arXiv subjects

Khanh Duy Nguyen

Publications and source records attributed to Khanh Duy Nguyen.

14 recordsLinked to original sources

arXiv2026

Signatures of a light-induced exciton condensate exhibiting BEC-BCS crossover

Exciton condensates provide a platform to study quasiparticle pairing, Bose-Einstein condensation-Bardeen-Cooper-Schrieffer (BEC-BCS) crossover, and excitonic topological phenomena. Achieving a nonequilibrium exciton condensate allows the ultimate tunability of these emergent phenomena. Yet, evidence of a light-induced, nonequilibrium exciton condensate and its BEC-BCS crossover remains elusive. Here, we use time- and angle-resolved photoemission spectroscopy to demonstrate signatures of a non-equilibrium exciton condensate and its BEC-BCS crossover in monolayer MnBi2Te4. Following optical excitation, a distinctive hole-like dispersion representing excitons emerges and persists for >20 ps. Strikingly, energy-domain sharpening in the valence band occurs 2 ps after time zero and exhibits a sharp onset at a threshold pump fluence of 0.84 mJ/cm2. The delayed and strongly nonlinear response is difficult to reconcile with transient field effects or conventional carrier-induced band shifts but is consistent with a model of exciton condensation governed by a Berezinskii-Kosterlitz-Thouless transition. The estimated threshold exciton density agrees quantitatively with the Nelson-Kosterlitz critical density. At higher fluences, the exciton feature develops a camel-back-shaped dispersion, consistent with the BEC-BCS crossover in the condensate framework. Our work establishes ultrathin MnBi2Te4 as a model system for studying nonequilibrium exciton condensates with a connection to superconductivity and exciton-driven topological phases.

cond-mat.mes-hall↗

arXiv2026

Millimeter-Scale, Atomically Controlled 2D Topological Insulators Revealed by Multimodal Spectroscopy

Quantum spin Hall insulators, or synonymously known as 2D topological insulators, are crucial 2D systems hosting topologically protected edge states. The working temperature of this topological quantum phase is dictated by the inverted bandgap. However, the previously identified large-gap 2D topological insulators are either extremely chemically unstable, or cannot be made with atomistic precision over macroscopic scales. Here, we establish two-quintuple-layer Bi2Te3 and MnBi2Te4/Bi2Te3 heterostructures as atomically controlled, millimeter-scale 2D topological insulators, enabled by precision layer-by-layer growth that yields a carpet-like morphology extending coherently over macroscopic distances. This carpet-like growth mode renders the films amenable to mechanical exfoliation and subsequent wet or dry transfer. Multimodal spectroscopies and microscopies reveal the integer-layer tuned electronic structure of (Bi2Te3)n with excellent agreement to theory. Photon-energy-dependent photoemission and time-resolved photoemission identify band inversion and band dynamics, respectively, while scanning tunneling spectroscopy resolves topological edge states, characteristic of the 2D topological insulator phase. Thickness- and photon-energy-dependent photoemission further validates MnBi2Te4/Bi2Te3 as a robust 2D topological insulator. The large inverted gaps of ~100 meV in (Bi2Te3)2 and ~150 meV in MnBi2Te4/Bi2Te3 suggest operation near ambient temperature. These results define a scalable materials platform for next-generation, low-loss quantum and energy-efficient devices.

cond-mat.mtrl-sci↗

arXiv2026

Interaction-driven flat band and charge order in Fe5GeTe2

Flat electronic bands enable fascinating emergent phenomena such as superconductivity and charge orders. A prevailing approach to realizing flat bands is to engineer lattice geometric constraints in twisted or kagome-like materials. An alternative approach is to utilize purely electronic-interaction-driven flat bands, yet a fundamental challenge is that extreme flatness requires ultrastrong interaction strength, which often leads to incoherent states. Here we demonstrate the concurrent formation of an interaction-driven flat band at the Fermi level and a $\sqrt{3}\times\sqrt{3}\,R30^\circ$ charge order in a van der Waals magnet Fe5GeTe2 using high-resolution angle-resolved photoemission spectroscopy. This charge order is manifested by band folding within 30 meV below the Fermi level, with its nesting driven by flat bands. The presence of this flat band throughout the Brillouin zone and the logarithmic temperature dependence of its spectral weight suggest a Kondo-like, coherent Fermi liquid emerging from strong correlations. Our work establishes a paradigm where an interaction-driven flat band promotes large-scale electronic ordering.

