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Kelin Gao

Publications and source records attributed to Kelin Gao.

At least 19 recordsLinked to original sources
arXiv2025

A Liquid-Nitrogen-Cooled Ca+ Ion Optical Clock with a Systematic Uncertainty of 4.4E-19

We report a single-ion optical clock based on the 4S_1/2-3D_5/2 transition of the 40Ca+ ion, operated in a liquid nitrogen cryogenic environment,achieving a total systematic uncertainty of 4.4E-19. We employ a refined temperature evaluation scheme to reduce the frequency uncertainty due to blackbody radiation (BBR), and the 3D sideband cooling has been implemented to minimize the second-order Doppler shift. We have precisely determined the average Zeeman coefficient of the 40Ca+ clock transition to be 14.345(40) Hz/mT^2, thereby significantly reducing the quadratic Zeeman shift uncertainty. Moreover, the cryogenic environment enables the lowest reported heating rate due to ambient electric field noise in trapped-ion optical clocks.

physics.atom-ph↗
arXiv2025

Coulomb Crystallization of Highly Charged Ni^12+ Ions in a Linear Paul Trap

Optical clocks have garnered widespread attention due to their unparalleled precision in time-frequency standards, geodetic measurements, and fundamental physics research. Among emerging developments, highly charged ion (HCI)-based optical clocks have attracted significant scientific interest owing to their exceptional resilience against electromagnetic perturbations and enhanced sensitivity to variations in the fine-structure constant ($α$). While the recent successful demonstration of an Ar$^{13+}$ optical clock has validated the feasibility of HCI-based systems, Ni$^{12+}$ -- featuring an ultranarrow clock transition linewidth -- stands out as a superior candidate for achieving HCI optical clocks with $10^{-19}$ level uncertainty and stability. In this work, we report the Coulomb crystallization of nickel highly charged ions (Ni-HCIs). Through a precision deceleration and sympathetic cooling protocol in a room-temperature Paul trap, high-energy Ni-HCI bunches were sympathetically cooled from megakelvin to the 100-millikelvin range using laser-cooled Be$^{+}$ ions. This work represents a pivotal step toward the realization of an optical clock based on the Ni$^{12+}$ ion.

physics.atom-ph↗
arXiv2023

Precision Measurement of M1 Optical Clock Transition in Ni12+

Highly charged ions (HCIs) have drawn significant interest in quantum metrology and in search for new physics. Among these, Ni12+ is considered as one of the most promising candidates for the next generation of HCI optical clocks, due to its two E1-forbidden transitions M1 and E2, which occur in the visible spectral range. In this work, we used the Shanghai-Wuhan Electron Beam Ion Trap to perform a high-precision measurement of the M1 transition wavelength. Our approach involved an improved calibration scheme for the spectra, utilizing auxiliary Ar+ lines for calibration and correction. Our final measured result of the M1 transition wavelength demonstrates a five-fold improvement in accuracy compared to our previous findings, reaching the sub-picometer level accuracy. In combination with our rigorous atomic-structure calculations to capture the electron correlations and relativistic effects, the quantum electrodynamic (QED) corrections were extracted. Moreover, comparing with an estimate of the one-electron QED contributions by using the GRASP2018 package, we found that the present experimental accuracy is high enough for testing the higher-order QED corrections for such a complex system with four electrons in the p subshell.

physics.atom-ph↗
arXiv2023

Towards a transportable Ca$^+$ optical clock with a systematic uncertainty of $4.8\times 10^{-18}$

We present a compact, long-term nearly continuous operation of a room-temperature Ca$^+$ optical clock setup towards a transportable clock, achieving an overall systematic uncertainty of $4.8\times 10^{-18}$ and an uptime rate of 97.8% over an 8-day period. The active liquid-cooling scheme is adopted, combined with the precise temperature measurement with 13 temperature sensors both inside and outside the vacuum chamber to ensure the accurate evaluation of the thermal environment for the optical clock. The environmental temperature uncertainty is evaluated as 293.31(0.4) K, corresponding to a blackbody radiation (BBR) frequency shift uncertainty of $4.6\times 10^{-18}$, which is reduced more than two times compared to our previous work. Through the frequency comparison between the room temperature Ca$^+$ optical clock and a cryogenic Ca$^+$ optical clock, the overall uncertainty of the clock comparison is $7.5\times 10^{-18}$, including a statistic uncertainty of $4.9\times 10^{-18}$ and a systematic uncertainty of $5.7\times 10^{-18}$. This work provides a set of feasible implementations for high-precision transportable ion optical clocks.

