arXiv subjects

Katsuya Hirota

Publications and source records attributed to Katsuya Hirota.

11 recordsLinked to original sources

arXiv2026

Development and Characterization of Low-Scattering Vanadium Nanoparticle Targets for Short-Range Interaction Searches

We developed high-purity vanadium-based nanoparticle targets for neutron scattering experiments aimed at exploring gravity-like short-range new interactions in the submicron regime. Vanadium and V-Ni nanoparticles were fabricated using top-down and bottom-up methods and quantitatively characterized by SEM-EDS, ICP-AES, NDIR and SAXS. Through the performance tests, an RF thermal plasma method was found to be the best from viewpoints of the reproducibility, dispersion of the radius, and contamination of metallic elements. The oxygen incorporation during fabrication was quantified, and its impact on the effective coherent scattering length was evaluated, leading to a minimum average coherent scattering length of $\mathrm{0.719(23)\,fm}$, comparable to that of natural vanadium. These results demonstrate that vanadium-based nanoparticle targets with controlled composition and nanostructure can be systematically designed and fabricated to suppress nuclear scattering backgrounds, thereby enabling experimentally viable coherent neutron scattering measurements for short-range interaction searches.

physics.ins-det↗

arXiv2026

First Constraint on P-odd/T-odd Cross Section in Polarized Neutron Transmission through Transversely Polarized $^{139}$La

We report the first constraint on time-reversal invariance violating (TRIV) effects in polarized neutron transmission through a transversely polarized $^{139}$La target. We formulate the transmission asymmetry within the density matrix formalism, explicitly incorporating the forward scattering amplitude of $^{139}$La including tensor polarization terms up to third-rank. The formalism is applied to existing transmission data originally obtained to measure the spin-dependent cross section near the $0.75$~eV $p$-wave resonance. Since these data were not optimized for P-odd/T-odd observables, the attainable sensitivity is intrinsically limited; nevertheless, they provide a useful test of the formalism on real experimental data. No statistically significant TRIV signal is observed. By analyzing the global $χ^2$ structure in the parameter space, we obtain an upper limit of $|W_T|<15~\mathrm{eV}$ at the 90\% confidence level. This corresponds to an upper limit on the resonance-averaged TRIV cross section of $|Δσ_{\not{T}\not{P}}|<8.3\times10^2~\mathrm{b}$. These results validate the present theoretical framework and provide guidance for future dedicated TRIV searches in polarized neutron transmission experiments.

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arXiv2022

Investigation of the neutron imaging applications using fine-grained nuclear emulsion

Neutron imaging is a non-destructive inspection technique with a wide range of applications. One of the important aspects concerning neutron imaging is achieving micrometer-scale spatial resolution. Developing a neutron detector with a high resolution is a challenging task. Neutron detectors, based on fine-grained nuclear emulsion, may be suitable for high resolution neutron imaging applications. High track density is a necessary requirement to improve the quality of neutron imaging. However, the available track analysis methods are difficult to apply under high track density conditions. Simulated images were used to determine the required track density for neutron imaging. It was concluded that a track density of the order of $10^4$ tracks per 100 $\times$ 100 $μ$m$^2$ is sufficient to utilize neutron detectors for imaging applications. The contrast resolution was also investigated for the image data sets with various track densities and neutron transmission rates. Moreover, experiments were performed for neutron imaging of the gadolinium-based gratings with known geometries. The structure of gratings was successfully resolved. The calculated 1$σ$ 10-90 \% edge response, using the gray scale optical images of the grating slit with a periodic structure of 9 $μ$m, was 0.945 $\pm$ 0.004 $μ$m.

