arXiv subjects

Keiya Shirahama

Publications and source records attributed to Keiya Shirahama.

18 recordsLinked to original sources

arXiv2022

$^4$He in Nanoporous Media: 4D XY Quantum Criticality at Finite Temperatures

We review our study of critical phenomena in superfluid $^4$He confined in nanoporous glasses. $^4$He in nanoporous media is an ideal ground to survey the quantum phase transition of bosons. In the present work, critical phenomena were examined using a newly developed hydrodynamic mechanical resonator. The critical exponent of superfluid density $ζ$ was found to be 1.0, in contrast to 0.67 in bulk $^4$He. We also demonstrate that the superfluid density is proportional to $|P - P_{\mathrm c}|^{ζ_p}$ with $ζ_p = 1$ at any finite temperatures. These are the decisive evidences for the 4D XY criticality, which should have been observed only at 0 K, at finite temperatures. We propose a mechanism of the quantum criticality at finite temperatures in terms of phase alignment among the nanoscale localized Bose condensates (LBECs) in nanopores. The proposed mechanism are discussed in the consideration of the correlation length compared with the quantum effect.

cond-mat.supr-con↗

arXiv2021

4D-XY Superfluid Transition and Dissipation in $^4$He Confined in Nanoporous Media

$^4$He confined in nanoporous Gelsil glass is a unique, strongly correlated Bose system exhibiting quantum phase transition (QPT) by controlling pressure. Previous studies revealed that the QPT occurs with four - dimensional (4D) XY criticality, which appears in the zero-temperature limit of the superfluid density. However, the $P-T$ phase diagram also suggested that 4D XY nature appears at finite temperatures. Here, we have determined the critical exponent of the superfluid density of $^4$He in two Gelsil samples that have pore diameter to be about 3 nm, using a newly developed mechanical resonator technique. The critical exponent $ζ$ in the powerlaw fitting $ρ_{\mathrm s} \propto \left| 1 - T/T_{\mathrm c} \right| ^ζ$, where $T_{\mathrm c}$ is the superfluid transition temperature, was found to be 1.0 $\pm$ 0.1 for all pressures realized in this experiment, 0.1 $<$ $P$ $<$ 2.4 MPa. This value of $ζ$ gives a decisive evidence that the finite-temperature superfluid transition belongs to 4D XY universality class. The emergence of the 4D XY criticality is explained by the existence of many nanoscale superfluid droplets, the so called localized Bose - Einstein condensates (LBECs), above $T_{\mathrm c}$. Due to the large energy cost for $^4$He atoms to move between the LBECs, the phase of the LBEC order parameters fluctuates not only in spatial (3D) but imaginary time ($+1$D) dimensions, resulting in the 4D XY criticality by a temperature near $T_{\mathrm c}$, which is determined by the finite size of the system in the imaginary time dimension. Below $T_{\mathrm c}$, macroscopic superfluidity grows in the nanopores of Gelsil by the alignment of the phases of the LBEC order parameters. An excess dissipation peak observed below $T_{\mathrm c}$ is well explained by this phase matching process.

cond-mat.other↗

arXiv2021

Evidence for 4D XY Quantum Criticality in $^4$He Confined in Nanoporous Media at Finite Temperatures

$^4$He confined in nanoporous media is a model Bose system that exhibits quantum phase transition (QPT) by varying pressure. We have precisely determined the critical exponent of the superfluid density of $^4$He in porous Gelsil glasses with pore size of 3.0 nm using the Helmholtz resonator technique. The critical exponent $ζ$ of the superfluid density was found to be 1.0 $\pm$ 0.1 for the pressure range 0.1 < P < 2.4 MPa. This value provides decisive evidence that the finite-temperature superfluid transition belongs to the four-dimensional (4D) XY universality class, in contrast to the classical 3D XY one in bulk liquid 4He, in which $ζ$ = 0.67. The quantum critical behavior at a finite temperature is understood by strong phase fluctuation in local Bose-Einstein condensates above the superfluid transition temperature. $^4$He in nanoporous media is a unique example in which quantum criticality emerges not only at 0 K but at finite temperatures.

