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Klaus Mølmer

Publications and source records attributed to Klaus Mølmer.

At least 73 records · Page 4Linked to original sources

Free-Fermion Multiply Excited Eigenstates and Their Experimental Signatures in 1D Arrays of Two-Level Atoms

One-dimensional (1D) subwavelength atom arrays display multiply excited subradiant eigenstates which are reminiscent of free fermions. So far, these states have been associated with subradiant states with decay rates $\propto N^{-3}$, with N the number of atoms, which fundamentally prevents detection of their fermionic features by optical means. In this Letter, we show that free-fermion states generally appear whenever the band of singly excited states has a quadratic dispersion relation at the band edge and, hence, may also be obtained with radiant and even superradiant states. 1D arrays have free-fermion multiply excited eigenstates that are typically either subradiant or (super)radiant, and we show that a simple transformation acts between the two families. Based on this correspondence, we propose different means for their preparation and analyze their experimental signature in optical detection.

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Gaussian theory for estimating fluctuating perturbations with back action evasive oscillator variables

We apply a Gaussian state formalism to track fluctuating perturbations that act on the position and momentum quadrature variables of a harmonic oscillator. Following a seminal proposal by Tsang and Caves [Phys. Rev. Lett. 105, 123601 (2010)], Einstein-Podolsky-Rosen correlations with the quadrature variables of an ancillary harmonic oscillator are leveraged to significantly improve the estimates as relevant sensor variables can be arbitrarily squeezed while evading adverse effects from the conjugate, anti-squeezed variables. Our real-time analysis of the continuous monitoring of the system employs a hybrid quantum-classical description of the quantum probe and the unknown classical perturbations, and it provides a general formalism to establish the achievements of the sensing scheme and how they depend on different parameters.

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Deterministic Photon Sorting in Waveguide QED Systems

Sorting quantum fields into different modes according to their Fock-space quantum numbers is a highly desirable quantum operation. In this Letter, we show that a pair of two-level emitters, chirally coupled to a waveguide, may scatter single- and two-photon components of an input pulse into orthogonal temporal modes with a fidelity $\gtrsim 0.9997$. We develop a general theory to characterize and optimize this process and observe an interesting dynamics in the two-photon scattering regime: while the first emitter gives rise to a complex multimode field, the second emitter recombines the field amplitudes and the net two-photon scattering induces a self-time reversal of the pulse mode. The presented scheme can be employed to construct logic elements for propagating photons, such as a deterministic nonlinear-sign gate with a fidelity $\gtrsim 0.9995$

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Cavity Quantum Electrodynamics Effects with Nitrogen Vacancy Center Spins in Diamond and Microwave Resonators at Room Temperature

Cavity quantum electrodynamics (C-QED) effects, such as Rabi splitting, Rabi oscillations and superradiance, have been demonstrated with nitrogen vacancy center spins in diamond in microwave resonators at cryogenic temperature. In this article we explore the possibility to realize strong collective coupling and the resulting C-QED effects with ensembles of spins at room temperature. Thermal excitation of the individual spins by the hot environment leads to population of collective Dicke states with low symmetry and a reduced collective spin-microwave field coupling. However, we show with simulations that the thermal excitation can be compensated by spin-cooling via optical pumping. The resulting population of Dicke states with higher symmetry implies strong coupling with currently available high-quality resonators and enables C-QED effects at room temperature with potential applications in quantum sensing and quantum information processing.

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Adiabatic theorem revisited: the unexpectedly good performance of adiabatic passage

Adiabatic passage employs a slowly varying time-dependent Hamiltonian to control the evolution of a quantum system along the Hamiltonian eigenstates. For processes of finite duration, the exact time evolving state may deviate from the adiabatic eigenstate at intermediate times, but in numerous applications it is observed that this deviation reaches a maximum and then decreases significantly towards the end of the process. We provide a straightforward theoretical explanation for this welcome but often unappreciated fact. Our analysis emphasizes a separate adiabaticity criterion for high fidelity state-to-state transfer and it points to new effective shortcut strategies for near adiabatic dynamics.

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Quantum estimation of a time dependent perturbation

We analyze the estimation of a time dependent perturbation acting on a continuously monitored quantum system. We describe the temporal fluctuations of the perturbation by a Hidden Markov Model, and we combine quantum measurement theory and classical filter theory into a time evolving hybrid quantum and classical trajectory. The forward-backward analysis that permits smoothed estimates of classical Hidden Markov Models has a counterpart in the theory of retrodiction and Past Quantum States. As a specific example, we apply our hybrid trajectory and Past Quantum State theory to the sensing of a fluctuating magnetic field by microwave interrogation of a single quantum spin.

