arXiv subjects

Kenji Watanabe

Publications and source records attributed to Kenji Watanabe.

At least 181 records · Page 10Linked to original sources

arXiv2026

Emission dipole orientation reveals dynamic single-molecule interactions with 2D crystals at solvent interfaces

Direct observation of individual fluorescent emitters is crucial for understanding and studying quantum materials, chemical reactions, and biological systems. However, current single-molecule tracking methods only focuses on the localizations of molecules, overlooking molecular configuration and orientation. In this work, we introduce a high-throughput polarized single-molecule localization microscopy that simultaneously resolves the locations and emission dipole orientations of single fluorescent emitters with nanometer precision. Using the interface between pristine hexagonal boron nitride (h-BN) and an organic solvent as a challenging platform, we capture over 10^5 fluorescent events and reveal distinct molecular interaction dynamics at room temperature. The measured dipole orientations align with the three-fold rotational symmetry of the h-BN lattice, and molecular dynamics in the liquid enivronment can be modulated electrochemically, suggesting a route for on-demand control of quantum emitters. We also find that lateral diffusion at the solid-liquid interface is far more dynamic than that of solid-state emitters. This simultaneous tracking of molecular conformation and photophysics advances the understanding of single-molecule interactions and enables real-time sensing through two-dimensional materials.

cond-mat.mes-hall↗

arXiv2026

Electrically Programmable Correlated Topology and Magnetism in a Moiré Trilayer

Strong electron-electron interactions underlie a wide range of quantum many-body phenomena, including magnetism, superconductivity, and charge fractionalization. A central goal is to achieve in situ control over lattice geometry, bandwidth, and band topology within a single platform. Here we realize such an electrically programmable quantum many-body system in an alternating twisted trilayer MoTe$_2$, where an out-of-plane displacement field continuously modifies the layer polarization, effective lattice, and topology of the moiré bands. At zero displacement field, the system realizes a triangular lattice hosting a correlated insulator at one hole per moiré unit cell ($ν= -1$). Doping this state produces strongly asymmetric magnetic responses: double-exchange-like ferromagnetism for $|ν| > 1$, and signatures of spin polarons and antiferromagnetism for $|ν| < 1$. At large displacement field, interlayer hybridization reconstructs the electronic structure into a honeycomb lattice with a flat Chern band, supporting integer and fractional Chern insulators. Magneto-optical measurements further reveal the signatures of gap closure and Landau-level formation from a spin-polarized Fermi surface near the crossover between the two regimes. These results establish a unified, electrically tunable platform in which correlated magnetism and topological states emerge from a single controllable band structure.

cond-mat.mes-hall↗

arXiv2026

Nontrivial Boundary-Mediated Superconducting Transport in a TRSB Topological Iron-Based Superconductor

The interplay of superconductivity, band topology, and spontaneous time-reversal-symmetry breaking (TRSB) is expected to enable topological superconducting boundary states. FeTe0.55Se0.45 provides a promising single-material platform because it combines superconductivity, nontrivial band topology, and spontaneous magnetization in the superconducting state. Here we report evidence for a boundary-mediated superconducting transport response in exfoliated Fe(Te,Se) devices. Polar Kerr measurements show that TRSB emerges below TKerr < Tc and coexists with superconductivity across multiple compositions, providing an independent symmetry-breaking scale for transport. Using crystallographically sharp, continuous edges and side-surface-dominant contacts, we find that topological FeTe0.55Se0.45 exhibits an anomalous conductance plateau absent in topologically trivial FeTe0.40Se0.60 and Fe1.02Te0.55Se0.45 under comparable measurements. This plateau requires uninterrupted sharp edges connecting source and drain, persists over micrometer-scale separations far exceeding the bulk coherence length, shows strongly suppressed thermal broadening, and collapses when the drain is moved to the top surface. Its temperature evolution follows the TRSB scale: the plateau remains weakly broadened below T*Kerr and disappears near TKerr rather than Tc. These doping-selective, edge-geometry-dependent, TRSB-correlated, and long-range nonlocal signatures establish experimental criteria for identifying boundary-mediated superconducting transport in FeTe0.55Se0.45 and motivate phase-sensitive and theoretical studies of its microscopic origin.

cond-mat.supr-con↗

arXiv2026

Contactless cavity sensing of superfluid stiffness in atomically thin 4Hb-TaS$_2$

