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Kenneth Choo

Publications and source records attributed to Kenneth Choo.

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Resonantly enhanced polariton-mediated superconductivity in a doped transition metal dichalcogenide monolayer

We present a proposal for achieving light-induced superconductivity using exciton polaritons - hybrid light-matter particles of excitons (bound electron-hole pairs) and microcavity photons. In contrast to previous theories of polariton-mediated superconductivity, which typically require multiple semiconductor layers, we show that superconductivity can be induced within a single semiconductor monolayer with inverted conduction bands, such as in the tungsten-based transition metal dichalcogenides. The key ingredient is that we can resonantly excite exciton polaritons into bands that are different from those occupied by the doped electrons, thus avoiding any Pauli blocking effects. Crucially, we can exploit the trion fine structure (i.e., multiple exciton-electron bound states) and tune the electron-polariton interactions via Feshbach resonances. Our theory of polariton-mediated superconductivity includes the energy dependence of the polariton-mediated interactions between electrons, as well as the polariton-induced changes to the electron quasiparticles. We find that superconductivity at elevated temperatures is within reach of current experiments.

cond-mat.mes-hall

Polaronic polariton quasiparticles in a dark excitonic medium

Exciton polaritons are hybrid particles of excitons (bound electron-hole pairs) and cavity photons, which are renowned for displaying Bose Einstein condensation and other coherent phenomena at elevated temperatures. However, their formation in semiconductor microcavities is often accompanied by the appearance of an incoherent bath of optically dark excitonic states that can interact with polaritons via their matter component. Here we show that the presence of such a dark excitonic medium can "dress" polaritons with density fluctuations to form coherent polaron-like quasiparticles, thus fundamentally modifying their character. We employ a many-body Green's function approach that naturally incorporates correlations beyond the standard mean-field theories applied to this system. With increasing exciton density, we find a reduction in the light-matter coupling that arises from the polaronic dressing cloud rather than any saturation induced by the fermionic constituents of the exciton. In particular, we observe the strongest effects when the spin of the polaritons is opposite that of the excitonic medium. In this case, the coupling to light generates an additional polaron quasiparticle - the biexciton polariton - which emerges due to the dark-exciton counterpart of a polariton Feshbach resonance. Our results can explain recent experiments on polariton interactions in two-dimensional semiconductors and potentially provide a route to tailoring the properties of exciton polaritons and their correlations.

cond-mat.mes-hall

Dissipative light-matter coupling and anomalous dispersion in nonideal cavities

We consider the scenario of an emitter embedded in a nonideal cavity. Using an input-output approach to describe the open system, we show that an effective dissipative coupling between the emitter and the cavity can emerge because of their interaction with a common photonic environment. The underlying mechanism is independent of the nature of the emitter and exists even at zero temperature; hence our results provide a pathway for accessing a range of non-Hermitian phenomena in a variety of light-matter coupled systems. In particular, we show that the effective dissipative coupling can lead to the phenomenon of level attraction between the emitter and cavity mode when the radiative decay rates exceed the conventional Rabi coupling. Our model thus provides a possible explanation for the anomalous dispersions and negative mass observed in recent photoluminescence measurements in semiconductor microcavities. Finally, we show that our effective non-Hermitian system can produce hybrid light-matter exceptional points and bound states in the continuum.

quant-ph