arXiv subjects

Kenya Shimada

Publications and source records attributed to Kenya Shimada.

At least 19 recordsLinked to original sources

arXiv2026

Disentangling bulk and surface states in the electronic structure of PtBi$_2$(0001)

Recent reports of surface-localized topological superconductivity in trigonal PtBi$_2$ highlight the importance of understanding its surface electronic structure. We investigate the bulk and surface band structure of PtBi$_2$ using angle-resolved photoemission spectroscopy (ARPES) and first-principles calculations. Through photon-energy- and polarization-dependent measurements, we disentangle bulk dispersions from surface states on the two distinct surface terminations of PtBi$_2$(0001). For both terminations, we assign several different surface states and find good agreement between experiment and calculations. Based on our calculations, we analyze the orbital composition in the surface and bulk bands and compare the results to polarization-dependent ARPES measurements. Together, our results provide a coherent picture of the surface electronic structure of PtBi$_2$ across both surface terminations.

cond-mat.str-el↗

arXiv2026

Topological Surface States and Anisotropic Magnetotransport in SnSb$_6$Te$_{10}$

We have investigated the electronic structure and magnetotransport properties of SnSb$_6$Te$_{10}$ single crystals using density functional theory (DFT), synchrotron-based angle-resolved photoemission spectroscopy (ARPES), and quantum transport measurements. Our DFT calculations reveal a clear spin-orbit coupling driven band inversion between the Sb-$p$ and Te-$p$ states together with a non-trivial $\mathbb{Z}_2$ topological invariant. The calculated surface-state dispersion and hexagonally warped Fermi surface contours agree well with the ARPES measurements. Temperature-dependent transport measurements indicate dominant electron-phonon scattering, while Hall measurements confirm hole-type carriers with carrier density of the order of $10^{21}$ cm$^{-3}$. Both transverse and longitudinal magnetotransport exhibit weak antilocalization behavior, while Shubnikov-de Haas oscillations observed for $H \parallel c$ yield a Berry phase close to $\pi$, consistent with Dirac-like surface states. Furthermore, angle-dependent magnetotransport measurements reveal pronounced anisotropy associated with an anisotropic Fermi surface topology and mixed bulk-surface transport behavior. Our combined theoretical and experimental results establish SnSb$_6$Te$_{10}$ as a strong topological insulator and a promising platform for investigating topological transport phenomena in layered telluride systems.

cond-mat.mtrl-sci↗

arXiv2026

Discovery of d-orbital order in Tb2CoAl4Ge2

Orbital order describes a quantum state where occupied orbitals line up in a periodic pattern. While orbital physics plays a fundamental and universal role in strongly correlated electron systems, the existence and particularly the band structure fingerprint of orbital order remain a long-standing mystery. Here, we report the discovery of rare earth 5d-orbital order developed by the surface states of intermetallic compound Tb2CoAl4Ge2. Angle-resolved photoemission spectroscopy reveals characteristic nematic features like Fermi surface deformation and band split. These experimental observations can be described by a ferro-orbital order term in the mean-field Hamiltonian. The structural and magnetic origin of such order is excluded by systematic high-resolution neutron powder diffraction and scanning tunnelling microscopy measurements. Our results provide strong evidence for a pure surface orbital order scenario avoiding complications from structural distortion as in colossal magnetoresistance manganites, magnetic order as in iron-based superconductors, and charge transfer p-orbital order in cuprates.

cond-mat.str-el↗

arXiv2026

Termination-Dependent Surface States and Magnetic Fingerprints of Chiral Helimagnet Cr1/3TaS2

