arXiv subjects

Kristiaan De Greve

Publications and source records attributed to Kristiaan De Greve.

50 records · Page 3Linked to original sources

arXiv2019

Quantum-Assisted Telescope Arrays

Quantum networks provide a platform for astronomical interferometers capable of imaging faint stellar objects. In a recent work [arXiv:1809.01659], we presented a protocol that circumvents transmission losses with efficient use of quantum resources and modest quantum memories. Here we analyze a number of extensions to that scheme. We show that it can be operated as a truly broadband interferometer and generalized to multiple sites in the array. We also analyze how imaging based on the quantum Fourier transform provides improved signal-to-noise ratio compared to classical processing. Finally, we discuss physical realizations including photon-detection-based quantum state transfer.

quant-ph↗

arXiv2019

Optical Interferometry with Quantum Networks

We propose a method for optical interferometry in telescope arrays assisted by quantum networks. In our approach, the quantum state of incoming photons along with an arrival time index is stored in a binary qubit code at each receiver. Nonlocal retrieval of the quantum state via entanglement-assisted parity checks at the expected photon arrival rate allows for direct extraction of the phase difference, effectively circumventing transmission losses between nodes. Compared to prior proposals, our scheme (based on efficient quantum data compression) offers an exponential decrease in required entanglement bandwidth. Experimental implementation is then feasible with near-term technology, enabling optical imaging of astronomical objects akin to well-established radio interferometers and pushing resolution beyond what is practically achievable classically.

quant-ph↗

arXiv2018

Electrical control of interlayer exciton dynamics in atomically thin heterostructures

Excitons in semiconductors, bound pairs of excited electrons and holes, can form the basis for new classes of quantum optoelectronic devices. A van der Waals heterostructure built from atomically thin semiconducting transition metal dichalcogenides (TMDs) enables the formation of excitons from electrons and holes in distinct layers, producing interlayer excitons with large binding energy and a long lifetime. Employing heterostructures of monolayer TMDs, we realize optical and electrical generation of long-lived neutral and charged interlayer excitons. We demonstrate the transport of neutral interlayer excitons across the whole sample that can be controlled by excitation power and gate electrodes. We also realize the drift motion of charged interlayer excitons using Ohmic-contacted devices. The electrical generation and control of excitons provides a new route for realizing quantum manipulation of bosonic composite particles with complete electrical tunability.

cond-mat.mes-hall↗

arXiv2018

Origins of diamond surface noise probed by correlating single spin measurements with surface spectroscopy

The nitrogen vacancy (NV) center in diamond exhibits spin-dependent fluorescence and long spin coherence times under ambient conditions, enabling applications in quantum information processing and sensing. NV centers near the surface can have strong interactions with external materials and spins, enabling new forms of nanoscale spectroscopy. However, NV spin coherence degrades within 100 nanometers of the surface, suggesting that diamond surfaces are plagued with ubiquitous defects. Prior work on characterizing near-surface noise has primarily relied on using NV centers themselves as probes; while this has the advantage of exquisite sensitivity, it provides only indirect information about the origin of the noise. Here we demonstrate that surface spectroscopy methods and single spin measurements can be used as complementary diagnostics to understand sources of noise. We find that surface morphology is crucial for realizing reproducible chemical termination, and use these insights to achieve a highly ordered, oxygen-terminated surface with suppressed noise. We observe NV centers within 10 nm of the surface with coherence times extended by an order of magnitude.

