arXiv subjects

Klaus Mølmer

Publications and source records attributed to Klaus Mølmer.

At least 37 records · Page 2Linked to original sources

arXiv2025

Stochastic Schrödinger equation for a homodyne measurement setup of strongly correlated systems

Starting from an experimentally feasible atomic setup, we derive a stochastic Schrödinger equation that captures the homodyne detection record of a strongly interacting system. Applying the rotating wave approximation to the linear atom-light coupling, we arrive at a reduced equation formulated solely in terms of atomic operators. In the appropriate limit, this equation converges to that of Gaussian continuous quantum measurement -- revealing that the complexities of real-world detection can, under certain conditions, echo the elegance of idealized theory. To illustrate the utility of this framework, we numerically study the Bose-Hubbard model under continuous observation, showing that time-domain analysis of the measurement signal uncovers rich dynamical features, including quantum jumps, that are obscured in ensemble-averaged spectral data.

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arXiv2025

Superradiant Echoes Induced by Multiple Re-phasing of NV Spin Sub-ensembles Grating at Room Temperature

In this Letter, we propose that superradiant echoes can be achieved at room temperature by applying a laser illumination and a microwave Hahn echo sequence to a diamond with a high concentration of nitrogen-vacancy (NV) centers placed in a dielectric microwave cavity. We identify that the combined action of two microwave driving pulses and a free evolution imprints a phase grating among NV spin sub-ensembles in frequency space, and multiple re-phasing of the grated spin sub-ensembles leads to multiple superradiant echoes through a collective coupling with the cavity. Furthermore, we show that the superradiant echoes can be actively tailored with the microwave pulses and the laser illumination by modifying the grating parameters, and the multiple re-phasing dynamics is analogous to the one leading to superradiant beats in optical clock system. In the future, the spin sub-ensembles grating and the resulting echoes can be further optimized with dynamical decoupling, which might pave the way for applications in quantum sensing.

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arXiv2025

Interactions in Quantum Networks with Pulse Propagation Delays

The finite speed of light of pulses implies propagation delays between the generation of light, the interaction with different elements along its path and the final detection at the output of networks and interferometers. We show that it is possible to take these delays into account with a theoretical method which evades quantization of the full continuum of field modes. We illustrate the use of this method by analyzing Ramsey excitation of an atom by a split and delayed quantum pulse.

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arXiv2025

Complementary Collective Spin Descriptions of Superradiant Ramsey Spectroscopy

A recent experiment demonstrated delayed superradiance from strontium-88 atoms, which are coupled to a longitudinal mode of a cavity while being excited by laser pulses propagating along a transversal direction [Nat. Commun. 15, 1084 (2024)]. A coherent picture of the atomic ensemble dynamics in this experiment requires complementary representations of the external driving dynamics and the superradiant dynamics. To complement previous analyses, we introduce these representations by considering in-phase and out-of-phase superpositions of transverse collective spin components of two atomic sub-ensembles, and analyze the dynamics with the corresponding collective Dicke states and Bloch vectors. This approach also explains Ramsey spectroscopy experiments with the ensemble, and it may be employed to explore other phenomena, such as weak-to-strong coupling phase transitions and triggered superradiance.

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arXiv2025

Theoretical framework for enhancing or enabling cooling of a mechanical resonator via the anti-Stokes or Stokes interaction and zero-photon detection

We develop a theoretical framework to describe how zero-photon detection may be utilized to enhance laser cooling via the anti-Stokes interaction and, somewhat surprisingly, enable cooling via the Stokes interaction commonly associated with heating. Our description includes both pulsed and continuous measurements as well as optical detection efficiency and open-system dynamics. For both cases, we discuss how the cooling depends on the system parameters such as detection efficiency and optomechanical cooperativity, and we study the continuous-measurement-induced dynamics, contrasting to single-photon detection events. For the Stokes case, we explore the interplay between cooling and heating via optomechanical parametric amplification, and we find the efficiency required to cool a mechanical oscillator via zero-photon detection. This work serves as a companion article to the recent experiment [E. A. Cryer-Jenkins, K. D. Major, et al., arXiv:2408.01734 (2024)], which demonstrated enhanced laser cooling of a mechanical oscillator via zero-photon detection on the anti-Stokes signal. The framework developed here provides new approaches for cooling mechanical resonators that can be applied to a wide range of areas including nonclassical state preparation, quantum thermodynamics, and avoiding the often unwanted heating effects of parametric amplification.

