arXiv subjects

Kenji Watanabe

Publications and source records attributed to Kenji Watanabe.

At least 739 records · Page 41Linked to original sources

arXiv2024

Rapid infrared imaging for rhombohedral graphene

The extrinsic stacking sequence based on intrinsic crystal symmetry in multilayer two-dimensional materials plays a significant role in determining their electronic and optical properties. Compared with Bernal-stacked (ABA) multilayer graphene, rhombohedral (ABC) multilayer graphene hosts stronger electron-electron interaction due to its unique dispersion at low-energy excitations and has been utiliazed as a unique platform to explore strongly correlated physics. However, discerning the stacking sequence has always been a quite time-consuming process by scanning mapping methods. Here, we report a rapid recognition method for ABC- stacked graphene with high accuracy by infrared imaging based on the distinct optical responses at infrared range. The optical contrast of the image between ABC and ABA stacked graphene is strikingly clear, and the discernibility is comparable to traditional optical Raman microscopy but with higher consistency and throughput. We further demonstrate that the infrared imaging technique can be integrated with dry transfer techniques commonly used in the community. This rapid and convenient infrared imaging technique will significantly improve the sorting efficiency for differently stacked multilayer graphene, thereby accelerating the exploration of the novel emergent correlated phenomena in ABC stacked graphene.

cond-mat.mes-hall↗

arXiv2024

Extended Quantum Anomalous Hall States in Graphene/hBN Moiré Superlattices

Electrons in topological flat bands can form novel topological states driven by the correlation effects. The penta-layer rhombohedral graphene/hBN moire superlattice has been shown to host fractional quantum anomalous Hall effect (FQAHE) at ~400 mK, triggering discussions around the underlying mechanism and the role of moire effects. In particular, novel electron crystal states with non-trivial topology have been proposed. Here we report DC electrical transport measurement in rhombohedral penta- and tetra-layer graphene/hBN moire superlattices at electronic temperatures down to ~40 mK. We observed two more FQAH states in the penta-layer devices than previously reported. In a new tetra-layer device, we observed FQAHE at filling factors v = 3/5 and 2/3 at 300 mK. With a small bias current and the lowest temperature, we observed a new extended quantum anomalous Hall (EQAH) state and magnetic hysteresis, where Rxy = h/e2 and vanishing Rxx span a wide range of moire filling factor v from 0.5 to up to 1.3. By increasing the temperature or current, FQAHE can be recovered -- suggesting the break-down of the EQAH states and a phase transition into the fractional quantum Hall liquid. Furthermore, we observed displacement field-induced quantum phase transitions from the EQAH states to Fermi liquid, FQAH liquid and the likely composite Fermi liquid. Our observation establishes a new topological phase of electrons with quantized Hall resistance at zero magnetic field, and enriches the emergent quantum phenomena in materials with topological flat bands.

cond-mat.mes-hall↗

arXiv2024

Twist-Programmable Superconductivity in Spin-Orbit Coupled Bilayer Graphene

The relative twist angle between layers of near-lattice-matched van der Waals materials is critical for the emergent correlated phenomena associated with moire flat bands. However, the concept of angle rotation control is not exclusive to moiré superlattices in which electrons directly experience a twist-angle-dependent periodic potential. Instead, it can also be employed to induce programmable symmetry-breaking perturbations with the goal of stabilizing desired correlated states. Here, we experimentally demonstrate `moireless' twist-tuning of superconductivity together with other correlated orders in Bernal bilayer graphene proximitized by tungsten diselenide. The alignment between the two materials systematically controls the strength of the induced Ising spin-orbit coupling (SOC), profoundly altering the phase diagram. As Ising SOC is increased, superconductivity onsets at a higher displacement field and features a higher critical temperature, reaching up to 0.5K. Within the main superconducting dome and in the strong Ising SOC limit, we find an unusual phase transition characterized by a nematic redistribution of holes among trigonally warped Fermi pockets and enhanced resilience to in-plane magnetic fields. The behavior of the superconducting phase is well captured by our theoretical model, which emphasizes the role of interband interactions between Fermi pockets arising due to interaction-enhanced symmetry breaking. Moreover, we identify two additional superconducting regions, one of which descends from an inter-valley coherent normal state and exhibits a Pauli-limit violation ratio exceeding 40, among the highest for all known superconductors. Our results provide new insights into ultra-clean graphene-based superconductors and underscore the potential of utilizing moireless-twist engineering across a range of van der Waals heterostructures.