cond-mat.mtrl-sci↗

arXiv2017

Atomically thin mirrors made of monolayer semiconductors

Transition metal dichalcogenide monolayers are promising candidates for exploring new electronic and optical phenomena and for realizing atomically thin optoelectronic devices. They host tightly bound electron-hole pairs (excitons) that can be efficiently excited by resonant light fields. Here, we demonstrate that a single monolayer of molybdenum diselenide (MoSe2) can dramatically modify light transmission near the excitonic resonance, acting as an electrically switchable mirror that reflects up to 85% of incident light at cryogenic temperatures. This high reflectance is a direct consequence of the excellent coherence properties of excitons in this atomically thin semiconductor, encapsulated by hexagonal boron nitride. Furthermore, we show that the MoSe2 monolayer exhibits power- and wavelength-dependent nonlinearities that stem from exciton-based lattice heating in the case of continuous-wave excitation and exciton-exciton interactions when fast, pulsed laser excitation is used. These observations open up new possibilities for studying quantum nonlinear optical phenomena and topological photonics, and for miniaturizing optical devices.

cond-mat.mes-hall↗

arXiv2015

Towards Quantum Repeaters with Solid-State Qubits: Spin-Photon Entanglement Generation using Self-Assembled Quantum Dots

In this chapter we review the use of spins in optically-active InAs quantum dots as the key physical building block for constructing a quantum repeater, with a particular focus on recent results demonstrating entanglement between a quantum memory (electron spin qubit) and a flying qubit (polarization- or frequency-encoded photonic qubit). This is a first step towards demonstrating entanglement between distant quantum memories (realized with quantum dots), which in turn is a milestone in the roadmap for building a functional quantum repeater. We also place this experimental work in context by providing an overview of quantum repeaters, their potential uses, and the challenges in implementing them.

quant-ph↗

arXiv2013

A high-speed optical link to entangle quantum dots

A long-distance quantum network for distributing entangled states would support novel information applications, such as unconditionally secure cryptography and distributed quantum computing. Realizing such a network requires hardware that can reliably and efficiently establish entanglement over long distances, despite challenges like loss and transmission delay. We propose a new scheme for distributing entanglement that increases communication rates one to two orders of magnitude over existing protocols. The method is less sensitive to overall system loss because it transmits many signals within one round-trip-time window and efficiently discriminates lost-photon events. While the scheme applies to many types of matter qubits, we analyze a specific implementation with optical quantum dots, showing that the method uses practical hardware consistent with recent experiments.

quant-ph↗

arXiv2013

Downconversion quantum interface for a single quantum dot spin and 1550-nm single-photon channel

Long-distance quantum communication networks require appropriate interfaces between matter qubit-based nodes and low-loss photonic quantum channels. We implement a downconversion quantum interface, where the single photons emitted from a semiconductor quantum dot at 910 nm are downconverted to 1560 nm using a fiber-coupled periodically poled lithium niobate waveguide and a 2.2-$μ$m pulsed pump laser. The single-photon character of the quantum dot emission is preserved during the downconversion process: we measure a cross-correlation $g^{(2)}(τ= 0) = 0.17$ using resonant excitation of the quantum dot. We show that the downconversion interface is fully compatible with coherent optical control of the quantum dot electron spin through the observation of Rabi oscillations in the downconverted photon counts. These results represent a critical step towards a long-distance hybrid quantum network in which subsystems operating at different wavelengths are connected through quantum frequency conversion devices and 1.5-$μ$m quantum channels.

quant-ph↗

arXiv2011

Coherent control and suppressed nuclear feedback of a single quantum dot hole qubit

Future communication and computation technologies that exploit quantum information require robust and well-isolated qubits. Electron spins in III-V semiconductor quantum dots, while promising candidates, see their dynamics limited by undesirable hysteresis and decohering effects of the nuclear spin bath. Replacing electrons with holes should suppress the hyperfine interaction and consequently eliminate strong nuclear effects. Using picosecond optical pulses, we demonstrate coherent control of a single hole qubit and examine both free-induction and spin-echo decay. In moving from electrons to holes, we observe significantly reduced hyperfine interactions, evidenced by the reemergence of hysteresis-free dynamics, while obtaining similar coherence times, limited by non-nuclear mechanisms. These results demonstrate the potential of optically controlled, quantum dot hole qubits.

quant-ph↗

arXiv2011

On the origin of non-monotonic doping dependence of the in-plane resistivity anisotropy in Ba(Fe$_{1-x}T_x$)$_2$As$_2$, $T$ = Co, Ni and Cu

