arXiv subjects

Keigo Arai

Publications and source records attributed to Keigo Arai.

15 recordsLinked to original sources

arXiv2026

Universal scaling of electrochemical information transfer at solid-liquid interfaces

Electrochemical potentials at solid-liquid interfaces govern diverse chemical and energy conversion processes; however, the extent to which their electrochemical influence extends into the solid remains unclear. Here, we show that the maximum accessible electrochemical information is governed by a single dimensionless screening parameter $u$, defined as the ratio of the effective electrostatic separation between the interface and probe to the electrostatic propagation length in the solid. The maximum Fisher information follows a universal inverse-square scaling with this parameter. This relation identifies electrostatic screening as a fundamental constraint on information transfer across solid-liquid interfaces and provides quantitative design principles for interfacial electrochemical sensing.

physics.app-ph↗

arXiv2026

Current-dipole detection of microscale metal defects

An effective electric current dipole provides a compact description of localized current disturbances and has been employed across a broad range of physical systems and length scales. Despite its extensive use in macroscopic systems, its applicability to microscale material diagnostics remains unexplored. In this study, we demonstrate that the current-dipole representation provides an effective physical framework for the detection and characterization of microscopic defects in conductive materials. When an external current is applied to a metal, defects locally perturb the current distribution, thus generating an effective in-plane current dipole that yields a characteristic magnetic-field pattern. By measuring the magnetic-field distribution above the metal and fitting it with a dipole model, we reconstruct the position and effective strength of the dipole, thereby enabling the inference of the defect location and an effective defect-volume metric. Using wide-field magnetic imaging as a measurement platform, we observe a defect-associated magnetic signal from a 38-um-long defect on the front surface of copper samples and identify a defect on the back surface using a 0.5-mm-thick copper plate. We further examine the applicability of this approach to magnetic materials, where permeability contrasts modify the field distribution. Our results establish current-dipole imaging as a general physical framework for magnetic detection of defects and highlight its potential for nondestructive inspection across a wide range of length scales.

physics.app-ph↗

arXiv2026

Diamond quantum-sensing platform with integrated boron-doped diamond microwave antenna and thermometer

Wide-field nitrogen-vacancy (NV) magnetic imaging at cryogenic temperatures requires microwave excitation and reliable knowledge of the temperature near the sensing region. Here, we report an integrated diamond quantum-sensing platform combining an ensemble of NV centers with a boron-doped diamond (BDD) microwave antenna and thermometer formed on the same diamond substrate. The BDD antenna provides microwave excitation for optically detected magnetic resonance measurements, and the BDD thermometer monitors the thermal environment near the NV sensing region. The BDD thermometer detected laser-induced local heating that was not clearly resolved by a stage-mounted thermometer. Using this platform, we imaged the temperature-dependent Meissner response of multiple cuprate superconductors while recording the temperature. These results demonstrate that the integrated BDD--NV platform provides a practical approach for cryogenic wide-field magnetic imaging with integrated microwave delivery and local thermometry.

physics.app-ph↗

arXiv2026

Fisher Glasses: Tail-Certified Quantum Metrology in Quenched Environments

Quantum metrological advantage is certified by averaged Fisher responses: contrast, susceptibility, or quantum Fisher information (QFI). This fails in quenched sensors, where slow environmental variables freeze within a session but vary between repetitions: shallow nitrogen-vacancy (NV) centers, superconducting qubits with slow two-level fluctuators, and semiconductor spin qubits in drifting charge noise. They sample session-resolved Fisher geometries, not an averaged channel. Certification conditions on the latent session, projects nuisance directions, inverts to attainable loss, then tail-certifies; this inverse upper-tail loss defines quenched tail-certified information. A no-go theorem: no averaged Fisher data determine this certificate; ensembles sharing averaged Fisher matrix, QFI, and projected information have finite or zero certified precision. A Fisher-zero integrability transition governs collapse: the inverse-loss tail exponent $β$ sets the boundary, with nonintegrable certified loss for $β\le 1$, even when annealed information is large or scaling. The certified quantum resource is response transverse to latent disorder, not raw amplification sharing its generator; universal design laws: safe windows, nondegenerate portfolios, Fisher reserves, action separation, Fisher-cut criteria. A shallow-NV Ramsey tournament shows average-QFI optimization is tail-catastrophic, whereas tail-certified designs recover nearly three orders of magnitude in certified information at equal shot budget and latent ensemble. These non-self-averaging phases are Fisher glasses, governed by Fisher-zero rare-event statistics.

