arXiv subjects

Kevin J. Resch

Publications and source records attributed to Kevin J. Resch.

At least 19 recordsLinked to original sources

arXiv2025

Entanglement certification using noncontextuality inequalities

By combining the assumptions of Bell locality with those of generalized noncontextuality, we define classes of noncontextuality inequalities for correlations arising in a bipartite Bell circuit. These classes are distinguished by which subsets of the full set of operational identities are taken as input to the principle of noncontextuality; certain natural subsets form a hierarchy that provides a new way of understanding and classifying quantum correlations, including entanglement, steering, and nonlocality. Each level of this hierarchy gives rise to a corresponding class of noncontextuality inequalities whose violation witnesses one of these forms of bipartite quantum resourcefulness, thereby yielding different sufficient conditions for entanglement. The resulting entanglement certification paradigm requires no prior characterization of the measurements, is independent of tomographic gauge freedom, and can certify any entangled state without auxiliary entangled sources. To illustrate its power, we show that noncontextuality inequalities can certify entanglement for families of two-qubit isotropic states for which Bell or steering inequalities are known to fail. We also show that, compared with the Bell test, this approach certifies a much larger fraction of entangled states, while the associated membership problem is more tractable. On the experimental side, we describe techniques to ensure nontrivial operational identities in the presence of noisy and imperfect implementations. We also identify the key assumption under which these techniques are valid, namely, a particular notion of tomographic completeness, which ensures that the operational identities are gauge-independent. Finally, we provide an experimental demonstration of the superior performance of this entanglement certification technique using polarization-entangled photons.

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arXiv2025

Experimental Test of the Principle of Tomographic Locality

The principle of tomographic locality states that the operational state of a multipartite system can be fully characterized by the statistics obtained from measurements that are local to the individual subsystems. This property holds in quantum theory and features prominently in axiomatic reconstructions of the theory, where it serves to rule out a wide class of alternatives. For instance, quantum theory with Hilbert spaces defined over the real field (rather than the complex field) is an example of a theory that is ruled out in this fashion. Given its foundational importance, it is worthwhile to subject this principle to a direct experimental test. Specifically, we consider an experiment on the polarization degrees of freedom of a pair of photonic modes in a prepare-and-measure scenario and analyze the resulting data within the framework of generalized probabilistic theories. The signature of a failure of tomographic locality is that there are pairs of states on the bipartite system that can only be distinguished by the statistics they yield for non-separable measurements. In the full quantum setting, we find no evidence of a violation of tomographic locality. As a test of our analysis method, we also verify that if we restrict attention to those states and measurements that lie within the fragment described by quantum theory over the real field, then a clear signature of the failure of tomographic locality is observed.

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arXiv2025

Enhanced resolution chirped-pulse interferometry

Chirped-pulse interferometry (CPI) is a classical low-coherence interferometry technique with automatic dispersion cancellation and improved resolution over white-light interference. Previous work has shown that CPI with linearly-chirped Gaussian laser pulses achieves a $\sqrt{2}$ improvement in resolution over conventional white-light interferometry, but this is less than the factor of 2 improvement exhibited by a comparable quantum technique. In this work, we show how a particular class of nonlinearly-chirped laser pulses can meet, and even exceed, the factor of 2 improvement resolution. This enhanced resolution CPI removes the remaining advantage of quantum interferometers in dispersion-cancelled interferometry.

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arXiv2024

Reply to "Comment on 'Experimentally adjudicating between different causal accounts of Bell-inequality violations via statistical model selection'"

Our article described an experiment that adjudicates between different causal accounts of Bell inequality violations by a comparison of their predictive power, finding that certain types of models that are structurally radical but parametrically conservative, of which a class of superdeterministic models are an example, overfit the data relative to models that are structurally conservative but parametrically radical in the sense of endorsing an intrinsically quantum generalization of the framework of causal modelling. In their comment (arXiv:2206.10619), Hance and Hossenfelder argue that we have misrepresented the purpose of superdeterministic models. We here dispute this claim by recalling the different classes of superdeterministic models we defined in our article and our conclusions regarding which of these are disfavoured by our experimental results. Their confusion on this point seems to have arisen in part from the fact that we characterized superdeterministic models within a causal modelling framework and from the fact that we referred to this framework as "classical" in order to contrast it with an intrinsically quantum alternative. In this reply, therefore, we take the opportunity to clarify these points. They also claim that if one is adjudicating between a pair of models, where one model can account for strictly more operational statistics than the other, the first model will tend to overfit the data relative to the second. Because this model inclusion relation can arise for pairs of models in a reductionist heirarchy, they conclude that overfitting should not be taken as evidence against the first model. We point out here that, contrary to this claim, one does not expect overfitting to arise generically in cases of model inclusion, so that it is indeed sometimes appropriate to consider overfitting as a criterion for adjudicating between such models.