cond-mat.supr-con↗

arXiv2024

Superconductivity and spin canting in spin-orbit proximitized rhombohedral trilayer graphene

Graphene and transition metal dichalcogenide flat-band systems show similar phase diagrams, replete with magnetic and superconducting phases. An abiding question has been whether magnetic ordering competes with superconductivity or facilitates pairing. The advent of crystalline graphene superconductors enables a new generation of controlled experiments to probe the microscopic origin of superconductivity. For example, recent studies of Bernal bilayer graphene show a dramatic increase in the observed domain and critical temperature $T_c$ of superconducting states in the presence of enhanced spin-orbit coupling; the mechanism for this enhancement, however, remains unclear. Here, we show that introducing spin-orbit coupling in rhombohedral trilayer graphene (RTG) via substrate proximity effect generates new superconducting pockets for both electron and hole doping, with maximal $T_c\approx$ 300mK three times larger than in RTG encapsulated by hexagonal boron nitride alone. Using local magnetometry and thermodynamic compressibility measurements, we show that superconductivity straddles an apparently continuous transition between a spin-canted state with a finite in-plane magnetic moment and a state with complete spin-valley locking. This transition is reproduced in our Hartree-Fock calculations, where it is driven by the competition between spin-orbit coupling and the carrier-density-tuned Hund's interaction. Our experiment suggests that the enhancement of superconductivity by spin-orbit coupling is driven not by a change in the ground state symmetry or degeneracy but rather by a quantitative change in the canting angle. These results align with a recently proposed mechanism for the enhancement of superconductivity in spin-orbit coupled rhombohedral multilayers, in which fluctuations in the spin-canting order contribute to the pairing interaction.

cond-mat.mes-hall↗

arXiv2024

Interplay of electronic crystals with integer and fractional Chern insulators in moiré pentalayer graphene

The rapid development of moiré quantum matter has recently led to the remarkable discovery of the fractional quantum anomalous Hall effect, and sparked predictions of other novel correlation-driven topological states. Here, we investigate the interplay of electronic crystals with integer and fractional Chern insulators in a moiré lattice of rhomobohedral pentalayer graphene (RPG) aligned with hexagonal boron nitride. At a doping of one electron per moiré unit cell, we see a correlated insulator with a Chern number that can be tuned between $C=0$ and $+1$ by an electric displacement field, accompanied by an array of other such insulators formed at fractional band fillings, $ν$. Collectively, these states likely correspond to trivial and topological electronic crystals, some of which spontaneously break the discrete translational symmetry of the moiré lattice. Upon applying a modest magnetic field, a narrow region forms around $ν=2/3$ in which transport measurements imply the emergence of a fractional Chern insulator, along with hints of weaker states at other fractional $ν$. In the same sample, we also see a unique sequence of incipient Chern insulators arising over a broad range of incommensurate band filling near two holes per moiré unit cell. Our results establish moiré RPG as a fertile platform for studying the competition and potential intertwining of electronic crystallization and topological charge fractionalization.

cond-mat.mes-hall↗

arXiv2024

An active metasurface enhanced with moiré ferroelectricity

Semiconductor moiré systems, characterized by their periodic spatial light emission, unveil a new paradigm of active metasurfaces. Here, we show that ferroelectric moiré domains formed in a twisted hexagonal boron nitride (t-hBN) substrate can modulate light emission from an adjacent semiconductor MoSe$_2$ monolayer, enhancing its functionality as an active metasurface. The electrostatic potential at the surface of the t-hBN substrate provides a simple way to confine excitons in the MoSe$_2$ monolayer. The excitons confined within the domains and at the domain walls are spectrally separated due to a pronounced Stark shift. Moreover, the patterned light emission can be dynamically controlled by electrically gating the ferroelectric domains, introducing a novel functionality beyond conventional semiconductor moiré systems. Our findings chart an exciting pathway for integrating nanometer-scale moiré ferroelectric domains with various optically active functional layers, paving the way for advanced nanophotonic applications.

cond-mat.mes-hall↗

arXiv2024

Nonlinear electrical transport unveils Fermi surface malleability in a moiré heterostructure