cond-mat.str-el↗

arXiv2025

SYNTHIA: Novel Concept Design with Affordance Composition

Text-to-image (T2I) models enable rapid concept design, making them widely used in AI-driven design. While recent studies focus on generating semantic and stylistic variations of given design concepts, functional coherence--the integration of multiple affordances into a single coherent concept--remains largely overlooked. In this paper, we introduce SYNTHIA, a framework for generating novel, functionally coherent designs based on desired affordances. Our approach leverages a hierarchical concept ontology that decomposes concepts into parts and affordances, serving as a crucial building block for functionally coherent design. We also develop a curriculum learning scheme based on our ontology that contrastively fine-tunes T2I models to progressively learn affordance composition while maintaining visual novelty. To elaborate, we (i) gradually increase affordance distance, guiding models from basic concept-affordance association to complex affordance compositions that integrate parts of distinct affordances into a single, coherent form, and (ii) enforce visual novelty by employing contrastive objectives to push learned representations away from existing concepts. Experimental results show that SYNTHIA outperforms state-of-the-art T2I models, demonstrating absolute gains of 25.1% and 14.7% for novelty and functional coherence in human evaluation, respectively.

cs.CV↗

arXiv2025

PARTONOMY: Large Multimodal Models with Part-Level Visual Understanding

Real-world objects are composed of distinctive, object-specific parts. Identifying these parts is key to performing fine-grained, compositional reasoning-yet, large multimodal models (LMMs) struggle to perform this seemingly straightforward task. In this work, we introduce PARTONOMY, an LMM benchmark designed for pixel-level part grounding. We construct PARTONOMY from existing part datasets and our own rigorously annotated set of images, encompassing 862 part labels and 534 object labels for evaluation. Unlike existing datasets that simply ask models to identify generic parts, PARTONOMY uses specialized concepts (e.g., agricultural airplane), and challenges models to compare objects' parts, consider part-whole relationships, and justify textual predictions with visual segmentations. Our experiments demonstrate significant limitations in state-of-the-art LMMs (e.g., LISA-13B achieves only 5.9% gIoU), highlighting a critical gap in their part grounding abilities. We note that existing segmentation-enabled LMMs (segmenting LMMs) have two key architectural shortcomings: they use special [SEG] tokens not seen during pretraining which induce distribution shift, and they discard predicted segmentations instead of using past predictions to guide future ones. To address these deficiencies, we train several part-centric LMMs and propose PLUM, a novel segmenting LMM that uses span tagging instead of segmentation tokens and that conditions on prior predictions in a feedback loop. We find that pretrained PLUM outperforms existing segmenting LMMs on reasoning segmentation, VQA, and visual hallucination benchmarks. In addition, PLUM finetuned on our proposed Explanatory Part Segmentation task is competitive with segmenting LMMs trained on significantly more segmentation data. Our work opens up new avenues towards enabling fine-grained, grounded visual understanding in LMMs.

cs.CV↗

arXiv2025

Spectroscopic evidence of intra-unit-cell charge redistribution in charge-neutral magnetic topological insulator Sb-doped MnBi6Te10

The magnetic topological insulator MnBi$_{6}$Te$_{10}$ has emerged as a promising candidate for realizing the quantum anomalous Hall effect (QAHE), owing to its ability to retain ferromagnetism through precise control of anti-site defects. The next important task for realizing the QAHE is to tune the chemical potential into the energy gap formed by the broken time-reversal symmetry. Here we reveal an intra-unit-cell charge redistribution even when the overall doping suggests a near-charge-neutral condition. By performing time- and angle-resolved photoemission spectroscopy (trARPES) on the optimally 18% Sb-doped MnBi$_{6}$Te$_{10}$, we observe transient surface photovoltage (SPV) effects on both the MnBi$_{2}$Te$_{4}$ and single-Bi$_{2}$Te$_{3}$ terminations. Furthermore, we observe a time-dependent splitting of the band structure indicating multiple SPV shifts with different magnitudes. This observation suggests that adjacent plateaus with nominally the same terminating layer exhibit a strong intra-unit-cell charge redistribution, resulting in spontaneous electrical polarization. This is consistent with static micro-ARPES measurements revealing significant doping deviations from the charge-neutral configuration. Our findings underscore the challenges of engineering the family of Mn-Bi-Te materials to realize QAHE purely through chemical doping. Achieving the desired topological quantum phase requires both a uniform carrier doping and a ferromagnetic ground state. Furthermore, the light-induced polarization within each unit cell of ferromagnetic Mn(Bi$_{0.82}$Sb$_{0.18}$)$_{6}$Te$_{10}$ may open new possibilities for optoelectronic and spintronics.