cond-mat.supr-con↗

arXiv2019

Multiple Diffusion-Freezing Mechanisms in Molecular Hydrogen Films

Molecular hydrogen is a fascinating candidate for quantum fluid showing bosonic and fermionic superfluidity. We have studied diffusion dynamics of thin films of H$_2$, HD and D$_2$ adsorbed on a glass substrate by measurements of elasticity. The elasticity shows multiple anomalies well below bulk triple point. They are attributed to three different diffusion mechanisms of admolecules and their "freezing" into localized state: classical thermal diffusion of vacancies, quantum tunneling of vacancies, and diffusion of molecules in the uppermost surface. The surface diffusion is active down to 1 K, below which the molecules become localized. This suggests that the surface layer of hydrogen films is on the verge of quantum phase transition to superfluid state.

cond-mat.str-el↗

arXiv2019

Elastic Anomaly of Thin Neon Film

Adsorbed molecular films provide two-dimensional systems that show various emergent phenomena that are not observed in bulk counterparts. We have measured the elasticity of thin neon films adsorbed on porous glass down to 1 K by the torsional oscillator technique. The shear modulus of a neon film anomalously increases at low temperatures with excess dissipation. This behavior indicates a crossover from a soft (fluidlike) state at high temperatures to a stiff (solidlike) state at low temperatures. The temperature dependence of the anomaly is qualitatively similar to that of the elastic anomaly of helium films found in our recent study. The dissipation peak temperature, however, becomes constant at about 5 K, contrary to the case of helium, in which it decreases to 0 K at a critical coverage of a quantum phase transition between a gapped localized phase and a mobile (superfluid) phase. It is concluded that neon films behave as a classical system that does not show a quantum phase transition or superfluidity, although the films may be strongly supercooled to temperatures much lower than the bulk triple point, 24.6 K. Our results suggest that the elastic anomaly is a universal phenomenon of atomic or molecular films adsorbed on disordered substrates.

cond-mat.str-el↗

arXiv2017

Effect of Rotation on Elastic Moduli of Solid $^4$He

We report measurements of elastic moduli of hcp solid $^4$He down to 15 mK when the samples are rotated unidirectionally. Recent investigations have revealed that the elastic behavior of solid $^4$He is dominated by gliding of dislocations and pinning of them by $^3$He impurities, which move in the solid like Bloch waves (impuritons). Motivated by the recent controversy of torsional oscillator studies, we have preformed direct measurements of shear and Young's moduli of annular solid $^4$He using pairs of quarter-circle shape piezoelectric transducers (PZTs) while the whole apparatus is rotated with angular velocity $Ω$ up to 4 rad/s. We have found that shear modulus $μ$ is suppressed by rotation below 80 mK, when shear strain applied by PZT exceeds a critical value, above which $μ$ decreases because the shear strain unbinds dislocations from $^3$He impurities. The rotation - induced decrement of $μ$ at $Ω= 4$ rad/s is about 14.7 (12.3) % of the total change of temperature dependent $μ$ for solid samples of pressure 3.6 (5.4) MPa. The decrements indicate that the probability of pinning of $^3$He on dislocation segment, $G$, decreases by several orders of magnitude. We propose that the motion of $^3$He impuritons under rotation becomes strongly anisotropic by the Coriolis force, resulting a decrease in $G$ for dislocation lines aligning parallel to the rotation axis.

cond-mat.other↗

arXiv2017

Superfluid-like TO Responses in Rotating Solid Helium

The irrotational nature of superfluid helium was discovered through its decoupling from the container under rotation. Similarly, the resonant period drop of a torsional oscillator (TO) containing solid helium was first interpreted as the decoupling of solid from the TO and appearance of supersolid. However, the resonant period can be changed by mechanisms other than supersolid, such as the elastic stiffening of solid helium that is widely accepted as the reason for the TO response. To demonstrate the irrotational nature more directly, the previous experiments superimposed the dc rotation onto the TO and revealed strong suppression on the TO response without affecting the shear modulus. This result is inconsistent with the simple temperature-dependent elasticity model and supports the supersolid scenario. Here, we re-examine the rotational effect on solid helium with a two-frequency rigid TO to clarify the conflicting observations. Surprisingly, most of the result of previous rotation experiments were not reproduced. Instead, we found a very interesting superfluid-like irrotational response that cannot be explained by elastic models.

