arXiv subjects

Krishnendu Maji

Publications and source records attributed to Krishnendu Maji.

5 recordsLinked to original sources

arXiv2026

Superconducting cavity probes sliding ferroelectricity in small-angle twisted WSe$_2$

Ferroelectricity is a property of materials that exhibit spontaneous charge polarization. Ferroelectricity in 2D materials is interesting because of their applications in memory devices and field-effect transistors. Recently, a new type of ferroelectricity, known as sliding ferroelectricity, has been discovered, in which parallel-stacked bilayers of hexagonal boron nitride (hBN) or transition metal dichalcogenides (TMDCs) develop an out-of-plane electric polarization. In this work, we probe the polarization of small-angle parallel stacked WSe$_2$ by measuring its high-frequency AC response, achieved by embedding it into a half-wave superconducting coplanar waveguide cavity. We observe a hysteretic response in the capacitance of the stack and quality factor of the cavity, confirming ferroelectric switching in the system. Our results further reveal relaxation effects associated with ferroelectric domain-wall motion. This cavity-based technique has potential applications in probing domain-wall dynamics in a ferroelectric system at high frequencies.

cond-mat.mes-hall↗

arXiv2025

Cavity based sensing of antiferromagnetic canting and nonzero-momentum spin waves in a van der Waals cavity-magnon-polariton system

Cavity-magnon-polaritons are hybrid excitations from the interaction between cavity photons and magnons, the quanta of collective spin oscillations. Along with the tunability of the magnon-photon coupling strength, fast information transfer and conversion speed are desired in hybrid devices. This can be achieved utilizing the propagating nature of spin waves with non-zero momentum for their ultra-fast time dynamics and reduced ohmic dissipation. Antiferromagnets are particularly interesting as hosts for magnons since stray-field interactions are minimized, and they support multiple modes with distinctive magnetic-field behavior across the phase diagram. CrCl3 is a van der Waals antiferromagnet having a strong easy-plane anisotropy and a weak in-plane easy-axis anisotropy. Despite some magnetic resonance studies, the impact of magnetic reorientation of spins in CrCl3 on cavity-magnon-polariton interaction strength as a function of magnetic field remains largely unexplored. In this study, we investigate the coupling between magnons in CrCl3 and photons in a coplanar waveguide resonator as a function of magnetic field. In particular, we find that the magnon-photon coupling strength varies nonmonotonically and distinctly with the magnetic field for both acoustic and optical magnons, enabling tuning of the coupling strength with an external magnetic field as a knob. We find the signature of spin-flop transition in two harmonics of the cavity due to a stronger dispersive coupling between optical magnons and cavity photons at lower fields. Additionally, we find standing modes formed by spin waves with nonzero momentum associated with the two hybrid magnons when the external field is applied at an angle with the crystal plane. These modes do not undergo substantial coupling with the cavity mode unlike the antiferromagnetic modes and can be used as low-loss propagation channels in hybrid devices.

cond-mat.mes-hall↗

arXiv2025

Diffuson-Dominated Thermal Transport Crossover from Ordered to Liquid-like Cu$_3$BiS$_3$:The Negligible Role of Ion Hopping

Fundamentally understanding lattice dynamics and thermal transport behavior in liquid-like, partially occupied compounds remains a long-standing challenge in condensed matter physics. Here, we investigate the microscopic mechanisms underlying the ultralow thermal conductivity in ordered/liquid-like Cu$_3$BiS$_3$ by combining experimental methods with first-principles calculations. We first experimentally synthesize and characterize the ordered structure and liquid-like, partially Cu-atom occupied Cu$_3$BiS$_3$ structure with increasing temperature. We then combine self-consistent phonon calculations, including bubble-diagram corrections, with the Wigner transport equation, considering both phonon propagation and diffuson contributions, to evaluate the anharmonic lattice dynamics and thermal conductivity in phase-change Cu$_3$BiS$_3$. Our theoretical model predicts an ultralow thermal conductivity of 0.34 W/m/K at 400 K, dominated by diffuson contributions, which accurately reproduces and explains the experimental data. Importantly, the machine-learning-based molecular dynamics (MD) simulations not only reproduced the partially Cu-atom occupied Cu$_3$BiS$_3$ structure with the space group $\mathrm{P2_12_12_1}$ but also successfully replicated the thermal conductivity obtained from experiments and Wigner transport calculations. This observation highlights the negligible impact of ionic mobility arising from partially occupied Cu sites on the thermal conductivity in diffuson-dominated thermal transport compounds. Our work not only sheds light on the minimal impact of ionic mobility on ultralow thermal conductivity in phase-change materials but also demonstrates that the Wigner transport equation accurately describes thermal transport behavior in partially occupied phases with diffuson-dominant thermal transport.

cond-mat.mtrl-sci↗

arXiv2025

Kerr non-linearity enhances the response of a graphene Josephson bolometer

Highly sensitive, broadband bolometers are of great interest because of their versatile usage in wide areas starting from dark matter search, radio astronomy, material science, and qubit readouts in cQED experiments. There have been different realizations of bolometers using superconducting thin films, nanowires, quantum dots, and various 2D materials in the recent past. The challenge is to have a single device that combines high sensitivity, broad bandwidth, a fast readout mechanism, and low noise. Here we demonstrate the first usage of a Josephson parametric amplifier (JPA) as a highly sensitive bolometer. Our key finding is the Kerr non-linearity of the JPA boosts the device's sensitivity. When the bolometer is biased in the non-linear regime, it enhances the sideband signals (~100 times), resulting in an order of magnitude improvement in sensitivity compared to the linear regime. In the non-linear biasing of the device, we achieve a NEP~500 aW/sqrt(Hz). Our bolometer offers a fast detection scheme with a thermal time constant of 4.26 us and an intrinsic JPA time constant of 70 ns. Our device's broadband and fast operation are key and new compared to previously studied graphene-based bolometers. In our device, the gate voltage tunability and the possibility of multiplexing combined with the sensitive bolometric performance offer an opportunity for integrated quantum sensor arrays. Our work demonstrates a way forward to enhance the performance of quantum sensors based on 2D materials by leveraging the inherent non-linear response.

cond-mat.mes-hall↗

arXiv2024

Superconducting Cavity-Based Sensing of Band Gaps in 2D Materials

The superconducting coplanar waveguide (SCPW) cavity plays an essential role in various areas like superconducting qubits, parametric amplifiers, radiation detectors, and studying magnon-photon and photon-phonon coupling. Despite its wide-ranging applications, the use of SCPW cavities to study various van der Waals 2D materials is relatively unexplored. The resonant modes of the SCPW cavity exquisitely sense the dielectric environment. In this work, we measure the charge compressibility of bilayer graphene coupled to a half-wavelength SCPW cavity. Our approach provides a means to detect subtle changes in the capacitance of the bilayer graphene heterostructure, which depends on the compressibility of bilayer graphene, manifesting as shifts in the resonant frequency of the cavity. This method holds promise for exploring a wide class of van der Waals 2D materials, including transition metal dichalcogenides (TMDs) and their moir\'e where DC transport measurement is challenging.

cond-mat.mes-hall↗