The exceptional tunability of two-dimensional van der Waals materials offers unique opportunities for exploring novel superconducting phases. However, in such systems, the measurement of superfluid phase stiffness, a fundamental property of a superconductor, is challenging because of the mesoscopic sample size. Here, we introduce a contact-free technique for probing the electrodynamic response, and thereby the phase stiffness, of atomically thin superconductors using on-chip superconducting microwave resonators. We demonstrate this technique on 4Hb-TaS$_2$, a van der Waals superconductor whose gap structure under broken mirror symmetry is under debate. In our cleanest few-layer device, we observe a superconducting critical temperature comparable to that of the bulk. The temperature evolution of the phase stiffness features nodeless behavior in the presence of broken mirror symmetry, inconsistent with the scenario of nodal surface superconductivity. With minimal fabrication requirements, our technique enables microwave measurements across wide ranges of two-dimensional superconductors.

cond-mat.supr-con↗

arXiv2026

On chip, multifunctional quantum sensing using single spins in a van der Waals crystal

Nanoscale thermometry and magnetometry are in high demand across a wide range of scientific and technological applications. In this context, optically addressable spins in solids have emerged at the forefront of on-chip quantum sensing. However, simultaneous quantum sensing of multiple parameters (e.g., temperature and magnetic field) using the same spin sensor remains challenging due to cross-sensitivity to multiple physical quantities. Here, we demonstrate independent dual sensing of temperature and magnetic field using single quantum emitters in hexagonal boron nitride (hBN). We experimentally verify the independent response of the zero-phonon line (ZPL) position to temperature and of optically detected magnetic resonance (ODMR) to magnetic fields. Furthermore, we demonstrate local temperature sensing of a microcircuit while simultaneously measuring an external magnetic field. Our results establish quantum emitters in hBN as a robust platform for multifunctional quantum sensing under realistic operating conditions.

quant-ph↗

arXiv2026

Electric-field-driven magnetic switching and tightly bound interlayer excitons in bilayer CrSBr

Electric field control of magnetic order in two-dimensional (2D) van der Waals magnets is a central goal for low-power spin-based technologies. In the ambient-stable antiferromagnet CrSBr, strong magnetic anisotropy and robust exciton-spin coupling provide a favorable platform, yet deterministic electric field control of its magnetic phases has not been achieved. Here we demonstrate electric-field-driven reversible switching between antiferromagnetic and ferromagnetic states in dual-gated bilayer CrSBr without intentional carrier doping. In parallel, photoluminescence measurements resolve a tightly bound interlayer exciton with an intrinsic dipole moment of only ~1 e angstrom. The electric field dependence of the magnetic phase transition reveals two coexisting mechanisms: a linear magnetoelectric effect in the antiferromagnetic state and an electric-field-modulated interlayer exchange coupling. Their interplay accounts for the asymmetric evolution of the critical magnetic field. Our results establish bilayer CrSBr as a promising 2D material for electrically controlled spin-optoelectronic functionalities.

cond-mat.mes-hall↗

arXiv2026

Anomalous magneto-optical response at $\mathrm{RuO_2 / WSe_2}$ van der Waals interface

Ruthenium dioxide ($\mathrm{RuO_2}$) has been proposed as an altermagnetic candidate, although its magnetic ground state remains controversial. Here, we probe weak interfacial magnetic states at the surface of (001)-oriented $\mathrm{RuO_2}$ films using the magnetic proximity effect (MPE) in a van der Waals heterostructure consisting of monolayer tungsten diselenide ($\mathrm{WSe_2}$) atop $\mathrm{RuO_2}$. Temperature-dependent magneto-optical spectroscopy reveals an anomalous excitonic energy shift and a deviation from conventional Varshni behavior below 55 K that are absent in an encapsulated $\mathrm{WSe_2}$ control sample. The anomalous shift reverses sign upon field cooling with opposite magnetic field polarity, indicating a magnetic origin. Polarization-resolved measurements further show a nearly field-independent and fluctuating valley splitting in $\mathrm{WSe_2 / RuO_2}$ in strong contrast to the conventional linear Zeeman splitting observed in the control bare $\mathrm{WSe_2}$ sample. These results suggest that the valley states are governed predominantly by interfacial exchange fields associated with weak surface magnetic states in $\mathrm{RuO_2}$, which do not produce a conventional linear Zeeman response within the applied magnetic field range. Importantly, this approach enables direct optical probing of emergent surface magnetism without introducing an additional ferromagnetic layer, positioning MPE-based optical probing as a tool for investigating weak surface magnetism and offering new possibilities for studying magnetic materials with controversial magnetic states.