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arXiv2025

Enhanced Laser Cooling of a Mechanical Resonator via Zero-Photon Detection

Throughout quantum science and technology, measurement is used as a powerful resource for nonlinear operations and quantum state engineering. In particular, single-photon detection is commonly employed for quantum-information applications and tests of fundamental physics. By contrast, and perhaps counter-intuitively, measurement of the absence of photons also provides useful information, and offers significant potential for a wide range of new experimental directions. Here, we propose and experimentally demonstrate cooling of a mechanical resonator below its laser-cooled mechanical occupation via zero-photon detection on the anti-Stokes scattered optical field and verify this cooling through heterodyne measurements. Our measurements are well captured by a stochastic master equation and the techniques introduced here open new avenues for cooling, quantum thermodynamics, quantum state engineering, and quantum measurement and control.

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arXiv2025

Probing Hilbert Space Fragmentation with Strongly Interacting Rydberg Atoms

Hilbert space fragmentation provides a mechanism to break ergodicity in closed many-body systems. Here, we propose a feasible scheme to explore this exotic paradigm on a Rydberg quantum simulator. We show that the Rydberg Ising model in the large detuning regime can be mapped to a generalized folded XXZ model featuring a strongly fragmented Hilbert space. The emergent Hamiltonian, however, displays distinct time scales for the transport of a magnon and a hole excitation. This interesting property facilitates a continuous tuning of the Krylov-subspace ergodicity, from the integrable regime, to the Krylov-restricted thermal phase, and eventually to the statistical bubble localization region. By further introducing nonlocal interactions, we find that both the fragmentation behavior and the ergodicity of the Krylov subspace can be significantly enriched. We also examine the role of atomic position disorders and identify a symmetry-selective many-body localization transition. We demonstrate that these phenomena manifest themselves in quench dynamics, which can be readily probed in state-of-the-art Rydberg array setups.

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arXiv2025

Boundary Time Crystals Induced by Local Dissipation and Long-Range Interactions

Driven-dissipative many-body system supports nontrivial quantum phases absent in equilibrium. As a prominent example, the interplay between coherent driving and collective dissipation can lead to a dynamical quantum phase that spontaneously breaks time-translation symmetry. This so-called boundary time crystal (BTC) is fragile in the presence of local dissipation, which can easily relax the system to a stationary state. In this work, we demonstrate a robust BTC that is intrinsically induced by local dissipation. We provide extensive numerical evidences to support existence of the BTC and study its behaviors in different regimes. In particular, with decreasing interaction range, we identify a transition from classical limit cycles to quantum BTCs featuring sizable spatial correlations. Our studies significantly broaden the scope of nonequilibrium phases and shed new light on experimental search for dynamical quantum matter.

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arXiv2024

Censorship of Quantum Resources in Quantum Networks

We may soon see agencies offering public access to quantum communication networks. In such networks it may be a feature that certain resources are available only to priority users or at a higher user fee, as governed by a protective agency overseeing the communication in the network. If the agency wants to restrict the general users to communicate by transmitting states that we categorize as free states of a quantum resource theory (QRT), it may employ resource-destroying (RD) channels that do not affect the free states. Such channels, however, only exist for the simplest of QRTs, putting fundamental limitations on how quantum resources can be regulated. In this work, we go beyond the present limitation by devising a nonlinear censorship protocol which makes use of classical information about the transmitted state. We study the requirement disabling malicious users from breaking the censorship. The protocol can establish an unbreakable censorship of imaginarity and entanglement, while no such censorship can be made for quantum discord and Bell nonlocality.

