mat.mes-hall↗

arXiv2024

Direct Comparison of Magnetic Penetration Depth in Kagome Superconductors AV$_3$Sb$_5$ (A = Cs, K, Rb)

We report measurements of the local temperature-dependent penetration depth, $\lambda(T)$, in the Kagome superconductors AV$_3$Sb$_5$ (A = Cs, K, Rb) using scanning superconducting quantum interference device (SQUID) microscopy. Our results suggest that the superconducting order in all three compounds is fully gapped, in contrast to reports of nodal superconductivity in KV$_3$Sb$_5$ and RbV$_3$Sb$_5$. Analysis of the temperature-dependent superfluid density, $\rho_s(T)$, shows deviations from the behavior expected for a single isotropic gap, but the data are well described by models incorporating either a single anisotropic gap or two isotropic gaps. Notably, the temperature dependences of $\lambda(T)$ and $\rho_s(T)$ in KV$_3$Sb$_5$ and RbV$_3$Sb$_5$ are qualitatively more similar to each other than to CsV$_3$Sb$_5$, consistent with the superconducting phase reflecting features of the normal-state band structure. Our findings provide a direct comparison of the superconducting properties across the AV$_3$Sb$_5$ family.

cond-mat.supr-con↗

arXiv2024

Direct Imaging of Transition-Edge Sensors with Scanning SQUID Microscopy

Significant advancements have been made in understanding the physics of transition-edge sensors (TESs) over the past decade. However, key questions remain, particularly a detailed understanding of the current-dependent resistance of these detectors when biased within their superconducting transition. We use scanning superconducting quantum interference device (SQUID) microscopy (SSM) to image the local diamagnetic response of aluminum-manganese alloy (Al-Mn) transition-edge sensors (TESs) near their critical temperature of approximately 175 mK. By doing so, we gain insights into how the device dimensions influence TES transition width, which in turn affects device operation and informs optimal device design. Our images reveal that the Al-Mn thin film near the niobium (Nb) leads exhibits an excess diamagnetic response at temperatures several milli-Kelvin (mK) higher than the bulk of the film farther from the contacts. A possible origin of this behavior is a longitudinal proximity effect between the Nb and Al-Mn where the TES acts as a weak link between superconducting leads. We discuss how this effect shapes the temperature dependence of the resistance as the spacing between the leads decreases. This work demonstrates that magnetic imaging with SSM is a powerful tool for local characterization of superconducting detectors.

cond-mat.supr-con↗

arXiv2024

Local magnetic response of superconducting Sr$\mathrm{_2}$RuO$\mathrm{_4}$ thin films and rings

We conduct local magnetic measurements on superconducting thin-film samples of Sr$\mathrm{_2}$RuO$\mathrm{_4}$ using scanning Superconducting Quantum Interference Device (SQUID) susceptometry. From the diamagnetic response, we extract the magnetic penetration depth, $λ$, which exhibits a quadratic temperature dependence at low temperatures. Although a quadratic dependence in high-purity bulk samples has been attributed to non-local electrodynamics, our analysis suggests that in our thin-film samples the presence of scattering is the origin of the quadratic dependence. While we observe micron-scale variations in the diamagnetic response and superconducting transition temperature, the form of the temperature dependence of $λ$ is independent of position. Finally, we characterize flux trapping in superconducting rings lithographically fabricated from the thin films, paving the way to systematic device-based tests of the superconducting order parameter in Sr$\mathrm{_2}$RuO$\mathrm{_4}$.

cond-mat.supr-con↗

arXiv2022

Current-induced switching of thin film $α$-Fe$_2$O$_3$ devices imaged using a scanning single-spin microscope

Electrical switching of Néel order in an antiferromagnetic insulator is desirable as a basis for memory applications. Unlike electrically-driven switching of ferromagnetic order via spin-orbit torques, electrical switching of antiferromagnetic order remains poorly understood. Here we investigate the low-field magnetic properties of 30 nm thick, c-axis oriented $α$-Fe$_2$O$_3$ Hall devices using a diamond nitrogen-vacancy (NV) center scanning microscope. Using the canted moment of $α$-Fe$_2$O$_3$ as a magnetic handle on its Néel vector, we apply a saturating in-plane magnetic field to create a known initial state before letting the state relax in low field for magnetic imaging. We repeat this procedure for different in-plane orientations of the initialization field. We find that the magnetic field images are characterized by stronger magnetic textures for fields along $[\bar{1}\bar{1}20]$ and $[11\bar{2}0]$, suggesting that despite the expected 3-fold magneto-crystalline anisotropy, our $α$-Fe$_2$O$_3$ thin films have an overall in-plane uniaxial anisotropy. We also study current-induced switching of the magnetic order in $α$-Fe$_2$O$_3$. We find that the fraction of the device that switches depends on the current pulse duration, amplitude and direction relative to the initialization field. Specifically, we find that switching is most efficient when current is applied along the direction of the initialization field.

