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Keng Tou Chu

Publications and source records attributed to Keng Tou Chu.

4 recordsLinked to original sources

Record magnetoresistance, enhanced superconductivity, and fermiology in WTe2

The diverse electronic properties of transition metal chalcogenides can be very sensitive to crystal imperfections. A new crystal growth technique, known as horizontal flux transport, offers a route to improved crystal quality. By refining this technique and applying it to the topological semimetal WTe2, we achieved crystals with an order of magnitude less disorder as determined by electrical transport and scanning tunneling microscopy measurements. At low temperatures these crystals exhibit the largest magnetoresistance reported in a metal. Exfoliated monolayers show quantum oscillations for the first time in the electrostatically doped metallic states, enabling determination of band degeneracies and the valley splitting induced by an electric field. Moreover, they exhibit a gated superconducting dome with a greatly enhanced critical temperature approaching 1.8 K. This advance opens up new avenues for employing WTe2 in topological electronics and gated superconducting devices, and promises comparable breakthroughs with other chalcogenides.

cond-mat.supr-con

Sliding Disassembly of van der Waals Heterostructures

Many recent advances in our understanding of two-dimensional (2D) electron systems stem from van der Waals (vdW) heterostructures. The assembly process relies on the weak bonding across interfaces between layered vdW compounds, making it possible to construct exceptionally clean heterostructures from chemically and structurally distinct materials - a challenging task for traditional thin-film growth techniques. Here we demonstrate an additional, dynamic degree of freedom afforded by vdW interfaces, wherein we use microstructured polymer stamps to disassemble and reconfigure vdW heterostructures by sliding. We apply this technique to alter the dielectric environment of monolayer graphene, perform scanning tunneling microscopy on semiconducting and air-sensitive monolayers, and manipulate strain-sensitive moiré materials. Together these demonstrations suggest a new paradigm for assembling and dynamically modifying van der Waals heterostructures, with the potential to reveal new insights into 2D electron systems.

cond-mat.mes-hall

Low-lying Electronic Structure of Rare-Earth Based Topological Nodal Line Semimetal Candidate DySbTe

Lanthanide (Ln) based LnSbTe materials have garnered significant attention due to rich interplay of long range magnetic ordering and topological properties, driven by unique crystalline symmetry, 4f electron interactions, and pronounced spin-orbit coupling (SOC) effects. DySbTe, as a heavier lanthanide-based member of the LnSbTe family, stands out with its SOC and larger on site interactions on its 4f electrons, which arise due to the heavier Dy element. Here, we present a comprehensive study on the low-temperature bulk physical properties and the electronic structure of DySbTe using magnetic susceptibility, heat capacity, and electrical resistivity measurements, along with high-resolution angle-resolved photoemission spectroscopy (ARPES), scanning tunneling microscopy and spectroscopy (STM/S), and density functional theory calculations. Our thermodynamic measurements revealed an antiferromagnetic ordering below TN = 7.45 K and a subsequent magnetic phase transition at TN1 = 7.15 K. Our transport studies indicate a semimetallic behavior with unusual feature in the ordered state. Our ARPES measurements revealed a diamond-shaped Fermi pocket centered at the G point, with band features that evolve distinctly across various binding energies. STM/S results indicate a minimum in the density of states at around 100 meV below the Fermi level, and ARPES measurements reveal a significant gap present around the X point, differentiating DySbTe from other LnSbTe compounds. These findings enhance our understanding of the SOC effects on the electronic structure and topological properties in the LnSbTe family, highlighting DySbTe as a promising candidate for exploring the interplay between topology and magnetism.

cond-mat.mes-hall

Visualizing the microscopic origins of topology in twisted molybdenum ditelluride

In moiré materials with flat electronic bands and suitable quantum geometry, strong correlations can give rise to novel topological states of matter. The nontrivial band topology of twisted molybdenum ditelluride (tMoTe$_2$) -- responsible for its fractional quantum anomalous Hall (FQAH) states -- is predicted to arise from a layer-pseudospin skyrmion lattice. Tracing the layer polarization of wavefunctions within the moiré unit cell can thus offer crucial insights into the band topology. Here, we use scanning tunneling microscopy and spectroscopy (STM/S) to probe the layer-pseudospin skyrmion textures of tMoTe$_2$. We do this by simultaneously visualizing the moiré lattice structure and the spatial localization of its electronic states. We find that the wavefunctions associated with the topological flat bands exhibit a spatially-dependent layer polarization within the moiré unit cell. This is in excellent agreement with our theoretical modeling, thereby revealing a direct microscopic connection between the structural properties of tMoTe$_2$ and its band topology. Our work enables new pathways for engineering FQAH states with strain, as well as future STM studies of the intertwined correlated and topological states arising in gate-tunable devices.

cond-mat.mes-hall