arXiv subjects

Kirsten Harth

Publications and source records attributed to Kirsten Harth.

17 recordsLinked to original sources

arXiv2023

Cooling of a granular gas mixture in microgravity

Granular gases are fascinating non-equilibrium systems with interesting features such as spontaneous clustering and non-Gaussian velocity distributions. Mixtures of different components represent a much more natural composition than monodisperse ensembles, but attracted comparably little attention so far. We present the first experimental observation and characterization of a mixture of rod-like particles with different sizes and masses in microgravity. Kinetic energy decay rates during granular cooling and collision rates were determined and Haff's law for homogeneous granular cooling was confirmed. Thereby, energy equipartition between the mixture components and between individual degrees of freedom is violated. Heavier particles keep a slightly higher average kinetic energy than lighter ones. Experimental results are supported by numerical simulations.

cond-mat.soft↗

arXiv2023

The structure of disintegrating defect clusters in smectic C freely suspended films

Disclinations or disclination clusters in smectic C freely suspended films with topological charges larger than one are unstable. They disintegrate, preferably in a spatially symmetric fashion, into single defects with individual charges +1, which is the smallest positive topological charge allowed in polar vector fields. While the opposite process of defect annihilation is well-defined by the initial defect positions, a disintegration starts from a singular state and the following scenario including the emerging regular defect patterns must be selected by specific mechanisms. We analyze experimental data and compare them with a simple model where the defect clusters adiabatically pass quasi-equilibrium solutions in one-constant approximation. It is found that the defects arrange in geometrical patterns that correspond very closely to superimposed singular defect solutions, without additional director distortions. The patterns expand by affine transformations where all distances between individual defects scale with the same time-dependent scaling factor proportional to the square-root of time.

cond-mat.soft↗

arXiv2022

The effect of obstacles near a silo outlet on the discharge of soft spheres

Soft smooth particles in silo discharge show peculiar characteristics, including, for example, non-permanent clogging and intermittent flow. This paper describes a study of soft, low-frictional hydro\-gel spheres in a quasi-2D silo. We enforce a more competitive behavior of these spheres during their discharge by placing an obstacle in front of the outlet of the silo. High-speed optical imaging is used to capture the process of discharge. All particles in the field of view are identified and tracked by means of machine learning software using a MASK R-CNN algorithm. With particle tracking velocimetry (PTV), the fields of velocity, egress time, packing fraction, and kinetic stress are analysed in this study. While in pedestrian dynamics, the placement of an obstacle in front of a narrow gate may reduce the stress near the exit and enable a more efficient egress, the effect is opposite for our soft grains. Placing an obstacle above the orifice always led to a reduction of the flow rates, in some cases even to increased clogging probabilities.

physics.flu-dyn↗

arXiv2021

Deformation and relaxation of viscous thin films under bouncing drops

Thin, viscous liquid films subjected to impact events can deform. Here we investigate free surface oil film deformations that arise due to the air pressure buildup under the impacting and rebouncing water drops. Using Digital Holographic Microscopy, we measure the 3D surface topography of the deformed film immediately after the drop rebound, with a resolution down to 20 nm. We first discuss how the film is initially deformed during impact, as a function of film thickness, film viscosity, and drop impact speed. Subsequently, we describe the slow relaxation process of the deformed film after the rebound. Scaling laws for the broadening of the width and the decay of the amplitude of the perturbations are obtained experimentally and found to be in excellent agreement with the results from a lubrication analysis. We finally arrive at a detailed spatio-temporal description of the oil film deformations that arise during the impact and rebouncing of water drops.

physics.flu-dyn↗

arXiv2021

A simple model system for self-propelled particles passing a bottleneck

We study the passage of active and passive granular particles through a bottleneck under gravitational bias. The grains are pharmaceutical capsules with nearly spherocylindrical shapes on a vibrating table. The vibrating plate is slightly tilted in order to break the in-plane symmetry and to give particles a motivation to move in a preferential direction on the plate. The passage through a narrow gate with openings comparable to the grain length is studied using video imaging, and particle positions and velocities are extracted from the recorded frames. We compare the behaviour of asymmetrically filled, active capsules with symmetrically filled, passive ones.