The in-plane resistivity anisotropy has been measured for detwinned single crystals of Ba(Fe$_{1-x}$Ni$_x$)$_2$As$_2$ and Ba(Fe$_{1-x}$Cu$_x$)$_2$As$_2$. The data reveal a non-monotonic doping dependence, similar to previous observations for Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$. Magnetotransport measurements of the parent compound reveal a non-linear Hall coefficient and a strong linear term in the transverse magnetoresistance. Both effects are rapidly suppressed with chemical substitution over a similar compositional range as the onset of the large in-plane resistivity anisotropy. It is suggested that the relatively small in-plane anisotropy of the parent compound in the spin density wave state is due to the presence of an isotropic, high mobility pocket of reconstructed Fermi surface. Progressive suppression of the contribution to the conductivity arising from this isotropic pocket with chemical substitution eventually reveals the underlying in-plane anisotropy associated with the remaining FS pockets.

cond-mat.supr-con↗

arXiv2010

Nuclear Feedback in a Single Electron-Charged Quantum Dot under Pulsed Optical Control

Electron spins in quantum dots under coherent control exhibit a number of novel feedback processes. Here, we present experimental and theoretical evidence of a feedback process between nuclear spins and a single electron spin in a single charged InAs quantum dot, controlled by the coherently modified probability of exciting a trion state. We present a mathematical model describing competition between optical nuclear pumping and nuclear spin-diffusion inside the quantum dot. The model correctly postdicts the observation of a hysteretic sawtooth pattern in the free-induction-decay of the single electron spin, hysteresis while scanning a narrowband laser through the quantum dot's optical resonance frequency, and non-sinusoidal fringes in the spin echo. Both the coherent electron-spin rotations, implemented with off-resonant ultrafast laser pulses, and the resonant narrow-band optical pumping for spin initialization interspersed between ultrafast pulses, play a role in the observed behavior. This effect allows dynamic tuning of the electron Larmor frequency to a value determined by the pulse timing, potentially allowing more complex coherent control operations.

quant-ph↗

arXiv2010

Evidence for an electron nematic phase transition in underdoped iron pnictide superconductors

Electrical resistivity measurements of detwinned single crystals of the representative iron arsenide Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ reveal a dramatic in-plane anisotropy associated with the tetragonal-to-orthorhombic structural transition that precedes the onset of long-range antiferromagnetic order. These results indicate that the structural transition in this family of compounds is fundamentally electronic in origin.

cond-mat.supr-con↗

arXiv2009

Pulsed Nuclear Pumping and Spin Diffusion in a Single Charged Quantum Dot

We report the observation of a feedback process between the nuclear spins in a single charged quantum dot and its trion transition, driven by a periodic sequence of optical pulses. The pulse sequence intersperses off-resonant ultrafast pulses for coherent electron-spin rotation and resonant narrow-band optical pumping. The feedback manifests as a hysteretic triangle-like pattern in the free-induction-decay of the single spin. We present a simple, quasi-analytic numerical model to describe this observation, indicating that the feedback process results from the countering effects of optical nuclear pumping and nuclear spin-diffusion inside the quantum dot. This effect allows dynamic tuning of the electron Larmor frequency to a value determined by the pulse timing, potentially allowing more complex coherent control operations.

quant-ph↗

arXiv2009

In-plane electronic anisotropy in underdoped Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ revealed by detwinning in a magnetic field

We present results of angle-dependent magnetoresistance measurements and direct optical images of underdoped Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ which reveal partial detwinning by action of a 14T magnetic field. Driven by a substantial magneto-elastic coupling, this result provides evidence for an electronic origin of the lattice distortion in underdoped iron pnictides. The observed anisotropy in these partially detwinned samples implies a substantial in-plane electronic anisotropy in the broken symmetry state, with a smaller resistivity along the antiferromagnetic ordering direction.

cond-mat.supr-con↗