arXiv subjects

Klaus Halterman

Publications and source records attributed to Klaus Halterman.

At least 19 recordsLinked to original sources

arXiv2022

Controllable nonreciprocal optical response and handedness-switching in magnetized spin orbit coupled graphene

Starting from a low-energy effective Hamiltonian model, we theoretically calculate the dynamical optical conductivity and permittivity tensor of a magnetized graphene layer with Rashba spin orbit coupling (SOC). Our results reveal a transverse Hall conductivity correlated with the usual nonreciprocal longitudinal conductivity. Further analysis illustrates that for intermediate magnetization strengths, the relative magnitudes of the magnetization and SOC can be identified experimentally by two well-separated peaks in the dynamical optical response (both the longitudinal and transverse components) as a function of photon frequency. Moreover, the frequency dependent permittivity tensor is obtained for a wide range of chemical potentials and magnetization strengths. Employing experimentally realistic parameter values, we calculate the circular dichroism of a representative device consisting of magnetized spin orbit coupled graphene and a dielectric insulator layer, backed by a metallic plate. The results reveal that this device has different relative absorptivities for right-handed and left-handed circularly polarized electromagnetic waves. It is found that the magnetized spin orbit coupled graphene supports strong handedness-switchings, effectively controlled by varying the chemical potential and magnetization strength with respect to the SOC strength.

cond-mat.mes-hall↗

arXiv2021

Supercurrent Diode Effect, Spin Torques, and Robust Zero-Energy Peak in Planar Half-Metallic Trilayers

We consider a Josephson junction with ${\rm F_1 F_2 F_3}$ ferromagnetic trilayers in the ballistic regime, where the magnetization in each ferromagnet ${\rm F}_i (i=1,2,3)$, can have arbitrary orientations and magnetization strengths. The trilayers are sandwiched between two $s$-wave superconductors with a macroscopic phase difference $Δφ$. A broad range of magnetization strengths of the central $\rm F_2$ layer are considered, from an unpolarized normal metal (N) to a half-metallic phase, supporting only one spin species. Our results reveal that when the magnetization configuration in ${\rm F_1 F_2 F_3}$ has three orthogonal components, a supercurrent can flow at $Δφ=0$, and a strong second harmonic in the current-phase relation appears. Upon increasing the magnetization strength in the central ferromagnet layer up to the half-metallic limit, the self-biased current and second harmonic component become dramatically enhanced, and the critical supercurrent reaches its maximum value. The higher harmonics in the current-phase relations can be controlled by the relative magnetization orientations, with negligible current damping compared to the corresponding ${\rm F_1 N F_3}$ counterparts. For a broad range of exchange field strengths in the central ferromagnet ${\rm F}_2$, the ground state of the system can be tuned to an arbitrary phase difference $φ_0$ by rotating the magnetization in the outer ferromagnet $\rm F_3$. For intermediate exchange field strengths in ${\rm F}_2$, a $φ_0$ state can arise that creates a superconducting diode effect, whereby $Δφ$ can be tuned to create a one-way dissipationless current flow. The density of states demonstrates the emergence of zero energy peaks for the mutually orthogonal magnetization configurations, which is strongest in the half-metallic phase.

cond-mat.supr-con↗

arXiv2021

Comparison of Optical Response from DFT Random Phase Approximation and Low-Energy Effective Model: Strained Phosphorene