cond-mat.mtrl-sci↗

arXiv2026

Propagating Collective Spin-valley Modes in Twisted WSe2

The emergence of neutral collective modes is a hallmark of correlated quantum phases but is often challenging to probe experimentally. In two-dimensional flatband systems, charge responses have been intensively investigated yet neutral excitations remain largely unexplored. In particular, intervalley coherent state (IVC) features a neutral Goldstone mode due to spontaneously broken valley U(1) symmetry. While IVC state has been proposed as a unifying theme across graphene and semiconductor based systems, its defining feature, the neutral Goldstone mode, remains elusive in experiment. Here we investigate space and time resolved transport of neutral modes in twisted WSe2 moire superlattices through a novel ultrafast imaging technique. We uncover two new propagating collective modes with very different velocities, which emerge near the van Hove singularity (VHS) in both intermediate (3.5 to 4 degree) and large (around 5 degree) angle twisted WSe2. The fast-propagating mode has a large speed of about 3 km/s and is consistent with a Goldstone mode for an IVC state, while the slow-moving mode is likely a gapped amplitude mode. They can be understood as the spin-valley analogues of collective modes of a superfluid, whose propagation is imaged for the first time in a condensed matter system. Our study demonstrates a powerful new approach for probing charge-neutral modes in quantum materials and offers key insights into the interplay between charge and spin-valley physics in moire superlattices.

cond-mat.mes-hall↗

arXiv2026

Trion Hall effect in electron-hole double layers

The realization of Coulomb coupled electron-hole double layers in 2D semiconductor heterostructures has enabled the thermodynamic and transport studies of equilibrium exciton fluids without a magnetic field. By doping the exciton fluid with additional electrons/holes, an equilibrium fluid of trions - three particle bound states of electrons and holes - further emerge, providing the platform to explore new transport phenomena associated with such composite particles. Here we report the observation of a Hall effect for trions in MoSe2/WSe2 heterobilayers, which support Coulomb-coupled electron and hole fluids with tunable densities. The Hall effect arises from a Lorentz force on trions under a perpendicular magnetic field. It is manifested in both Hall drag measurements and standard Hall effect measurements on just one of the semiconductor layers. For negatively charged trions, an electron Hall effect is observed even in a hole doped WSe2 monolayer due to the presence of trion drags. The trion Hall effect also disappears when the trions are ionized at elevated temperatures and/or high trion densities. Our work opens the door for realizing quantum oscillations and the quantum Hall effect for trions.

cond-mat.mes-hall↗

arXiv2026

Graphene Josephson diodes from inherent asymmetric disorder

Josephson diodes are non-reciprocal superconducting devices characterized by different switching currents depending on the current flow direction. They recently attracted considerable theoretical and experimental attention, in view of their possible application as rectifying elements in the field of superconducting electronics, and as probes to investigate symmetry breaking mechanisms in mesoscopic systems. In this work, we show that graphene Josephson junctions provide rectification of supercurrent with an efficiency exceeding 20%. The effect appears applying a mT out-of-plane magnetic field and is enhanced close to the nodes of the Fraunhofer interference pattern. Our theoretical model identifies long-range scattering potentials in the junction as the symmetry-breaking mechanism, which yields supercurrent rectification in highly transparent junctions. While graphene stands as an ultra-clean transmission medium, our work shows that unavoidable residual disorder in a clean two-dimensional system is sufficient to promote this effect. Tailoring of the inversion (mirror) symmetry breaking could be obtained via proper design of external gates.

cond-mat.supr-con↗

arXiv2026

Superconductivity near quarter and half filling of a strongly correlated triangular Hubbard band in twisted trilayer WSe2

The triangular-lattice Hubbard model is one of the paradigmatic settings for studying correlated electronic systems with geometric frustration that can give rise to a variety of phases. Recently, twisted bilayer TMD systems have emerged as attractive experimental platforms for realising such a model in the moderate-correlation regime. Alternating twisted trilayer TMD systems are expected to realise stronger correlations than bilayer systems owing to their mirror symmetry. Here we report the discovery of superconductivity near quarter- and half-filling, together with various correlated phases, in alternating twisted trilayer WSe2 (TTWSe2). At half filling, a robust correlated insulating state persists over a broad range of displacement fields, signalling the strongly correlated regime. Upon doping, superconductivity emerges over an extended region of the phase diagram. Near quarter filling, another superconducting state appears flanked by correlated metals. Our results establish the TTWSe2 system as a compelling platform for studying strongly correlated triangular-lattice Hubbard physics.