Van Hove singularities enhance many-body interactions and induce collective states of matter ranging from superconductivity to magnetism. In magic-angle twisted bilayer graphene, van Hove singularities appear at low energies and are malleable with density, leading to a sequence of Lifshitz transitions and resets observable in Hall measurements. However, without a magnetic field, linear transport measurements have limited sensitivity to the band's topology. Here, we utilize nonlinear longitudinal and transverse transport measurements to probe these unique features in twisted bilayer graphene at zero magnetic field. We demonstrate that the nonlinear responses, induced by the Berry curvature dipole and extrinsic scattering processes, intricately map the Fermi surface reconstructions at various fillings. Importantly, our experiments highlight the intrinsic connection of these features with the moiré bands. Beyond corroborating the insights from linear Hall measurements, our findings establish nonlinear transport as a pivotal tool for probing band topology and correlated phenomena.

cond-mat.mes-hall↗

arXiv2024

Multiplet Supercurrents in a Josephson Circuit

Multiterminal Josephson junctions are a promising platform to host synthetic topological phases of matter and Floquet states. However, the energy scales governing topological protection in these devices are on the order of the spacing between Andreev bound states. Recent theories suggest that similar phenomena may instead be explored in circuits composed of two-terminal Josephson junctions, allowing for the topological protection to be controlled by the comparatively large Josephson energy. Here, we explore a Josephson circuit, in which three superconducting electrodes are connected through Josephson junctions to a common superconducting island. We demonstrate the dynamic generation of multiplet resonances, which have previously been observed in multiterminal Josephson junctions. The multiplets are found to be robust to elevated temperatures and are confirmed by exhibiting the expected Shapiro step quantization under a microwave drive. We also find an unexpected novel supercurrent, which couples a pair of contacts that are both voltage-biased with respect to the common superconducting island. We show that this supercurrent results from synchronization of the phase dynamics and pose the question whether it should also carry a topological contribution.

cond-mat.mes-hall↗

arXiv2024

High-Temperature Quantum Valley Hall Effect with Quantized Resistance and a Topological Switch

Edge states of a topological insulator can be used to explore fundamental science emerging at the interface of low dimensionality and topology. Achieving a robust conductance quantization, however, has proven challenging for helical edge states. Here we show wide resistance plateaus in kink states - a manifestation of the quantum valley Hall effect in Bernal bilayer graphene - quantized to the predicted value at zero magnetic field. The plateau resistance has a very weak temperature dependence up to 50 Kelvin and is flat within a dc bias window of tens of mV. We demonstrate the electrical operation of a topology-controlled switch with an on/off ratio of 200. These results demonstrate the robustness and tunability of the kink states and its promise in constructing electron quantum optics devices.

cond-mat.mes-hall↗

arXiv2024

Noise-induced stabilization of dynamical states with broken time-reversal symmetry

Under a high frequency drive, Josephson junctions demonstrate "Shapiro steps" of quantized voltage. These are dynamically stabilized states, in which the phase across the junction locks to the external drive. We explore the stochastic switching between two symmetric steps at $\frac{\hbarω}{2e}$ and $-\frac{\hbarω}{2e}$. Surprisingly, the switching rate exhibits a pronounced non-monotonicity as a function of temperature, violating the general expectation that transitions should become faster with temperature. We explain this behavior by realizing that the system retains memory of the dynamic state from which it is switching, thereby breaking the conventional simplifying assumptions about separations of time scales.