The engineering of the optical response of materials is a paradigm that demands microscopic-level accuracy and reliable predictive theoretical tools. Here we compare and contrast the dispersive permittivity tensor, using both a low-energy effective model and density functional theory (DFT). As a representative material, phosphorene subject to strain is considered. Employing a low-energy model Hamiltonian with a Green's function current-current correlation function, we compute the dynamical optical conductivity and its associated permittivity tensor. For the DFT approach, first-principles calculations make use of the first-order random-phase approximation. Our results reveal that although the two models are generally in agreement within the low-strain and low-frequency regime, the intricate features associated with the fundamental physical properties of the system and optoelectronic device implementation such as band gap, Drude absorption response, vanishing real part, absorptivity, and sign of permittivity over the frequency range show significant discrepancies. Our results suggest that the random-phase approximation employed in widely used DFT packages should be revisited and improved to be able to predict these fundamental electronic characteristics of a given material with confidence. Furthermore, employing the permittivity results from both models, we uncover the pivotal role that phosphorene can play in optoelectronics devices to facilitate highly programable perfect absorption of electromagnetic waves by manipulating the chemical potential and exerting strain and illustrate how reliable predictions for the dielectric response of a given material are crucial to precise device design.

cond-mat.mtrl-sci↗

arXiv2021

Supergap and subgap enhanced currents in asymmetric {S_1FS_2} Josephson junctions

We have theoretically studied the supercurrent profiles in three-dimensional normal metal and ferromagnetic Josephson configurations, where the magnitude of the superconducting gaps in the superconducting leads are unequal, i.e., $Δ_1\neq Δ_2$, creating asymmetric $S_1NS_2$ and $S_1FS_2$ systems. Our results reveal that by increasing the ratio of the superconducting gaps $Δ_2/Δ_1$, the critical supercurrent in a ballistic $S_1NS_2$ system can be enhanced by more than $100\%$, and reaches a saturation point, or decays away, depending on the junction thickness, magnetization strength, and chemical potential. The total critical current in a diffusive $S_1NS_2$ system was found to be enhanced by more than $50\%$ parabolically, and reaches saturation by increasing one of the superconducting gaps. In a uniform ferromagnetic junction, the supercurrent undergoes reversal by increasing $Δ_2/Δ_1>1$. Through decomposing the total supercurrent into its supergap and subgap components, our results illustrate their crucial relative contributions to the Josephson current flow. It was found that the competition of subgap and supergap currents in a $S_1FS_2$ junction results in the emergence of second harmonics in the current-phase relation. In contrast to a diffusive asymmetric Josephson configuration, the behavior of the supercurrent in a ballistic system with $Δ_2/Δ_1=1$ can be properly described by the subgap current component only, in a wide range of parameter sets, including Fermi level mismatch, magnetization strength, and junction thickness. Interestingly, when $Δ_2/Δ_1>1$, our results have found multiple parameter sets where the total supercurrent is driven by the supergap component. Therefore, our comprehensive study highlights the importance of subgap and supergap supercurrent components in both the ballistic and diffusive regimes.

cond-mat.supr-con↗

arXiv2020

Strain-Engineered Widely-Tunable Perfect Absorption Angle in Black Phosphorus from First-Principles

Using the density functional theory of electronic structure, we compute the anisotropic dielectric response of bulk black phosphorus subject to strain. Employing the obtained permittivity tensor, we solve Maxwell's equations and study the electromagnetic response of a layered structure comprising a film of black phosphorus stacked on a metallic substrate. Our results reveal that a small compressive or tensile strain, $\sim 4\%$, exerted either perpendicular or in the plane to the black phosphorus growth direction, efficiently controls the epsilon-near-zero response, and allows a perfect absorption tuning from low-angle of the incident beam $θ=0^\circ$ to high values $θ\approx 90^\circ$ while switching the energy flow direction. Incorporating a spatially inhomogeneous strain model, we also find that for certain thicknesses of the black phosphorus, near-perfect absorption can be achieved through controlled variations of the in-plane strain. These findings can serve as guidelines for designing largely tunable perfect electromagnetic wave absorber devices.