quant-ph↗

arXiv2026

Wide-field NV magnetometry under simultaneous high-pressure and high-temperature conditions

We demonstrate wide-field optically detected magnetic resonance (ODMR) under simultaneous high-pressure and high-temperature conditions using nitrogen-vacancy (NV) centers. Although NV-center magnetometry has been widely used for spatially resolved magnetic-field imaging, its application to extreme environments combining pressure and temperature remains challenging. In this work, we show that ODMR can be observed at 5 GPa and 500 K, demonstrating the feasibility of NV spin readout under such combined extreme conditions. We further perform wide-field ODMR of iron at 7 GPa and 500 K, where the stray magnetic field from the sample is spatially visualized through the pressure cell. These results establish NV-center magnetometry as a promising platform for imaging magnetic phenomena in materials under high-pressure and high-temperature environments.

physics.app-ph↗

arXiv2026

Deployment-complete benchmarking

Benchmarks increasingly guide deployment, procurement and scientific screening, yet a score supports only the response it records, not necessarily the deployment action. We introduce deployment-complete benchmarking, which tests whether benchmark evidence determines a deployment action. A benchmark is complete for a claim exactly when the action is constant on each evidence fiber; mixed fibers expose missing deployment information, and completion curves quantify the evidence required to resolve ambiguity. In controlled response spaces, benchmark-channel conformal coverage of 94.98% transferred poorly to an unmeasured deployment channel (10.07%), whereas response-rank intervals achieved 94.91% coverage; even zero benchmark error certified only 45.4% of candidates at the largest residual size. Public audits revealed incompleteness, including 97.9% mixed Tox21 fibers and zero median certifiable fraction in main Matbench and JARVIS audits. In held-out replays, certify-then-acquire reduced false decisions from 1.19% to 0.027% in Tox21 and from 20.3% to 0.128% in JARVIS, while changing model choice and identifying deployment-relevant probes. Deployment-ready benchmarks should report evidence, supported actions, ambiguity and completion cost rather than scores alone.

cs.LG↗

arXiv2026

Crystallographic Symmetry Generates Phononic Holonomic Gates with Biased-Erasure Channels

Solid-state processors require control layers whose errors are legible to quantum-error-correction decoders. We show that crystallographic symmetry can provide such a layer in strain-active Lambda manifolds. When the projected strain tensor and Lambda-transition operators share a multiplicity-one two-dimensional irreducible representation, symmetry fixes the linear strain interaction to a scalar dot product. Two phase-locked mechanical modes synthesize a circular strain field, enabling complex phononic Lambda-leg control without local microwave near fields. On this manifold we construct a superadiabatic echo-lune holonomic gate using Lambda-leg control and a resonant double-quantum counterdiabatic tone. Rotating-frame simulations of a nitrogen-vacancy center give 99.88% conditional average fidelity in 1.833 microseconds, or 99.40% when leakage is counted as error. A resonant gigahertz high-overtone bulk acoustic resonator analysis translates the Hamiltonian into Rabi-rate, linewidth, and envelope-tracking requirements. The bright-state structure organizes noise: A2-sector perturbations are parity-filtered into an optically distinguishable auxiliary state, whereas transverse E-sector faults are echo suppressed and retained as a decoder stress axis. The extracted channel has 0.47% erasure probability and 0.168% residual Z error. In XZZX code-capacity simulations, this biased-erasure model yields a nominal 64% fit-extrapolated data-qubit reduction relative to an unstructured Rabi baseline. Repeated-round detector-model diagnostics preserve the nominal distance-9 proxy and identify missed erasures, transverse floors, leakage/flag timing, and strong crosstalk as validation limits. Extensions to orbital Lambda systems and bright-projector phonon-bus diagnostics identify crystallographic symmetry as a principle for co-designing phononic actuation, leakage, noise bias, and quantum decoding.

quant-ph↗

arXiv2026

Probing the Meissner effect in single crystals of $\mathbf{Bi_2Sr_2Ca_2Cu_3O_{10+δ}}$ via wide-field quantum microscopy under high pressure