cond-mat.soft↗

arXiv2021

Silo discharge of mixtures of soft and rigid grains

We study the outflow dynamics and clogging phenomena of mixtures of soft, elastic low-friction spherical grains and hard frictional spheres of similar size in a quasi-two-dimensional (2D) silo with narrow orifice at the bottom. Previous work has demonstrated the crucial influence of elasticity and friction on silo discharge. We show that the addition of small amounts, even as low as 5\%, of hard grains to an ensemble of soft, low-friction grains already has significant consequences. The mixtures allow a direct comparison of the probabilities of the different types of particles to clog the orifice. We analyze these probabilities for the hard, frictional and the soft, slippery grains on the basis of their participation in the blocking arches, and compare outflow velocities and durations of non-permanent clogs for different compositions of the mixtures. Experimental results are compared with numerical simulations. The latter strongly suggest a significant influence of the inter-species particle friction.

cond-mat.soft↗

arXiv2020

Intermittent flow and transient congestions of soft spheres passing narrow orifices

Soft, low-friction particles in silos show peculiar features during their discharge. The outflow velocity and the clogging probability both depend upon the momentary silo fill height, in sharp contrast to silos filled with hard particles. The reason is the fill-height dependence of the pressure at the orifice. We study the statistics of silo discharge of soft hydrogel spheres. The outflow is found to become increasingly fluctuating and even intermittent with decreasing orifice size, and with decreasing fill height. In orifices narrower than two particle diameters, outflow can stop completely, but in contrast to clogs formed by rigid particles, these congestions may dissolve spontaneously. We analyze such non-permanent congestions and attribute them to slow reorganization processes in the container, caused by viscoelasticity of the material.

cond-mat.soft↗

arXiv2020

Drop Impact on Hot Plates: Contact times, Lift-off and the Lamella Rupture

When a liquid drop impacts on a heated substrate, it can remain deposited, or violently boil in contact, or lift off with or without ever touching the surface. The latter is known as the Leidenfrost effect. The duration and area of the liquid--substrate contact is highly relevant for the heat transfer, as well as other effects such as corrosion. However, most experimental studies rely on side view imaging to determine contact times, and those are often mixed with the time until the drop lifts off from the substrate. Here, we develop and validate a reliable method of contact time determination using high-speed X-ray and Total Internal Reflection measurements. We exemplarily compare contact and lift-off times on flat silicon and sapphire substrates. We show that drops can rebound even without formation of a complete vapor layer, with a wide range of lift-off times. On sapphire, we find a local minimum of lift-off times much shorter than by capillary rebound in the comparatively low-temperature regime of transition boiling / thermal atomization. We elucidate the underlying mechanism related to spontaneous rupture of the lamella and receding of the contact area.

physics.flu-dyn↗

arXiv2020

Initial solidification dynamics of spreading droplets

When a droplet is brought in contact with an undercooled surface, it wets the substrate and solidifies at the same time. The interplay between the phase transition effects and the contact-line motion, leading to its arrest, remains poorly understood. Here we reveal the early solidification patterns and dynamics of spreading hexadecane droplets. Total internal reflection (TIR) imaging is employed to temporally and spatially resolve the early solidification behaviour. With this, we determine the conditions leading to the contact-line arrest. We quantify the overall nucleation behaviour, \textit{i.e.} the nucleation rate and the crystal growth speed, and show its sensitivity to the applied undercooling of the substrate. By combining the Johnson-Mehl-Avrami-Kolmogorov nucleation theory and scaling relations for the spreading, we can calculate the temporal evolution of the solid area fraction, which is in good agreement with our observations. We also show that for strong enough undercooling it is the rapid growth of the crystals which determines the eventual arrest of the spreading contact line.