cond-mat.mtrl-sci↗

arXiv2020

Waveguide Modes in Weyl Semimetals with Tilted Dirac Cones

We theoretically study unattenuated electromagnetic guided wave modes in centrosymmetric Weyl semimetal layered systems. By solving Maxwell's equations for the electromagnetic fields and using the appropriate boundary conditions, we derive dispersion relations for propagating modes in a finite-sized Weyl semimetal. Our findings reveal that for ultrathin structures, and proper Weyl cones tilts, extremely localized guided waves can propagate along the semimetal interface over a certain range of frequencies. This follows from the anisotropic nature of the semimetal where the diagonal components of the permittivity can exhibit a tunable epsilon-near-zero response. From the dispersion diagrams, we determine experimentally accessible regimes that lead to high energy-density confinement in the Weyl semimetal layer. Furthermore, we show that the net system power can vanish all together, depending on the Weyl cone tilt and frequency of the electromagnetic wave.These effects are seen in the energy transport velocity, which demonstrates a substantial slowdown in the propagation of electromagnetic energy near critical points of the dispersion diagrams. Our results can provide guidelines in designing Weyl semimetal waveguides that can offer efficient control in the velocity and direction of energy flow.

physics.optics↗

arXiv2020

Evolution of Pair Correlation Symmetries and Supercurrent Reversal in Tilted Weyl Semimetals

We study the effective symmetry profiles of superconducting pair correlations and the flow of charge supercurrent in ballistic Weyl semimetal systems with a tilted dispersion relation. Utilizing a microscopic method in the ballistic regime and starting from both opposite-pseudospin and equal-pseudospin phonon-mediated opposite-spin electron-electron couplings, we calculate the anomalous Green's function to study various superconducting pair correlations that Weyl semimetal systems may develop. The momentum-space profile reveals that by properly manipulating the parameters of Weyl semimetal systems, including the tilting parameter, the effective symmetry class of even-parity s-wave (odd-parity p-wave) superconducting correlations can be converted into a d-wave (f-wave) symmetry class that consists of equal-pseudospin and opposite-pseudospin channels. We also find that the supercurrent in a ballistic Weyl Josephson junction can be made to vanish or switch directions, depending on the tilt of the Weyl cones, in addition to the relevant parameters characterizing the Weyl semimetal and junction. We show that inversion symmetry breaking terms introduce transitions that result in the appearance of self-biased current at zero difference between the macroscopic phases of the superconducting segments, creating a phi0 Josephson state. Weyl semimetal systems are shown to offer several experimentally tunable parameters to control the induction of higher harmonics into the current phase relations.

cond-mat.supr-con↗

arXiv2018

Induced Energy Gap in Finite-Sized Superconductor/Ferromagnet Hybrids

We theoretically study self-consistent proximity effects in finite-sized systems consisting of ferromagnet ($\rm F$) layers coupled to an $s$-wave superconductor ($\rm S$). We consider both $\rm SF_1F_2$ and $\rm SH$ nanostructures, where the $\rm F_1 F_2$ bilayers are uniformly magnetized, and the ferromagnetic $\rm H$ layer possesses a helical magnetization profile. We find that when the $\rm F_1 F_2$ layers are weakly ferromagnetic, a hard gap can emerge when the relative magnetization directions are rotated from parallel to antiparallel. Moreover, the gap is most prominent when the thicknesses of $\rm F_1$ and $\rm F_2$ satisfy $\rm d_{F1}\leq d_{F2}$, respectively. For the $\rm SH$ configuration, increasing the spatial rotation period of the exchange field can enhance the induced hard gap. Our investigations reveal that the origin of these findings can be correlated with the propagation of quasiparticles with wavevectors directed along the interface. To further clarify the source of the induced energy gap, we also examine the spatial and energy resolved density of states, as well as the spin-singlet, and spin-triplet superconducting correlations, using experimentally accessible parameter values. Our findings can be beneficial for designing magnetic hybrid structures where a tunable superconducting hard gap is needed.