Chiral helimagnets based on intercalated transition-metal dichalcogenides, characterized by nano-scale spin ordering, provide a powerful route to engineer chiral spin textures (e.g. the topologically protected magnetic solitons) and emergent electronic functionality at reduced dimensions, where surface and interface states often dominate device operation. However, despite growing interest, direct experimental studies of termination-dependent surface electronic structures and their temperature-driven magnetic evolution remain largely unexplored, hindering a microscopic understanding of the electronic states that is crucial for the development of low-dimensional spintronic devices. Here, for the first time, taking Cr1/3TaS2 as a representative example, we systematically investigate the termination-dependent surface electronic states of the chiral helimagnets and uncover their distinct temperature evolution across the magnetic transition (TC~142K) by combining high-resolution ARPES with a micro-focused beam and surface-state-resolved first-principles calculations. The TaS2-terminated surface hosts folded monolayer-like TaS2 bands under the $\sqrt3\times\sqrt3$ superlattice potential and a shallow triangular electron pocket at the superlattice $\bar K$ point arising from Cr-Ta orbital hybridization. In contrast, the Cr-terminated surface exhibits reconstructed hole pockets with pronounced magnetic band splitting. This splitting disappears above TC and closely follows the chiral helimagnetic order parameter, providing a direct spectroscopic fingerprint of chiral helimagnetic order. In addition, multiple ultranarrow Cr-d-derived surface flat bands are resolved. These findings establish Cr1/3TaS2 as a model system in which surface electronic states are strongly coupled to chiral magnetism, opening new opportunities for chiral spintronic and valleytronic micro/nanodevices.

cond-mat.mtrl-sci↗

arXiv2026

Orbital Selective Dirac-like States in EuAgAs Revealed by Polarization Dependent ARPES and DFT

Magnetic topological semimetals provide a promising platform for emergent quantum phenomena driven by the interplay between magnetism and relativistic fermions, including anomalous transport effects and tunable topological phases. Here, we investigate the electronic structure and orbital character of EuAgAs, a magnetic topological Dirac semimetal candidate, using density functional theory (DFT) and polarization dependent angle resolved photoemission spectroscopy (ARPES). Fermi surface mapping and constant energy contours measured at 9 eV reveal ring like features that systematically expand with increasing binding energy, consistent with nearly linear low energy Dirac like dispersion. ARPES measurements at different photon energies hint at the presence of a van Hove singularity predicted by DFT calculations. Furthermore, this indicates that the photoemission matrix elements are highly sensitive to the excitation energy, allowing different photon energies to selectively probe distinct orbital characters. Polarization dependent ARPES measurements performed in s- and p-polarized geometries exhibit pronounced variations in spectral intensity, indicating symmetry selective orbital contributions to electronic states. These matrix element driven intensity modulations are well reproduced by DFT calculations. Furthermore, the observed Dirac like states remain nearly unchanged over the temperature range from 9 K to 30 K, suggesting that the magnetic ordering has minimal influence on the electronic structure. Our combined experimental and theoretical results provide detailed insight into the orbital selective electronic structure of EuAgAs and its implications for magnetic topological quantum states.

cond-mat.mes-hall↗

arXiv2026

Emergent surface resonance from charge density wave symmetry breaking in TiSe2

Surface confined electronic states provide a fertile ground for discovering emergent phenomena that have no counterpart in the bulk, offering new routes to manipulate correlations, symmetry breaking, and dimensionality at the atomic scale. Here, we show that charge density wave (CDW) symmetry breaking can yield a surface states in 1T-TiSe2. Micro angle resolved photoemission spectroscopy resolves a sharp, two dimensional surface resonant state (SRS) that emerges within the CDW reconstructed low energy spectrum. The SRS exhibits notable temperature dependence and its spectral weight collapses around 160 K, while CDW transition temperature TCDW is commonly reported as 202 K. Slab DFT+U calculations reproduce a surface localized resonance when CDW folding brings valence and conduction states into near degeneracy, suggesting a correlation tuned, surface selective origin. These results point to a form of correlation-tuned surface resonance in a layered CDW compound and suggest a framework for engineering low dimensional quantum states in van der Waals materials via symmetry breaking and electronic structure tuning.

cond-mat.mtrl-sci↗

arXiv2026

Unusual Dual Flat Bands and two-dimensional Dirac-node Arc State in Kagome Metal Ni3In2S2

