Dielectric Evidence for Possible Type-II Multiferroicity in alpha-RuCl3
$α$-RuCl$_3$ is a Mott insulator with a honeycomb lattice with strong spin-orbit coupling. We report dielectric measurements on $α$-RuCl$_3$ single crystals under field. At zero field, the dielectric constant, $ε$, drops rapidly when cooled through the magnetic transition temperature T$_N$. With increasing field, the onset of the drop in $ε$ tracks the T$_N$. Such behavior is absent with field above a critical value H$_c$ ~ 7.5 T, indicating the onset of a quantum phase transition. Our data suggest that the dielectric constant can be used as a probe of magnetic ordering in $α$-RuCl$_3$, and $α$-RuCl$_3$ is a possible type-II multiferroics.
cond-mat.str-el↗