cond-mat.supr-con↗

arXiv2018

Epsilon-Near-Zero Response and Tunable Perfect Absorption in Weyl Semimetals

We theoretically study the electromagnetic response of type-I and type-II centrosymmetric Weyl semimetals. We derive an anisotropic permittivity tensor with off-diagonal elements to describe such gyrotropic media. Our findings reveal that for appropriate Weyl cones tilts, the real part of the transverse component of the permittivity can exhibit an epsilon-near-zero response. The tilt parameter can also control the amount of loss in the medium, ranging from lossless to dissipative when transitioning from type-I to type-II. Similarly, by tuning either the frequency of the electromagnetic field or the chemical potential in the system, an epsilon-near-zero response can appear as the permittivity of the Weyl semimetal transitions between positive and negative values. Employing the obtained permittivity tensor, we consider a setup where the Weyl semimetal is deposited on a perfect conductive substrate and study the refection and absorption characteristics of this layered configuration. We show that by choosing the proper geometrical and material parameters, devices can be created that perfectly absorb electromagnetic energy over a wide angular range of incident electromagnetic waves.

cond-mat.str-el↗

arXiv2018

Spin Transport in Half-Metallic Ferromagnet-Superconductor Junctions

We investigate the charge and spin transport in half-metallic ferromagnet ($F$) and superconductor ($S$) nanojunctions. We utilize a self-consistent microscopic method that can accommodate the broad range of energy scales present, and ensures proximity effects that account for the interactions at the interfaces are accurately determined. Two experimentally relevant half-metallic junction types are considered: The first is a $F_1 F_2 S$ structure, where a half-metallic ferromagnet $F_1$ adjoins a weaker conventional ferromagnet $F_2$. The current is injected through the $F_1$ layer by means of an applied bias voltage. The second configuration involves a $S F_1 F_2 F_3 S$ Josephson junction whereby a phase difference $Δφ$ between the two superconducting electrodes generates the supercurrent flow. In this case, the central half-metallic $F_2$ layer is surrounded by two weak ferromagnets $F_1$ and $F_3$. By placing a ferromagnet with a weak exchange field adjacent to an $S$ layer, we are able to optimize the conversion process in which opposite-spin triplet pairs are converted into equal-spin triplet pairs that propagate deep into the half-metallic regions in both junction types. For the tunnel junctions, we study the bias-induced local magnetization, spin currents, and spin transfer torques for various orientations of the relative magnetization angle $θ$ in the $F$ layers. We find that the bias-induced equal-spin triplet pairs are maximized in the half-metal for $θ\approx90^\circ$ and as part of the conversion process, are anticorrelated with the opposite-spin pairs. We show that the charge current density is maximized, corresponding to the occurrence of a large amplitude of equal-spin triplet pairs, when the exchange interaction of the weak ferromagnet is about $0.1E_F.$

cond-mat.supr-con↗

arXiv2018

Half-Metallic Superconducting Triplet Spin MultiValves

We study spin switching effects in finite-size superconducting multivalve structures. We examine $\rm F_1F_2SF_3$ and $\rm F_1F_2SF_3F_4$ hybrids where a singlet superconductor ($\rm S$) layer is sandwiched among ferromagnet ($\rm F$) layers with differing thicknesses and magnetization orientations. Our results reveal a considerable number of experimentally viable spin valve configurations that lead to on-off switching of the superconducting state. For $\rm S$ widths on the order of the superconducting coherence length $ξ_0$, non-collinear magnetization orientations in adjacent $\rm F$ layers with multiple spin-axes leads to a rich variety of triplet spin-valve effects. Motivated by recent experiments, we focus on samples where magnetizations in the $\rm F_1$ and $\rm F_4$ layers exist in a fully spin-polarized half metallic phase, and calculate the superconducting transition temperature, spatially and energy resolved density of states, and the spin-singlet and spin-triplet superconducting correlations. Our findings demonstrate that superconductivity in these devices can be completely switched on or off over a wide range of magnetization misalignment angles due to the generation of equal-spin and opposite-spin triplet pairings.