cond-mat.mtrl-sci↗

arXiv2022

Superfluid response of an atomically thin, gate-tuned van der Waals superconductor

A growing number of two-dimensional superconductors are being discovered in the family of layered van der Waals (vdW) materials. Due to small sample volume, their characterization has been largely limited to electrical transport measurements. As a consequence, characterization of the diamagnetic response of the superfluid to an applied magnetic field, a defining property of any superconductor, has been lacking. Here, we use a local magnetic probe to directly measure the superfluid response of the tunable, gate-induced superconducting state in MoS$_2$. We find that the backgate changes the superconducting transition temperature non-monotonically whereas the superfluid stiffness at low temperature and the normal state conductivity monotonically increase with backgate voltage. In some devices, we find direct signatures in agreement with a Berezinskii-Kosterlitz-Thouless transition, whereas in others we find a broadened, shallow onset of the superfluid response. We show that the observed behavior is consistent with disorder playing an important role in determining the superconducting properties in superconducting MoS$_2$. Our work demonstrates that magnetic property measurements are within reach for vdW superconductors and reveals that the superfluid response significantly deviates from simple BCS-like behavior.

cond-mat.supr-con↗

arXiv2021

Direct visualization of electronic transport in a quantum anomalous Hall insulator

A quantum anomalous Hall (QAH) insulator is characterized by quantized Hall and vanishing longitudinal resistances at zero magnetic field that are protected against local perturbations and independent of sample details. This insensitivity makes the microscopic details of the local current distribution inaccessible to global transport measurements. Accordingly, the current distributions that give rise to the transport quantization are unknown. Here we use magnetic imaging to directly visualize the transport current in the QAH regime. As we tune through the QAH plateau by electrostatic gating, we clearly identify a regime in which the sample transports current primarily in the bulk rather than along the edges. Furthermore, we image the local response of the magnetization to electrostatic gating. Combined, these measurements suggest that incompressible regions carry the current within the QAH regime. Our observations indicate that the self-consistent electrostatics of the sample play a central role in determining the current distribution. Identifying the appropriate microscopic picture of electronic transport in QAH insulators and other topologically non-trivial states of matter is a crucial step towards realizing their potential in next-generation quantum devices.

cond-mat.mes-hall↗

arXiv2021

Reconstruction of Current Densities from Magnetic Images by Bayesian Inference

Electronic transport is at the heart of many phenomena in condensed matter physics and material science. Magnetic imaging is a non-invasive tool for detecting electric current in materials and devices. A two-dimensional current density can be reconstructed from an image of a single component of the magnetic field produced by the current. In this work, we approach the reconstruction problem in the framework of Bayesian inference, i.e. we solve for the most likely current density given an image obtained by a magnetic probe. To enforce a sensible current density priors are used to associate a cost with unphysical features such as pixel-to-pixel oscillations or current outside the device boundary. Beyond previous work, our approach does not require analytically tractable priors and therefore creates flexibility to use priors that have not been explored in the context of current reconstruction. Here, we implement several such priors that have desirable properties. A challenging aspect of imposing a prior is choosing the optimal strength. We describe an empirical way to determine the appropriate strength of the prior. We test our approach on numerically generated examples. Our code is released in an open-source \texttt{python} package called \texttt{pysquid}.

physics.data-an↗

arXiv2021

Electrically tunable and reversible magnetoelectric coupling in strained bilayer graphene