Kagome materials are at the frontier of condensed matter physics. An ideal kagome lattice features only one geometrically frustrated flat band spanning the entire momentum space and a single Dirac cone at the Brillouin-zone corners. However, for the first time, here we observe unusual flat-band and Dirac physics in the newly discovered "322" kagome material Ni3In2S2 by combining high-resolution synchrotron- and laser-based angle-resolved photoemission spectroscopy with a micro-focused beam, scanning tunneling microscopy, and first-principles calculations. We resolve two distinct electronic flat-band states located in close proximity to the Fermi level: a robust Topological Surface Flat Band at ~40 meV below the Fermi level on the Sulfur-terminated surface, originating from weak topological insulator states, and a kagome lattice-derived flat band at ~100 meV binding energy with an ultranarrow bandwidth (~5 meV). Instead of the single Dirac cone, the Indium-terminated surface hosts a rare two-dimensional Dirac-node arc state, where the gapless Dirac nodes extend along an open one-dimensional line crossing the Brillouin-zone boundary, exhibiting sharp linear dispersion, exceptionally high Fermi velocity, and pronounced circular dichroism. These findings establish Ni3In2S2 as a unique topological kagome metal in which multiple flat-band states of different physical origin coexist with an unusual Dirac-node arc, opening an avenue for discovering flat-band--driven and topology-enabled quantum phenomena.

cond-mat.mtrl-sci↗

arXiv2025

Non-altermagnetic spin texture in MnTe

Recently, altermagnets have emerged as promising candidates in spintronics, uniquely combining large spin-polarized electronic states with zero net magnetization. A prominent example is $\alpha$-MnTe, whose altermagnetic spin splitting, i.e., the degeneracy lift in momentum space induced by collinear magnetic order, has been experimentally observed. However, the direct evidence of its $g$-wave spin polarization, the key property for altermagnetic spintronics, is thus far lacking. By combining high-resolution spin- and angle-resolved photoemission spectroscopy (SARPES) with first-principles calculations, we reveal a $k_z$-independent, Rashba-like spin texture in $\alpha$-MnTe. Our results indicate that the observed spin polarization is primarily governed by spin-orbit coupling, whereas the magnetic order contributes to the splitting of energy bands but plays a much less dominant role in spin polarization due to the multi-domain nature. From this result, we further establish a way to prescreen altermagnet candidates that favor the formation of large antiferromagnetic domains based on symmetry analysis. Our work elucidates the interplay between magnetic order and spin-orbit coupling in governing spin polarization in altermagnet candidates, and thereby advances the materials design paradigm for spin-functional devices.

cond-mat.mtrl-sci↗

arXiv2025

Spectroscopic Evidence for Electron-Boson Coupling in Half-metallic CrO2

We report quasiparticle properties of the half-metal ferromagnet CrO2 by means of high-resolution angle-resolved photoemission spectroscopy (ARPES). We clearly observed the Fermi surface (FS) and band dispersion in good agreement with the previous reports. Moreover, the ARPES band dispersion reveals a distinct kink structure around 68 meV, providing the first spectroscopic evidence for the elementary excitations in CrO2. The energy scale of this feature is comparable to the Debye temperature and the $A\subm{1g}$ phonon mode, suggesting the electron-phonon interaction. From the detailed analysis, we have extracted the self-energy and found two characteristic structures in the real part of the self-energy. Assuming the existence of the electron-magnon interaction as well as the electron-phonon interaction, we could reproduce the evaluated real and imaginary parts of the self-energy as well as ARPES intensity. Our findings reveal the renormalized quasiparticle (QP) dynamics in CrO$_2$ and provide valuable insights into the fundamental many-body interactions governing half-metallic ferromagnets.

cond-mat.str-el↗

arXiv2025

Reconstruction of the occupied and unoccupied electronic states driven by quantum charge fluctuations in electron doped cuprate superconductors

The origin of electron-boson interactions is central to understanding high-$T_c$ superconductivity in cuprates. While phonons and magnetic fluctuations are widely considered as candidates for mediating electron pairing, the role of charge fluctuations -- one of the fundamental electronic degrees of freedom -- remains unclear. Here, we investigate the electronic structure of the electron-doped cuprate Nd$_{2-x}$Ce$_x$CuO$_4$ using angle-resolved photoemission spectroscopy and angle-resolved inverse photoemission spectroscopy, which reveal the occupied and unoccupied states, respectively. We identify emergent spectral features on both occupied and unoccupied states that are consistent with excitations driven by quantum charge fluctuations. The results obtained in this study offer direct experimental insight into charge fluctuations in cuprates, thereby paving the way towards clarifying their fine electronic structure and the mechanism of high-$T_c$ superconductivity.