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arXiv2023

Ultrafast Measurement of Energy-Time Entanglement with an Optical Kerr Shutter

Recent experimental progress in quantum optics has enabled measurement of single photons on ultrafast timescales, beyond the resolution limit of single photon detectors. The energy-time degree of freedom has emerged as a promising avenue for quantum technologies, as entanglement between the frequency and temporal properties of two photons can be fully explored and utilized. Here, we implement optical Kerr shutters in single mode fibers to map out the sub-picosecond correlations of energy-time entangled photon pairs. These measurements, in addition to joint spectral measurements of the photon pair state, are used to verify entanglement by means of the violation of a time-bandwidth inequality.

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arXiv2021

Experimentally bounding deviations from quantum theory in the landscape of generalized probabilistic theories

Many experiments in the field of quantum foundations seek to adjudicate between quantum theory and speculative alternatives to it. This requires one to analyze the experimental data in a manner that does not presume the correctness of the quantum formalism. The mathematical framework of generalized probabilistic theories (GPTs) provides a means of doing so. We present a scheme for determining which GPTs are consistent with a given set of experimental data. It proceeds by performing tomography on the preparations and measurements in a self-consistent manner, i.e., without presuming a prior characterization of either. We illustrate the scheme by analyzing experimental data for a large set of preparations and measurements on the polarization degree of freedom of a single photon. We find that the smallest and largest GPT state spaces consistent with our data are a pair of polytopes, each approximating the shape of the Bloch Sphere and having a volume ratio of $0.977 \pm 0.001$, which provides a quantitative bound on the scope for deviations from quantum theory. We also demonstrate how our scheme can be used to bound the extent to which nature might be more nonlocal than quantum theory predicts, as well as the extent to which it might be more or less contextual. Specifically, we find that the maximal violation of the CHSH inequality can be at most $1.3\% \pm 0.1$ greater than the quantum prediction, and the maximal violation of a particular inequality for universal noncontextuality can not differ from the quantum prediction by more than this factor on either side. The most significant loophole in this sort of analysis is that the set of preparations and measurements one implements might fail to be tomographically complete for the system of interest.

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arXiv2021

Experimentally adjudicating between different causal accounts of Bell inequality violations via statistical model selection

Bell inequalities follow from a set of seemingly natural assumptions about how to provide a causal model of a Bell experiment. In the face of their violation, two types of causal models that modify some of these assumptions have been proposed: (i) those that are parametrically conservative and structurally radical, such as models where the parameters are conditional probability distributions (termed 'classical causal models') but where one posits inter-lab causal influences or superdeterminism, and (ii) those that are parametrically radical and structurally conservative, such as models where the labs are taken to be connected only by a common cause but where conditional probabilities are replaced by conditional density operators (these are termed 'quantum causal models'). We here seek to adjudicate between these alternatives based on their predictive power. The data from a Bell experiment is divided into a training set and a test set, and for each causal model, the parameters that yield the best fit for the training set are estimated and then used to make predictions about the test set. Our main result is that the structurally radical classical causal models are disfavoured relative to the structurally conservative quantum causal model. Their lower predictive power seems to be due to the fact that, unlike the quantum causal model, they are prone to a certain type of overfitting wherein statistical fluctuations away from the no-signalling condition are mistaken for real features. Our technique shows that it is possible to witness quantumness even in a Bell experiment that does not close the locality loophole. It also overturns the notion that it is impossible to experimentally test the plausibility of superdeterminist models of Bell inequality violations.

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arXiv2021

Remote state preparation of single photon orbital angular momentum lattices

Optical beams with periodic lattice structures have broadened the study of structured waves. In the present work, we generate spin-orbit entangled photon states with a lattice structure and use them in a remote state preparation protocol. We sequentially measure spatially-dependent correlation rates with an electron-multiplying intensified CCD camera and verify the successful remote preparation of spin-orbit states by performing pixel-wise quantum state tomography. Control of these novel structured waves in the quantum regime provides a method for quantum sensing and manipulation of periodic structures.