We investigated the pressure dependence of the superconducting transition temperature ($T_{\rm c}$) in optimally doped Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+δ}$ (Bi-2223) single crystals using different pressure-transmitting media. Previous high-pressure studies have reported conflicting behaviors, ranging from a resurgence of $T_{\rm c}$ of optimally doped Bi-2223 in fluid media to an insulating-like transition in solid media. However, a direct comparison of the effects of different pressure-transmitting media is lacking. Here, we employed wide-field quantum microscopy based on nitrogen-vacancy centers to probe the magnetic response under high pressure, utilizing cBN and KBr as media. We observed that a diamagnetic response near 70 K, indicative of the superconducting transition, persisted up to 23 GPa in KBr, whereas it disappeared above 11 GPa and 70 K in cBN. These results demonstrate the high sensitivity of Bi-2223 to the pressure environment and highlight the critical role of hydrostatic pressure in cuprate superconductors.

cond-mat.supr-con↗

arXiv2026

Optically detected magnetic resonance of nitrogen-vacancy centers in microdiamonds inside nanopolycrystalline diamond anvil cell

We demonstrated optically detected magnetic resonance (ODMR) of nitrogen-vacancy (NV) centers in microdiamonds inside a diamond anvil cell pressurized with nanopolycrystalline diamond (NPD) anvils. NPD exhibits high optical transparency, superior hardness, and low thermal conductivity, making it suitable for optical and spectroscopic measurements under high-pressure and high-temperature conditions. We observed the ODMR signal from an ensemble of NV centers under conditions where NV centers in microdiamonds served as markers for pressures exceeding 30 GPa, with a culet diameter of 600 $μ$m. We also performed ODMR measurements on multiple microdiamonds sealed inside a sample chamber and found that the resonance frequency varied with the pressure distribution. The combination of NPD and microdiamonds containing NV centers is auspicious for pressure and magnetic sensing under concurrent high-pressure and high-temperature conditions.

cond-mat.mtrl-sci↗

arXiv2025

Coherent control of solid-state defect spins via patterned boron-doped diamond circuit

Monolithic integration, which refers to the incorporation of all device functionalities within a single material, shows significant potential for creating scalable solid-state quantum devices. This study demonstrated the coherent control of nitrogen-vacancy (NV) spins using an electronic circuit monolithically integrated within diamond: a patterned, conductive boron-doped diamond (BDD) microwave waveguide. First, we validated the high-frequency performance of the circuit by characterizing its impedance up to the microwave range, confirming its capability for efficient microwave transmission. Then, using this monolithically integrated BDD--NV hybrid system, we performed optically detected magnetic resonance and observed noticeable Rabi oscillations driven by the metallic BDD circuit. Importantly, we verified that the BDD antenna has a minimal detrimental impact on the NV spins; microwave-induced heating is negligible under both pulsed and continuous driving, and the spin relaxation time ($T_1$) remains unperturbed. This approach paves the way for a new class of compact, robust, and versatile quantum platforms suitable for sensing and information processing in various environments.

physics.app-ph↗

arXiv2023

Fast coherent control of nitrogen-14 spins associated with nitrogen-vacancy centers in diamonds using dynamical decoupling

A nitrogen-vacancy (NV) center in a diamond enables the access to an electron spin, which is expected to present highly sensitive quantum sensors. Although exploiting a nitrogen nuclear spin improves the sensitivity, manipulating it using a resonant pulse requires a long gate time owing to its small gyromagnetic ratio. Another technique to control nuclear spins is a conditional rotation gate based on dynamical decoupling, which is faster but unavailable for nitrogen spins owing to the lack of transverse hyperfine coupling with the electron spin. In this study, we generated effective transverse coupling by applying a weak off-axis magnetic field. An effective coupling depends on the off-axis field; the conditional rotation gate on the nitrogen-14 spins of an NV center was demonstrated within 4.2 μs under an 1.8% off-axis field and a longitudinal field of approximately 280 mT. We estimated that a population transfer from the electron to nitrogen spins can be implemented with 8.7 μs. Our method is applicable to an ensemble of NV centers, in addition to a single NV center.

quant-ph↗

arXiv2022

Controllable tunability of a Chern number within the electronic-nuclear spin system in diamond