physics.atom-ph↗
arXiv2023

Absolute frequency measurements with a robust, transportable ^{40}Ca^{+} optical clock

We constructed a transportable 40Ca+ optical clock (with an estimated minimum systematic shift uncertainty of 1.3*10^(-17) and a stability of 5*10^(-15)/sqrt{tau} ) that can operate outside the laboratory. We transported it from the Innovation Academy for Precision Measurement Science and Technology, Chinese Academy of Sciences, Wuhan to the National Institute of Metrology, Beijing. The absolute frequency of the 729 nm clock transition was measured for up to 35 days by tracing its frequency to the second of International System of Units. Some improvements were implemented in the measurement process, such as the increased effective up-time of 91.3 % of the 40Ca+ optical clock over a 35-day-period, the reduced statistical uncertainty of the comparison between the optical clock and hydrogen maser, and the use of longer measurement times to reduce the uncertainty of the frequency traceability link. The absolute frequency measurement of the 40Ca+ optical clock yielded a value of 411042129776400.26 (13) Hz with an uncertainty of 3.2*10^(-16), which is reduced by a factor of 1.7 compared with our previous results. As a result of the increase in the operating rate of the optical clock, the accuracy of 35 days of absolute frequency measurement can be comparable to the best results of different institutions in the world based on different optical frequency measurements.

physics.atom-ph↗
arXiv2022

Measurement of infrared magic wavelength for an all-optical trapping of $^{40}$Ca$^{+}$ ion clock

For the first time, we experimentally determine the infrared magic wavelength for the $^{40}$Ca$^{+}$ $4s\, ^{2}\!S_{1/2} \rightarrow 3d\,^{2}\!D_{5/2}$ electric quadrupole transition by observation of the light shift canceling in $^{40}$Ca$^{+}$ optical clock. A "magic" magnetic field direction is chosen to make the magic wavelength insensitive to both the linear polarization purity and the polarization direction of the laser. The determined magic wavelength for this transition is 1056.37(9)~nm, which is not only in good agreement with theoretical predictions but also more precise by a factor of about 300. Using this measured magic wavelength we also derive the differential static polarizability to be $-44.32(32)$~a.u., which will be an important input for the evaluation of the blackbody radiation shift at room temperatures. Our work paves a way for all-optical-trapping of $^{40}$Ca$^{+}$ optical clock.

physics.atom-ph↗
arXiv2021

Highly charged Nd$^{9+}$ Ion: A potential candidate of $\upmu$Hz linewidth optical clocks for probing fundamental physics

An active optical clock based on highly charged Nd$^{9+}$ ion is proposed for the first time. The clock can offer ultra-narrow linewidth at the $\upmu$Hz-level which is more than two-order of magnitude below the currently recorded laser linewidth. Operating at 605(90) nm superradiation lasing transition between the $5p^2~4f$ ground state and one of the long-lived $5p~4f^2$ excited state, the proposed active clock is inherently immune against the cavity noise which provides high stability. The clock serves as a sensitive probe with high sensitivity to variation of the fine-structure constant with accuracies below 10$^{-19}$ level. Sophisticated relativistic many-body methods are employed to predict related atomic properties that have corroborated the above findings.

physics.atom-ph↗
arXiv2021

A liquid nitrogen-cooled Ca^+ optical clock with systematic uncertainty of 3*10^-18