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arXiv2020

Quantum simulation of Unruh-DeWitt detectors with nonlinear optics

We propose a method for simulating an Unruh-DeWitt detector, coupled to a 1+1-dimensional massless scalar field, with a suitably-engineered $χ^{(2)}$ nonlinear interaction. In this simulation, the parameter playing the role of the detector acceleration is played by the relative inverse-group-velocity gradient inside the nonlinear material. We identify experimental parameters that tune the detector energy gap, acceleration, and switching function. This system can simulate time-dependent acceleration, time-dependent detector energy gaps, and non-vacuum initial detector-field states. Furthermore, for very short materials, the system can simulate the weak anti-Unruh effect, in which the response of the detector decreases with acceleration. While some Unruh-related phenomena have been investigated in nonlinear optics, this is the first proposal for simulating an Unruh-DeWitt detector in these systems.

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arXiv2020

Talbot Effect of orbital angular momentum lattices with single photons

The self-imaging, or Talbot Effect, that occurs with the propagation of periodically structured waves has enabled several unique applications in optical metrology, image processing, data transmission, and matter-wave interferometry. In this work, we report on the first demonstration of a Talbot Effect with single photons prepared in a lattice of orbital angular momentum (OAM) states. We observe that upon propagation, the wavefronts of the single photons manifest self-imaging whereby the OAM lattice intensity profile is recovered. Furthermore, we show that the intensity at fractional Talbot distances is indicative of a periodic helical phase structure corresponding to a lattice of OAM states. This phenomenon is a powerful addition to the toolbox of orbital angular momentum and spin-orbit techniques that have already enabled many recent developments in quantum optics.

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arXiv2019

Reconstructing ultrafast energy-time entangled two-photon pulses

The generation of ultrafast laser pulses and the reconstruction of their electric fields is essential for many applications in modern optics. Quantum optical fields can also be generated on ultrafast time scales, however, the tools and methods available for strong laser pulses are not appropriate for measuring the properties of weak, possibly entangled pulses. Here, we demonstrate a method to reconstruct the joint-spectral amplitude of a two-photon energy-time entangled state from joint measurements of the frequencies and arrival times of the photons, and the correlations between them. Our reconstruction method is based on a modified Gerchberg-Saxton algorithm. Such techniques are essential to measure and control the shape of ultrafast entangled photon pulses.

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arXiv2018

Ultrafast quantum interferometry with energy-time entangled photons

Many quantum advantages in metrology and communication arise from interferometric phenomena. Such phenomena can occur on ultrafast time scales, particularly when energy-time entangled photons are employed. These have been relatively unexplored as their observation necessitates time resolution much shorter than conventional photon counters. Integrating nonlinear optical gating with conventional photon counters can overcome this limitation and enable subpicosecond time resolution. Here, using this technique and a Franson interferometer, we demonstrate high-visibility quantum interference with two entangled photons, where the one- and two-photon coherence times are both subpicosecond. We directly observe the spectral and temporal interference patterns, measure a visibility in the two-photon coincidence rate of $(85.3\pm0.4)\%$, and report a CHSH-Bell parameter of $2.42\pm0.02$, violating the local-hidden variable bound by 21 standard deviations. The demonstration of energy-time entanglement with ultrafast interferometry provides opportunities for examining and exploiting entanglement in previously inaccessible regimes.

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arXiv2018

Quantum-coherent mixtures of causal relations

Understanding the causal influences that hold among parts of a system is critical both to explaining that system's natural behaviour and to controlling it through targeted interventions. In a quantum world, understanding causal relations is equally important, but the set of possibilities is far richer. The two basic ways in which a pair of time-ordered quantum systems may be causally related are by a cause-effect mechanism or by a common cause acting on both. Here, we show a coherent mixture of these two possibilities. We realize this nonclassical causal relation in a quantum optics experiment and derive a set of criteria for witnessing the coherence based on a quantum version of Berkson's effect, whereby two independent causes can become correlated upon observation of their common effect. The interplay of causality and quantum theory lies at the heart of challenging foundational puzzles, including Bell's theorem and the search for quantum gravity.

