arXiv subjects

Kevin J. Weatherill

Publications and source records attributed to Kevin J. Weatherill.

At least 19 recordsLinked to original sources

arXiv2025

Simultaneous optical and multi-band terahertz imaging using an atomic quantum sensor

We demonstrate simultaneous imaging at 0.549 THz and 1.012 THz with an optical overlay using a two-species atomic-vapour-based technique. The atomic vapour, comprising laser-pumped rubidium and caesium atoms contained within the same cell, is used to convert two narrowband terahertz signals to optical frequencies which can then be detected using standard CMOS sensors. We use the system to image and perform spectral analysis of material samples. As atomic vapour is optically transparent, by using optically-transparent terahertz lenses, we can achieve simultaneous optical imaging, allowing for potential integration of terahertz sensitivity into a range of optical imaging devices.

physics.atom-ph↗

arXiv2025

Temporally-multiplexed dual-frequency terahertz imaging at kilohertz frame rates

We present a temporally-multiplexed dual-colour terahertz (THz) imaging technique using THz-to-optical conversion in atomic vapour. By rapidly alternating the pump laser frequency, we sequentially excite two atomic states, each absorbing a different THz frequency: 0.5 THz and 1.1 THz. Each THz field induces optical fluorescence at a distinct wavelength, enabling the creation of a sequence of alternating, interleaved images for each frequency. Synchronizing the laser switching with camera acquisition allows video capture at 1,000 frames per second for both frequencies. The system's speed is limited only by laser power and fibre switching hardware. The presented method can be scaled to image more THz frequencies through the addition of further laser frequencies, paving the way for THz hyperspectral imaging in many real-world settings.

physics.atom-ph↗

arXiv2025

Virtually structured illumination for terahertz super-resolution imaging

We demonstrate structured illumination super-resolution imaging in the Terahertz (THz) frequency band using the Virtually Structured Detection (VSD) method. Leveraging our previously reported high-speed, high-sensitivity atomic-based THz imager, we achieve a resolution enhancement of 74(3)% at 0.55 THz, without the aid of deconvolution methods. We show a high-speed THz imaging system is compatible with the use of advanced optical techniques, with potential disruptive effects on applications requiring both high speed and high spatial resolution imaging in the THz range.

physics.optics↗

arXiv2025

Determination of Quantum Defects and Core Polarizability of Atomic Cesium via Terahertz and Radio-Frequency Spectroscopy in Thermal Vapor

We present new measurements of quantum defects and core polarizabilities in cesium ($^{133}$Cs), based on transition frequency measurements between Rydberg states ($14 \leq n \leq 38$) obtained through terahertz (THz) and radio-frequency spectroscopy in a thermal atomic vapor. %By detuning resonant fields coupling neighbouring Rydberg states, we observe a detuning-dependent asymmetry in the line shape which can be used to extract the frequency of the transition. We perform a global fitting of our measurements to extract quantum defects of the $s_{1/2}$, $p_{1/2}$, $p_{3/2}$, $d_{3/2}$, $d_{5/2}$, $f_{5/2}$, $f_{7/2}$, $g_{7/2}$ and $g_{9/2}$ electronic states. Transitions between high angular momentum states ($4 \leq \ell \leq 8$) were measured to extract the Cs$^{+}$ dipole and quadrupole polarizabilities. We find $α_{d} = 15.729(18)$ $a_{0}^{3}$ and $α_{q} = 76.3(1.9)$ $a_{0}^{5}$ respectively. Using these results, and accounting for the covariances between parameters in the global fit, the energies for $n\ell_{j}$ Rydberg states can be estimated to a precision of a few MHz or less.