Here we present a liquid nitrogen-cooled Ca^+ optical clock with an overall systematic uncertainty of 3*10^-18. In contrast with the room-temperature Ca^+ optical clock that we have reported previously, the temperature of the blackbody radiation (BBR) shield in vacuum has been reduced to 82(5) K using liquid nitrogen. An ion trap with a lower heating rate and improved cooling lasers were also introduced. This allows cooling the ion temperature to the Doppler cooling limit during the clock operation, and the systematic uncertainty due to the ion's secular (thermal) motion is reduced to < 1*10^-18. The uncertainty due to the probe laser light shift and the servo error are also reduced to < 1*10^-19 and 4*10^-19 with the hyper-Ramsey method and the higher-order servo algorithm, respectively. By comparing the output frequency of the cryogenic clock to that of a room-temperature clock, the differential BBR shift between the two was measured with a fractional statistical uncertainty of 7*10^-18. The differential BBR shift was used to calculate the static differential polarizability, and it was found in excellent agreement with our previous measurement with a different method. This work suggests that the BBR shift of optical clocks can be well suppressed in a liquid nitrogen environment. This is advantageous because conventional liquid-helium cryogenic systems for optical clocks are more expensive and complicated. Moreover, the proposed system can be used to suppress the BBR shift significantly in other types of optical clocks such as Yb^+, Sr^+, Yb, Sr, etc.

physics.atom-ph↗
arXiv2019

Observation of Edge Solitons in Photonic Graphene

Edge states emerge in diverse areas of science, offering new opportunities for the development of novel electronic or optoelectronic devices, sound and light propagation controls in acoustics and photonics. Previous experiments on edge states and exploration of topological phases in photonics were carried out mostly in linear regimes, but the current belief is that nonlinearity introduces new striking features into physics of edge states, lead-ing to the formation of edge solitons, optical isolation, and topological lasing, to name a few. Here we experimentally demonstrate edge solitons at the zigzag edge of a reconfigurable photonic graphene lattice created via the effect of electromagneti-cally induced transparency in an atomic vapor cell with controllable nonlinearity . To obtain edge solitons, Raman gain was introduced to compensate strong absorption experienced by the edge state during propagation. Our observations pave the way to ex-perimental exploration of topological photonics on nonlinear, reconfigurable platform.

physics.optics↗
arXiv2019

A low-energy compact Shanghai-Wuhan electron beam ion trap for extraction of highly charged ions

A low-energy, compact and superconducting electron beam ion trap (the Shanghai-Wuhan EBIT or SW-EBIT) for extraction of highly charged ions is presented. The magnetic field in the central drift tube of the SW-EBIT is approximately 0.21 T produced by a pair of high-temperature superconducting coils. The electron-beam energy of the SW-EBIT is in the range of 30-4000 eV, and the maximum electron-beam current is up to 9 mA. Acting as a source of highly charged ions, the ion-beam optics for extraction is integrated, including an ion extractor and an einzel lens. A Wien filter is then used to measure the charge-state distribution of the extracted ions. In this work, the tungsten ions below the charge state of 15 have been produced, extracted, and analyzed. The charge-state distributions and spectra in the range of 530-580 nm of tungsten ions have been measured simultaneously with the electron-beam energy of 279 eV and 300 eV, which preliminarily indicates that the 549.9 nm line comes from $W^{14+}$.

physics.atom-ph↗
arXiv2015

Measurement of magic wavelengths for the 40Ca+ clock transition

We demonstrate experimentally the existence of magic wavelengths and determine the ratio of the oscillator strengths for a single trapped ion. For the first time, two magic wavelengths for the 40Ca+ clock-transition are measured simultaneously with high precision, giving Lamda|mj|=1/2 = 395.7992(7) nm and Lamda|mj|=3/2 = 395.7990(7) nm. By tuning a laser to an intermediate wavelength between two transitions (4s1/2-4p1/2 and 4s1/2-4p3/2) of 40Ca+, the sensitivity of the clock transition Stark shift to the oscillator strengths for the resonance transition has been greatly enhanced. With the measured magic wavelengths, we determine the ratio of the oscillator strengths to sub-0.5% accuracy. Our experimental method may be applied to measure magic wavelengths for other ion clock-transitions, and, promisingly, the measurement of these magic wavelengths paves the way to building lattice ion clocks.

physics.atom-ph↗
arXiv2013

Analytical energy spectrum for hybrid mechanical systems

We investigate the energy spectrum for hybrid mechanical systems described by non-parity-symmetric quantum Rabi models. A set of analytical solutions in terms of the confluent Heun functions and their analytical energy spectrum are obtained. The analytical energy spectrum includes regular and exceptional parts, which are both confirmed by direct numerical simulation. The regular part is determined by the zeros of the Wronskian for a pair of analytical solutions. The exceptional part is relevant to the isolated exact solutions and its energy eigenvalues are obtained by analyzing the truncation conditions for the confluent Heun functions. By analyzing the energy eigenvalues for exceptional points, we obtain the analytical conditions for the energy-level-crossings, which correspond to two-fold energy degeneracy.