cond-mat.mes-hall↗

arXiv2024

Exciton diffusion in two-dimensional chiral perovskites

Two-dimensional (2D) organic-inorganic hybrid perovskites emerged as a versatile platform for light-emitting and photovol-taic applications due to their unique structural design and chemical flexibility. Their properties depend heavily on both the choice of the inorganic lead halide framework and the surrounding organic layers. Recently, the introduction of chiral cations into 2D perovskites has attracted major interest due to their potential for introducing chirality and tuning the chiro-optical response. Importantly, the optical properties in these materials are dominated by tightly bound excitons that also serve as primary carriers for the energy transport. The mobility of photoinjected excitons is thus important from the perspectives of fundamental material properties and optoelectronic applications, yet remains an open question. Here, we demonstrate exciton propagation in a 2D chiral perovskite methylbenzylammonium lead iodide (MBA2PbI4) using transient photoluminescence microscopy and reveal density-dependent transport over more than 100 nanometers at room temperature with diffusion coeffi-cients as high as 2 cm2/s. We observe two distinct regimes of initially rapid diffusive propagation and subsequent localiza-tion. Moreover, perovskites with enantiomer pure cations are found to exhibit faster exciton diffusion compared to the race-mic mixture, correlated with the impact of the material composition on disorder. Altogether, the observations of efficient exciton diffusion at room temperature highlight the potential of 2D chiral perovskites to merge chiro-optical properties with strong light-matter interaction and efficient energy transport.

cond-mat.mtrl-sci↗

arXiv2024

Robust field-free switching using large unconventional spin-orbit torque in an all-van der Waals heterostructure

The emerging all-van der Waals (vdW) magnetic heterostructure provides a new platform to control the magnetization by the electric field beyond the traditional spintronics devices. One promising strategy is using unconventional spin-orbit torque (SOT) exerted by the out-of-plane polarized spin current to enable deterministic magnetization switching and enhance the switching efficiency. However, in all-vdW heterostructures, large unconventional SOT remains elusive and the robustness of the field-free switching against external magnetic field hasn't been examined, which hinder further applications. Here we demonstrate the field-free switching in an all-vdW heterostructure combining a type-II Weyl semimetal TaIrTe4 and above-room-temperature ferromagnet Fe3GaTe2. The fully field-free switching can be achieved at 2.56 x 10^10 A per m2 at 300K and a large SOT effective field efficiency of the out-of-plane polarized spin current generated by TaIrTe4 is determined to be 0.37. Moreover, we find that the switching polarity cannot be changed until the external in-plane magnetic field reaches 252mT, indicating a robust switching against the magnetic field. The numerical simulation suggests the large unconventional SOT reduces the switching current density and enhances the robustness of the switching. Our work shows that all-vdW heterostructures are promising candidates for future highly efficient and stable SOT-based devices.

cond-mat.mes-hall↗

arXiv2024

Electrically tunable layer-hybridized trions in doped WSe$_2$ bilayers

Doped van der Waals heterostructures host layer-hybridized trions, i.e. charged excitons with layer-delocalized constituents holding promise for highly controllable optoelectronics. Combining a microscopic theory with photoluminescence (PL) experiments, we demonstrate the electrical tunability of the trion energy landscape in naturally stacked WSe$_2$ bilayers. We show that an out-of-plane electric field modifies the energetic ordering of the lowest lying trion states, which consist of layer-hybridized $Λ$-point electrons and layer-localized K-point holes. At small fields, intralayer-like trions yield distinct PL signatures in opposite doping regimes characterized by weak Stark shifts in both cases. Above a doping-asymmetric critical field, interlayer-like species are energetically favored and produce PL peaks with a pronounced Stark red-shift and a counter-intuitively large intensity arising from efficient phonon-assisted recombination. Our work presents an important step forward in the microscopic understanding of layer-hybridized trions in van der Waals heterostructures and paves the way towards optoelectronic applications based on electrically controllable atomically-thin semiconductors.

cond-mat.mes-hall↗

arXiv2024

Field-Tunable Valley Coupling and Localization in a Dodecagonal Semiconductor Quasicrystal

Quasicrystals are characterized by atomic arrangements possessing long-range order without periodicity. Van der Waals (vdW) bilayers provide a unique opportunity to controllably vary atomic alignment between two layers from a periodic moiré crystal to an aperiodic quasicrystal. Here, we reveal a remarkable consequence of the unique atomic arrangement in a dodecagonal WSe2 quasicrystal: the K and Q valleys in separate layers are brought arbitrarily close in momentum space via higher-order Umklapp scatterings. A modest perpendicular electric field is sufficient to induce strong interlayer K-Q hybridization, manifested as a new hybrid excitonic doublet. Concurrently, we observe the disappearance of the trion resonance and attribute it to quasicrystal potential driven localization. Our findings highlight the remarkable attribute of incommensurate systems to bring any pair of momenta into close proximity, thereby introducing a novel aspect to valley engineering.