physics.atom-ph↗

arXiv2024

Single photonic qutrit in a collective Rydberg polariton

We report on the coherent creation, control and read-out of a single photonic qutrit in a Rydberg ensemble. In each measurement, an optical photon is stored as a Rydberg polariton through electromagnetically induced transparency. Employing two microwave fields, the polariton is driven into an arbitrary superposition of three collective states, each encoded in a Rydberg state. The collective state is mapped into a photonic time-bin qutrit with the microwave field and read out sequentially. The complete sequence, including preparation, control, and read-out, is less than 1.8~$μ$s, which mitigates decoherence significantly. We measure the coherence of the qutrit with non-destructive Ramsey interferometry, which is preferable for quantum information processing, and find good quantitative agreement with the theoretical model. The ability to write, process and read out the single photonic qutrit on microsecond time scales with microwave coupled Rydberg states demonstrates the coherent connectivity among the high Hilbert space of the qutrit.Our study is an important step in exploring qutrit based quantum information processes and quantum simulation of topological physics with microwave coupled Rydberg atom ensembles.

quant-ph↗

arXiv2023

Simultaneous multi-band radio-frequency detection using high-orbital-angular-momentum states in a Rydberg-atom receiver

We demonstrate simultaneous detection of radio-frequency (RF) fields ranging from the very high-frequency (VHF) band (128 MHz) to terahertz frequencies (0.61 THz) using a caesium Rydberg-atom receiver. The RF fields are concurrently applied to a series of atomic transitions involving states of increasing orbital angular momentum, where the energy separations become progressively smaller, allowing access to a very wide range of radio frequencies. We show that the optical response of the system in the presence of the RF fields can be reproduced theoretically using a simple Lindblad-master-equation approach. Furthermore, we demonstrate experimentally that a series of amplitude-modulated tones can be detected simultaneously using multiple carrier frequencies. This demonstration opens the way for RF communications across multiple bands simultaneously using a single optical receiver.

physics.atom-ph↗

arXiv2022

Rapid readout of terahertz orbital angular momentum beams using atom-based imaging

We demonstrate the rapid readout of terahertz (THz) orbital angular momentum (OAM) beams using an atomic-vapour based imaging technique. OAM modes with both azimuthal and radial indices are created using phase-only transmission plates. The beams undergo terahertz to optical conversion in an atomic vapour, before being imaged in the far field using an optical CCD camera. In addition to the spatial intensity profile, we also observe the self-interferogram of the beams by imaging through a tilted lens, allowing the sign and magnitude of the azimuthal index to be read out directly. Using this technique, we can reliably read out the OAM mode of low-intensity beams with high fidelity in 10 ms. Such a demonstration is expected to have far-reaching consequences for proposed applications of terahertz OAM beams in communications and microscopy.

physics.optics↗

arXiv2021

The Robustness of a Collectively Encoded Rydberg Qubit

We demonstrate a collectively-encoded qubit based on a single Rydberg excitation stored in an ensemble of $N$ entangled atoms. Qubit rotations are performed by applying microwave fields that drive excitations between Rydberg states. Coherent read-out is performed by mapping the excitation into a single photon. Ramsey interferometry is used to probe the coherence of the qubit, and to test the robustness to external perturbations. We show that qubit coherence is preserved even as we lose atoms from the polariton mode, preserving Ramsey fringe visibility. We show that dephasing due to electric field noise scales as the fourth power of field amplitude. These results show that robust quantum information processing can be achieved via collective encoding using Rydberg polaritons, and hence this system could provide an attractive alternative coding strategy for quantum computation and networking.

physics.atom-ph↗

arXiv2020

Single-Photon Stored-Light Interferometry

We demonstrate a single-photon stored-light interferometer, where a photon is stored in a laser-cooled atomic ensemble in the form of a Rydberg polariton with a spatial extent of $10 \times1\times1μm^3$. The photon is subject to a Ramsey sequence, i.e. `split' into a superposition of two paths. After a delay of up to 450 ns, the two paths are recombined to give an output dependent on their relative phase. The superposition time of 450 ns is equivalent to a free-space propagation distance of 135 m. We show that the interferometer fringes are sensitive to external fields, and suggest that stored-light interferometry could be useful for localized sensing applications.