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A Superradiant Maser with Nitrogen-Vacancy Center Spins

Recent experiments have demonstrated Rabi-oscillations, superradiant pulses and stimulated emission from negatively-charged nitrogen-vacancy ($\mathrm{NV}^{-}$) center spins in microwave resonators. These phenomena witness the kind of collective and strong coupling which has been prerequisite for observation of superradiant lasing in the optical frequency regime. In this article, we investigate the possibility to employ coherence, present in both the collective $\mathrm{NV}^{-}$ spin ensemble and the microwave field, to achieve a superradiant maser. Our calculations show that a superradiant maser with a linewidth below millihertz can be achieved with moderate kilohertz incoherent pumping of over $10^{14}$ spins kept at low temperature. We show that the superradiant masing prevails in the presence of inhomogeneous broadening, and we present numerical and analytical studies of the dependence of the phenomenon on the various physical parameters.

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Active Frequency Measurement on Superradiant Strontium Clock Transitions

We develop a stochastic mean-field theory to describe active frequency measurements of pulsed superradiant emission, studied in recent experiments with strontium-87 atoms trapped in an optical lattice inside an optical cavity [M. Norcia, et al., Phys. Rev. X 8, 21036 (2018)]. Our theory reveals the intriguing dynamics of atomic ensembles with multiple transition frequencies, and it reproduces the superradiant beats signal, noisy power spectra, and frequency uncertainty in remarkable agreement with the experiments. Moreover, by reducing the number of atoms, elongating the superradiant pulses and shortening the experimental duty cycle, we predict a short-term frequency uncertainty $9\times10^{-16} \sqrt{τ/s}$, which makes active frequency measurements with superradiant transitions comparable with the record performance of current frequency standards [M. Schioppo, et al., Nat. Photonics, 11, 48 (2017)]. Our theory combines cavity-quantum electrodynamics and quantum measurement theory, and it can be readily applied to explore conditional quantum dynamics and describe frequency measurements for other processes such as steady-state superradiance and superradiant Raman lasing.

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How well can we guess the outcome of measurements of non-commuting observables?

According to Heisenberg's uncertainty relation, there is an ultimate limit to how precisely we may predict the outcome of position and momentum measurements on a quantum system. We show that this limit may be violated by an arbitrarily large factor if one aims, instead, to guess the unknown value of a past measurement. For experiments on a single quantum system, the precise assignment of past position and momentum measurement outcomes is accompanied by large uncertainty about their linear combinations, while we show that entanglement with an ancillary system permits accurate retrodiction of any such linear combination. Finally, we show that the outcomes of experiments that jointly measure multiple linear combinations of position and momentum observables by means of ancillary probe particles can also be guessed with no formal lower limit. We present quantitative results for projective measurements and for generalized measurements where all components are prepared in Gaussian states.

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Roadmap for Rare-earth Quantum Computing

Several platforms are being considered as hardware for quantum technologies. For quantum computing (QC), superconducting qubits and artificially trapped ions are among the leading platforms, but many others also show promise, e.g. photons, cold atoms, defect centers including Rare-Earth (RE) ions. So far, results are limited to the regime of noisy intermediate scale qubits (NISQ), with a small number of qubits and a limited connectivity, and it is likely that future QC hardware will utilize several existing platforms in different ways. Thus, it currently makes sense to invest resources broadly and explore the full range of promising routes to quantum technology. Rare-earth ions in solids constitute one of the most versatile platforms for future quantum technology. One advantage is good coherence properties even when confined in strong natural traps inside a solid-state matrix. This confinement allows very high qubit densities and correspondingly strong ion-ion couplings. In addition, although their fluorescence is generally weak, cavity integration can enhance the emission greatly and enable very good connections to photonic circuits, including at the telecom wavelengths, making them promising systems for long-term scalability. The primary aim of this roadmap is to provide a complete picture of what components a RE quantum computer would consist of, to describe the details of all parts required to achieve a scalable system, and to discuss the most promising paths to reach it. In brief, we find that clusters of 50-100 single RE ions can act as high fidelity qubits in small processors, occupying only about (10 nm)^3. Due to the high capacity for integration of the RE systems, they be optically read out and connected to other such clusters for larger scalability. We make suggestions for future improvements, which could allow the REQC platform to be a leading one.

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Ancilla mediated qubit readout and heralded entanglement between rare-earth dopant ions in crystals

Owing to their long excited state lifetimes, rare-earth ions in crystals are widely used in quantum applications. To allow optical readout of the qubit state of individual ions, we propose to dope the crystal with an additional nearby ancilla ion with a shorter radiative lifetime. We show how a Bayesian analysis exhausts the information about the state of the qubit from the optical signal of the ancilla ion. We study the effects of incoherent processes and propose ways to reduce their effect on the readout. Finally, we extend the architecture to ions residing in two remote cavities, and we show how continuous monitoring of fluorescence signals from the two ancilla ions leads to entanglement of the qubit ions.