cond-mat.supr-con↗

arXiv2017

Magnetization-control and transfer of spin-polarized Cooper pairs into a half-metal manganite

The pairing state and critical temperature (T$_c$) of a thin s-wave superconductor (S) on two or more ferromagnets (F) are controllable through the magnetization-alignment of the F layers. Magnetization misalignment can lead to spin-polarized triplet pair creation, and since such triplets are compatible with spin-polarized materials they are able to pass deeply into the F layers and so, cause a decrease in T$_c$. Various experiments on S/F$_1$/F$_2$ "triplet spin-valves" have been performed with the most pronounced suppression of T$_c$ reported in devices containing the half-metal ferromagnet (HMF) CrO$_2$ (F$_2$) albeit using out-of-plane magnetic fields to tune magnetic non-collinearity [Singh et al., Phys. Rev. X 5, 021019 (2015)]. Routine transfer of spin-polarized triplets to HMFs is a major goal for superconducting spintronics so as to maximize triplet-state spin-polarization. However, CrO$_2$ is chemically unstable and out-of-plane fields are undesirable for superconductivity. Here, we demonstrate magnetization-tuneable pair conversion and transfer of spin-polarized triplet pairs to the chemically stable mixed valence manganite La$_{2/3}$Ca$_{1/3}$MnO$_3$ in a pseudo spin-valve device using in-plane magnetic fields. The results match microscopic theory and offer full control over the pairing state.

cond-mat.supr-con↗

arXiv2016

Dynamical tuning between nearly perfect reflection, absorption, and transmission of light via graphene/dielectric structures

Exerting well-defined control over the reflection $(R)$, absorption $(A)$, and transmission $(T)$ of electromagnetic waves is a key objective in quantum optics. To this end, one often utilizes hybrid structures comprised of elements with different optical properties in order to achieve features such as high $R$ or high $A$ for incident light. A desirable goal would be the possibility to tune between all three regimes of nearly perfect reflection, absorption, and transmission within the same device, thus swapping between the cases $R\to 1$, $A\to1$, and $T\to1$ dynamically. We here show that a dielectric interfaced with a graphene layer on each side allows for precisely this: by tuning only the Fermi level of graphene, all three regimes can be reached in the THz regime and below. Moreover, we show that the inclusion of cylindrical defects in the system offers a different type of control of the scattering of electromagnetic waves by means of the graphene layers.

physics.optics↗

arXiv2016

Pure Odd Frequency Superconductivity at the Cores of Proximity Vortices

After more than a decade, direct observation of the odd frequency triplet pairing state in super- conducting hybrid structures remains elusive. We propose an experimentally feasible setup that can unambiguously reveal the zero energy peak due to proximity-induced equal spin superconducting triplet correlations. We theoretically investigate a two dimensional Josephson junction in the diffu- sive regime. The nanostructure consists of a normal metal sandwiched between two ferromagnetic layers with spiral magnetization patterns. By applying an external magnetic field perpendicular to the junction plane, vortices nucleate in the normal metal. The calculated energy and spatially resolved density of states, along with the pair potential, reveal that remarkably, only triplet Cooper pairs survive in the vortex cores. These isolated odd frequency triplet correlations result in well defined zero energy peaks in the local density of states that can be identified through tunneling spectroscopy experiments. Moreover, the diffusive regime considered here rules out the possibility of Andreev bound states in the vortex core as contributors to the zero energy peaks.

cond-mat.str-el↗

arXiv2016

Graphene-based extremely wide-angle tunable metamaterial absorber

We investigate the absorption properties of graphene-based anisotropic metamaterial structures where the metamaterial layer possesses an electromagnetic response corresponding to a near-zero permittivity. We find that through analytical and numerical studies, near perfect absorption arises over an unusually broad range of beam incidence angles. Due to the presence of graphene, the absorption is tunable via a gate voltage, providing dynamic control of the energy transmission. We show that this strongly enhanced absorption arises due to a coupling between light and a fast wave-mode propagating along the graphene/metamaterial hybrid.