physics.atom-ph↗

arXiv2019

Ultra-high-speed Terahertz Imaging Using Atomic Vapour

Terahertz (THz) technologies, generally defined as operating in the 0.1-10THz range, bridge the gap between electronic and photonic devices. Because THz radiation passes readily through materials such as plastics, paper and cloth it can be employed in non-destructive testing, and as it is non-ionising it is considered safe for security and biomedical applications. There is significant demand for high speed THz imaging across a range of applications but, despite ongoing efforts, fast full-field imaging remains an unfulfilled goal. Here we demonstrate a THz imaging system based upon efficient THz-to-optical conversion in atomic vapour, where full-field images can be collected at ultra-high speeds using conventional optical camera technology. For a 0.55 THz field we show an effective 1 cm $^{2}$ sensor with near diffraction-limited spatial resolution and a minimum detectable power of 190 $\pm$ 30 fW s$^{-1/2}$ per 40x40$μ$m pixel capable of video capture at 3000 frames per second. This combination of speed and sensitivity represents a step change in the state of the art of THz imaging, and will likely lead to its uptake in wider industrial settings. With further improvements we expect that even higher frame rates of up to 1 MHz would be possible.

physics.atom-ph↗

arXiv2017

Terahertz-driven phase transition applied as a room-temperature terahertz detector

There are few demonstrated examples of phase transitions that may be driven directly by terahertz-frequency electric fields, and those that are known require field strengths exceeding 1 MVcm$^{-1}$. Here we report a room-temperature phase transition driven by a weak ($\ll 1$ Vcm$^{-1}$), continuous-wave terahertz electric field. The system consists of caesium vapour under continuous optical excitation to a high-lying Rydberg state, which is resonantly coupled to a nearby level by the terahertz electric field. We use a simple model to understand the underlying physical behaviour, and we demonstrate two protocols to exploit the phase transition as a narrowband terahertz detector: the first with a fast (20 $μ$s) nonlinear response to nano-Watts of incident radiation, and the second with a linearised response and effective noise equivalent power (NEP) $\leq 1$ pWHz$^{-1/2}$. The work opens the door to a new class of terahertz devices controlled with low field intensities and operating around room temperature.

physics.atom-ph↗

arXiv2017

Probing interactions of thermal Sr Rydberg atoms using simultaneous optical and ion detection

We demonstrate a method for probing interaction effects in a thermal beam of strontium atoms using simultaneous measurements of Rydberg EIT and spontaneously created ions or electrons. We present a Doppler-averaged optical Bloch equation model that reproduces the optical signals and allows us to connect the optical coherences and the populations. We use this to determine that the spontaneous ionization process in our system occurs due to collisions between Rydberg and ground state atoms in the EIT regime. We measure the cross section of this process to be 0.6 $\pm$ 0.2 $σ_{\rm{geo}}$, where $σ_{\rm{geo}}$ is the geometrical cross section of the Rydberg atom. This results adds complementary insight to a range of recent studies of interacting thermal Rydberg ensembles.

physics.atom-ph↗

arXiv2016

Real-Time Near-Field Terahertz Imaging with Atomic Optical Fluorescence

Terahertz (THz) near-field imaging is a flourishing discipline [1], with applications from fundamental studies of beam propagation [2,3] to the characterisation of metameterials [4,5] and waveguides [6,7]. Beating the diffraction limit typically involves rastering structures or detectors with length scale shorter than the radiation wavelength; in the THz domain this has been achieved using a number of techniques including scattering tips [8,9] and apertures [10]. Alternatively, mapping THz fields onto an optical wavelength and imaging the visible light removes the requirement for scanning a local probe, speeding up image collection times [11,12]. Here we report THz to optical conversion using a gas of highly excited `Rydberg' atoms. By collecting THz-induced optical fluorescence we demonstrate a real-time image of a THz standing wave and we use well-known atomic properties to calibrate the THz field strength. The mono-atomic gas does not distort the THz field and offers the potential to immerse structures within the THz-to-optical conversion medium.