cond-mat.mes-hall↗

arXiv2025

A Topological Superconductor Tuned by Electronic Correlations

A topological superconductor, characterized by either a chiral order parameter or a chiral topological surface state in proximity to bulk superconductivity, is foundational to topological quantum computing. As in other topological phases of matter, electronic correlations can tune topological superconductivity via modifications of the low-energy Fermiology. Such tuning has not been realized so far. Here we uncover a unique topological superconducting phase in competition with electronic correlations in 10-unit-cell thick FeTe$_{x}$Se$_{1-x}$ films grown on SrTiO$_{3}$ substrates. When the Te content $x$ exceeds $0.7$, we observe a rapid increase of the effective mass for the Fe $d_{xy}$ band, with the emergence of a superconducting topological surface state confirmed by high-resolution angle-resolved photoemission spectroscopy; however, near the FeTe limit, the system enters an incoherent regime where the topological surface state becomes unidentifiable and superconductivity is suppressed. Theory suggests that the electron-electron interactions in the odd-parity $xy^-$ band with a strong $d_{xy}$ character lead to an orbital-selective correlated phase. Our work establishes FeTe$_{x}$Se$_{1-x}$ thin films as a unique platform where electronic correlations sensitively modulate topological superconductivity, suggesting opportunities to use tunable electron-electron interactions to engineer new topological phases in a broad class of materials.

cond-mat.supr-con↗

arXiv2024

Schema-Guided Culture-Aware Complex Event Simulation with Multi-Agent Role-Play

Complex news events, such as natural disasters and socio-political conflicts, require swift responses from the government and society. Relying on historical events to project the future is insufficient as such events are sparse and do not cover all possible conditions and nuanced situations. Simulation of these complex events can help better prepare and reduce the negative impact. We develop a controllable complex news event simulator guided by both the event schema representing domain knowledge about the scenario and user-provided assumptions representing case-specific conditions. As event dynamics depend on the fine-grained social and cultural context, we further introduce a geo-diverse commonsense and cultural norm-aware knowledge enhancement component. To enhance the coherence of the simulation, apart from the global timeline of events, we take an agent-based approach to simulate the individual character states, plans, and actions. By incorporating the schema and cultural norms, our generated simulations achieve much higher coherence and appropriateness and are received favorably by participants from a humanitarian assistance organization.

cs.AI↗

arXiv2024

Distinguishing Surface and Bulk Electromagnetism via Their Dynamics in an Intrinsic Magnetic Topological Insulator

The indirect exchange interaction between local magnetic moments via surface electrons has been long predicted to bolster the surface ferromagnetism in magnetic topological insulators (MTIs), which facilitates the quantum anomalous Hall effect. This unconventional effect is critical to determining the operating temperatures of future topotronic devices. However, the experimental confirmation of this mechanism remains elusive, especially in intrinsic MTIs. Here we combine time-resolved photoemission spectroscopy with time-resolved magneto-optical Kerr effect measurements to elucidate the unique electromagnetism at the surface of an intrinsic MTI MnBi2Te4. Theoretical modeling based on 2D Ruderman-Kittel-Kasuya-Yosida interactions captures the initial quenching of a surface-rooted exchange gap within a factor of two but over-estimates the bulk demagnetization by one order of magnitude. This mechanism directly explains the sizable gap in the quasi-2D electronic state and the nonzero residual magnetization in even-layer MnBi2Te4. Furthermore, it leads to efficient light-induced demagnetization comparable to state-of-the-art magnetophotonic crystals, promising an effective manipulation of magnetism and topological orders for future topotronics.

cond-mat.str-el↗

arXiv2024

SmartBook: AI-Assisted Situation Report Generation for Intelligence Analysts

Timely and comprehensive understanding of emerging events is crucial for effective decision-making; automating situation report generation can significantly reduce the time, effort, and cost for intelligence analysts. In this work, we identify intelligence analysts' practices and preferences for AI assistance in situation report generation to guide the design strategies for an effective, trust-building interface that aligns with their thought processes and needs. Next, we introduce SmartBook, an automated framework designed to generate situation reports from large volumes of news data, creating structured reports by automatically discovering event-related strategic questions. These reports include multiple hypotheses (claims), summarized and grounded to sources with factual evidence, to promote in-depth situation understanding. Our comprehensive evaluation of SmartBook, encompassing a user study alongside a content review with an editing study, reveals SmartBook's effectiveness in generating accurate and relevant situation reports. Qualitative evaluations indicate over 80% of questions probe for strategic information, and over 90% of summaries produce tactically useful content, being consistently favored over summaries from a large language model integrated with web search. The editing study reveals that minimal information is removed from the generated text (under 2.5%), suggesting that SmartBook provides analysts with a valuable foundation for situation reports

