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Keita Arimitsu

Publications and source records attributed to Keita Arimitsu.

3 recordsLinked to original sources

Molecular Structure Optimization based on Electrons-Nuclei Quantum Dynamics Computation

A new concept of the molecular structure optimization method based on quantum dynamics computations is presented. Nuclei are treated as quantum mechanical particles, as are electrons, and the many-body wave function of the system is optimized by the imaginary time evolution method. A demonstration with a 2-dimensional H$^+_2$ molecule shows that the optimized nuclear positions can be specified with a small number of observations. This method is considered to be suitable for quantum computers, the development of which will realize its application as a powerful method.

quant-ph↗

Distinctive class of dissipation-induced phase transitions and their universal characteristics

Coupling a system to a nonthermal environment can profoundly affect the phase diagram of the closed system, giving rise to a special class of dissipation-induced phase transitions. Such transitions take the system out of its ground state and stabilize a higher-energy stationary state, rendering it the sole attractor of the dissipative dynamics. In this work, we present a unifying methodology, which we use to characterize this ubiquitous phenomenology and its implications for the open system dynamics. Specifically, we analyze the closed system's phase diagram, including symmetry-broken phases, and explore their corresponding excitations' spectra. Opening the system, the environment can overwhelm the system's symmetry-breaking tendencies, and changes its order parameter. As a result, isolated distinct phases of similar order become connected, and new phase-costability regions appear. Interestingly, the excitations differ in the newly-connected regions through a change in their symplectic norm, which is robust to the introduction of dissipation. As a result, by tuning the system from one phase to the other across the dissipation-stabilized region, the open system fluctuations exhibit an exceptional point-like scenario, where the fluctuations become overdamped, only to reappear with an opposite sign in the dynamical response function of the system. The overdamped region is also associated with squeezing of the fluctuations. We demonstrate the pervasive nature of such dissipation-induced phenomena in two prominent examples, namely in parametric resonators and in light-matter systems. Our work draws a crucial distinction between quantum phase transitions and their zero-temperature open system counterparts.

quant-ph↗

Modification of the effective action approach for the Leggett mode

The modified procedure to get the effective action is discussed. Careful observation of phase of electrons leads to the conclusion that Hubbard-Stratonovich field should be pair wavefunction, instead of gap. The modified theory is valid for arbitrary strong interband coupling while the earlier approach only deals with weak interband coupling. This paper also discusses experimental observation of the Leggett mode: Raman spectroscopy. The spectral peak which corresponds to the Leggett mode is calculated in earlier the earlier and the modified theory, which shows that they are much different.

cond-mat.supr-con↗