Chern numbers are gaining traction as they characterize topological phases in various physical systems. However, the resilience of the system topology to external perturbations makes it challenging to experimentally investigate transitions between different phases. In this study, we demonstrate the transitions of Chern number from 0 to 3, synthesized in an electronic-nuclear spin system associated with the nitrogen-vacancy (NV) centre in diamond. The Chern number is characterized by the number of degeneracies enclosed in a control Hamiltonian parameter sphere. The topological transitions between different phases are depicted by varying the radius and offset of the sphere. We show that the measured topological phase diagram is not only consistent with the numerical calculations but can also be mapped onto an interacting three-qubit system. The NV system may also allow access to even higher Chern numbers, which can be applied to exploring exotic topology or topological quantum information.

quant-ph↗

arXiv2021

Millimetre-scale magnetocardiography of living rats using a solid-state quantum sensor

A key challenge in cardiology is the non-invasive imaging of electric current propagation occurring in the cardiovascular system at an intra-cardiac scale. A promising approach for directly mapping the current dynamics is to monitor the associated stray magnetic field. However, in this magnetic field approach, the spatial resolution deteriorates significantly as the standoff distance between the target and the sensor increases. Existing sensors usually remain relatively far from the target and provide only centimetre-scale resolution because their operating temperature is not biocompatible. Here we demonstrate millimetre-scale magnetocardiography of living rats using a solid-state quantum sensor based on nitrogen-vacancy centres in diamond. The essence of the method is a millimetre proximity from the sensor to heart surface, which enhances the cardiac magnetic field to greater than nanoteslas and allows the mapping of these signals with intra-cardiac resolution. From the acquired magnetic images, we also estimate the source electric current vector, flowing from the right atria base via the Purkinje fibre bundle to the left ventricular apex. Our results establish the solid-state quantum sensor's capability to probe cardiac magnetic signals from mammalian animals and reveal their intra-cardiac electrodynamics. This technique will enable the study of the origin and progression of myriad cardiac arrhythmias including flutter, fibrillation, and tachycardia.

physics.med-ph↗

arXiv2018

Geometric phase magnetometry using a solid-state spin

Magnetometry is a powerful technique for the non-invasive study of biological and physical systems. A key challenge lies in the simultaneous optimization of magnetic field sensitivity and maximum field range. In interferometry-based magnetometry, a quantum two-level system acquires a dynamic phase in response to an applied magnetic field. However, due to the 2π periodicity of the phase, increasing the coherent interrogation time to improve sensitivity results in reduced field range. Here we introduce a route towards both large magnetic field range and high sensitivity via measurements of the geometric phase acquired by a quantum two-level system. We experimentally demonstrate geometric-phase magnetometry using the optically addressable electronic spin associated with the nitrogen vacancy (NV) color center in diamond. Our approach enables unwrapping of the 2π phase ambiguity, decoupling of magnetic field range from sensitivity, and enhancement of the field range by about 400 times. We also find additional improvement in sensitivity in the nonadiabatic regime, and study how geometric-phase decoherence depends on adiabaticity. Our results show that the geometric phase can be a versatile tool for quantum sensing applications.

quant-ph↗

arXiv2016

Selective addressing of solid-state spins at the nanoscale via magnetic resonance frequency encoding

The nitrogen-vacancy (NV) centre in diamond is a leading platform for nanoscale sensing and imaging, as well as quantum information processing in the solid state. To date, individual control of two NV electronic spins at the nanoscale has been demonstrated. However, a key challenge is to scale up such control to arrays of NV spins. Here we apply nanoscale magnetic resonance frequency encoding to realize site-selective addressing and coherent control of a four-site array of NV spins. Sites in the array are separated by 100 nm, with each site containing multiple NVs separated by ~15 nm. Microcoils fabricated on the diamond chip provide electrically tuneable magnetic-field gradients ~0.1 G/nm. Tailored application of gradient fields and resonant microwaves allow site-selective NV spin manipulation and sensing applications, including Rabi oscillations, imaging, and nuclear magnetic resonance (NMR) spectroscopy with nanoscale resolution. Microcoil-based magnetic resonance of solid-state spins provides a practical platform for quantum-assisted sensing, quantum information processing, and the study of nanoscale spin networks.

quant-ph↗