cs.CL↗

arXiv2023

RESIN-EDITOR: A Schema-guided Hierarchical Event Graph Visualizer and Editor

In this paper, we present RESIN-EDITOR, an interactive event graph visualizer and editor designed for analyzing complex events. Our RESIN-EDITOR system allows users to render and freely edit hierarchical event graphs extracted from multimedia and multi-document news clusters with guidance from human-curated event schemas. RESIN-EDITOR's unique features include hierarchical graph visualization, comprehensive source tracing, and interactive user editing, which is more powerful and versatile than existing Information Extraction (IE) visualization tools. In our evaluation of RESIN-EDITOR, we demonstrate ways in which our tool is effective in understanding complex events and enhancing system performance. The source code, a video demonstration, and a live website for RESIN-EDITOR have been made publicly available.

cs.HC↗

arXiv2023

PopSim: An Individual-level Population Simulator for Equitable Allocation of City Resources

Historical systematic exclusionary tactics based on race have forced people of certain demographic groups to congregate in specific urban areas. Aside from the ethical aspects of such segregation, these policies have implications for the allocation of urban resources including public transportation, healthcare, and education within the cities. The initial step towards addressing these issues involves conducting an audit to assess the status of equitable resource allocation. However, due to privacy and confidentiality concerns, individual-level data containing demographic information cannot be made publicly available. By leveraging publicly available aggregated demographic statistics data, we introduce PopSim, a system for generating semi-synthetic individual-level population data with demographic information. We use PopSim to generate multiple benchmark datasets for the city of Chicago and conduct extensive statistical evaluations to validate those. We further use our datasets for several case studies that showcase the application of our system for auditing equitable allocation of city resources.

cs.CY↗

arXiv2017

Essential Properties of Fluorinated Graphene and Graphene Nanoribbons

A systematic study is conducted on the fluorination-enriched essential properties of 2D graphene and 1D graphene nanoribbons using the first-principles method. The combined effects, which arise from the significant chemical bonds in C-C, F-C and F-F bonds, the finite-size quantum confinement, and the edge structure, can greatly diversify geometric structures, electronic properties and magnetic configurations. By the detailed analyses, the critical orbital hybridizations in determining the essential properties are accurately identified from the atom-dominated energy bands, the spatial charge distributions, and the orbital-projected density of states. The top-site F-C bonds, with the multi-orbital hybridizations, create the non-uniform buckled honeycomb lattice. There exist the C-, F- and (C, F)-dominated energy bands. Fluorinated graphene belongs either to the p-type metals (with/without the ferromagnetic spin arrangement) or to the large-gap semiconductors (without magnetism), depending on the concentration and distribution of adatoms. Specially, fluorinated graphene nanoribbons, with armchair/zigzag edge, presents five kinds of spin-dependent properties, covering the non-magnetic and ferromagnetic metals, non-magnetic semiconductors, and anti-ferromagnetic semiconductors with/without the spin splitting. The various band-edge states in 2D and 1D systems appear as the rich and unique structures in density of states. Part of theoretical predictions are consistent with the experimental measurements, and the others are worthy of the further examinations. Also, the fluorination-created diverse properties clearly indicate the high potentials in various applications that will be discussed in detail, e.g., electronic and spintronic nanodevices.

cond-mat.mtrl-sci↗

arXiv2013

Skyrmions in the Skyrme model revisited

The possible boundary value problems of the skyrmions are reexamined in the original Skyrme model with two new viewpoints. The first one suggests to replace the infinity boundary point by the finite radius R, which is related to the density of the surrounding nuclear matter. The second viewpoint suggests to combine the global analysis with the numerical computation to give better results by avoiding the errors. It is interesting that the half integer topological skyrmions do exist in the model. Finally, the static properties of all possible skyrmions are calculated with the model parameters Subscript[F, \[Pi]] = 186 MeV, Subscript[m, \[Pi]]= 138 MeV and 1.57 < e < 4.17. The baryon masses are found to be too high compared to the experimental values, while the mass splitting between them is too small. On the other hand, the isoscalar radii and the axial coupling constant can be fitted with the experimental data with an error of 20% within the Balachandra's bound.

hep-ph↗