The valleys in hexagonal two-dimensional systems with broken inversion symmetry carry an intrinsic orbital magnetic moment. Despite this, such systems possess zero net magnetization unless additional symmetries are broken, since the contributions from both valleys cancel. A nonzero net magnetization can be induced through applying both uniaxial strain to break the rotational symmetry of the lattice and an in-plane electric field to break time-reversal symmetry owing to the resulting current. This creates a magnetoelectric effect whose strength is characterized by a magnetoelectric susceptibility, which describes the induced magnetization per unit applied in-plane electric field. Here, we predict the strength of this magnetoelectric susceptibility for Bernal-stacked bilayer graphene as a function of the magnitude and direction of strain, the chemical potential, and the interlayer electric field. We estimate that an orbital magnetization of ~5400 $μ_{\text{B}}/μ\text{m}^2$ can be achieved for 1% uniaxial strain and a 10 $μ\text{A}$ bias current, which is almost three orders of magnitude larger than previously probed experimentally in strained monolayer MoS$_2$. We also identify regimes in which the magnetoelectric susceptibility not only switches sign upon reversal of the interlayer electric field but also in response to small changes in the carrier density. Taking advantage of this reversibility, we further show that it is experimentally feasible to probe the effect using scanning magnetometry.

cond-mat.mes-hall↗

arXiv2021

Scanning SQUID microscopy in a cryogen-free dilution refrigerator

We report a scanning superconducting quantum interference device (SQUID) microscope in a cryogen-free dilution refrigerator with a base temperature at the sample stage of at least 30 mK. The microscope is rigidly mounted to the mixing chamber plate to optimize thermal anchoring of the sample. The microscope housing fits into the bore of a superconducting vector magnet, and our design accommodates a large number of wires connecting the sample and sensor. Through a combination of vibration isolation in the cryostat and a rigid microscope housing, we achieve relative vibrations between the SQUID and sample that allow us to image with micrometer resolution over a 150 $μ$m range while the sample stage temperature remains at base temperature. To demonstrate the capabilities of our system, we show images acquired simultaneously of the static magnetic field, magnetic susceptibility, and magnetic fields produced by a current above a superconducting micrometer-scale device.

cond-mat.mes-hall↗

arXiv2019

Gate-Tunable Graphene Hall Sensors with High Magnetic Field Sensitivity

Solid-state magnetic field sensors are important to both modern electronics and fundamental materials science. Many types of these sensors maintain high sensitivity only in a limited range of temperature and background magnetic field, but Hall-effect sensors are in principle able to operate over a broad range of these conditions. Here, we fabricate and characterize micrometer-scale graphene Hall sensors demonstrating high magnetic field sensitivity from liquid-helium to room temperature and in background magnetic field up to several Tesla. By tuning the charge carrier density with an electrostatic gate, we optimize the magnetic field sensitivity for different working conditions. From measurements of the Hall coefficient and the Hall voltage noise at 1 kHz, we estimate an optimum magnetic field sensitivity of 80 nT Hz$^{-1/2}$ at 4.2 K, 700 nT Hz$^{-1/2}$ at room temperature, and 3 $μ$T Hz$^{-1/2}$ in 3 T background magnetic field at 4.2 K. Our devices perform competitively with the best existing Hall sensor technologies at room temperature, outperform any Hall sensors reported in the literature at 4.2 K, and demonstrate high sensitivity for the first time in a few Tesla applied magnetic field.

cond-mat.mes-hall↗

arXiv2019

Spin Seebeck imaging of spin-torque switching in antiferromagnetic Pt/NiO heterostructures

As electrical control of Néel order opens the door to reliable antiferromagnetic spintronic devices, understanding the microscopic mechanisms of antiferromagnetic switching is crucial. Spatially-resolved studies are necessary to distinguish multiple nonuniform switching mechanisms; however, progress has been hindered by the lack of tabletop techniques to image the Néel order. We demonstrate spin Seebeck microscopy as a sensitive, table-top method for imaging antiferromagnetic order in thin films, and apply this technique to study spin-torque switching in NiO/Pt and Pt/NiO/Pt heterostructures. We establish the interfacial antiferromagnetic spin Seebeck effect in NiO as a probe of surface Néel order, resolving antiferromagnetic spin domains within crystalline twin domains. By imaging before and after applying current-induced spin torque, we resolve spin domain rotation and domain wall motion, acting simultaneously. We correlate the changes in spin Seebeck images with electrical measurements of the average Néel orientation through the spin Hall magnetoresistance, confirming that we image antiferromagnetic order.

cond-mat.mtrl-sci↗