cond-mat.supr-con↗

arXiv2026

On-chip superconducting GHz RF reflectometry of the capacitance response in bilayer graphene

In dual-gated bilayer graphene, a perpendicular displacement field opens a band gap that modifies both the channel conductance and the electronic compressibility, motivating measurements that resolve resistive and capacitive responses on the same device. We integrate an hBN-encapsulated bilayer graphene heterostructure with an on-chip superconducting Nb lumped-element LC resonator and carry out RF reflectometry near 4.25 GHz. DC transport and finite-bias spectroscopy on the same device provide a transport reference. Top and bottom gates independently set the carrier density and displacement field. The DC and RF gate maps share the same gate-dependent features, with finite-bias measurements revealing a region of suppressed conductance whose bias extent grows with the displacement field, consistent with a field-induced gap. The gate-dependent resonance-frequency shift is converted to the effective capacitance seen by the resonator using an equivalent-circuit model. The capacitance shows a minimum near the conductance-suppressed region, consistent with reduced electronic compressibility in the gapped bilayer graphene, and exhibits an electron-hole asymmetry. The on-chip configuration probes the gate-dependent admittance of a dual-gated van der Waals heterostructure, providing capacitance-sensitive information that complements DC transport within a single device.

cond-mat.mes-hall↗

arXiv2026

Monolithic hybrid quantum dot devices in superconducting twisted bilayer graphene

Gate-tunable superconductivity in magic-angle twisted bilayer graphene (MATBG) has enabled the realization of superconducting devices, such as Josephson junctions, within a single crystal. This interface-free platform provides a reconfigurable and scalable architecture that overcomes limitations of conventional superconducting-semiconducting systems. Incorporating single-electron control enables access to regimes in which flat-band superconductivity competes with strong Coulomb repulsion, providing a platform for studying correlated physics phenomena. Here, we report a new class of quantum devices that combines electrostatic confinement with tunable superconductivity in a monolithic MATBG architecture. Within a single device, we demonstrate two complementary hybrid systems: superconducting islands and proximitized quantum dots. The superconducting island exhibits $2e$-periodic transport, indicating a well-defined gap protected against quasiparticle poisoning. The proximitized quantum dot hosts subgap Andreev states together with a strongly parity-modulated supercurrent.

cond-mat.mes-hall↗

arXiv2026

Ising Dirac fermions across a topological phase transition

Dirac fermions have attracted significant interest due to their relativistic dispersions and close connections to topological physics, yet they are generally expected to be gapped in two-dimensional systems with strong Ising spin orbit coupling, making their realization in such materials an outstanding challenge. Here we report the emergence of six fold degenerate Dirac fermions in an Ising moire system across a quantum spin Hall transition in twisted WSe2. In a 3.65 degree device, we observe a quantum spin Hall phase at high electric fields with nearly quantized resistance h/(2e2), and a Dirac semimetal phase over a broad range of electric fields near zero field. Magnetotransport measurements of the Dirac phase exhibit a half-integer Landau fan sequence, characteristic of Dirac fermions, with six-fold degeneracy on the hole-doped side and two fold degeneracy on the electron-doped side. Temperature dependence shows weakly metallic behavior consistent with a semimetallic state. Our twist-angle-dependent transport measurements map out a complete phase diagram and identify a critical twist angle of 3.3 degree, establishing the phase boundary between the quantum spin Hall and Dirac semimetal regimes. Our work establishes a new route to realizing Dirac fermions in strongly spin orbit coupled moire systems through a topological phase transition, providing a promising platform for high mobility spintronics.

cond-mat.mes-hall↗

arXiv2026

Engineering electrically-switchable quantum anomalous Hall states by spin-orbit coupling

Nonvolatile gate-driven switching of quantum anomalous Hall (QAH) states in graphene moiré systems provides a promising route toward topological electronics based on chiral edge states. However, deliberate use of this switching mechanism requires control over both the magnetic properties and metastability of QAH states. While previous demonstrations mostly relied on the intrinsic magnetic energy landscape of moiré devices, here we show that this landscape can be engineered through proximity coupling to WSe2. We find that proximitizing twisted monolayer-bilayer graphene by WSe2 reshapes the magnetization reversals responsible for nonvolatile electrical switching of QAH states. We attribute this effect to the proximity-induced spin-orbit coupling (SOC), which can lock spin and valley and modify the magnetization of the competing states involved in switching compared with non-proximitized graphene systems. Our findings establish proximity-induced SOC as a new way to engineer magnetic properties and switchable magnetic states in graphene-based systems. We further demonstrate that strong magnetic metastability in tMBG allows the magnetic states to be gate-tuned between QAH and metallic regimes, and between QAH states with Chern numbers |C| = 2 and 1 without resetting the magnetic state. This functionality points toward new device architectures based on QAH chiral edge states.