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arXiv2017

Direct characterization of ultrafast energy-time entangled photon pairs

Energy-time entangled photons are critical in many quantum optical phenomena and have emerged as important elements in quantum information protocols. Entanglement in this degree of freedom often manifests itself on ultrafast timescales making it very difficult to detect, whether one employs direct or interferometric techniques, as photon-counting detectors have insufficient time resolution. Here, we implement ultrafast photon counters based on nonlinear interactions and strong femtosecond laser pulses to probe energy-time entanglement in this important regime. Using this technique and single-photon spectrometers, we characterize all the spectral and temporal correlations of two entangled photons with femtosecond resolution. This enables the witnessing of energy-time entanglement using uncertainty relations and the direct observation of nonlocal dispersion cancellation on ultrafast timescales. These techniques are essential to understand and control the energy-time degree of freedom of light for ultrafast quantum optics.

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arXiv2017

Quantum to classical transitions in causal relations

The landscape of causal relations that can hold among a set of systems in quantum theory is richer than in classical physics. In particular, a pair of time-ordered systems can be related as cause and effect or as the effects of a common cause, and each of these causal mechanisms can be coherent or not. Furthermore, one can combine these mechanisms in different ways: by probabilistically realizing either one or the other or by having both act simultaneously (termed a physical mixture). In the latter case, it is possible for the two mechanisms to be combined quantum-coherently. Previous work has shown how to experimentally realize one example of each class of possible causal relations. Here, we make a theoretical and experimental study of the transitions between these classes. In particular, for each of the two distinct types of coherence that can exist in mixtures of common-cause and cause-effect relations--coherence in the individual causal pathways and coherence in the way the causal relations are combined--we determine how it degrades under noise and we confirm these expectations in a quantum-optical experiment.

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arXiv2017

Storage of polarization-entangled THz-bandwidth photons in a diamond quantum memory

Bulk diamond phonons have been shown to be a versatile platform for the generation, storage, and manipulation of high-bandwidth quantum states of light. Here we demonstrate a diamond quantum memory that stores, and releases on demand, an arbitrarily polarized $\sim$250 fs duration photonic qubit. The single-mode nature of the memory is overcome by mapping the two degrees of polarization of the qubit, via Raman transitions, onto two spatially distinct optical phonon modes located in the same diamond crystal. The two modes are coherently recombined upon retrieval and quantum process tomography confirms that the memory faithfully reproduces the input state with average fidelity $0.784\pm0.004$ with a total memory efficiency of $(0.76\pm0.03)\%$. In an additional demonstration, one photon of a polarization-entangled pair is stored in the memory. We report that entanglement persists in the retrieved state for up to 1.3 ps of storage time. These results demonstrate that the diamond phonon platform can be used in concert with polarization qubits, a key requirement for polarization-encoded photonic processing.

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arXiv2017

Observation of genuine three-photon interference

Multiparticle quantum interference is critical for our understanding and exploitation of quantum information, and for fundamental tests of quantum mechanics. A remarkable example of multi-partite correlations is exhibited by the Greenberger-Horne-Zeilinger (GHZ) state. In a GHZ state, three particles are correlated while no pairwise correlation is found. The manifestation of these strong correlations in an interferometric setting has been studied theoretically since 1990 but no three-photon GHZ interferometer has been realized experimentally. Here we demonstrate three-photon interference that does not originate from two-photon or single photon interference. We observe phase-dependent variation of three-photon coincidences with 90.5 \pm 5.0 % visibility in a generalized Franson interferometer using energy-time entangled photon triplets. The demonstration of these strong correlations in an interferometric setting provides new avenues for multiphoton interferometry, fundamental tests of quantum mechanics and quantum information applications in higher dimensions.

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arXiv2016

Spectrally engineering photonic entanglement with a time lens

In the same manner that free-space propagation and curved glass lenses are used to shape the spatial properties of light, a combination of chromatic dispersion and devices known as time lenses may be used to reshape its temporal properties. These techniques have found extensive application in classical optical signal processing based on nonlinear optics. A new set of challenges presents itself when processing quantum signals, including noise suppression and high fidelity requirements. In this work, we construct a single-photon time lens based on dispersion and nonlinear sum-frequency generation to image the spectral waveform of half of an entangled photon pair. We find that the joint spectrum of the photon pair has strongly negative frequency correlations before the time lens and strongly positive correlations afterwards, verifying that the process has an overall negative spectro-temporal magnification. The temporal imaging of energy-time entangled systems opens up a host of new possible techniques for distinctly quantum tasks in the frequency domain, including state engineering, and our results demonstrate that the upconversion time lens is an essential part of the single-photon waveform manipulation toolkit.

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