cond-mat.mtrl-sci↗

arXiv2024

Direct visualization of defect-controlled diffusion in van der Waals gaps

Diffusion processes govern fundamental phenomena such as phase transformations, doping, and intercalation in van der Waals (vdW) bonded materials. Here, we quantify the diffusion dynamics of W atoms by visualizing the motion of individual atoms at three different vdW interfaces: BN/vacuum, BN/BN, and BN/WSe2, by recording scanning transmission electron microscopy movies. Supported by density functional theory calculations, we infer that in all cases diffusion is governed by intermittent trapping at electron beam-generated defect sites. This leads to diffusion properties that depend strongly on the number of defects. These results suggest that diffusion and intercalation processes in vdW materials are highly tunable and sensitive to crystal quality. The demonstration of imaging, with high spatial and temporal resolution, of layers and individual atoms inside vdW heterostructures offers possibilities for direct visualization of diffusion and atomic interactions, as well as for experiments exploring atomic structures, their in-situ modification, and electrical property measurements of active devices combined with atomic resolution imaging.

cond-mat.mtrl-sci↗

arXiv2024

Emergence of electric-field-tunable interfacial ferromagnetism in 2D antiferromagnet heterostructures

Van der Waals (vdW) magnet heterostructures have emerged as new platforms to explore exotic magnetic orders and quantum phenomena. Here, we study heterostructures of layered antiferromagnets, CrI3 and CrCl3, with perpendicular and in-plane magnetic anisotropy, respectively. Using magneto-optical Kerr effect microscopy, we demonstrate out-of-plane magnetic order in the CrCl3 layer proximal to CrI3, with ferromagnetic interfacial coupling between the two. Such an interlayer exchange field leads to higher critical temperature than that of either CrI3 or CrCl3 alone. We further demonstrate significant electric-field control of the coercivity, attributed to the naturally broken structural inversion symmetry of the heterostructure allowing unprecedented direct coupling between electric field and interfacial magnetism. These findings illustrate the opportunity to explore exotic magnetic phases and engineer spintronic devices in vdW heterostructures.

cond-mat.mtrl-sci↗

arXiv2024

Strongly interacting Hofstadter states in magic-angle twisted bilayer graphene

Magic-angle twisted bilayer graphene (MATBG) hosts a multitude of strongly correlated states at partial fillings of its flat bands. In a magnetic field, these flat bands further evolve into a unique Hofstadter spectrum renormalized by strong Coulomb interactions. Here, we study the interacting Hofstadter states spontaneously formed within the topological magnetic subbands of an ultraclean MATBG device, notably including symmetry-broken Chern insulator (SBCI) states and fractional quantum Hall (FQH) states. The observed SBCI states form a cascade with their Chern numbers mimicking the main sequence correlated Chern insulators. The FQH states in MATBG form in Jain sequence; however, they disappear at high magnetic field, distinct from conventional FQH states which strengthen with increasing magnetic field. We reveal a unique magnetic field-driven phase transition from composite fermion phases to a dissipative Fermi liquid. Our theoretical analysis of the magnetic subbands hosting FQH states predicts non uniform quantum geometric properties far from the lowest Landau level. This points towards a more natural interpretation of these FQH states as in-field fractional Chern insulators of the magnetic subbands.

cond-mat.mes-hall↗

arXiv2024

Electrically tunable moiré magnetism in twisted double bilayers of chromium triiodide

Moiré superlattices in van der Waals structures can be used to control the electronic properties of the material and lead to emergent correlated and topological phenomena. Its first demonstration in van der Waals magnets exhibited noncollinear states and domain structures with, however, limited manipulation. Here we report electrically tunable moiré magnetism in twisted double bilayers - that is, a bilayer plus a bilayer with a twist angle between them - of layered antiferromagnet CrI3. Using magneto-optical Kerr effect microscopy, we observe the coexistence of antiferromagnetic and ferromagnetic order with nonzero net magnetization - a hallmark of moiré magnetism. Such magnetic state extends over a wide range of twist angles (with transitions at around 0° and above 20°) and exhibits a nonmonotonic temperature dependence. We further demonstrate voltage-assisted magnetic switching. The observed nontrivial magnetic states and unprecedented control by twist angle, temperature and electrical gating are supported by the simulated phase diagram of the moiré magnetism.

cond-mat.mtrl-sci↗