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Collective emission of photons from dense, dipole-dipole interacting atomic ensembles

We study the collective radiation properties of cold, trapped ensembles of atoms. We consider the high density regime with the mean interatomic distance being comparable to, or smaller than, the wavelength of the resonant optical radiation emitted by the atoms. We find that the emission rate of a photon from an excited atomic ensemble is strongly enhanced for an elongated cloud. We analyze collective single-excitation eigenstates of the atomic ensemble and find that the absorption/emission spectrum is broadened and shifted to lower frequencies as compared to the non-interacting (low density) or single atom spectrum. We also analyze the spatial and temporal profile of the emitted radiation. Finally, we explore how to efficiently excite the collective super-radiant states of the atomic ensemble from a long-lived storage state in order to implement matter-light interfaces for quantum computation and communication applications.

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Time-dependent atomic magnetometry with a recurrent neural network

We propose to employ a recurrent neural network to estimate a fluctuating magnetic field from continuous optical Faraday rotation measurement on an atomic ensemble. We show that an encoder-decoder architecture neural network can process measurement data and learn an accurate map between recorded signals and the time-dependent magnetic field. The performance of this method is comparable to Kalman filters while it is free of the theory assumptions that restrict their application to particular measurements and physical systems.

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Subradiant emission from regular atomic arrays: universal scaling of decay rates from the generalized Bloch theorem

The Hermitian part of the dipole-dipole interaction in infinite periodic arrays of two-level atoms yields an energy band of singly excited states. In this Letter, we show that a dispersion relation, $ω_k-ω_{k_\ex} \propto (k-k_{\ex})^s$, near the band edge of the infinite system leads to the existence of subradiant states of finite one-dimensional arrays of $N$ atoms with decay rates scaling as $N^{-(s+1)}$. This explains the recently discovered $N^{-3}$ scaling and it leads to the prediction of power law scaling with higher power for special values of the lattice period. For the quantum optical implementation of the Su-Schrieffer-Heeger (SSH) topological model in a dimerized emitter array, the band-gap-closing inherent to topological transitions changes the value of $s$ in the dispersion relation and alters the decay rates of the subradiant states by many orders of magnitude.

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Retrodiction beyond the Heisenberg uncertainty relation

In quantum mechanics, the Heisenberg uncertainty relation presents an ultimate limit to the precision by which one can predict the outcome of position and momentum measurements on a particle. Heisenberg explicitly stated this relation for the prediction of "hypothetical future measurements", and it does not describe the situation where knowledge is available about the system both earlier and later than the time of the measurement. We study what happens under such circumstances with an atomic ensemble containing $10^{11}$ $^{87}\text{Rb}$ atoms, initiated nearly in the ground state in presence of a magnetic field. The collective spin observables of the atoms are then well described by canonical position and momentum observables, $\hat{x}_A$ and $\hat{p}_A$ that satisfy $[\hat{x}_A,\hat{p}_A]=i\hbar$. Quantum non-demolition measurements of $\hat{p}_A$ before and of $\hat{x}_A$ after time $t$ allow precise estimates of both observables at time $t$. The capability of assigning precise values to multiple observables and to observe their variation during physical processes may have implications in quantum state estimation and sensing.

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Radiation Eigenmodes of Dicke Superradiance

We calculate the field eigenmodes of the superradiant emission from an ensemble of $N$ two-level atoms. While numerical techniques are effective due to the symmetry of the problem, we develop also an analytical method to approximates the modes in the limit of a large number of emitters. We find that Dicke superradiant emission is restricted to a small number of modes, with a little over 90\% of the photons emitted in a single dominant mode.

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Crowdsourcing human common sense for quantum control

Citizen science methodologies have over the past decade been applied with great success to help solve highly complex numerical challenges. Here, we take early steps in the quantum physics arena by introducing a citizen science game, Quantum Moves 2, and compare the performance of different optimization methods across three different quantum optimal control problems of varying difficulty. Inside the game, players can apply a gradient-based algorithm (running locally on their device) to optimize their solutions and we find that these results perform roughly on par with the best of the tested standard optimization methods performed on a computer cluster. In addition, cluster-optimized player seeds was the only method to exhibit roughly optimal performance across all three challenges. This highlights the potential for crowdsourcing the solution of future quantum research problems.

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Self-stimulated pulse echo trains from inhomogeneously broadened spin ensembles

We show experimentally and describe theoretically how a conventional magnetic resonance Hahn echo sequence can lead to a self-stimulated pulse echo train when an inhomogeneously broadened spin ensemble is coupled to a resonator. Effective strong coupling between the subsystems assures that the first Hahn echo can act as a refocussing pulse on the spins, leading to self-stimulated secondary echoes. Within the framework of mean field theory, we show that this process can continue multiple times leading to a train of echoes. We introduce an analytical model that explains the shape of the first echo and numerical results that account well for the experimentally observed shape and strength of the echo train and provides insights into the collective effects involved.

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