cond-mat.soft↗

arXiv2020

Self-Similar Liquid Lens Coalescence

A basic feature of liquid drops is that they can merge upon contact to form a larger drop. In spite of its importance to various applications, drop coalescence on pre-wetted substrates has received little attention. Here, we experimentally and theoretically reveal the dynamics of drop coalescence on a thick layer of a low-viscosity liquid. It is shown that these so-called "liquid lenses" merge by the self-similar vertical growth of a bridge connecting the two lenses. Using a slender analysis, we derive similarity solutions corresponding to the viscous and inertial limits. Excellent agreement is found with the experiments without any adjustable parameters, capturing both the spatial and temporal structure of the flow during coalescence. Finally, we consider the crossover between the two regimes and show that all data of different lens viscosities collapse on a single curve capturing the full range of the coalescence dynamics.

physics.flu-dyn↗

arXiv2020

Fast-freezing kinetics inside a droplet impacting on a cold surface

Freezing or solidification of impacting droplets is omnipresent in nature and technology, be it a rain droplet falling on a supercooled surface, be it in inkjet printing where often molten wax is used, be it in added manufacturing or in metal production processes or in extreme ultraviolet lithography (EUV) for the chip production where molten tin is used to generate the EUV radiation. For many of these industrial applications, a detailed understanding of the solidification process is essential. Here, by adopting a totally new optical technique in the context of freezing, namely TIR (Total-Internal-Reflection), we elucidate the freezing kinetics during the solidification of a droplet while it impacts on an undercooled surface. We show for the first time that at sufficiently high undercooling a peculiar freezing morphology exists that involves sequential advection of frozen fronts from the centre of the droplet to its boundaries. This phenomenon is examined by combining elements of classical nucleation theory to the large scale hydrodynamics on the droplet scale, bringing together two subfields which traditionally have been quite separated. Furthermore, we report a peculiar self-peeling phenomenon of a frozen splat that is driven by the existence of a transient crystalline state during solidification.

cond-mat.soft↗

arXiv2019

Annihilation of Point Defect Pairs in Freely Suspended Liquid-Crystal Films

We study the annihilation of topological defect pairs in the quasi-twodimensional (2D) geometry of freely suspended smectic films. This elementary process is at the basis of all models describing the statistics of complex defect patterns. We prepare pairs with opposite topological charges and retrieve the interaction mechanisms from their trajectories. The square-root dependence of the defect separation on the time until annihilation and the asymmetry in propagation velocities of the opponents predicted by theory are confirmed. The importance of defect orientations is demonstrated. Trajectories are in general curved, depending on the mutual orientations (phase mismatch) of the defects and on the orientation of the pair respective to the far, undisturbed director. The experiments provide the basis for an adaption of the theoretical models to the real complexity of the annihilation.

cond-mat.soft↗

arXiv2019

Wrinkling of freely floating smectic films

We demonstrate spontaneous wrinkling as a transient dynamical pattern in thin freely floating smectic liquid-crystalline films. The peculiarity of such films is that, while flowing liquid-like in the film plane, they cannot quickly expand in the direction perpendicular to that plane. At short time scales they therefore behave in two dimensions like quasi-incompressible membranes. Such films can develop a transient undulation instability or form bulges in response to lateral compression. Optical experiments with freely floating bubbles on parabolic flights and in ground lab experiments are reported. The characteristic wavelengths of the wrinkles are in the submillimeter range. We demonstrate the dynamic nature of the pattern formation mechanism and develop a basic model for the wavelength selection and wrinkle orientation.

cond-mat.soft↗

arXiv2018

Marangoni flow in freely suspended liquid films

We demonstrate controlled material transport driven by temperature gradients in thin freely suspended smectic films. The films with submicrometer thicknesses and lateral extensions of several millimeters were studied in microgravity during suborbital rocket flights. In-plane temperature gradients cause two specific Marangoni effects, directed flow and convection patterns. At low gradients, practically thresholdless, flow transports material with a normal (negative) temperature coefficient of the surface tension, $dσ/dT<0$, from the hot to the cold film edge. That material accumulates at the cold film border. In materials with positive temperature coefficient, $dσ/dT>0$, the reverse transport from the cold to the hot edge is observed. We present a model that describes the effect quantitatively.