cond-mat.other↗

arXiv2016

Simultaneous investigation of shear modulus and torsional resonance of solid 4He

We investigate the origin of a resonant period drop of a torsional oscillator (TO) containing solid ${}^{4}$He by inspecting its relation to a change in elastic modulus. To understand this relationship directly, we measure both phenomena simultaneously using a TO with a pair of concentric piezoelectric transducers inserted in its annulus. Although the temperature, ${}^{3}$He concentration, and frequency dependence are essentially the same, a marked discrepancy in the drive amplitude dependence is observed. We find that this discrepancy originates from the anisotropic response of polycrystalline solid ${}^{4}$He connected with low-angle grain boundaries by studying the shear modulus parallel to and perpendicular to the driving direction.

cond-mat.other↗

arXiv2011

Suppression of Superfluidity of $^4$He in a Nanoporous Glass by Preplating a Kr Layer

Helium in nanoporous media has attracted much interest as a model Bose system with disorder and confinement. Here we have examined how a change in porous structure by preplating a monolayer of krypton affects the superfluid properties of $^4$He adsorbed or confined in a nanoporous Gelsil glass, which has a three-dimensional interconnected network of nanopores of 5.8 nm in diameter. Isotherms of adsorption and desorption of nitrogen show that monolayer preplating of Kr decreases the effective pore diameter to 4.7 nm and broadens the pore size distribution by about eight times from the sharp distribution of the bare Gelsil sample. The superfluid properties were studied by a torsional oscillator for adsorbed film states and pressurized liquid states, both before and after the monolayer Kr preplating. In the film states, both the superfluid transition temperature $T_{\mathrm c}$ and the superfluid density decrease about 10 percent by Kr preplating. The suppression of film superfluidity is attributed to the quantum localization of $^4$He atoms by the randomness in the substrate potential, which is caused by the preplating--induced broadening of the pore size distribution. In the pressurized liquid states, the superfluid density $ρ_{\mathrm s}$ is found to increase by 10 percent by Kr preplating, whereas $T_{\mathrm c}$ is decreased by 2 percent at all pressures. The unexpected enhancement of $ρ_{\mathrm s}$ might indicate the existence of an unknown disorder effect for confined $^4$He.

cond-mat.other↗

arXiv2010

Gigantic Maximum of Nanoscale Noncontact Friction

We report measurements of noncontact friction between surfaces of NbSe$_{2}$ and SrTiO$_{3}$, and a sharp Pt-Ir tip that is oscillated laterally by a quartz tuning fork cantilever. At 4.2 K, the friction coefficients on both the metallic and insulating materials show a giant maximum at the tip-surface distance of several nanometers. The maximum is strongly correlated with an increase in the spring constant of the cantilever. These features can be understood phenomenologically by a distance-dependent relaxation mechanism with distributed time scales.

cond-mat.mtrl-sci↗

arXiv2010

Quantum Critical Phenomena of 4He in Nanoporous Media

The superfluid transition in liquid 4He filled in Gelsil glass observed in recent experiments is discussed in the framework of quantum critical phenomena. We show that quantum fluctuations of phase are indeed important at the experimentally studied temperature range owing to the small pore size of Gelsil, in contrast to 4He filled in previously studied porous media such as Vycor glass. As a consequence of an effective particle-hole symmetry, the quantum critical phenomena of the system are described by the 4D XY universality class, except at very low temperatures. The simple scaling agrees with the experimental data remarkably well.

cond-mat.stat-mech↗

arXiv2007

Superfluidity of $^4$He Confined in Nano-Porous Media

We have examined superfluid properties of $^4$He confined to a nano-porous Gelsil glass that has nanopores 2.5 nm in diameter. The pressure-temperature phase diagram was determined by torsional oscillator, heat capacity and pressure studies. The superfluid transition temperature $T_{\mathrm c}$ approaches zero at 3.4 MPa, indicating a novel "quantum" superfluid transition. By heat capacity measurements, the nonsuperfluid phase adjacent to the superfluid and solid phases is identified to be a nanometer-scale, localized Bose condensation state, in which global phase coherence is destroyed. At high pressures, the superfluid density has a $T$-linear term, and $T_{\mathrm c}$ is proportional to the zero-temperature superfluid density. These results strongly suggest that phase fluctuations in the superfluid order parameter play a dominant role on the phase diagram and superfluid properties.

cond-mat.mes-hall↗

arXiv2007

Thermodynamic Evidence for Nanoscale Bose-Einstein Condensation in ^4He Confined in Nanoporous Media