cond-mat.str-el↗

arXiv2025

Flat bands and temperature-driven phase transition in quasi-one-dimensional zigzag chains

Flat-band materials have garnered extensive attention due to their captivating properties associated with strong correlation effects. While flat bands have been discovered in several types of 2D materials, their existence in 1D systems remains elusive. Here, we propose a 1D frustrated lattice, specifically the 1D zigzag lattice, as a platform for hosting flat bands. This lattice can be experimentally realized by growing CuTe chains on Cu(111). The presence of flat bands was confirmed by tight-binding model analysis, first-principles calculations, and angle-resolved photoemission spectroscopy measurements. In addition, we discovered a temperature-driven phase transition at approximately 250 K. Detailed analyses demonstrate that the system has a Tomonaga-Luttinger liquid behavior, accompanied by spin-charge separation effects. Our work unveils new prospects for investigating strongly correlated electron behaviors and topological properties in the 1D limit.

cond-mat.str-el↗

arXiv2025

Hedgehog-like spin texture in Sb-doped MnBi$_2$Te$_4$

We employ spin- and angle-resolved photoemission spectroscopy and circular-dichroism ARPES to systematically investigate the spin texture of Sb-doped MnBi$_2$Te$_4$. Our results display a hedgehog-like spin texture in this system which is signified by reversed-orienting out-of-plane spins at the Dirac gap. Our finding reveals the presence of time-reversal symmetry breaking, implying the possibility for realization of high-temperature quantum anomalous Hall effect.

cond-mat.mtrl-sci↗

arXiv2024

Electronic states in superconducting type-II Dirac semimetal: 1T-PdSeTe

We have investigated the surface and bulk electronic structures of the superconducting type-II Dirac semimetal 1T-PdSeTe. The superconducting transition temperature $T_C = 3.2$ K was almost twice as high as $T_C = 1.6$ K in 1T-PdTe$_2$. Scanning transmission electron microscopy measurements showed homogeneously mixed Se and Te atoms in the chalcogen layers, consistent with the CdI$_2$-type crystal structure. Angle-resolved photoemission spectroscopy measurements and density functional theory calculations indicated the existence of the topological surface states, and the overall band structures were similar to those of 1T-PdTe$_2$. These results suggest that CdI$_2$-type lattice symmetry dictates the band dispersion, regardless of atomic disorder in the chalcogen layers. As the electronic band dispersion and the local structures were persistent upon substitution, the enhancement of $T_C$ is likely associated with the chemical pressure. Our results provide insight into the effects of the solid solution on the surface and bulk electronic states as well as the superconducting transition temperature.

cond-mat.supr-con↗

arXiv2024

Evidence for Two-dimensional Weyl Fermions in Air-Stable Monolayer PtTe$_{1.75}$

The Weyl semimetals represent a distinct category of topological materials wherein the low-energy excitations appear as the long-sought Weyl fermions. Exotic transport and optical properties are expected because of the chiral anomaly and linear energy-momentum dispersion. While three-dimensional Weyl semimetals have been successfully realized, the quest for their two-dimensional (2D) counterparts is ongoing. Here, we report the realization of 2D Weyl fermions in monolayer PtTe$_{1.75}$, which has strong spin-orbit coupling and lacks inversion symmetry, by combined angle-resolved photoemission spectroscopy, scanning tunneling microscopy, second harmonic generation, X-ray photoelectron spectroscopy measurements, and first-principles calculations. The giant Rashba splitting and band inversion lead to the emergence of three pairs of critical Weyl cones. Moreover, monolayer PtTe$_{1.75}$ exhibits excellent chemical stability in ambient conditions, which is critical for future device applications. The discovery of 2D Weyl fermions in monolayer PtTe$_{1.75}$ opens up new possibilities for designing and fabricating novel spintronic devices.

cond-mat.mes-hall↗

arXiv2024

Crystal-symmetry-paired spin-valley locking in a layered room-temperature antiferromagnet