physics.flu-dyn↗

arXiv2017

Free Cooling of a Granular Gas in Three Dimensions

Granular gases as dilute ensembles of particles in random motion are not only at the basis of elementary structure-forming processes in the universe and involved in many industrial and natural phenomena, but also excellent models to study fundamental statistical dynamics. A vast number of theoretical and numerical investigations have dealt with this apparently simple non-equilibrium system. The essential difference to molecular gases is the energy dissipation in particle collisions, a subtle distinction with immense impact on their global dynamics. Its most striking manifestation is the so-called granular cooling, the gradual loss of mechanical energy in absence of external excitation. We report an experimental study of homogeneous cooling of three-dimensional (3D) granular gases in microgravity. Surprisingly, the asymptotic scaling $E(t)\propto t^{-2}$ obtained by Haff's minimal model [J. Fluid Mech. 134, 401 (1983)] proves to be robust, despite the violation of several of its central assumptions. The shape anisotropy of the grains influences the characteristic time of energy loss quantitatively, but not qualitatively. We compare kinetic energies in the individual degrees of freedom, and find a slight predominance of the translational motions. In addition, we detect a certain preference of the grains to align with their long axis in flight direction, a feature known from active matter or animal flocks, and the onset of clustering.

physics.flu-dyn↗

arXiv2017

Realization of hydrodynamic experiments on quasi-2D liquid crystal films in microgravity

Freely suspended films of smectic liquid crystals are unique examples of quasi two-dimensional fluids. Mechanically stable and with quantized thickness of the order of only a few molecular layers, smectic films are ideal systems for studying fundamental fluid physics, such as collective molecular ordering, defect and fluctuation phenomena, hydrodynamics, and nonequilibrium behavior in two dimensions (2D), including serving as models of complex biological membranes. Smectic films can be drawn across openings in planar supports resulting in thin, meniscus-bounded membranes, and can also be prepared as bubbles, either supported on an inflation tube or floating freely. The quantized layering renders smectic films uniquely useful in 2D fluid physics. The OASIS team has pursued a variety of ground-based and microgravity applications of thin liquid crystal films to fluid structure and hydrodynamic problems in 2D and quasi-2D systems. Parabolic flights and sounding rocket experiments were carried out in order to explore the shape evolution of free floating smectic bubbles, and to probe Marangoni effects in flat films. The dynamics of emulsions of smectic islands (thicker regions on thin background films) and of microdroplet inclusions in spherical films, as well as thermocapillary effects, were studied over extended periods within the OASIS (Observation and Analysis of Smectic Islands in Space) project on the International Space Station. We summarize the technical details of the OASIS hardware and give preliminary examples of key observations.

cond-mat.soft↗

arXiv2012

Shear induced alignment and dynamics of elongated granular particles

The alignment, ordering and rotation of elongated granular particles was studied in shear flow. The time evolution of the orientation of a large number of particles was monitored in laboratory experiments by particle tracking using optical imaging and x-ray computed tomography. The experiments were complemented by discrete element simulations. The particles develop an orientational order. In the steady state the time and ensemble averaged direction of the main axis of the particles encloses a small angle with the streamlines. This shear alignment angle is independent of the applied shear rate, and it decreases with increasing grain aspect ratio. At the grain level the steady state is characterized by a net rotation of the particles, as dictated by the shear flow. The distribution of particle rotational velocities was measured both in the steady state and also during the initial transients. The average rotation speed of particles with their long axis perpendicular to the shear alignment angle is larger, while shear aligned particles rotate slower. The ratio of this fast/slow rotation increases with particle aspect ratio. During the initial transient starting from an unaligned initial condition, particles having an orientation just beyond the shear alignment angle rotate opposite to the direction dictated by the shear flow.

cond-mat.soft↗