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arXiv2022

Study on the reusability of fluorescent nuclear track detectors using optical bleaching

Fluorescent nuclear track detectors (FNTDs) based on Al${_2}$O${_3}$:C,Mg crystals are luminescent detectors that can be used for dosimetry and detection of charged particles and neutrons. These detectors can be utilised for imaging applications where a reasonably high track density, approximately of the order of 1 $\times$ $10^4$ tracks in an area of 100 $\times$ 100 $μ$m$^2$, is required. To investigate the reusability of FNTDs for imaging applications, we present an approach to perform optical bleaching under the required track density conditions. The reusability was assessed through seven irradiation-bleaching cycles. For the irradiation, the studied FNTD was exposed to alpha-particles from an $^{241}$Am radioactive source. The optical bleaching was performed by means of ultraviolet laser light with a wavelength of 355 nm. Three dedicated regions on a single FNTD with different accumulated track densities and bleaching conditions were investigated. After every irradiation-bleaching cycle, signal-to-noise ratio was calculated to evaluate FNTD performance. It is concluded that FNTDs can be reused at least seven times for applications where accumulation of a high track density is required.

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arXiv2022

A Novel Nuclear Emulsion Detector for Measurement of Quantum States of Ultracold Neutrons in the Earth's Gravitational Field

Hypothetical short-range interactions could be detected by measuring the wavefunctions of ultracold neutrons (UCNs) on a mirror bounded by the Earth's gravitational field. The Searches require detectors with higher spatial resolution. We are developing a UCN detector for the with a high spatial resolution, which consists of a Si substrate, a thin converter layer including $^{10}$B$_{4}$C, and a layer of fine-grained nuclear emulsion. Its resolution was estimated to be less than 100 nm by fitting tracks of either $^{7}$Li nuclei or $α$-particles, which were created when neutrons interacted with the $^{10}$B$_{4}$C layer. For actual measurements of the spatial distributions, the following two improvements were made: The first was to establish a method to align microscopic images with high accuracy within a wide region of 65 mm $\times$ 0.2 mm. We created reference marks of 1 $μ$m and 5 $μ$m diameter with an interval of 50 $μ$m and 500 $μ$m, respectively, on the Si substrate by electron beam lithography and realized a position accuracy of less than 30 nm. The second was to build a holder that could maintain the atmospheric pressure around the nuclear emulsion to utilize it under vacuum during exposure to UCNs. The intrinsic resolution of the improved detector was estimated by evaluating the blur of a transmission image of a gadolinium grating taken by cold neutrons as better than 0.56 $\pm$ 0.08 $μ$m, which included the grating accuracy. A test exposure to UCNs was conducted to obtain the spatial distribution of UCNs in the Earth's gravitational field. Although the test was successful, a blurring of 6.9 $μ$m was found in the measurements, compared with a theoretical curve. We identified the blurring caused by the refraction of UCNs due to the roughness of the upstream surface of the substrate. Polishing of the surface makes the resolution less than 100 nm.

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arXiv2021

Pendellösung Interferometry Probes the Neutron Charge Radius, Lattice Dynamics, and Fifth Forces

Structure factors describe how incident radiation is scattered from materials such as silicon and germanium and characterize the physical interaction between the material and scattered particles. We use neutron pendellösung interferometry to make precision measurements of the (220) and (400) neutron-silicon structure factors, and achieve a factor of four improvement in the (111) structure factor uncertainty. These data provide measurements of the silicon Debye-Waller factor at room temperature and the mean square neutron charge radius $\langle r_n^2 \rangle = -0.1101 \pm 0.0089 \, \mathrm{fm}^2$. Combined with existing measurements of the Debye-Waller factor and charge radius, the measured structure factors also improve constraints on the strength of a Yukawa-modification to gravity by an order of magnitude over the 20 pm to 10 nm length scale range.

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arXiv2019

Measurement of the total neutron scattering cross section ratios of noble gases of natural isotopic composition using a pulsed neutron beam