Recent theoretical efforts predicted a type of unconventional antiferromagnet characterized by the crystal symmetry C (rotation or mirror), which connects antiferromagnetic sublattices in real space and simultaneously couples spin and momentum in reciprocal space. This results in a unique C-paired spin-valley locking (SVL) and corresponding novel properties such as piezomagnetism and noncollinear spin current even without spin-orbit coupling. However, the unconventional antiferromagnets reported thus far are not layered materials, limiting their potential in spintronic applications. Additionally, they do not meet the necessary symmetry requirements for nonrelativistic spin current. Here, we report the realization of C-paired SVL in a layered room-temperature antiferromagnetic compound, Rb1-{\delta}V2Te2O. Spin resolved photoemission measurements directly demonstrate the opposite spin splitting between C-paired valleys. Quasi-particle interference patterns reveal the suppression of inter-valley scattering due to the spin selection rules, as a direct consequence of C-paired SVL. All these experiments are well consistent with the results obtained from first-principles calculations. Our observations represent the first realization of layered antiferromagnets with C-paired SVL, enabling both the advantages of layered materials and possible control through crystal symmetry manipulation. These results hold significant promise and broad implications for advancements in magnetism, electronics, and information technology.

cond-mat.str-el↗

arXiv2024

Observation of Spin Splitting in Room-Temperature Metallic Antiferromagnet CrSb

Recently, unconventional antiferromagnets that enable the splitting of electronic spins have been theoretically proposed and experimentally realized, where the magnetic sublattices containing moments pointing at different directions are connected by a novel set of symmetries. Such spin splitting (SS) is substantial, $k$-dependent, and independent of the spin-orbit coupling strength, making these magnets promising materials for antiferromagnetic spintronics. Here, combined with angle-resolved photoemission spectroscopy (ARPES) and density functional theory (DFT) calculations, we perform a systematic study on CrSb, a metallic spin-split antiferromagnet candidate with $T_N$ = 703 K. Our data reveals the electronic structure of CrSb along both out-of-plane and in-plane momentum directions, which renders anisotropic $k$-dependent SS and agrees well with the calculational results. The magnitude of such SS reaches up to at least 0.8 eV at non-high-symmetry momentum points, which is significantly higher than the largest known SOC-induced SS. This compound expands the choice of materials in the field of antiferromagnetic spintronics and is likely to stimulate subsequent investigations of high-efficiency spintronic devices that are functional at room temperature.

cond-mat.mtrl-sci↗

arXiv2023

Electronic Transport Studies of Ag-doped Bi2Se3 Topological Insulator

The structural, magnetotransport, and angle-resolved photoemission spectroscopy (ARPES) of Ag-doped Bi2Se3 single crystals are presented. Temperature dependent resistivity exhibits metallic behavior with a slope change above 200 K for Ag-doped Bi2Se3. The magnetoresistance shows positive quadratic dependence at low fields satisfying Kohler's rule. Hall resistivity measurement shows that electrons are dominant charge carriers. Furthermore, these results agree well with the ARPES spectra observed at T = 20 K, where the Fermi level lies inside the bulk conduction band. The Dirac point of the topological surface states is shifted toward higher binding energy (~ 0.12 eV) for Ag-doped samples as compared to pristine Bi2Se3.

cond-mat.str-el↗

arXiv2023

Chiral Dirac fermion in a collinear antiferromagnet

In a Dirac semimetal, the massless Dirac fermion has zero chirality, leading to surface states connected adiabatically to a topologically trivial surface state as well as vanishing anomalous Hall effect (AHE). Recently, it is predicted that in the nonrelativistic limit of certain collinear antiferromagnets, there exists a type of chiral Dirac-like fermion, whose dispersion manifests four-fold degenerate crossing points formed by spin-degenerate linear bands, with topologically protected Fermi arcs. Such unconventional chiral fermion, protected by a hidden SU(2) symmetry in the hierarchy of an enhanced crystallographic group, namely spin space group, is not experimentally verified yet. Here, by angle-resolved photoemission spectroscopy measurements, we reveal the surface origin of the electron pocket at the Fermi surface in collinear antiferromagnet CoNb3S6. Combining with neutron diffraction and first-principles calculations, we suggest a multidomain collinear AFM configuration, rendering the the existence of the Fermi-arc surface states induced by chiral Dirac-like fermions. Our work provides spectral evidence of the chiral Dirac-like fermion caused by particular spin symmetry in CoNb3S6, paving an avenue for exploring new emergent phenomena in antiferromagnets with unconventional quasiparticle excitations.

cond-mat.mtrl-sci↗