quant-ph↗
arXiv2013

Sequential Landau-Zener transitions in spin-orbit coupled systems

We investigate the Landau-Zener (LZ) process in spin-orbit coupled systems of single or multiple two-level (spin-$\frac{1}{2}$) particles. The coupling between internal spin states and external vibrational states, a simple spin-orbit coupling (SOC), is induced by applying a spin-dependent harmonic trap. Because of the SOC, the single-particle energy-level structures are modified by the Franck-Condon (FC) effects, in which some avoided energy-level-crossings (ELCs) are almost closed and some ELCs are opened. The close of avoided ELCs and the open of ELCs result in the FC blockade and the vibrational transitions, respectively. For a given low sweeping rate, the sequential LZ transitions of ladder-like population transition can be induced by strong SOC. We derive an analytical formula for the final population which is well consistent with the numerical results. For a given strong SOC, the sequential LZ transitions are submerged in the non-adiabatic transitions if the sweeping rate is sufficiently high. Further, we study LZ transitions of multiple interacting two-level Bose particles in a spin-dependent harmonic trap. The interplay between the SOC effects and the interaction effects is explored.

cond-mat.mes-hall↗
arXiv2011

Franck-Condon Physics in A Single Trapped Ion

We propose how to explore the Franck-Condon (FC) physics via a single ion confined in a spin-dependent potential, formed by the combination of a Paul trap and a magnetic field gradient. The correlation between electronic and vibrational degrees of freedom, called as electron-vibron coupling, is induced by a nonzero gradient. For a sufficiently strong electron-vibron coupling, the FC blockade of low-lying vibronic transitions takes place. We analyze the feasibility of observing the FC physics in a single trapped ion, and demonstrate various potential applications of the ionic FC physics in quantum state engineering and quantum information processing.

physics.atom-ph↗
arXiv2005

Quantification of complementarity in multi-qubit systems

Complementarity was originally introduced as a qualitative concept for the discussion of properties of quantum mechanical objects that are classically incompatible. More recently, complementarity has become a \emph{quantitative} relation between classically incompatible properties, such as visibility of interference fringes and "which-way" information, but also between purely quantum mechanical properties, such as measures of entanglement. We discuss different complementarity relations for systems of 2-, 3-, or \textit{n} qubits. Using nuclear magnetic resonance techniques, we have experimentally verified some of these complementarity relations in a two-qubit system.

quant-ph↗
arXiv2004

Condensate fraction of molecules for a spin mixture of ultracold fermionic atoms

The condensate fraction of molecules for ultracold Fermi gases is investigated for the magnetic field below the Feshbach resonant magnetic field. Assuming that there is no loss of particles and energy during the adiabatic magnetic-field sweep, a simple theory is used to interpret the measured condensate fraction in the experiments by JILA group (Phys. Rev. Lett. 92, 040403 (2004)) and MIT group (Phys. Rev. Lett. 92, 120403 (2004)). Our theory shows that the condensate fraction of molecules is dependent on the initial condition of the system and especially on the process of the magnetic-field sweep.

cond-mat.soft↗
arXiv2004

"Spectral Implementation" for creating a labeled pseudo-pure state and the Bernstein-Vazirani's algorithm in a four-qubit nuclear magnetic resonance quantum processor

A quantum circuit is introducted to describe the preparation of a labeled pseudo-pure state by mutiplet-component excitation scheme which has been experimentally implemented on a 4-qubit nuclear magnetic resonance quantum processor. Meanwhile, we theoretically analyze and numerically inverstigate the low-power selective single-pulse implementation of a controlled-rotation gate, which manifests its validity in our experiment. Based on the labeled pseudo-pure state prepared, a 3-qubit Bernstein-Vazirani algorithm has been experimentally demonstrated by spectral implementation. The "answers" of the computations are indentified from the split speak positions in the spectra of the observer spin, which are equivalent to projective measurements required by the algorithms.

quant-ph↗