Precision measurements of slow neutron cross sections with atoms have several scientific applications. In particular the n-$^{4}$He s-wave scattering length is important to know both for helping to constrain the nuclear three-body interaction and for the proper interpretation of several ongoing slow neutron experiments searching for other types of neutron-atom interactions. We present new measurements of the ratios of the neutron differential scattering cross sections for natural isotopic-abundance mixtures of the noble gases He, Ar, Kr, and Xe to natural isotopic abundance Ne. These measurements were performed using a recently developed neutron scattering apparatus for gas samples located on a pulsed slow neutron beamline which was designed to search for possible exotic neutron-atom interactions and employs both neutron time of flight information and a position-sensitive neutron detector for scattering event reconstruction. We found agreement with the literature values of scattering cross sections inferred from Ar/Ne, Kr/Ne and Xe/Ne differential cross section ratios over the $q$ range of $1 - 7$ nm$^{-1}$. However for the case of He/Ne we find that the cross section inferred differs by 11.3% (7.6 $σ$) from previously-reported values inferred from neutron phase shift measurements, but is in reasonable agreement with values from other measurements. The very large discrepancy in the He/Ne ratio calls for a new precision measurement of the n-$^{4}$He scattering length using neutron interferometry.

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arXiv2018

A Search for deviations from the inverse square law of gravity at nm range using a pulsed neutron beam

We describe an experimental search for deviations from the inverse square law of gravity at the nanometer length scale using neutron scattering from noble gases on a pulsed slow neutron beamline. By measuring the neutron momentum transfer ($q$) dependence of the differential cross section for xenon and helium and comparing to their well-known analytical forms, we place an upper bound on the strength of a new interaction as a function of interaction length $λ$ which improves upon previous results in the region $λ< 0.1\,$nm, and remains competitive in the larger $λ$ region. A pseudoexperimental simulation developed for this experiment and its role in the data analysis described. We conclude with plans for improving sensitivity in the larger $λ$ region.

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arXiv2018

Fundamental physics activities with pulsed neutron at J-PARC(BL05)

"Neutron Optics and Physics (NOP/ BL05)" at MLF in J-PARC is a beamline for studies of fundamental physics. The beamline is divided into three branches so that different experiments can be performed in parallel. These beam branches are being used to develop a variety of new projects. We are developing an experimental project to measure the neutron lifetime with total uncertainty of 1 s (0.1%). The neutron lifetime is an important parameter in elementary particle and astrophysics. Thus far, the neutron lifetime has been measured by several groups; however, different values are obtained from different measurement methods. This experiment is using a method with different sources of systematic uncertainty than measurements conducted to date. We are also developing a source of pulsed ultra-cold neutrons (UCNs) produced from a Doppler shifter are available at the unpolarized beam branch. We are developing a time focusing device for UCNs, a so called "rebuncher", which can increase UCN density from a pulsed UCN source. At the low divergence beam branch, an experiment to search an unknown intermediate force with nanometer range is performed by measuring the angular dependence of neutron scattering by noble gases. Finally the beamline is also used for the research and development of optical elements and detectors. For example, a position sensitive neutron detector that uses emulsion to achieve sub-micrometer resolution is currently under development. We have succeeded in detecting cold and ultra-cold neutrons using the emulsion detector.

physics.ins-det↗

arXiv2017

Characterization of Germanium Detectors for the Measurement of the Angular Distribution of Prompt gamma-rays at the ANNRI in the MLF of the J-PARC

In this study, the germanium detector assembly, installed at the Accurate Neutron-Nuclear Reaction measurement Instruments (ANNRI) in the Material and Life Science Facility (MLF) operated by the Japan Proton Accelerator Research Complex (J-PARC), has been characterized for extension to the measurement of the angular distribution of individual gamma-ray transitions from neutron-induced compound states. We have developed a Monte Carlo simulation code using the GEANT4 toolkit, which can reproduce the pulse-height spectra of gamma-rays from radioactive sources and (n,gamma) reactions. The simulation is applicable to the measurement of gamma-rays in the energy region of 0.5-11.0 MeV.

physics.ins-det↗

arXiv2017

Precise neutron lifetime experiment using pulsed neutron beams at J-PARC

The neutron lifetime is one of the basic parameters in the weak interaction, and is used for predicting the light element abundance in the early universe. Our group developed a new setup to measure the lifetime with the goal precision of 0.1% at the polarized beam branch BL05 of MLF, J-PARC. The commissioning data was acquired in 2014 and 2015, and the first set of data to evaluate the lifetime in 2016, which is expected to yield a statistical uncertainty of O(1)%. This paper presents the current analysis results and the future plans to achieve our goal precision.

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