arXiv subjects

Kim G. L. Pedersen

Publications and source records attributed to Kim G. L. Pedersen.

8 recordsLinked to original sources

arXiv2018

Non-adiabatic effects in periodically driven-dissipative open quantum systems

We present a general method to calculate the quasi-stationary state of a driven-dissipative system coupled to a transmission line (and more generally, to a reservoir) under periodic modulation of its parameters. Using Floquet's theorem, we formulate the differential equation for the system's density operator which has to be solved for a single period of modulation. On this basis we also provide systematic expansions in both the adiabatic and high-frequency regime. Applying our method to three different systems -- two- and three-level models as well as the driven nonlinear cavity -- we propose periodic modulation protocols of parameters leading to a temporary suppression of effective dissipation rates, and study the arising non-adiabatic features in the response of these systems.

quant-ph↗

arXiv2017

Few photon scattering on Bose-Hubbard lattices

We theoretically investigate the scattering of few photon light on Bose-Hubbard lattices using diagrammatic scattering theory. We explicitly derive general analytical expressions for the lowest order photonic correlation functions, which we apply numerically to several different lattices. We focus specifically on non-linear effects visible in the intensity-intensity correlation function and explain bunching and anti-bunching effects in dimers, chains, rings and planes. The numerical implementation can be applied to arbitrary Bose-Hubbard graphs, and we provide it as an attachment to this publication.

quant-ph↗

arXiv2017

Kondo blockade due to quantum interference in single-molecule junctions

Molecular electronics offers unique scientific and technological possibilities, resulting from both the nanometre scale of the devices and their reproducible chemical complexity. Two fundamental yet different effects, with no classical analogue, have been demonstrated experimentally in single-molecule junctions: quantum interference due to competing electron transport pathways, and the Kondo effect due to entanglement from strong electronic interactions. Here we unify these phenomena, showing that transport through a spin-degenerate molecule can be either enhanced or blocked by Kondo correlations, depending on molecular structure, contacting geometry and applied gate voltages. An exact framework is developed, in terms of which the quantum interference properties of interacting molecular junctions can be systematically studied and understood. We prove that an exact Kondo-mediated conductance node results from destructive interference in exchange-cotunneling. Nonstandard temperature dependences and gate-tunable conductance peaks/nodes are demonstrated for prototypical molecular junctions, illustrating the intricate interplay of quantum effects beyond the single-orbital paradigm.

cond-mat.mes-hall↗

arXiv2017

Control over few photon pulses by a time-periodic modulation of the photon-emitter coupling

We develop a Floquet scattering formalism for the description of quasistationary states of microwave photons in a one-dimensional waveguide interacting with a nonlinear cavity by means of a periodically modulated coupling. This model is inspired by the recent progress in engineering of tunable coupling schemes with superconducting qubits. We argue that our model can realize the quantum analogue of an optical chopper. We find strong periodic modulations of the transmission and reflection envelopes in the scattered few-photon pulses, including photon compression and blockade, as well as dramatic changes in statistics. Our theoretical analysis allows us to explain these non-trivial phenomena as arising from non-adiabatic memory effects.

quant-ph↗

arXiv2016

Quantum choppers

An optical chopper periodically interrupts a classical light beam. We propose a realizable quantum version of the optical chopper, where the time-periodic driving of the light-matter coupling is achieved through a nonlinear three wave mixing element. We theoretically investigate how our scheme can be used for the controllable shaping of few photon light. Using Floquet dynamics, we find strong periodic modulations of the transmission and reflection envelopes in the scattered few-photon pulses, including photon compression and blockade, as well as dramatic changes in the quantum light statistics. Our theoretical analysis allows us to explain these non-trivial phenomena as arising from non-adiabatic memory effects.

quant-ph↗

arXiv2015

On the illusory connection between cross-conjugation and quantum interference

Quantum interference, be it destructive or constructive, has a substantial influence on the magnitude of molecular conductance and consequently there is significant interest in predicting these effects. It is commonly thought that cross-conjugated paths result in suppressed conductance due to destructive quantum interference. Using Hückel theory and DFT calculations we investigate systems that break this cross-conjugation rule of thumb. We predict and rationalize how a class of conjugated molecules containing closed loops can exhibit destructive interference despite being linearly conjugated and exhibit constructive interference despite being cross-conjugated. The arguments build on the graphical rules derived by Markussen et al. [1] and the hitherto neglected effects of closed loops in the molecular structure. Finally, we identify the 1,3 connected Azulene molecule as belonging to the closed-loop class and argue that this explains recent measurements of its electrical conductance.

cond-mat.mes-hall↗

arXiv2015

Using superlattice potentials to probe long-range magnetic correlations in optical lattices

In Pedersen et al. (2011) we proposed a method to utilize a temporally dependent superlattice potential to mediate spin-selective transport, and thereby probe long and short range magnetic correlations in optical lattices. Specifically this can be used for detecting antiferromagnetic ordering in repulsive fermionic optical lattice systems, but more generally it can serve as a means of directly probing correlations among the atoms by measuring the mean value of an observable, the number of double occupied sites. Here, we provide a detailed investigation of the physical processes which limit the effectiveness of this "conveyer belt method". Furthermore we propose a simple ways to improve the procedure, resulting in an essentially perfect (error-free) probing of the magnetic correlations. These results shows that suitably constructed superlattices constitute a promising way of manipulating atoms of different spin species as well as probing their interactions.

cond-mat.quant-gas↗

arXiv2014

Quantum Interference in Off-Resonant Transport through Single Molecules

We provide a simple set of rules for predicting interference effects in off-resonant transport through single-molecule junctions. These effects fall in two classes, showing respectively an odd or an even number of nodes in the linear conductance within a given molecular charge state, and we demonstrate how to decide the interference class directly from the contacting geometry. For neutral alternant hydrocarbons, we employ the Coulson-Rushbrooke-McLachlan pairing theorem to show that the interference class is decided simply by tunneling on and off the molecule from same, or different sublattices. More generally, we investigate a range of smaller molecules by means of exact diag- onalization combined with a perturbative treatment of the molecule-lead tunnel coupling. While these results generally agree well with GW calculations, they are shown to be at odds with simpler mean-field treatments. For molecules with spin-degenerate ground states, we show that for most junctions, interference causes no transmission nodes, but argue that it may lead to a non-standard gate-dependence of the zero-bias Kondo resonance.

cond-mat.mes-hall↗