We report the measurements of the heat capacity of ^4He confined in nanoporous Gelsil glass that has nanopores of 2.5-nm diameter at pressures up to 5.3 MPa. The heat capacity has a broad peak at a temperature much higher than the superfluid transition temperature obtained using the torsional oscillator technique. The peak provides a definite thermodynamic evidence for the formation of localized Bose-Einstein condensates (LBECs) on nanometer length scales. The temperature dependence of heat capacity is well described by the excitations of phonons and rotons, supporting the existence of LBEC.

cond-mat.mes-hall↗

arXiv2007

Microwave-Absorption-Induced Heating of Surface State Electrons on Liquid 3He

A resonance-induced change in the resistivity of the surface state electrons (SSE) exposed to the microwave (MW) radiation is observed. The MW frequency corresponds to the transition energy between two lowest Rydberg energy levels. All measurements are done with electrons over liquid 3He in a temperature range 0.45-0.65 K, in which the electron relaxation time and the MW absorption linewidth are determined by collisions with helium vapor atoms. The input MW power is varied by two orders of magnitude, and the resistivity is always found to increase. This effect is attributed to the heating of electrons with the resonance MW radiation. The temperature and the momentum relaxation rate of the hot electrons are calculated as a function of the MW power in the cell, and the Rabi frequency is determined from the comparison of the theoretical result with the experiment. In addition, the broadening of the absorption signal caused by the heating is studied experimentally, and the results are found to be in good agreement with our calculations.

cond-mat.other↗

arXiv2007

Liquid-Solid Transition and Phase Diagram of ^4He Confined in Nanoporous Glass

We have studied the liquid - solid (L-S) phase transition of ^4He confined in nanoporous glass, which has interconnected nanopores of 2.5 nm in diameter. The L-S boundary is determined by the measurements of pressure and thermal response during slow cooling and warming. Below 1 K, the freezing pressure is elevated to 1.2 MPa from the bulk freezing pressure, and appears to be independent of temperature. The T-independent L-S boundary implies the existence of a localized Bose-Einstein condensation state, in which long-range superfluid coherence is destroyed by narrowness of the nanopores and random potential.

cond-mat.mes-hall↗

arXiv2007

Microwave Absorption of Surface-State Electrons on Liquid $^3$He

We have investigated the intersubband transitions of surface state electrons (SSE) on liquid $^3$He induced by microwave radiation at temperatures from 1.1 K down to 0.01 K. Above 0.4 K, the transition linewidth is proportional to the density of $^3$He vapor atoms. This proportionality is explained well by Ando's theory, in which the linewidth is determined by the electron - vapor atom scattering. However, the linewidth is larger than the calculation by a factor of 2.1. This discrepancy strongly suggests that the theory underestimates the electron - vapor atom scattering rate. At lower temperatures, the absorption spectrum splits into several peaks. The multiple peak structure is partly attributed to the spatial inhomogeneity of the static holding electric field perpendicular to the electron sheet.

cond-mat.mes-hall↗

arXiv2006

Observation of non-classical rotational inertia in bulk solid 4He

In recent torsional oscillator experiments by Kim and Chan (KC), a decrease of rotational inertia has been observed in solid 4He in porous materials and in a bulk annular channel. This observation strongly suggests the existence of "non-classical rotational inertia" (NCRI), i.e. superflow, in solid 4He. In order to study such a possible "supersolid" phase, we perform torsional oscillator experiments for cylindrical solid 4He samples. We have observed decreases of rotational inertia below 200 mK for two solid samples (pressures P = 4.1 and 3.0 MPa). The observed NCRI fraction at 70 mK is 0.14 %, which is about 1/3 of the fraction observed in the annulus by KC. Our observation is the first experimental confirmation of the possible supersolid finding by KC.

cond-mat.other↗

arXiv2001

Sliding Dynamics of the Wigner Crystal on Liquid He

The Wigner crystal on liquid He accompanies with periodic corrugation of the He surface; dimples. The dynamics of the crystal is coupled with the motion and the deformation of the dimples. Nonlinear phenomena found in AC Corbino conductivity are attributed to the collective sliding of the electrons out of the dimples. In order to inspect the dynamical transition to the sliding state, we have developed a novel experimental method using a so-called "t^2 pulse", whose leading and trailing edges change in proportion to the square of time; V = at^2. Since the force exerting upon the crystal is proportional to the time derivative of the input voltage, dV/dt, the t^2-pulsed method is expected to realize a continuous sweep of the driving force, resulting in the real-time observation of the sliding transition. The observed response shows clearly the sliding, revealing that the external force to the crystal determines the sliding transition.

cond-mat.mes-hall↗