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Keiko Kato

Publications and source records attributed to Keiko Kato.

2 recordsLinked to original sources

Photoelectron spectroscopy of 3s3p doubly excited helium dressed with strong near-infrared laser fields

We report time-resolved photoelectron spectroscopy of the $3s3p$ doubly excited states of helium dressed by an intense near-infrared (NIR) laser field. Using synchronized XUV free-electron-laser and 800-nm NIR laser pulses, we observe a pronounced delay-dependent shift of resonance-related spectral minima together with the emergence of additional structures around the NIR sideband energy. \textit{Ab initio} theoretical calculations support these observations and identify the features as signatures of NIR-induced coupling of the bright ($3s3p {}^{1}P^{o}$) autoionizing state to nearby dark ($^{1}D^{e}$ and $^{1}S^{e}$) resonances below the $N = 3$ threshold. A multichannel Fano resonance analysis of the measured spectra yields delay-dependent line-shape parameters and resonance energies, establishing a quantitative route to characterize and control correlated two-electron resonances in strong laser fields.

physics.atom-ph

Effect of n- and p-type Doping on Coherent Phonons in GaN

Effect of doping on the carrier-phonon interaction in wurtzite GaN is investigated by pump-probe reflectivity measurements using 3.1 eV light in near resonance with the fundamental band gap of 3.39 eV. Coherent modulations of the reflectivity due to the E2 and the A1(LO) modes, as well as the 2A1(LO) overtone are observed. Doping of acceptor and more so for donor atoms enhances the dephasing of the polar A1(LO) phonon via coupling with plasmons, with the effect of donors being stronger. Doping also enhances the relative amplitude of the coherent A1(LO) phonon with respect to that of the high-frequency E2 phonon, though it does not affect the relative intensity in Raman spectroscopic measurements. This enhanced coherent amplitude indicates that transient depletion field screening (TDFS), in addition to impulsive stimulated Raman scattering (ISRS), contribute to generation of the coherent polar phonons even for sub-band gap excitation. Because the TDFS mechanism requires photoexcitation of carriers, we argue that the interband transition is made possible at the surface with photon energies below the bulk band gap through the Franz-Keldysh effect.

cond-mat.mtrl-sci