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arXiv2024

Subtraction and Addition of Propagating Photons by Two-Level Emitters

Coherent manipulation of quantum states of light is key to photonic quantum information processing. In this Letter, we show that a passive two-level nonlinearity suffices to implement non-Gaussian quantum operations on propagating field modes. In particular, the collective light-matter interaction can efficiently extract a single photon from a multi-photon input wave packet to an orthogonal temporal mode. We accurately describe the single-photon subtraction process by elements of an intuitive quantum-trajectory model. By employing this process, quantum information protocols gain orders of magnitude improved efficiency over heralded schemes with linear optics. The reverse process can be used to add photons one-by-one to a single wave-packet mode and compose arbitrarily large Fock states with a finite total success probability $>96.7\%$.

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arXiv2024

Characterization of the multimode nature of single-photon sources based on spontaneous parametric down conversion

Single-photon sources are necessary components for many prospective quantum technologies. One candidate for a single-photon source is spontaneous parametric down conversion combined with a heralding photon detection. The heralded light pulse from such a source, is typically treated as single-mode, this treatment, however, is incomplete. We develop a full multimode description based on the exact Bogoliubov treatment of the down conversion process. We then provide a perturbative and effective treatment, which illustrates the most important physical mechanisms and permits analytical estimates of the success probability and purity of single-photon states under practical heralding conditions, both without relying on the precise detection time of the heralding photon and when accepting photons only in a narrow window around the time of the detection. This permits us to characterize the emitted light under three different assumptions for the pump pulse. For spontaneous parametric down conversion with a very short pump pulse, we find the single-mode description to be accurate, while for longer pump pulses and continuous pumping, a multimode description is necessary. Our findings can be used to guide the design of quantum information protocols based on heralded single-photon sources, as their performance may depend on the multimode nature of the sources.

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arXiv2024

Superradiance from Nitrogen Vacancy Centers Coupled to An Ultranarrow Optical Cavity

Nitrogen-vacancy (NV) centers in diamond have been successfully coupled to various optical structures to enhance their radiation by the Purcell effect. The participation of many NV centers in these studies may naturally lead to cooperative emission and superradiance, and our recent experimental study with a diamond membrane in a fiber-based ultra-narrow optical cavity demonstrated nonlinear radiation power and fast photon bunching which are signatures of such collective effects. In this theoretical article, we go beyond the simple model used in the previous study to address more phenomena, such as the appearance of bunching shoulders in the second-order correlation function, Rabi splitting in the steady-state spectrum, and population dynamics on excited Dicke states, which for moderate pumping explains the observed collective effects. Overall, our results can guide further experiments with NV centers, and they are also relevant for other solid-state color centers, such as silicon-vacancy centers in diamond and silicon carbide, boron-vacancy centers and carbon-related centers in hexagonal boron-nitride.

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arXiv2024

Chiral Quantum-Optical Elements for Waveguide-QED with Sub-wavelength Rydberg-Atom Arrays

We describe an approach to achieve near-perfect unidirectional light-matter coupling to an effective quantum emitter that is formed by a subwavelength array of atoms in the Rydberg-blockade regime. The nonlinear reflection and transmission of such two-dimensional superatoms are exploited in different interferometric setups for the deterministic generation of tunable single photons and entangling two-photon operations with high fidelities, $\mathcal{F}\gtrsim0.999$. The described setup can function as a versatile nonlinear optical element in a free-space photonic quantum network with simple linear elements and without the need of additional mode confinement, optical resonators, or optical isolators.