cond-mat.mes-hall↗

arXiv2026

Tuning proximity-induced spin-orbit coupling in graphene/WSe$_{2}$ heterostructures

Recently, proximity-induced spin-orbit coupling (SOC) has been observed in heterostructures consisting of monolayer graphene (ML-G) and transition metal dichalcogenides (TMDCs) such as WSe$_{2}$. Successful tuning of SOC in graphene/WSe$_{2}$ heterostructures by applying mechanical pressure and electric fields was also demonstrated in previous studies. In addition, theoretical calculations predicted a strong dependence of the proximity-induced SOC on the twist angle between graphene and TMDC. Here, we put these predictions to experimental test in ML-G/ML-WSe$_{2}$/hBN-heterostructures, where the twist angle is determined by aligning fractured edges, and by crystallographic etching of graphene. By performing weak anti-localization measurements, we determine the strength of the Rasbha-type SOC ($λ_\mathrm{R}$) and the valley-Zeeman-type SOC ($λ_\mathrm{VZ}$). Our experiments confirm a strong twist angle dependence of the proximity-induced SOC in agreement with theoretical predictions. Finally, we demonstrate the tunability of the SOC strength via mechanical pressure, which is in agreement with earlier findings.

cond-mat.mes-hall↗

arXiv2026

Observation of a Mott quantum spin Hall insulator in twisted WSe2

Quantum spin Hall (QSH) insulators and Mott insulators are conventionally regarded as distinct insulating phases, arising from band topology and strong Coulomb interactions, respectively. Here, we report the observation of QSH edge transport in a magnetic-field-stabilized Mott insulating state at half filling of the second moire band in a 2.29 degree twisted WSe2 device. This state exhibits a resistance plateau identical to that of the single-particle QSH state at full filling of the first moire valence band, indicating the same number of helical edge channels. Electrical transport measurements reveal nearly quantized resistance that is insensitive to vertical electric field, out-of-plane magnetic field, and temperature below 5 K. Pronounced nonlocal transport and strong negative in-plane magnetoconductance further support helical edge conduction, establishing robust edge transport in the strongly correlated regime. Temperature-dependent Hall measurements reveal a characteristic temperature scale of approximately 10 K, corresponding to an energy scale of about 1 meV. Our results demonstrate that spin-conserved QSH edge states can persist in a half filled, strongly correlated insulating phase and under external magnetic field, opening a route toward interaction-resilient topological transport in moire quantum materials.

cond-mat.mes-hall↗

arXiv2026

Supermoiré Chern mosaic in helical trilayer WSe2

Helically twisted multilayers offer access to moiré physics beyond the single-superlattice paradigm, yet their correlated and topological transport properties remain largely unexplored in semiconductor moiré materials. Here we report magnetotransport measurements of helical trilayer WSe2, in which two coupled moiré patterns relax into a supermoiré landscape composed of inequivalent local topological domains with distinct electronic structures and unequal spatial areas. By electrostatic tuning, we identify a trilayer-hybridized regime where interactions and real-space reconstruction combine to generate a plethora of magnetic and topological states absent in the twisted bilayers. At moiré filling factor $ν$ = -1, we observe a ferromagnetic insulating state that is robust against magnetic field and accompanied by a non-quantized anomalous Hall response ~-4 kOhms. This behaviour is consistent with a time-reversal-symmetry-breaking supermoiré Chern mosaic, in which the Hall response arises from the non-cancelling contributions of local domains with opposite Chern character arranged by the relaxed structure. Under strong magnetic fields, a symmetry-broken Chern insulating state (C = 1) emerges near $ν$ = -2/3, displaying a much larger positive Hall response together with strongly enhanced longitudinal resistance, suggestive of field-reconstructed topological minibands and domain-boundary scattering. These results establish relaxed supermoiré semiconductor trilayers as a platform for spatially organized magnetism and topology beyond the bilayer limit.

cond-mat.str-el↗