physics.optics↗

arXiv2016

Half-Metallic Superconducting Triplet Spin Valve

We theoretically study a finite size $SF_1NF_2$ spin valve, where a normal metal ($N$) insert separates a thin standard ferromagnet ($F_1$) and a thick half-metallic ferromagnet ($F_2$). For sufficiently thin superconductor ($S$) widths close to the coherence length $ξ_0$, we find that changes to the relative magnetization orientations in the ferromagnets can result in substantial variations in the transition temperature $T_c$, consistent with experiment [Singh et al., Phys. Rev. X 5, 021019 (2015)]. Our results demonstrate that, in good agreement with the experiment, the variations are largest in the case where $F_2$ is in a half-metallic phase and thus supports only one spin direction. To pinpoint the origins of this strong spin-valve effect, both the equal-spin $f_1$ and opposite-spin $f_0$ triplet correlations are calculated using a self-consistent microscopic technique. We find that when the magnetization in $F_1$ is tilted slightly out-of-plane, the $f_1$ component can be the dominant triplet component in the superconductor. The coupling between the two ferromagnets is discussed in terms of the underlying spin currents present in the system. We go further and show that the zero energy peaks of the local density of states probed on the $S$ side of the valve can be another signature of the presence of superconducting triplet correlations. Our findings reveal that for sufficiently thin $S$ layers, the zero energy peak at the $S$ side can be larger than its counterpart in the $F_2$ side.

cond-mat.supr-con↗

arXiv2015

Zero Energy Peak and Triplet Correlations in Nanoscale SFF Spin-Valves

Using a self-consistent Bogoliubov-de Gennes approach, we theoretically study the proximity-induced density of states (DOS) in clean SFF spin-valves with noncollinear exchange fields. Our results clearly demonstrate a direct correlation between the presence of a zero energy peak (ZEP) in the DOS spectrum and the persistence of spin-1 triplet pair correlations. By systematically varying the geometrical and material parameters governing the spin-valve, we point out to experimentally optimal system configurations where the ZEPs are most pronounced, and which can be effectively probed via scanning tunneling microscopy. We complement these findings in the ballistic regime by employing the Usadel formalism in the full proximity limit to investigate their diffusive SFF counterparts. We determine the optimal normalized ferromagnetic layer thicknesses which result in the largest ZEPs. Our results can serve as guidelines in designing samples for future experiments.

cond-mat.str-el↗

arXiv2015

Charge and Spin Currents in Ferromagnetic Josephson junctions

We determine, using a self consistent method, the charge and spin currents in ballistic Josephson junctions consisting of ferromagnetic ($F$) layers sandwiched between superconducting ($S$) electrodes ($SFS$-type junctions). When there are two $F$ layers, we also consider the experimentally relevant configuration where a normal ($N$) nonmagnetic spacer layer separates them. We study the current-phase relationships as functions of geometrical parameters that are accessible experimentally including the angles that characterize the relative orientation of the magnetization in the $F$ layers. Our self-consistent method ensures that the proper charge conservation laws are satisfied. As we vary the phase difference $Δφ$ between the two outer $S$ electrodes, multiple harmonics in the current phase relations emerge, their extent depends on the interface scattering strength and the relative $F$ layer widths and magnetization orientations. By manipulating the relative $F$ layer magnetization orientations, we find that the charge supercurrent can reverse directions or vanish altogether. These findings are discussed in the context of the generation and long-range nature of triplet pair correlation. We also investigate the spin currents and associated spin transfer torques throughout the junction. For noncollinear relative magnetizations, the non-conserved spin currents in a given $F$ region gives rise to net torques that can switch directions at particular magnetic configurations or $Δφ$ values. The details of the spin current behavior are shown to depend strongly on the degree of magnetic inhomogeneity in the system.

cond-mat.supr-con↗