physics.atom-ph↗

arXiv2016

Dressed-state electromagnetically induced transparency for light storage in uniform phase spin-waves

We present, experimentally and theoretically, a scheme for dressed-state electromagnetically induced transparency (EIT) in a three-step cascade system where a four-level system is mapped into an effective three-level system. Theoretical analysis reveals that the scheme provides coherent state control via adiabatic following and provides a generalized protocol for light storage in uniform phase spin-waves that are insensitive to motional dephasing. The three-step driving enables a number of other features including spatial selectivity of the excitation region within the atomic medium, and kick-free and Doppler-free excitation that produces narrow resonances in thermal vapor. As a proof of concept we present an experimental demonstration of the generalized EIT scheme using the $6S_{1/2} \rightarrow 6P_{3/2} \rightarrow 7S_{1/2} \rightarrow 8P_{1/2}$ excitation path in thermal cesium vapor. This technique could be applied to cold and thermal ensembles to enable longer storage times for Rydberg polaritons.

physics.atom-ph↗

arXiv2016

Intrinsic Optical Bistability in a Strongly-Driven Rydberg Ensemble

We observe and characterize intrinsic optical bistability in a dilute Rydberg vapor. The bistability is characterized by sharp jumps between states of low and high Rydberg occupancy with jump up and down positions displaying hysteresis depending on the direction in which the control parameter is changed. We find that the shift in frequency of the jump point scales with the fourth power of the principal quantum number. Also, the width of the hysteresis window increases with increasing principal quantum number, before reaching a peak and then closing again. The experimental results are consistent with predictions from a simple theoretical model based on semiclassical Maxwell-Bloch equations including the effect of broadening and frequency shifts. These results provide insight to the dynamics of driven dissipative systems.

physics.atom-ph↗

arXiv2016

Driven-dissipative many-body systems with mixed power-law interactions: Bistabilities and temperature-driven non-equilibrium phase transitions

We investigate the non-equilibrium dynamics of a driven-dissipative spin ensemble with competing power-law interactions. We demonstrate that dynamical phase transitions as well as bistabilities can emerge for asymptotic van der Waals interactions, but critically rely on the presence of a slower decaying potential-core. Upon introducing random particle motion, we show that a finite gas temperature can drive a phase transition with regards to the spin degree of freedom and eventually leads to mean-field behaviour in the high-temperature limit. Our work reconciles contrasting observations of recent experiments with Rydberg atoms in the cold-gas and hot-vapour domain, and introduces an efficient theoretical framework in the latter regime.

physics.atom-ph↗

arXiv2015

Observation of interference effects via four photon excitation of highly excited Rydberg states in thermal cesium vapor

We report on the observation of electromagnetically induced transparency (EIT) and absorption (EIA) of highly excited Rydberg states in thermal Cs vapor using a four-step excitation scheme. The advantage of this four-step scheme is that the final transition to the Rydberg state has a large dipole moment and one can achieve similar Rabi frequencies to two- or three-step excitation schemes using two orders of magnitude less laser power. This scheme enables new applications such as dephasing free Rydberg excitation. The observed lineshapes are in good agreement with simulations based on multilevel optical Bloch equations.

physics.atom-ph↗

arXiv2014

Probing an excited-state atomic transition using hyperfine quantum beat spectroscopy

We describe a method to observe the dynamics of an excited-state transition in a room temperature atomic vapor using hyperfine quantum beats. Our experiment using cesium atoms consists of a pulsed excitation of the D2 transition, and continuous-wave driving of an excited-state transition from the 6P$_{3/2}$ state to the 7S$_{1/2}$ state. We observe quantum beats in the fluorescence from the 6P$_{3/2}$ state which are modified by the driving of the excited-state transition. The Fourier spectrum of the beat signal yields evidence of Autler-Townes splitting of the 6P$_{3/2}$, F = 5 hyperfine level and Rabi oscillations on the excited-state transition. A detailed model provides qualitative agreement with the data, giving insight to the physical processes involved.

physics.atom-ph↗