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arXiv2024

Jaynes-Cummings interaction with a traveling light pulse

The Jaynes-Cummings model provides a simple and accurate description of the interaction between a two-level quantum emitter and a single mode of quantum radiation. Due to the multimode continuum of eigenmodes in free space and in waveguides, the Jaynes-Cummings model should not be expected to properly describe the interaction between an emitter and a traveling pulse of quantum radiation. In this article, we review a cascaded quantum system approach that accurately describes the interaction of a quantum system with an incident quantum pulse of radiation. This approach leads to different formulations of the theory, each of a similar structure as the Jaynes-Cummings model but with important modifications.

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arXiv2024

Exact Numerical Solution of Stochastic Master Equations for Conditional Spin Squeezing

Stochastic master equations are often used to describe conditional spin squeezing of atomic ensemble, but are limited so far to the systems with few atoms due to the exponentially increased Hilbert space. In this article, we present an exact numerical solution of these equations for systems with identical atoms by mapping identical density matrix elements to a single quantity characterized by collective quantum numbers, and apply it to the system with hundred atoms in a bad cavity subject to a homodyne detection. We demonstrate that the spin squeezing can be vividly illustrated by the Gaussian-like distribution of the collective density matrix elements, and we examine the influence of the probe field strength and polarization, the detection efficiency, the spontaneous emission rate and the number of atoms. Our exact approach can play an important role in gauging the approximate approaches applied for systems with more atoms, such as Gaussian-state formalism and stochastic mean-field approach, and it permits also exploration of entanglement effects beyond these approaches.

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arXiv2024

Continuous field tracking with machine learning and steady state spin squeezing

Entanglement plays a crucial role in proposals for quantum metrology, yet demonstrating quantum enhancement in sensing with sustained spin entanglement remains a challenging endeavor. Here, we combine optical pumping and continuous quantum nondemolition measurements to achieve a sustained spin squeezed state with $\bm{4 \times 10^{10}}$ hot atoms. A metrologically relevant steady state squeezing of $\bm{-3.23 \pm 0.24}$ dB using prediction and retrodiction is maintained for about one day. We employ the system to track different types of continuous time-fluctuating magnetic fields, where we construct deep learning models to decode the measurement records from the optical signals. Quantum enhancement due to the steady spin squeezing is verified in our atomic magnetometer. These results represent important progress towards applying long-lived quantum entanglement resources in realistic settings.

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arXiv2023

Parametric Amplification of a Quantum Pulse

Creating and manipulating quantum states of light requires nonlinear interactions, but while nonlinear optics is inherently multi-mode, quantum optical analyses are often done with single-mode approximations. We present a multi-mode theory for the transformation of a quantum pulse by Hamiltonians that are quadratic in the field creation and annihilation operators. Our theory describes nonlinear processes, such as parametric amplification and squeezing, as well as all linear processes, such as dispersion and beam splitting. We show that a single input pulse feeds only two distinct output modes and, for certain quantum states, just one. Our theory provides the quantum states in the output modes, which are crucial for the application of pulses in quantum optics and quantum information.

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arXiv2023

Cavity-mediated collective emission from few emitters in a diamond membrane

When an ensemble of quantum emitters couples to a common radiation field, their polarizations can synchronize and a collective emission termed superfluorescence can occur. Entering this regime in a free-space setting requires a large number of emitters with a high spatial density as well as coherent optical transitions with small inhomogeneity. Here we show that by coupling nitrogen-vacancy (NV) centers in a diamond membrane to a high-finesse microcavity, also few, incoherent, inhomogeneous, and spatially separated emitters - as are typical for solid state systems - can enter the regime of collective emission. We observe a super-linear power dependence of the emission rate as a hallmark of collective emission. Furthermore, we find simultaneous photon bunching and antibunching on different timescales in the second-order auto-correlation function, revealing cavity-induced interference in the quantized emission from about fifteen emitters. We develop theoretical models for mesoscopic emitter numbers to analyze the behavior in the Dicke state basis and find that the population of collective states together with cavity enhancement and filtering can explain the observations. Such a system has prospects for the generation of multi-photon quantum states, and for the preparation of entanglement in few-emitter systems.

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